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Abstract
In this paper, the Life Cycle Assessment (LCA) methodology is applied to Portuguese printing and writing paper in order to
compare the environmental impact of the use of two kinds of fuels (heavy fuel oil and natural gas) in the pulp and paper production
processes. The results of inventory analysis and impact assessment show that the pulp and paper production processes play an
important role in almost all of the analysed parameters, which do not always result in an important contribution to the corresponding
impact categories. The substitution of heavy fuel oil by natural gas in the pulp and paper production processes seems to be environmentally positive. 2002 Elsevier Science Ltd. All rights reserved.
Keywords: LCA; Pulp; Paper; Eucalyptus globulus; Natural gas; Heavy fuel oil
1. Introduction
The concept of sustainability is becoming increasingly
important in the Portuguese pulp and paper industry,
which is one of the most important economic activities
in Portugal. In order to improve its environmental performance, this industry has made important investments,
not only in the production process itself, but also in the
flue gases and liquid effluents treatment systems. Besides
this concern regarding pollution prevention, one of the
issues of most relevance in the context of sustainability
is the consumption of energy. Traditionally, Portuguese
mills have used fuel oil as a fossil fuel in the chemical
recovery system in pulp production and for on-site
energy production in paper manufacturing. However, a
new source of primary energy is now becoming available
for the Portuguese industry with the recent installation
of a national grid of natural gas. The utilisation of this
alternative fossil fuel instead of fuel oil constitutes an
interesting option from both the environmental and economic point of view. This is particularly true in paper
production where energy production in a combined cycle
Corresponding author. Tel.: +351 234 370 200; fax: +351 234
429 290.
E-mail address: arroja@dao.ua.pt (L. Arroja).
seems appealing for reasons related to energy rationalisation issues. More than being aware of the consequences
of natural gas utilisation in the mills, it is important to
evaluate the global impact of this process modification
through the whole paper life cycle. Life Cycle Assessment (LCA) is thus the most appropriate tool to achieve
this purpose, allowing a global overview of this activity.
In this study, LCA methodology was applied to Portuguese production of printing and writing paper in order
to evaluate its environmental performance and also to
make a comparative environmental assessment of fuel
oil and natural gas, respectively, as energy sources in
the manufacturing process.
2. Methodology
This study was performed using a methodological
framework based on ISO (International Organization for
Standardization) recommendations [14]. According to
ISO, LCA is divided into four phases: goal and scope
definition, inventory analysis, impact assessment and
interpretation.
The goal and scope definition is extremely important
since the study will be carried out according to the statements made in this phase. The goal must refer the
intended application and audience, and the reasons for
0959-6526/02/$ - see front matter 2002 Elsevier Science Ltd. All rights reserved.
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conducting the study. In the scope definition, the following items, among others, should be described: system
under study, functional unit (FU), system boundaries,
allocation procedures, impact assessment methodologies,
data quality requirements and assumptions.
The inventory analysis involves data collection on raw
materials and energy consumption, emissions to air,
water and soil and solid waste generation.
The impact assessment phase assigns inventory results
to impact categories and quantifies the system potential
contribution to different environmental impacts.
Finally, in the interpretation phase, the inventory
analysis and impact assessment results are discussed and
the significant environmental issues are identified to
reach conclusions and recommendations consistent with
the goal and scope requirements.
Fig. 1.
System boundaries.
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2.2.8. Transports
This subsystem includes the circulation, between subsystems, of wood, softwood pulp, paper, wastepaper,
chemicals and fuels by 16 tonne, 28 tonne and garbage
trucks, ocean ships and electric trains. The travelled distances were provided by the involved bodies and the
emission factors were obtained from the literature [8].
2.2.6.2. Landfilling
70% of the landfill sites considered in this final disposal alternative include systems
for leachate control, collection and treatment, and 30%
represent uncontrolled tipping, the latter meaning that
landfill sites are not lined with an impermeable layer or
layers, and do not include systems for leachate control,
collection and treatment. In both cases the landfill gas
is neither burnt nor used for energy recovery. Inventory
data were based on data from literature [11] allocated to
the paper fraction of municipal solid waste (MSW) on
a causality basis. When leachate treatment occurs, liquid
emissions were calculated considering Portuguese wastewater discharge legislation.
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Table1
Impact categories and corresponding parameters
Impact category
Parameters
3. Results
3.1. Inventory analysis results
It is possible to make a first interpretation at the inventory analysis level based on individual parameters. The
inventory results consist of an exhaustive list of parameters, but in this paper only the parameters commonly
discussed from an environmental point of view are analysed: non-renewable and renewable energy consumption, non-renewable carbon dioxide (CO2), nitrogen
oxides (NOx), sulfur dioxide (SO2), chemical oxygen
demand (COD) and adsorbable organic halogens (AOX).
Figs. 24 show the energy consumption, the air emissions and the water emissions at the different stages of
the paper life cycle, for the actual scenario and for the
natural gas scenario. It is important to note that only the
Fig. 2.
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Fig. 4.
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Fig. 5.
4. Conclusions
Based on the inventory analysis and impact assessment results, the following conclusions can be drawn
concerning the contribution of the different processes to
the printing and writing paper life cycle environmental
impact, which was one the reasons stated for carrying
out this study:
the printing and writing paper production is the most
important contributor to non-renewable CO2 emissions due to on-site energy production, which does
not correspond, however, to a major contribution to
the overall global warming potential. Actually, in Portugal this impact category is dominated by CH4 emissions from wastepaper landfilling. On-site energy production in the paper production subsystem is the
major source of SO2 emissions, which makes it the
most significant contributor to the acidification impact
category. This subsystem is also the main consumer
of non-renewable energy and, as a result, it is responsible for the most important share of the global system
[4]
[5]
Acknowledgements
[6]
[7]
[8]
[9]
[10]
[11]
References
[1] International Organization for Standardization (ISO), Environmental management Life cycle assessment Principles and
framework. ISO 14040, 1997.
[2] International Organization for Standardization (ISO), Environmental management Life cycle assessment Goal and scope
definition and inventory analysis. ISO 14041, 1998.
[3] International Organization for Standardization (ISO), Environ-
[12]
[13]
[14]
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