AECL-9881 ^ R ^

ATOMIC ENERGY mS& ENERGIE ATOMIQUE

OF CANADA LIMITED ^fi9 DU CANADA LIMITEE
Research Company ^ ^ ^ ^ Societe de Recherche

DERIVATION OF INITIAL RADIONUCUDE INVENTORIES FOR THE SAFETY ASSESSMENT

OF THE DISPOSAL OF USED CANDU® FUEL

OBTENTION DES INVENTAIRES INITIAUX DE RADIONUCLIDES POUR DEVALUATION DE L'EVACUATION

DU COMBUSTIBLE IRRADIE DE REACTEUR CANDU® QUANT A LA SURETE

J. C. Tait, I. C. Gould, G. B. Wilkin

Whit«sh«ll Nucl«ar R«s«arch Etablisstmant d* recherches

Establishment nucl«air«s d« Whiteshell
Pinawa, Manitoba ROE UO
August 1989 aout
Copyright ® Atomic Energy of Canada Limited, 1989.
 ATOMIC ENERGY OF CANADA LIMITED

DERIVATION OF INITIAL RADIONUCLIDE INVENTORIES FOR THE SAFETY ASSESSMENT

OF THE DISPOSAL OF USED CANDU®FUEL

by

J.C. Tait, I.C. Gauld and G.B. Uilkin

Vhiteshell Nuclear Research Establishnent

Pinava, Manitoba ROE 1L0
1989
AECL-9881
 OBTENTION DES INVENTAIRES INITIAUX DE RADIONUCLIDES POUR L'ÉVALUATION
DE L'ÉVACUATION DU COMBUSTIBLE IRRADIÉ DE RÉACTEUR CÀNDU©
QUANT À LA SÛRETÉ

par

J.C. Tait, I.C. Gauld et G.B. Vilkin

RÉSUMÉ

On s'est servi du programme ORIGEN-S de calcul de la production et diminution de radionuclides pour

prédire la masse, la radioactivité et la chaleur de désintégration des radionuclides produits dans le
combustible d'UO2 du réacteur Bruce "A" et sa gaine de zircaloy ainsi que des radionuclides produits
par activation neutronique des impuretés de ce combustible et de cette gaine. La compilation a été
réalisée pour fournir des résultats d'inventaires initiaux de radionuclides à utiliser pour l'évalua-
tion de l'évacuation du combustible irradié de réacteur CANDU quant à la sûreté. En outre, on
présente une comparaison des résultats avec ceux obtenus à l'aide du programme de calcul CANIGEN-II.

Énergie atomique du Canada limitée

Établissement de recherches nucléaires de Vhiteshell
Pinava, Manitoba ROE 1L0
1989
AECL-9881
 DERIVATION OF INITIAL RADIONUCLIDE INVENTORIES
FOR THE SAFETY ASSESSMENT OF THE DISPOSAL
OF USED CANDU® FUEL

by

J.C. T a i t , I . C . Gauld and G.B. Villein

ABSTRACT

The ORIGEN-S radionuclide generation and depletion code has been used to predict the mass, activity and
decay heat of radionuclides produced in Bruce "A" U0 2 reactor fuel and the Zircaloy cladding and of
radionuclides produced by neutron activation of impurities in both the U0 2 fuel and the Zircaloy
cladding. This compilation has been produced to provide initial radionuclide inventory data for use in
the safety assessment of the disposal of used CANDU fuel. The methods used to generate the inventories
are described. A comparison of the results vith thon generated using the CANIGEN-II code is also
presented.

Atomic Energy of Canada Limited

Vhiteshell Nuclear Research Establishment
Pinava, Manitoba ROE 1L0
1989
AECL-9881
 CONTENTS

Page

1. INTRODUCTION 1

2. COMPUTER COuo SELECTION 2

2.1 ORIGEN-S CODE 3
2.2 ORIGEN-S CODE COMPARISONS AND VALIDATION 4

3. CALCULATION OF STABLE ELEMENT AND RADIONUCLIDE INVENTORIES 6

3.1 UO 2 FUEL 7
3.2 ZIRCALOT AND IMPURITIES IN UO 2 AND ZIRCALOY 7

3.3 DERIVATION OF INITIAL INVENTORIES 8

4. RADIONUCLIDE INVENTORY TABLES 9

ACKNOWLEDGEMENTS 10

REFERENCES 11

TABLES 14

APPENDIX A U0 2 FUEL - ACTINIDES AND FISSION PRODUCTS A.I

APPENDIX B U0 2 FUEL - IMPURITY ACTIVATION PRODUCTS B.I

continued...
 CONTENTS (concluded)

Page
APPENDIX C ACTIVATION PRODUCTS FOR ZIRCALOY-4 CLADDING AND IMPURITIES IN ZIRCALOY-4 C.I

APPENDIX D PROGRAM INPUT DATA AND OUTPUT VERIFICATION DATA D.I

APPENDIX E CREATION AND BENCHMARKING OF ORIGEN-S CROSS-SECTION DATA LIBRARIES FOR USE IN
BRUCE "A" CANDU FUEL BURNUP CALCULATIONS E.I

APPENDIX F CALCULATION OF THE ACTINIDE, FISSION PRODUCT, AND NEUTRON ACTIVATION PRODUCT
INVENTORIES IN USED BRUCE "A" CANDU FUEL F.I
 LIST OF TABLES
Page
TABLE 1 COMPARISON OF PREDICTED INVENTORIES (g/kg U) 14
TABLE 2 BRUCE "A" FUEL ASSEMBLY AND REACTOR CORE SPECIFICATIONS 23
TABLE 3 ZIRCALOY IMPURITIES (MAXIMUM PERMITTED LEVEL) 25
TABLE 4 UO 2 FUEL IMPURITIES 25
TABLE 5 RADIONUCLIDE INVENTORIES (MASS) OF IRRADIATED CANDU UO2 FUEL - ORIGEN-S CODE 26
TABLE 6 RADIONUCLIDE ACTIVITY OF IRRADIATED CANDU UO2 FUEL - ORIGEN-S CODE 27
1. INTRODUCTION

Atomic Energy of Canada Limited (ABCL) is assessing the concept of used U0 2 fuel disposal deep in the
plutonic rock of the Canadian Precambrian Shield. This concept involves sealing intact used-fuel bundles
in corrosion-resistant metal containers and placing them in boreholes in an underground vault (Dormuth,
1987; Hancox, 1988). The only credible scenario for the release of radionuclides to the environment is
corrosion of the containers and subsequent dissolution of radionuclides in the groundvater, where they
could be transported through the geosphere to the biosphere. The objective of the safety assessment of
the disposal concept is to perform a pathways analysis to estimate the dose consequence to man from
exposure to any released radionuclides that reach the biosphere from the vault. In addition, the safety
of the storage of used fuel and transportation of used fuel to a waste packaging centre and disposal site
is being assessed. These assessments will require information on the quantities of radionuclides present
in a used-fuel bundle. The purpose of this report is to provide a tabulation of initial radionuclide
inventories in the used U0 2 fuel and its Zircaloy sheath, and to outline the conditions and assumptions
used in calculating these inventories.

The sources for radiotoxic elements in the disposal of used fuel are the U0 2 fuel, the Zircaloy bundle
components, and impurities in both the Zircaloy and 00 2 . The used fuel contains both stable and
radioactive isotopes that arise from fission and neutron activation of the U0 2 in the reactor.
Additional stable and radioactive isotopes are generated in the Zircaloy and U0 2 fuel as a result of
neutron activation of zirconium and of inherent manufacturing impurities in the Zircaloy sheath and U0 2 .
The remainder of the components cf the engineered barriers in the disposal system may contain non-
radioactive toxic materials; however, these materials vill not be considered here, but are dealt with in
a separate report (Nehta, in preparation).
 - 2 -

2. COMPUTER CODE SELECTION

The stable and radioactive nuclide inventories at discharge from the reactor in Bruce "A" fuel have
previously been calculated using the isotope generation and depletion code CANIGEN (Smith et al., 1987).
The mass, activity, decay heat and gamma-source inventories were presented as a function of cooling time
for burnups of SOS, 68S, 86S and 1045 GJ/kg initial U 1 for both used-fuel bundles and fuel that had been
reprocessed to remove 99.5* (U + Pu) after various discharge times from the reactor.

The ability of the CANIGEN code to accurately predict isotopic concentrations was partially verified by
comparison with selected U and Pu isotope analyses of used fuel and by comparison of measured decay heats
and radiation fields with values predicted by CANIGEN. The predicted isotopic mass for U and Pu agreed
to within - IX of the analytical values and the predictions of decay heat and radiation fields agreed to
vithin - 13% and - 152, respectively, of the measured values. The CANIGEN code predictions were also
compared with other independent codes such as FISSPROD and ORIGEN. The details of the comparisons and
the methodology and error analysis for the calculations using CANIGEN were presented by Smith et al.
(1987).

The original ORIGEN code (Bell, 1973) was developed to characterize the bulk properties of used nuclear
fuel. It has since been updated to produce two separate codes - 0RIGEN2 (Croff, 1980a, 1980b, 1982,
1983) and ORIGEN-S (Hermann and Vestfall, 1984; Ryaan, 1984). All three ORIGEN codes use the same basic
model, numerical methods, decay data, and photon data. The major difference is that the updated codes
use cross-sections and fission product yield data that are significantly improved compared to those of
ORIGEN. The 0RIGEN2 code uses burnup-dependent libraries (delivered with the code) developed for

1/ Burnup is defined as GJ/kg of initial uranium, but vill be abbreviated hereafter as GJ/kg U
 - 3-

specific reactor types and fuel cycles. The majority of these libraries are based on the uranium-fueled
pressurized-vater reactors (PWRs) and boiling-water reactors (BVRs) using the once-through fuel cycle.
The ORIGEN-S code was developed to provide the user with the capability of producing reactor-specific,
burnup-dependent cross-section libraries. This is accomplished through the facilities of the SCALE code
system (NUREG, 1982), which includes the COUPLE code (Hermann, 1984). These libraries have received
heavy use in applications that require data-library flexibility, including the calculation of the decay
heats used in the USNRC Regulatory Guide 3.54 (USNRC, 1984).

The development and support of the CANIGEN code has been discontinued at AECL in favour of the more
recent isotope generation/depletion code ORIGEN-S, discussed above. The rationale for this decision is
that the ORIGEN-S code is more versatile for the development of new reactor types, is capable of
providing additional calculations not available with CANIGEN (e.g., activation of impurities in Zircaloy
and U0 2 , and neutron energy spectra) and has a more recent and more extensive radionuclide library
database than that available to CANIGEN. The ORIGEN-S code was used at AECL to produce new radionuclide
inventories for the reference burnup case (685 GJ/kg U) for used-fuel disposal and also to provide
inventories for activation products arising from impurities in the Zircaloy and U0 2 . These inventories
vill be used in the safety assessment of the nuclear fuel waste disposal concept.

2.1 ORIGEN-S CODE

In order to produce radionuclide inventory tables, it was necessary to generate a new cross-section
library for Bruce CANDU® 2 fuel to be used by ORIGEN-S. The original nuclear data library supplied with
ORIGEN-S was modified using the SCALIAS-3.1 (RSIC, 1986) cross-section processing system (a subset of the
SCALE system) to transform the library intc one that describes the CANDU heavy-water-moderated PVR.

2/ CANada Deuttrium Uranium. Registered in the U.S. Patent and Trademark Office.
COUPLE was used to update the library using multi-group fluxes and cross-sections determined with an
XSDRNPM-S transport calculation. The inventory calculations were then carried out with this new library
and ORIGEN-S, run stand-alone in fixed-power mode, to a burn-up of 685 GJ/kg U. A comparison was then
made between isotope inventories (one year after exit from the reactor) predicted by the ORIGEN-S,
CANIGEN (Smith et al., 1987) and VIMS codes. VIMS is a detailed physics lattice-cell transport and
burnup code used within AECL for reactor design and development (Askew et al., 1966; Donnelly, 1986) and
uses state-of-the-art ENDF/B-V cross-section data. The details of reactor conditions used, fuel assembly
specifications and details of the comparative cases are described in Appendix E.

During this comparative process, several differences were observed between the predicted ORIGEN-S
inventories and those predicted by the CANIGEN and VIMS codes. The source of these differences involves
the original ORIGEN-S library data for the 236 Pu decay chain (missing production channel from decay of
23
*Np), and 214 Pu decay chain (missing neutron capture data for 2 4 3 Fu). The ORIGEN-S database was revised
to produce new cross-section library data for the Bruce fuel calculations performed here (see Appendices
E and F ) .

2.2 ORIGEN-S CODE COMPARISONS AND VALIDATION

The results from the ORIGEN-S (with corrected library), CANIGEN (Smith et al., 1987) and VIMS
calculations a, presented in Table 1, for an exit burnup of 685 GJ/kg U and a cooling time of one year,
as ratios of ORIGEN/CANIGEN, CANIGEN/VTHS and ORIGEN/VIMS. It should be noted that, in the database used
for the CANIGEN case, the concentration of 2 3 4 U in the unirradiated fuel was assumed to be zero. For
consistency, the initial 2 3 4 U concentration was also assumed to be zero in the ORIGEN-S and VIM"
comparative runs. (Note thrt in the ORIGEN-S results reported in Appendices A to C, the initial
concentration of 234 U was included at its natural abundance of 0.0054Z.) The inventories calculated by
ORIGEN-S (Table 1) are in reasonable agreement with the CANIGEN results, with the exception of some cf
 - 5 -

the actinides in the 232 U, 233 U and 234 U decay chains, where differences of factors of four or more are
observed. In these instances, however, the significance of these differences is minimized by the
extremely lov activity of the isotopes involved (usually less than 10~3 Bq/kg U). Such low
concentrations are bordering on the detection limits of the best analytical techniques and it would be
extremely difficult to verify, with any certainty, which code was predicting the sore accurate value.
Generally, the code predictions agree to within a factor of two for the U and transuranic isotopes.
Concentrations of the fission products generally agree to within a factor of about 1.2, with the
exception of 152 Gd and 129 Xe (a stable isotope and a short-lived daughter isotope of 1 2 9 I , respectively).
ORIGEN-5 tends to predict higher concentrations than CANIGEN, particularly for the actinides, and thus,
for the majority of nuclides, it is more conservative to use ORIGEN-S results in the safety assessment
calculations. Overall agreement between the limited isotope library of the VIMS code and the CANIGEN and
ORIGEN-S codes is very good.

Several studies have been conducted comparing calculated and measured decay heats. Hermann, Parks and
Ryman (1986) report that ORIGEN-S overpredicts by about 5X. Heeb (1986) reports that 0RIGEN2 predictions
are within 3X of measurements for cooling times of less than ten years when detailed pover histories are
used, and that the code overpredicts by as much as 20Z when average power histories are used. A complete
survey of available measurements and comparisons to calculations is found in DOE/RW (1987).

The ORIGEN-S, CANIGEN and VIMS codes predict slightly different radionuclide inventories. The
differences, however, are mostly due to isotope cross-section differences in their respective database
libraries or are due to the different methods employed by each code to calculate the neutron-flux
spectrum at different periods throughout the burnup of the fuel, and the methods used to account for the
self-shielding effects of the strong resonance absorbing radionuclides as their concentrations increase
with burnup. A more comprehensive discussion of the differences between ORIGEN-S and CANIGEN results is
presented in Appendix E.
 - 6 -

It should be emphasized that all codes that have been used to predict isotopic concentrations or bulk
properties of used fuel have not been developed from the viewpoint of long-term waste management, but
rather to describe the neutronics of the reactor and bulk property behaviour for short ti«es after fuel
discharge from the reactor. For example, many isotopes that may be of importance from a waste management
perspective have little or no importance for modelling reactor neutronics, or for predicting short-term
decay heats or radiation fields. As a result, the cross-section data, production/decay-chain data and
half-life data may not have been verified for radionuclides that are unimportant to reactor physics
calculations, used-fuel transportation or interim fuel storage facilities. Verification of this library
data is important for prediction of isotope concentrations or decay heats for long-term waste management
purposes. Codes such as 0RIGEN2 and ORIGEN-S are currently being verified for light-water reactor (LVR)
fuel through a quality-assured fuel characterization program in the United States waste management
program (Roddy and Mailen, 1987). Only limited analytical data are currently available for CANDU fuels
(Smith et al., 1987) and none are available for fuel cladding. Over the next several years, the ORIGEN-S
code needs to be validated by performing rigorous chemical and isotopic analyses, and physical property
measurements on typical CANDU used-fuel bundles and the results compared with the predicted ORIGEN-S
isotopic concentrations and bulk property values. In addition, the cross-section and production/decay-
chain data in the code libraries need to be verified. A program has been initiated to verify the
databases for the code and validate the predicted inventories by radiochemical analysis.

3. CALCULATION OP STABLE ELEMENT AND RADIONUCLIDE INVENTORIES

The radionuclides that need to b« considered for the safety assessment of fuel disposal can be
categorized according to their origins:
 - 7 -

(i) fission of uranium and heavier fissile elements (to give fission products), and neutron
activation of uranium and heavier elements (to give actinides) in the U0 2 fuel; and

(ii) neutron activation of Zircaloy cladding, fuel bundle structural materials, and impurities in
the Zircaloy and U0 2 .

3.1 UP, FUEL

The inventory of stable and radioactive nuclides in used U0 2 fuel will be a function of the burnup and
pover history of the fuel, the cooling time out-of-reactor and thfc fuel type. The reference fuel chosen
to demonstrate the concept of used-fuel disposal is Bruce "A" U0 2 fuel irradiated to a burnup of
685 GJ/kg U and cooled for ten years after discharge from the reactor (Baumgartner, 1989). The
specifications for the fuel elements, fuel assemblies, and reactor operating conditions for the reference
burnup are given in Table 2 (see Appendices E and F for details).

3.2 ZIRCALOY AND IMPURITIES IN UP, AND ZIRCALOY

The concentrations of impurities in U0 2 and Zircaloy vere taken from Crosthvaite (unpublished report) and
are reproduced in Tables 3 and 4. These concentrations are similar to those chosen by Hehta (1982) for
the second interim safety assessment of a used-fuel disposal vault (Wuschke et al., 1985). In both
cases, the upper range of the "allowed limits" for impurities was assumed for the calculation of
inventories. Although U and Th could have been considered as impurities in the Zircaloy and U0 2 ,
respectively, they vere not included in the calculation as their inventory was many orders of magnitude
lover than that present or generated in the used fuel itself.
 - 8 -

3.3 DERIVATION OF INITIAL INVENTORIES

In calculating the inventories (grams or moles), activities (bequerels) and decay heats (vatts) of
radionuclides for both the used U0 2 fuel and activation of impurities in the U0 2 and Zircaloy, a cutoff
value of 1 x 10" 20 units/kg U or Zircaloy (units = g, nol, Ci 3 , or V) has been arbitrarily imposed to
limit the number of radionuclides reported in the calculations. This limit is many orders of magnitude
belov any value that could be reasonably verified by analytical measurements.

In the comparative runs described above, ORIGEN-S did not use burnup-dependent cross-sections, but rather
cross-sections determined for fresh-fuel conditions. The effect of this limitation vill be most
pronounced in the resonance self-shielding in the strong-resonance absorbing nuclides. Burnup-dependent
libraries vere inherently part of the CANIGEN analysis. This deficiency was recognized in the ORIGEN-S
calculation method, and as a result, two burnup-dependent libraries vere created for the inventories
reported here, to allov for a mid-burnup correction to the cross-section data (See Appendix F). The
first irradiation cycle vas performed to half-burnup using a cross-section library generated from fuel
compositions representative of the cycle midpoint, i.e., at 25X burnup. The second irradiation cycle vas
continued using a separate library created from the second cycle mid-point compositions. As a result of
this more rigorous modification to the ORIGEN-S calculation method, inventories for isotopes, such as
" 3 P u , 2 "Pu, "°Pu, 2<2-An, " 3 A m and 2 "Am, that differed by as much as 80* from the CANIGEN results
(Table 1) nov agree to within 30*. In general, most other actinide inventories moved closer to the
CANIGEN inventories; however, some moved slightly further avay from the CANIGEN values, but these changes
vere generally less than 20*. It is likely that additional cycling of the libraries including three or
•ore burnup correction steps vould result in further improvements. (Note that the SAS2 control module in
SCALIAS-3.1 (NUREG, 1982) developed for producing burnup-dependent libraries is not currently available

3/ 1 Ci - 37 GBq
 - 9 -

at AECL. Thus, the tvo-cycle libraries used here were created manually.) Addition of further cycling
steps, and any other changes that are indicated as being necessary based on comparisons of predicted
inventories with analytical results will be implemented during the ORIGEN-S code validation program.

4. RADIONUCLIDE INVENTORY TABLES

The results generated by the ORIGEN-S code (as corrected and enhanced as described above) for used fuel
at a burnup of 685 GJ/kg U are presented in Appendix A (See Appendix F for details). The results are
presented as actinide and fission product inventories: mass in mol/kg U and g/kg U; activities in Bq/kg U
and Ci/kg U; and decay heat in V/kg U.

The results for activation of impurities in UO, are presented similarly in Appendix B and the results for
the activation of the Zircaloy and impurities in the Zircaloy are presented in Appendix C. (No decay heat
results are presented for the U0 2 or Zircaloy impurities.)

The input parameters to the ORIGEN-S code and the program ouput verification data are presented in
Appendix D.

It should be noted again that a particular radionuclide vill not necessarily appear in every appendix
table, since each table has a cutoff value of 1 x 10~ 20 . The inclusion of a radionuclide in the tables
vill thus be dependent on the units.

A summary of the fission product and selected actinide masses and activities for Bruce fuel vith a burnup
of 685 GJ/kg U and cooled for ten years is presented in Tables 5 and 6.
ACKNOWLEDGEMENTS

The authors vish to thank D. Chen, L.H. Johnson and K. Mehta for helpful suggestions and review of this
report.
 - 11 -

REFERENCES

Askew, J.R., F.J. Payers, and P.B. Kemshell. 1966. A General Description of the Lattice Code VIMS.
JBNES 4, 564.
Bauogartner, P. 1989. Technical Specifications for a Used Fuel Disposal Centre. Atomic Energy of
Canada Limited Technical Record*, TR-A10.
Bell, M.J. 1973. ORIGEN - The ORNL Isotope Generation and Depletion Code. Oak Ridge National
Laboratory Report, ORNL-4628.
Croff, A.G. 1980a. A Revised and Updated Version of the Oak Ridge Isotope Generation and Depletion
Code. Oak Ridge National Laboratory Report, 0RNL-5621.
Croff, A.G. 1980b. A User's Manual for the 0RIGEN2 Computer Code. Oak Ridge National Laboratory
Report, ORNL/TM-7175, 1980.
Croff, A.G. 1982. 0RIGEN2 - Isotope Generation and Depletion Code - Matrix Exponential Method. Oak
Ridga National Laboratory Report, ORNL-CCC-371.
Croff, A.G. 1983. ORIGEN2: A Versatile Computer Code for Calculating the Nuclide Compositions and
Characteristics of Nuclear Materials. Nucl. Tech. 62, 335.
DOE/Rtf REPORT. 1987. Characteristics of Spent Fuel, High-Level Waste, and Other Radioactive Vastes
which May Require Long-Term Isolation. U.S. Department of Energy Report, Office of Civilian
Radioactive Vaste Management, DOE/RV-0184, Vol. 2, Appendix 1A.
Donnelly, J.V. 1986. WIMS-CRNLJ A Users Manual for the Chalk River Version of VIMS. Atomic Energy of
Canada Limited Report, AECL-8955.
Dormuth, R.tf. (ed.) 1987. Canadian Nuclear Fuel Vaste Management Program. Rad. Vaste Manage. Nucl.
Fuel Cycle, 8 (2-3).
Bancox, V.T . .losing the Circle: Returning Used Uranium Fuel to the Geologic Environment.
Presented at the Canadian Nuclear Society Symposium on Uranium and Electricity. Saskatoon, Sask.,
1988 Sept. 18-21.
 - 12 -

Heeb, C M . 1986. Comparison of Spent Fuel Decay Heat Rate 0RIGEN2 Predictions and Calorimeter
Measurements. Presented at the Third International Spent Fuel Storage Technology
Symposium/Workshop, 1986 April 8-10, Seattle, VA.
Hermann, O.V. 1984. COUPLE: SCALE System Module to Process Problem-Dependent Cross Sections and Neutron
Spectral Data for ORIGEN-S Analysis. Oak Ridge National Laboratory Report, NUREG/CR-0200, Rev. 2,
Vol. 2, Section F6.
Hermann, O.M., R.M. Westfall. 1984. ORIGEN-S: SCALE System Module to Calculate Fuel Depletion, Actinide
Transmutation, Fission Product Buildup and Decay, and Associated Radiation Source Terms. Oak
Ridge National Laboratory Report, NUREG/CR-0200, Rev. 2, Vol. 2, Section F7.
Hermann, O.V., C.V. Parks, J.C. Flyman. 1986. Spent Fuel Decay Heat Calculations Using ORIGEN-S.
Presented at the Third International Spent Fuel Storage Technology Symposium/Workshop, April 8-10,
1986, Seattle, VA.
Mehta, K. 1982. Nuclide Inventory for Nuclear Fuel Waste Management: Post-Closure Phase. Atomic Energy
of Canada Limited Report, AECL-6830.
Mehta, K. In preparation. Identification and Treatment of Nuclides and Nuclide-Chains for Post-Closure
SYVAC Assessment. Atomic Energy of Canada Limited Report.
NUREG. 1982. SCALE: A Modular Code System for Performing Standardized Computer Analyses for Licensing
Evaluation. NUREG/CR-0200, Oak Ridge National Laboratory Report. Volumes I, II, and III. Revised
1983 and 1984.
Roddy, J.W. and J.C. Mailen. 1987. Radiological Characteristics of Light-Water Reactor Spent Fuel: A
Literature Survey of Experimental Data. Oak Ridge National Laboratory Report, ORNL/TM-10105.
RSIC. 1986. SCALIAS 3.1: Selected FORTRAN 77 Modules From SCALE 3.1. RSIC Code Package CCC-47S.
Ryman, J.C. 1984. ORIGEN-S Data Libraries. NUREG/CR-0200, Rev. 2, Vol. 3, Section M6.
Smith, B.J., J.C. Tait and R. von Massov. 1987. Radioactive Decay Properties of BRUCE "A" CANDU™ U0 2
Fuel and Fuel Recycle Waste. Atomic Energy of Canada Limited Report, AECL-9072.
 - 13 -

Wuschke, D.M., P.A. Gillespie, K.K. Mehta, V.F. Heinrich, D.M. LeNeveu, V.M. Guvanasen, G.R. Sherman,
D.C. Donahue, B.V. Goodwin, T.H. Andres and R.B. Lyon. 1985. Second Interim Assessment of the
Canadian Concept for Nuclear Fuel Vaste Disposal. Volume 4: Post-Closure Assessment. Atomic
Energy of Canada Limited Report, AECL-8373-A.
USNRC. 1984. Spent Fuel Heat Generation in an Independent Spent Fuel Storage Installation. Regulatory
Guide 3.54. U.S. Nuclear Regulatory Commission, Vashington, DC.
* Unrestricted, unpublished report available from SDDO, Atomic Energy of Canada Limited Research Company,
Chalk River, Ontario KOJ 1J0.
 - 14 -
TABLE 1
COMPARISON OF PREDICTED INVENTORIES (g/kg U)
BRUCE "A" FUEL, BURNUP 685 GJ/kg U, ONE YEAR COOLED

Ratio
Muclide CANIGEN* ORIGEN-S VIMS ORIGEN-S/ ORIGEN-S/ CANIGEN/
CANIGEN VIMS VIMS

Cf 251 2.39e-15 1.92e-15 0.80

Cf 250 1.57e-14 7.70e-15 0.49
Cf 249 4.92e-14 2.60e-14 0.53
Bk 249 3.84C-14 2.04e-14 0.53
Cm 248 2.86e-ll 1.43e-U 0.50
Cm 247 1.31e-09 6.04e-10 0.46
Ca 246 2.22e-07 1.90e-07 0.86
Ca 245 2.29e-06 1.99e-06 0.87
Ca 244 2.34e-04 2.37e-O4 1.01
Ca 243 4.81e-06 4.43e-06 0.92
Ca 242 1.12e-04 1.12e-04 1.00
Aa 243 2.87e-03 3.19e-O3 3.67e-03 1.11 0.87 0.78
Aa 242a 1.73e-05 3.19e-05 1.42e-05 1.84 2.25 1.22
Aa 242 2.08e-10 3.82e-10 1.84
Aa 241 l.lle-02 1.64e-02 1.27e-02 1.48 1.29 0.87
Pu 244 1.35e-06 l.Ole-06 0.75
Pu 243 4.75e-20 2.15e-20 0.45
Pu 242 6.65e-02 8.18e-02 7.44e-02 1.23 1.10 0.89
Pu 241 1.99e-01 2.93c-01 2.25e-01 1.47 1.30 0.88
Pu 240 l.Ue+00 9.02e-01 1.06e+00 0.79 0.85 1.08
Pu 239 2.7Oe+OO 2.56*1-00 2.6U+OO 0.95 0.98 1.03
Pu 238 4.53e-03 4.68e-03 4.24e-03 1.03 1.10 1.07
Pu 236 1.45e-07 2.3U-08 1.39«-08 0.16 1.66 10.41
continued...
 - 15 -

TABLE 1 (continued)

Ratio
Nuclide CANIGEN* ORIGEN-S VIMS ORIGEN-S/ ORIGEN-S/ CANIGEN/
CANIGEN VIMS VIMS
Np 240m 2.28e-19 1.69e-19 0.74
Np 239 2.47e-09 2.74e-09 1.11
Np 237 3.09e-02 3.45e-02 2.84e-02 1.12 1.21 1.09
U 240 2.57e-17 1.93e-17 0.75
U 238 9.85e+02 9.85e+02 9.85e+02 1.00 1.00 1.00
U 237 5.68e-09 9.08e-09 1.60
U 236 7.64e-01 7.65e-01 7.58e-01 1.00 1.01 1.01
0 235 2.07e+0O 2.00e+00 2.12e+OO 0.97 0.94 0.98
U 234 3.99e-05 7.54e-05 3.62e-05 1.89 2.08 1.10
U 233 1.62e-08 3.2Oe-O8 1.98
U 232 4.63e-08 7.93e-09 0.17
Pa 234a 4.82e-13 4.82e-13 1.00
Pa 233 1.05e-09 1.17e-09 1.11
Pa 231 3.96e-09 3.81e-09 0.96
Th 234 1.43e-08 1.43e-08 1.00
Th 232 3.04e-08 3.06e-08 1.01
Th 231 8.43e-12 8.15e-12 0.97
Th 230 6.53«-ll 1.97e-10 3.02
Th 229 4.88e-14 2.89e-13 5.92
Th 228 2.36e-10 4.27e-ll 0.18
Th 227 1.63e-16 1.72e-16 1.06
Ac 228 1.09e-22 1.19e-22 1.09
Ac 227 7.49e-14 7.40e-14 0.99
Ac 225 1.55e-19 1.06e-18 6.84
Ra 228 8.94e-19 9.79e-19 1.10
Ra 226 2.28c-16 1.03e-15 4.52
Ra 225 2.44e-19 1.57e-18 6.43
continued...
 - 16 -
TABLE 1 (continued)

Ratio
Huclide CANIGEN* ORIGEN-S VIMS ORIGEN-S/ ORIGEN-S/ CANIGSN/
CANIGEN VIMS VIMS
Ra 224 1.18e-12 2.2Oe-13 0.19
Ra 223 9.28e-17 1.05e-16 1.13
Rn 222 1.41e-21 6.63e-21 4.70
Rn 220 2.05e-16 3.79e-17 0.18
Rn 219 3.65e-22 4.12e-22 1.13
Pr 221 5.08e-23 3.47e-22 6.83
Po 218 7.67e-25 3.60e-24 4.69
Po 216 5.43e-19 1.00e-19 0.18
Po 215 1.61e-25 1.82e-25 1.13
Po 214 6.74e-31 3.18e-30 4.72
Po 212 6.80e-25 1.26e-25 0.19
Po 213 6.64e-31 4.77e-30 7.18
Po 210 1.26e-22 1.17e-21 9.29
At 217 5.54e-27 3.82e-26 6.90
Bi 214 4.89e-24 2.31e-23 4.72
Bi 213 4.69e-22 3.18e-21 6.78
Bi 212 1.29e-14 2.39e-15 0.19
Bi 211 1.14e-20 1.28e-20 1.12
Bi 210 1.48e-23 l.O8e-22 7.30
Bi 209 1.43e-18 7.97e-17 55.73
Pb 214 6.62e-24 3.1U-23 4.70
Pb 212 1.36e-13 2.52e-14 0.19
Pb 211 1.93e-19 2.17e-19 1.12
Pb 210 2.57e-20 1.75e-19 6.81
continued...
 - 17 -

TABLE 1 (continued)

Ratio
Nuclide CANIGEN* ORIGEN-S VIMS ORIGEN-S/ ORIGEN-S/ CANIGEN/
CANIGEN VIMS VIMS
Pb 209 1.98e-21 1.33e-20 6.72
Pb 208 3.19e-ll 6.32e-12 0.20
Pb 207 9.61e-16 1.19e-15 1.24
Pb 206 4.50e-23 6.24e-22 13.87
Tl 209 4.84e-25 3.25e-24 6.71
Tl 208 2.29e-16 4.27e-17 0.19
Tl 207 2.50e-20 2.8Oe-2O 1.12
H 3 1.74e-05 1.37e-05 0.79
As 75 2.75e-05 3.00e-05 1.09
Ge 76 7.57e-05 3.30e-05 1.10
Se 77 1.78e-04 1.96e-04 1.10
Se 78 4.73e-04 5.07e-04 1.07
Se 79 1.17e-03 1.30e-03 1.11
Se 80 2.98e-03 3.21e-03 1.08
Se 82 7.24e-03 7.86e-03 1.09
Br 79 1.62e-08 2.19e-08 1.35
Br 81 4.90e-03 5.33e-03 1.09
Rr 83 9.12«-03 9.92t-03 9.8Oe-O3 1.09 1.01 0.93
Rr 84 2.2Oe-O2 2.43c-02 1.10
Rr 85 5.05C-03 5.60e-03 1.11
Rr 86 3.76e-02 4.19t-02 1.11
Rb 85 2.06«-02 2.29«-O2 1.11
Rb 87 4.91e-02 5.48C-02 1.12
continued...
 - 18 -

TABLE 1 (continued)

Ratio
Nuclide CANIGEN* 0RIGEN-S VIMS ORIGEN-S/ RIGEN-S/ CANIGEN/
CANIGEN VIMS VIMS
Sr 88 7. lle-02 7.92e-02 1.11
Sr 89 2. 17e-04 1.88e-O4 0.87
Sr 90 1.13e-01 1.26e-01 1.12
Y 89 9.39e-02 1.05e-01 1.12
Y 90 2.84e-05 3.16e-05 1.11
Y 91 5.56e-04 5.71e-04 1.03
Zr 90 3.63e-03 4.Ue-03 1.14
Zr 91 1.23e-01 1.37e-01 1.11
Zr 92 1.34e-01 1.47e-01 1.10
Zr 93 1.54e-01 1.68e-01 1.09
Zr 94 1 64e-01 1.79e-01 1.09
Zr 95 1.27e-03 1.29e-03 1.02
Zr 96 1 76e-01 1.89e-01 1.07
Nb 93 7 54e-09 1.18e-O8 1.56
Nb 93a 8 52e-08 9.57e-08 1.12
Nb 95 1.50e-03 1.60e-03 1.07
No 95 1.70e-01 1.84e-01 1.83e-01 1.08 1.01 0.93
No 96 1.13e-03 1.31e-03 1.16
No 97 1.81e-01 1.93e-01 1.07
No 98 1.85e-01 1.96e-01 1.95e-01 1.06 1.01 0.95
No 100 2•15e-01 2.26e-01 1.05
Tc 99 1.92e-01 2.05e-01 2.03e-01 1.07 1.01 0.94
Ru 100 6.08e-03 6.89c-03 1.13
Ru 101 1.81c-01 1.89e-01 1.89e-01 1.04 1.00 0.96
Ru 102 1.74e-01 1.80«-01 1.03
continued...
 - 19 -
TABLE 1 (continued)

Ratio
Nuclide CANIGEN* ORIGEN-S VIMS ORIGEN-S/ ORIGEN-S/ CANIGEN/
CANIGEN VIMS VIMS
Ru 103 8.09e-05 7.53e-05 7.33e-05 0.93 1.03 1.10
Ru 104 1.35e-01 1.33e-01 0.99
Ru 106 3.51e-02 3.30e-02 0.94
Rh 103 1.54e-01 1.55e-01 1.53e-01 1.01 1.02 1.01
Rh 106 3.3Oe-08 3.10e-08 0.94
Pd 105 8.39e-02 9.08e-02 9.01e-02 1.08 1.01 0.93
Fd 106 7.62e-02 6.42e-02 0.84
Pd 107 5.96e-02 5.48e-02 0.92
Pd 108 4.02e-02 3.72e-02 3.78e-02 0.93 0.98 1.06
Pd 110 1.16e-02 1.06e-02 0.91
Ag 107 7.95e-09 7.27e-09 0.91
Ag 109 2.27e-02 2.16e-02 2.87e-02 0.95 0.75 0.79
Ag 1 1 0 B 3.26e-05 3.04e-05 0.93
Cd 110 3.33e-03 2.54e-03 0.76
Cd 111 5.33e-03 4.87e-03 0.91
Cd 112 2.37e-03 2.19e-03 0.92
Cd 113B 2.77e-05 3.12e-05 1.13
Cd 113 3.23e-05 3.39e-05 2.77e-O5 1.05 1.23 1.17
Cd 114 2.81e-03 2.66e-03 0.95
Cd 116 8.75e-04 8.68e-04 0.99
In 115 6.55e-04 6.6Oe-OA 6.78e-04 1.01 0.97 0.97
Sn 117 8.77e-04 8.75e-04 1.00
Sn 118 9.02e-04 9.07e-04 1.01
Sn 119a 4.40e-06 3.69e-06 0.84
Sn 119 9.05e-04 9.04e-04 1.00
Sn 120 9.26e-04 9.32e-04 1.01
continued..
 - 20 -

TABLE 1 (continued)

Ratio
Hudide CANIGEN* ORIGEN-S VIMS ORIGEN-S/ RIGEN-S/ CANIGEN/
CANIGEN VIMS VIMS
Sn 1 2 1 B 9.35e-07 7.26e-07 0.78
Sn 122 1.04e-03 1.04e-03 1.00
Sn 123 5.16e-05 2.50e-05 0.48
Sn 124 1.55e-03 1.57e-03 1.01
Sn 126 4.87e-03 4.98e-03 1.02
Sb 121 9.67e-04 9.83e-04 1.02
Sb 123 1.13e-03 1.19e-03 1.05
Sb 124 6.38e-08 8.92e-08 1.40
Sb 125 2.17e-03 2.23e-03 1.03
Sb 126 2.31e-10 2.37e-10 1.03
Te 1 2 5 B 3.06e-05 3.10e-05 1.01
Te 125 7.89e-04 7.87e-04 1.00
Te 126 1.56e-04 1.41e-04 0.90
Te 127a 1.06e-04 1.00e-04 0.94
Te 128 2.43e-02 2.50e-02 1.03
Te 1 2 9 B 1.35e-06 8.52e-O7 0.63
Te 130 8.23e-02 8.50e-02 1.03
I 127 1.18e-02 1.23c-02 1.18e-02 1.04 1.04 1.00
I 129 4.35e-02 4.49e-02 1.03
I 131 1.72e-16 1.70e-16 1.92e-16 0.99 0.89 0.90
Xc 129 2.35e-09 3.12t-O7 132.77
Xc*131 1.24e-01 1.31e-01 1.06
Xt 132 2.20e-01 2.3Ot-Ol 1.05
Xt 134 3.28t-01 3.51t-01 1.07
Xc 136 5.75e-01 6.02t-01 1.05
Cs 133 2.81e-01 3.02«-01 2.9SC-01 1.07 1.02 0.95
C« 134 9.23c-03 8.06t-03 7.88t-03 0.87 1.02 1.17
continutd...
 - 21 -
TABLE 1 (continued)

Ratio
Nuclide CANIGEN* ORIGEN-S VIMS ORIGEN-S/ ORIGEN-S/ CANIGEN/
CANIGEN VIMS VIMS
Cs 135 2.01e-02 2.37e-02 2.25e-02 1.18 1.05 0.89
Cs 137 2.80e-01 2.94e-01 1.05
Ba 134 4.57e-O3 4.00e-03 0.88
Ba 135 1.08e-06 1.56e-06 1.44
Ba 137a 4.26e-08 4.48e-08 1.05
Ba 137 8.50e-03 9.05e-03 1.06
Ba 138 2.81e-01 3.00e-01 1.07
La 139 2.73e-01 2.90e-01 2.86e-01 1.06 1.01 0.95
Ce 140 2.73e-01 3.05e-01 1.12
Ce 141 2.26e-05 2.26e-05 1.00
Ce 142 2.53e-01 2.71e-01 1.07
Ce 144 6.94e-02 7.3le-02 7.23e-02 1.05 1.01 0.96
Pr 141 2.52e-01 2.69e-01 1.07
Pr 143 1.67e-10 1.75e-10 1.05
Pr 144 2.93e-06 3.09e-06 1.05
Pr 144a 1.46e-08 1.54e-08 1.05
Nd 142 1.80e-03 2.18e-03 1.21
Nd 143 1.89e-01 2.05e-01 1.89e-01 1.08 1.08 1.00
Nd 144 2.05e-01 2.22e-01 2.28e-01 1.08 0.97 0.90
Nd 145 1.58e-01 1.70e-01 1.67e-01 1.08 1.02 0.95
Nd 146 1.43e-01 1.51.-01 1.49e-01 1.06 1.01 0.96
Nd 147 7.6Oe-13 8.65e-13 7.12e-13 1.14 1.21 1.07
Nd 148 8.37e-02 8.7U-02 9.15e-02 1.04 0.95 0.91
Nd 150 4.17e-02 4.24«-02 4.24e-02 1.02 1.00 0.98
continued..
 - 22 -
TABLE 1 (concluded)

Ratio
Ruclide CANIGEN* ORIGEN-S W1MS ORIGEN-S/ ORIGBN-S/ CANIGEN/
CANIGEN VIMS VIMS
Pa 147 6.06e-02 6.38e-02 6.04e-02 1.05 1.06 1.00
Pa 148 7.62e-09 4.64e-09 6.45e-09 0.61 0.72 1.18
Pa 148a 8.50e-07 6.34e-07 7.02e-07 0.75 0.90 1.21
Sa 147 2.37e-02 2.54e-02 2.41e-02 1.07 1.06 0.98
Sa 148 1.06e-02 9.95*-03 9.61e-03 0.94 1.04 1.10
Sa 149 1.69e-03 1.76e-03 1.60e-03 1.04 1.10 1.06
Sa 150 6.23e-02 6.82e-02 6.39e-02 1.09 1.07 0.98
Sa 151 2.67e-03 2.51e-03 2.74e-03 0.94 0.92 0.97
Sa 152 4.16e-02 4.43e-02 4.40e-02 1.06 1.01 0.95
SB 154 1.03G-02 8.76e-03 0.85
Eu 151 2.1Oe-05 2.02e-05 2.20e-05 0.96 0.92 0.95
Eu 152 1.03e-06 1.82e-06 1.77
Eu 153 1.92e-02 2,O2e-O2 2.10e-02 1.05 0.96 0.91
Eu 154 3.7Oe-03 3.73e-03 3.06e-03 1.01 1.22 1.21
Eu 155 1.7Oe-03 1.58e-03 1.19e-03 0.93 1.32 1.42
Eu 156 7.99e-ll 8.69e-ll 6.44e-ll 1.09 1.35 1.24
Gd 152 2.15e-08 2.09e-06 97.21
Gd 154 3.92e-04 3.78e-04 0.96
Gd 155 2.66e-04 2.39e-04 3.64e-04 0.90 0.66 0.73
Gd 156 8.14«-03 9.02e-03 6.60e-03 1.11 1.37 1.23
Gd 157 5.5O«-05 2.16t-05 1.27e-05 0.39 1.71 4.34
Gd 158 5.84C-03 3.12t-03 0.53
Gd 160 2.78C-04 2.43e-04 0.87
Tb 159 5.87t-04 5.36e-04 0.91

(Saith «t al., 1987)

 - 23 -
TABLE 2
BRUCE "A" FUEL ASSEMBLY AND REACTOR CORE SPECIFICATIONS

Fuel Element
Fuel (natural UO 2 ) 234
composition 0.0054 vt.Z 235
U
0.7110 vt.Z 23
U
99.2836 vt.Z «U
radius 0.6077 cm 2
area (cross section) 1.1602 cm
density 10.3590 g/cm3
temperature (average) 1155 K
Cladding (Zircaloy-4)
outside radius 0.6538 cm
thickness 0.0419 cm
air-gap radius (outside) 0.6119 cm
air-gap thickness 0.0042 cm
temperature 546 R
Fuel Assembly
Number of elements 37 (one central)
radii (to element centre)
inner ring (31-36) 1.4885 cm
intermediate ring (19-30) 2.8755 cm
outer ring (1-18) 4.3305 cm

continued...
 - 24 -

TABLE 2 (concluded)

Reactor Core
Coolant and aoderator (D20)
aoderator teaperature 359 R
coolant teaperature 549 R
Pressure tube (Zircaloy-4)
inside radius 5.169 ca
thickness 0.406 ca
teaperature 549 R
Insulating gap (C02)
inside radius 5.575 ca
thickness 0.873 ca
teaperature 359 R
Calandria (Zircaloy-4)
inside radius 6.448 ca
thickness 0.140 ca
temperature 359 R
 - 25 -

TABLE 3 TABLE 4
ZIRCALOY* IMPURITIES (MAXIMUM PERMITTED LEVEL) UP, FUEL IMPURITIES

Element Mg/g Z r " Element pg/g Zr** Element ug/g u Element vg/g u
Sn 17 000.0 Fe 2 400.0
Al 75.0 Mn 50.0 Al 50.0 Fe 100.0
B 0.5 Mo 50.0 B 0.3 Hg 50.0
Cd 0.5 Ni 70.0 Cd 0.2 Mn 10.0
C 270.0 Nb 100.0 Ca 50.0 Mo 4.0
Co 20.0 N
2 80.0 C 100.0 Ni 30.0
Cu 50.0 Si 120.0 Cr 25.0 Si 60.0
Hf 100.0 Ta 200.0 Cu 20.0 Ag 1.0
H
J 25.0 Ti 50.0 Dy 0.15 Th 200.0
Pb 130.0 V 100.0 Gd 0.1
Mg 20.0 U 3.5
1 500.0 V 50.0 0* 134 454.0 50.0
°2
(Zr) 977 735.0 Cr 1 300.0
* Total Zircaloy-4 per bundle - 2.286 kg Atomic oxygen in UO, fuel
** Read as Zircaloy-4
 - 26 -
TABLE 5
RADIONUCLIDE INVENTORIES (MASS) OP IRRADIATED CANDU UP, FUEL
ORIGEN-S CODE
Bruce "A" fuel, 685 GJ/kg initial U burnup, 10 years cooled

Unirradiated Irradiated - Cooled 10 years

g/kg U g/kg U X initial U g/bundle*
Actinides
238JJ 992.836 984.92 98.50 18 641.5
23«u 0.77 0.08 14.6
235JJ 7.110 2.02 0.20 38.2
234 0 0.054 0.04 0.004 0.8
Pu (total) 4.00 0.40 75.7
Other actinides 0.13 0.01 2.5
Total actinides 1000.0 991.88 99.19 18 773.3

Fission products
Active 1.58 0.16 29.9
Inactive 6.54 0.65 123.8
Total fission
products 8.12 0.81 153.7
* 18 927 g U/bundle (Crosthwaite, unpublished report)
 - 27 -

TABLE 6

RADIONUCLIDE ACTIVITY OF IRRADIATED CANDU UP, FUEL

ORIGEN-S CODE

Bruce "A" fuel, 685 GJ/kg initial U burnup, 10 years cooled

Bq/kg u Bq/bundle Ci*/kg U Ci/bundle

238JJ 1.22 10 7 2. 32 10« 3 .31 io- 54 6.26 io-3

X X X X

X X X X
X XX

X X X X
236 0 1.84 10« 3.48 107 4 .97 io- 9.41 IO-«5
23S 0 1.61 105 3.05 10« 4 .36 io-< 8.25 io-3
234 0 9.95 10« 1 88 10« 2 .69 IO-« 5.09 10-

X
Other U 1.34 X 107 2 54 X 10s 3.62 X IO-« 6.85 X io-3
Pu (total) 5.55 X 10" 1.05 X 10" 1.50 X 101 2.84 X 102
«iAm 1.11 X 10 10 2.09 X 10" 2.99 X IO- 1 5.66 X 10°
Other actinides 5.40 X 10« 1.02 X 10 10 1.46 X io- 2 2.76 X io-1
Total actinides 5.66 X 10" 1.07 X 10" 1.53 X 10* 2.90 X 102
Total fission
products 2.85 X 10" 5.39 X 10" 7.70 X 101 1.46 X 103

' 1 Ci - 37 GBq
 - A.I
-/u
APPENDIX A

UP, FUEL - ACITNTOES AND FISSION PRODUCTS

Fuel Bruce "A" Reactor

Burnup 685 GJ/kg initial U
Neutron Flux 1.26 z 1014 n-cm-^s- 1
Power 0.034664 MW/kg initial U
Irradiation Time 228.72 d

Burnup-Dependent Library
ORIGEN-S Code
 - A.3 -

CONTENTS

UO 2 Fuel - Actinides Mass : (m>l/kg initial U) A.4

UO 2 Fuel - Fission Products Mass : (uol/kg initial U) A.7
UO 2 Fuel - Actinides Mass : (g/kg initial U) A. 13
UO 2 Fuel - Fission Products Mass : (g/kg initial U) A. 16
U0 2 Fuel Actinides Activity : (Bq/kg initial U) A. 22
UO 2 Fuel Fission Products Activity : (Bq/kg initial U) A. 25
UO 2 Fuel Actinides Decay Heat : (W/kg initial U) A. 28
UO 2 Fuel Fission Products Decay Heat : (W/kg initial U) A. 31
UO 2 Fuel Actinides Activity : (Ci/kg initial U) A. 34
UO 2 Fuel Fission Products Activity : (Ci/kg initial U) A. 37
U02 Fuel - Actinides Mass; sol/kg i n i t a l U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10* Year 10 6 Year

Cf 252 4.:25e-18 3.27e-18 1.14e-18 3.07e-19 2. 22e-20 1.66e-29 0.OOe+00 0.OOe+00 0.OOe+00
Cf 251 9..49e-18 9.48e-18 9.45e-18 9.41e-18 9.34e-18 8.78e-18 4. 38e-18 4. 21e-21 0.OOe+00
Cf 250 3.i85e-17 3.71e-17 3.00e-17 2. 3Oe-17 1.35e-17 1.95e-19 1.04e-25 4. 2Oe-26 0.OOe+00
Cf 249 6.81e-18 1.27e-16 2. 2Oe-16 2. 22e-16 2. 18e-16 1.86e-16 3.14e-17 5.87e-25 0.OOe+00
Bk 249 2. 19e-16 9.95e-17 4. 20e-18 8.04e-20 2. 94e-23 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00

Cm 248 6.49e-14 6.49e-14 6.49e-14 6.49e-14 6.49e-14 6.49e-14 6.48e-14 6.36e-14 8.40e-15
Cm 247 2. 64e-12 2. 64e-12 2. 64e-12 2. 64e-12 2. 64e-12 2. 64e-12 2. 64e-12 2. 64e-12 2. 52e-12
Cm 246 63e-10 7. 63e-10 7. 63e-10 7. 62e-10 7. 61e-10 7. 52e-10 6.59e-10 1.76e-10 0.OOe+00
Cm 245 7.88e-09 7. 88e-09 7. 87e-09 7. 87e-09 7. 87e-09 7. 81e-O9 7. 26e-09 3.49e-09 0.OOe+00
Cm 244 8.85e-07 8.64e-07 7. 41e-07 6.12e-07 4. 17e-O7 1.95e-08 2. 13e-23 0.OOe+00 0.OOe+00
Cm 243 1.44e-08 1.40e-08 1.27e-08 1.13e-08 8.83e-09 1.26e-09 3.92e-19 0.OOe+00 0.OOe+00
Cm 242 1.61e-06 3.48e-07 9.30e-10 2. 24e-10 2. 14e-10 1.49e-10 2. 45e-12 3.67e-30 0.OOe+00
Am 243 1.08e-05 1.08e-05 1.08e-05 1.08e-05 1.08e-05 1.07e-05 9.85e-06 4.,23e-06 1.19e-15
Am 242 3.74e-08 1.15e-12 1.,13e-12 1.lle-12 1.06e-12 7.,35e-13 1.21e-14 1..81e-32 0.OOe+00
Am 242m 9.69e-08 9.64e-08 9.47e-08 9.25e-O8 8.84e-08 6., 14e-08 1.Ole-09 1.,51e-27 0.,OOe+00
Am 241 7.,03e-06 5.,08e-05 2.,06e-04 3.62e-04 5.,77e-04 8.,36e-04 2. 00e-04 2.,85e-lO 0.,OOe+00

Pu 244 3.,51e-09 3.,51e-09 3.,51e-09 3.,51e-09 3.,51e-09 3..51e-09 3.51e-O9 3,,51e-09 3..48e-09
Pu 242 2..50e-04 2.,50e-04 2,.50e-04 2..50e-04 2,.50e-04 2..50e-04 2. 50e-04 2 ,46e-04 3..96e-05
Pu 241 9.,52e-04 9,.08e-04 7 .52e-04 5,.94e-04 3,.71e-04 8 .52e-06 1,.26e-ll 6 .O4e-12 0 .OOe+00
Pu 240 4..29e-03 4..29e-03 4 .29e-O3 4..29e-O3 4 .29e-03 4 .25e-03 3.,86e-03 1.49e-03 2..75e-13
Pu 239 1.lle-02 1.16e-02 1.16e-O2 1,.I5e-O2 1.15e-02 1.15e-02 1,.12e-O2 8 .67e-03 7.46e-15
Pu 238 1.94e-05 2 .13e-O5 2 .10e-05 2.O2e-O5 1.86e-05 9.92e-06 8 ,59e-09 1.72e-27 0.OOe+00
Pu 236 1.68e-10 1.34e-10 5.05e-ll 1•50e-ll 1.32e-12 4.69e-21 0 .OOe+00 0.OOe+00 0.OOe+00
Np 239 4 .83e-04 9.45e-12 9 •45e-12 9.44e-12 9.43e-12 9.36e-12 8 .60e-12 3.69e-12 1.04e-21
Np 238 8 .O3e-O7 1.76e-14 1.73e-14 1.69e-14 1.62e-14 1.12e-14 1•85e-16 0 .OOe+00 0.OOe+00
Np 237 1•50e-04 1.61e-04 1•61e-04 1.64e-04 1.71e-O4 2.74e-04 9.20e-04 1.12e-03 8.10e-04
U 240 6 .83e-20 6 .83e-20 6 .83e-20 6.83e-2O 6 .83e-2O 6 .83e-2O 6 .83e-20 6 .83e-20 6.78e-20
U 238 4 .14e+00 4. 14e+00 4 . 14e+00 4.14e+00 4.14e+00 4. 14e+00 4 .14e+00 4. 14e+00 4. 14e+00
U 237 1.06e-05 2.86e-ll 2.37e-ll 1.87e-ll 1.17e-U 2.68e-13 3.95e-19 1.90e-19 0.OOe+00
U 236 3 .25e-03 3.25e-03 3.25e-03 3.25e-O3 3.26e-O3 3.3Oe-O3 3.68e-03 6 .06e-03 7.33e-03
U 235 8 .57e-O3 8.57e-O3 8 .57e-03 8.58e-03 8.58e-03 8.61e-03 8 .9Oe-O3 1.15e-02 2.Ole-02
U 234 1,83e-04 1.83e-04 1.83e-04 1.84e-04 1.86e-04 1.94e-04 2.04e-04 2.05e-04 2.25e-04
U 233 3 .98e-10 4 .54e-10 6.63e-10 9.26e-10 1•47e-O9 7.19e-09 2.O3e-O7 3.39e-06 6.37e-O5
U 232 2.Ue-11 5.79e-ll 1.37e-10 1.65e-10 1.63e-10 7.59e-ll 1.31e-14 0t. OOe+00 0.OOe+00
a~« A /
U0 2 Fuel - Actinides Mass: aol/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 10* Year

Pa 234 1.80e-15 1.13e-15 1.13e-15 1.13e-15 1.13e-15 1.13e-15 1.13e-15 1.13e-15 1.13e-15
Pa 234m 2.06e-15 2.06e-15 2.06e-l5 2.06e-15 2.06e-15 2.06e-15 2.06e-15 2.06e-15 2.06e-15
Pa 233 4.14e-12 5.55e-12 5.57e-12 5.65e-12 5.92e-12 9.48e-12 3.18e-ll 3.86e-ll 2.80e-ll
Pa 231 4.79e-ll 5.70e-ll 9.08e-ll 1.33e-10 2.18e-10 8.94e-10 8.56e-09 9.00e-08 9.36e-07

Th 234
Th 232 3.58e-ll 1.32e-10 5.17e-10 9.99e-10 1.96e-09 9.72e-09 l.O3e-O7 1.45e-06 2.19e-04
Th 231 6.34e-13 3.55e-14 3.55e-14 3.55e-14 3.55e-14 3.56e-14 3.68e-14 4.74e-14 8.32e-14
Th 230 3.19e-10 8.37e-10 2.91e-09 5.52e-09 1.08e-08 5.40e-08 5.73e-07 5.55e-06 7.27e-O5
Th 229 3.14e-15 5.02e-15 1.48e-14 3.22e-14 8.45e-14 1.52e-12 3.46e-10 5.40e-08 2.95e-06
Th 228 3.96e-14 3.64e-13 2.39e-12 3.91e-12 4.37e-12 2.07e-12 3.71e-16 1.97e-16 2.99e-14
Th 227 4.59e-19 3.14e-18 1.65e-17 3.96e-17 1.04e-16 9.83e-16 1.32e-14 1.39e-13 1.44e-12

Ac 228 4.81e-26 5.23e-25 6.80e-24 2.13e-23 6.13e-23 4.84e-22 5.11e-21 7.22e-20 1.09e-17
Ac 227 2.60e-16 1.35e-15 7.09e-15 1.71e-14 4.46e-14 4.23e-13 5.69e-12 5.98e-ll 6.22e-10
Ac 225 1.90e-19 1.87e-20 5.53e-20 1.2Oe-19 3.15e-19 5.65e-18 1.29e-15 2.01e-13

Ra 228 3.96e-22 3Oe-21 5.59e-20 1.75e-19 5.04e-19 3.98e-18 4.21e-17 5.93e-16 8.98e-14
Ra 226 9.81e-16 18e-15 7.36e-14 2.63e-13 9.93e-13 2.38e-ll 2.23e-09 8.96e-08 1.51e-06
Ra 225 3.39e-19 77e-20 8.19e-20 1.78e-19 4.67e-19 8.36e-18 1.91e-15 2.98e-13 1.63e-ll
Ra 224 1.95e-16 91e-15 1.25e-14 2.05e-14 2.29e-14 1.09e-14 1.95e-18 1.03e-18 1.56e-16
Ra 223 2.36e-19 1.94e-18 l.O2e-17 2.45e-17 6.41e-17 6.09e-16 8.18e-15 8.60e-14 8.95e-13

Pr 223 6.84e-24 3.55e-23 1.86e-22 4.48e-22 1.17e-21 l.lle-20 1.50e-19 1.57e-18 1.636-17
Pr 221 6.34e-23 6.24e-24 1.84e-23 4.01e-23 1.05e-22 1.88e-21 4.30e-19 3.676-15

Rn 222 6.14e-21 4.04e-20 4.32e-19 1.72e-18 6.50e-18 1.56e-16 1.46e-14 5.86e-13 9.88e-12
Rn 220 3.42e-20 3.35e-l9 2.20e-18 3.60e-18 4.03e-18 1.91e-18 3.42e-22 1.82e-22 2.75e-2O
Rn 219 9.48e-25 7.79e-24 4.09e-23 9.84e-23 2.57e-22 2.44e-21 3.28e-20 3.45e-19 3.59«-18

At 217 7.11e-27 7.00e-28 2.07e-27 4.50e-27 1.18e-26 2.11e-25 4.82e-23 7.53e-21 4.11e-19

Po 218 3.40e-24 2.24e-23 2.67e-22 9.53e-22 3.606-21 8.646-20 8.106-18 3.25e-16 5.486-15
Po 216 9.23e-23 9.04e-22 5.93e-21 9.72e-21 1.096-20 5.15e-21 9.236-25 4.906-25 7.426-23
Po 210 3.02e-22 1.10e-20 9.70e-19 6.31e-18 4.30e-17 3.136-15 5.296-13 2.126-11 3.586-10

Bi 214 2.226-23 1.46e-22 1.74e-21 6.226-21 2.356-20 5.646-19 5.286-17 2.126-15 3.576-K
Bi 213 6.03«-22 5.936-23 1.75e-22 3.816-22 1.006-21 1.796-20 4.096-18 6.396-16 3.496-14
Bi 212 2.24c-18 2.196-17 1.446-16 2.356-16 2.636-16 1.256-16 2.246-20 1.196-20 1.806-18
Bi 211 3.06e-23 2.S2C-22 1.326-21 3.176-21 8.306-21 7.886-20 1.066-18 1.116-17 1.166-16
U0 2 Fuel - Actinides Mass: sol/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10 4 Year 10* Year

Bi 210 4.83e-23 8.83e-22 3.51e-20 2.28e-19 1.56e-18 1.13e-16 1.92e-14 7.68e-13 1.30e-ll
Bi 209 7.26e-19 1.60e-18 5.20e-18 1.6Oe-17 6.91e-17 4.86e-15 9.40e-12 1.75e-08 2.46e-04

Pb 214 2.99e-23 1.97e-22 2.34e-21 8.37e-21 3.16e-20 59e-19 7.12e-17 2.85e-15 4.81e-14
Pb 212 2.36e-17 2.31e-16 1.51e-15 2.48e-15 2.77e-15 31e-15 2.36e-19 1.25e-19 1.89e-17
Pb 211 5.19e-22 4.26e-21 2.24e-20 5.38e-20 1.41e-19 33e-18 1.79e-17 1.89e-16 .96e-15
Pb 210 8.61e-20 1.44e-18 5.71e-17 3.71e-16 2.53e-15 84e-13 1.25e-09 .10e-08
Pb 209 2.58e-21 2.54e-22 7.50e-22 l-63e-21 4.27e-21 66e-2O 1.75e-17 2.73e-15 .49e-13
Pb 208 2.36e-15 6.78e-14 2..06e-12 7.99e-12 2.36e-ll 14e-10 1.92e-10 1.92e-10 .61e-09
Pb 207 8.31e-19 2.39e-17 5..3Oe-16 2.40e-15 1.19e-14 5.73e-13 8.77e-ll 9.34e-09 .88e-05
Pb 206 6.89e-23 7.19e-21 2.18e-18 2.88e-17 4.03e-16 1.61e-13 3.22e-10 1.63e-07 6.03e-04

Tl 209 6.28e-25 6.18e-26 1.83e-25 3.97e-25 1.04e-24 1.87e-23 4.26e-21 6.65e-19 3.63e-17
Tl 208 4.07e-20 3.99e-19 2.62e-18 4.29e-18 4.79e-18 2.27e-18 4.07e-22 2.16e-22 3.27e-20
Tl 207 6.83e-23 5.62e-22 2.95e-21 7.09e-21 1.85e-20 1.76e--19 2.36e-18 2.49e-17 2.58e-16
He 4 6.26e-07 2.96e-06 8.11e-06 1.53e-05 3.26e-05 2.08e-04 1.55e-03 6.71e-03 2.41e-02
TOTAL 4.17e+00 4.17e+00 4.17e+00 4.17e+00 4.17e+00 4.17e+00 4.17e+00 4.17e+00 4.19e+00

Page A.6
U0 2 Fuel - Fission Products Mass: aol/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10* Year 10 6 Year
H 3 4.83e-06 4.57e-06 3.65e-06 2.76e-O6 1.57e-O6 1.76e-08 0.00e+00 0.00e+00 0.00e+00
Ge 72 2.00e-08 2.04e-08 2.04e-08 2.04e-08 2.04e-08 2.04e-08 2.04e-08 2.04e-08 2.04e-08
Ge 73 5.31e-08 5.32e-08 5.32e-08 5.32e-08 5.32e-08 5.32e-08 5.32e-08 5.32e-08 5.32e-08
Ge 74 1.47e-07 1.47e-07 1.47e-07 1.47e-07 1.47e-O7 1.47e-07 1.47e-07 1.47e-07 1.47e-07
Ge 76 1.09e-06 1.09e-06 1.09e-06 1.09e-06 1.09e-06 1.09e-06 1.09e-06 1.09e-06 1.09e-06
As 75 3.98e-07 3.98e-07 3.98e-07 3.98e-07 3.98e-07 3.98e-07 3.98e-07 3.98e-07
Se 76 ,40e-09 3.45e-0? 3.45e-09 3.45e-O9 3.45e-09 3.45e-09 3.45e-09 3.45e-09 3.45e-09
Se 77 ,50e-06 2.53e-06 2.53e-06 2.53e-06 2.53e-O6 2.53e-06 2.53e-06 2.53e-06 2.53e-06
Se 78 .4be-06 6.46e-06 6.46e-06 6.46e-06 6.46e-06 6.46e-06 6.46e-06 6.46e-06 6.46e-06
Se 79 ,64e-05 1.64e-05 1.,64e-05 1.64e-O5 1.64e-05 1.64e-05 1.62e-05 1.47e-05 3.80e-10
Se 80 .00e-05 4.00e-05 4..00e-05 4.00e-05 4.00e-05 4.0Oe-05 4.00e-05 4.00e-05 4.00e-05
Se 82 9.59e-05 9.59e-05 9.59e-05 9.59e-05 9.59e-05 9.59e-05 9.59e-05 9.59e-05 9.59e-05
Br 79 1.01e-10 2.75e-10 9.74e-10 1.85e-09 3.59e-09 1.76e-O8 1.74e-07 1.66e-06 1.64e-05
Br 81 6.56e-05 6.56e-05 6.56e-05 6.56e-05 6.56e-05 6.56e-05 6.56e-05 6.56e-05 6.56e-05
Kr 80 9.26e-10 9.27e-10 9.27e-10 9.27e-10 9.27e-10 9.27e-10 9.27e-10 9.27e-10 9.27e-10
Kr 81 6.73e-ll 6.73e-ll 6.73e-ll 6.73e-ll 6.73e-ll 6.72e-ll 6.70e-ll 6.51e-ll 2.48e-12
Kr 82 9.75e-O7 9.92e-O7 9.92e-07 9.92e-O7 9.92e-07 9..92e-07 9..92e-07 9.92e-07 9.92e-O7
Kr 83 1..19e-04 1.20e-04 1.20e-04 1.2Oe-O4 1.20e-04 1..20e-04 1.,20e-04 1.20e-04 1.20e-04
Kr 84 2..90e-04 2.90e-04 2.90e-04 2.90e-04 2.90e-04 2..90e-04 2.9Oe-04 2.90e-04 2.90e-04
Kr 85 7..03e-05 6.60e-05 5.10e-05 3.69e-05 1.93e-05 1..09e-07 O.OOe+00 0-OOe+OO 0.00e+0O
Kr 86 4.88e-04 4.88e-04 4.88e-04 4.88e-04 4.88e-04 4.88e-04 4.88e-04 4.88e-04 4.88e-04
Rb 85 2.65e-04 2.70e-04 2.85e-04 2.99e-04 3.16e-04 3.36e-04 3.36e-04 3.36e-04 3.36e-04
Rb 86 7.21e-08 9.23e-14 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 O.OOe-fOO
Rb 87 6.31e-04 6.31e-04 6.31e-O4 6.31e-O4 6.31e-04 6.31e-04 6.31e-04 6.31e-04 6.31e-04
Sr 86 3.03e-07 3.75e-O7 3.75e-O7 3.75e-O7 3.75e-07 3.75e-07 3.75e-07 3.75e-O7 3.75e-O7
Sr 87 5.06e-09 5.07e-O9 5.07e-09 5.07e-09 5.07e-09 5.07e-09 5.08e-09 5.16e-09 1.44e-08
Sr 88 9.02e-04 9.02e-04 9.02e-04 9.02e-04 9.02e-04 9.02e-04 9.02e-04 9.02e-04 9.02e-04
Sr 89 3.19e-04 2.12e-O6 4.14e-15 5.37e-26 0.00e+00 O.OOe+00 0.00e+00 0.00e+00 0.00e+0O
Sr 90 1.43e-03 1.40e-03 1.27e-O3 1.13e-O3 8.91e-04 1.33e-04 6.58e-14 O.OOe+00 0.00e+00
Y 89 8.66e-04 1.18e-03 1.19e-03 1.19e-03 1.19e-03 1.19e-03 1.19e-03 1.19e-03 1.19e-O3
Y 90 3.93e-07 3.51e-07 3.19e-O7 2.84e-07 2.23e-O7 3.33e-08 1.65e-17 O.OOe+OO O.OOe+OO
Y 91 4.74e-04 6.3Oe-O6 1.92e-13 7.68e-23 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+OO
Pave A.7
U0 2 Fuel - Fission Products Mass: aol/kg inital D

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 10s Year

Zr 90 1.23e-05 4.61e-05 1.73e-04 3.16e-04 5.56e-04 1.31e-O3 1.45e-03 1.45e-03 1.45e-03

Zr 91 04e-03 51e-03 51e-03 51e-03 ,51e-03 1.51e-03 1.51e-03 1.51e-O3 1.51e-O3
Zr 92 60e-03 60e-03 60e-03 60e-03 .60e-03 1.6Oe-O3 1.60e-03 1.60e-03 1.60e-O3
Zr 93 80e-03 81e-03 1.81e-03 81e-03 ,81e-03 1.81e-03 1.80e-03 1.80e-03 1.15e-03
Zr 94 90e-03 90e-03 90e-03 90e-03 ,9Oe-03 1.9Oe-O3 1.90e-03 1.90e-03 1.90e-03
Zr 95 7.14e-04 36e-05 82e-12 4.64e-21 .O2e-38 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Zr 96 1.97e-03 1.97e-O3 1.97e-03 1.97e-03 1.97e-03 1.97e-03 1.97e-03 1.97e-03 1.97e-O3

Nb 93 5.19e-ll 1.26e-10 7.76e-10 2.26e-09 6.85e-09 6.70e-08 8.03e-07 8.15e-06 6.58e-04

Nb 93m 2.86e-10 1.03e-09 3.65e-09 6.26e-09 9.85e-09 1.52e-08 1.52e-08 1.52e-08 9.69e-09
Nb 94 2..49e-09 2.49e-09 2.49e-09 2.49e-09 2.49e-09 2.482-09 2.41e-09 1.77e-09 3.69e-24
Nb 95 3..62e-04 1.68e-O5 2.22e-12 5.67e-21 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Nb 95m 2.85e-07 5.71e-09 7.62e-16 1.94e-24 0.00e+00 0.00e+00 Q.00e+00 0.00e+00 0.00e+00

Mo 95 8.94e-04 1.94e-03 1.97e-03 1.97e-03 1.97e-03 97e-03 1.97e-O3 1.97e-03 1.97e-O3

Mo 96 1.40e-05 1.41e-05 1.41e-05 1.41e-05 1.41e-05 41e-05 1.41e-05 1.41e-05 1.41e-05
Mo 97 1.98e-03 1.99e-03 1.99e-O3 1.99e-03 1.99e-03 99e-03 1.99e-03 1.99e-03 1.99e-03
Mo 98 2.00e-03 2.00e-03 2.00e-03 2.00e-03 2.00e-03 OOe-O3 2.00e-03 2.00e-03 2.00e-03
Mo 100 2.26e-03 2.26e-O3 2.26e-03 2.26e-03 2.26e-03 2.26e-03 2.26e-03 2.26e-03 2.26e-O3

Tc 99 2.03e-03 2.07e-O3 2.07e-03 2.07e-03 2.07e-03 2.07e-03 2.06e-03 2.00e-03 7.98e-05

Ru 99 03e-09 8.75e-09 57e-08 93e-08 ,37e-07 6.75e-07 6.72e-06 6.62e-05 ,99e-03

Ru 100 22e-05 7.22e-05 22e-05 22e-05 .22e-05 7.22e-05 22e-05 7.22e-05 ,22e-O5
Ru 101 87e-O3 1.87e-O3 87e-O3 87e-03 .87e-03 1.87e-03 87e-O3 1.87e-O3 .87e-O3
Ru 102 76e-03 1..76e-O3 76e-O3 76e-O3 .76e-03 1.76e-03 76e-O3 1.76e-O3 .76e-O3
Ru 103 59e-04 7.,29e-O7 63e-18 ,66e-32 0.00e+00 0.00e+00 00e+00 0.00e+00 0.00e+00
Ru 104 28e-03 1.,28e-03 28e-03 ,28e-03 1.28e-03 1.28e-03 28e-03 1.28e-O3 1.28e-O3
Ru 106 6.17e-04 3.10e-04 1.98e-05 6.36e-07 6.56e-10 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Rh 103 1.05e-03 1.51e-O3 1.51e-03 1.51e-03 1.51e-03 1.51e-03 1.51e-03 1.51e-03 1.51e-03
Rh 103m 4.11e-07 6.52e-10 4.14e-21 4.17e-35 0.00e+00 0.00e+00 0.0Oe+O0 O.OOe+00 O.OOe+00
Rh 106 9.46e-10 2.91e-10 1.86e-ll 5.98e-13 6.17e-16 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00

Pd 104 1.71e-04 1.71e-04 1.71e-04 1.71e-04 1.71e-04 1.71e-04 1.71e-04 1.71e-04 1.71e-04
Pd 105 8.48e-04 8.61e-04 8.61e-04 8.61e-04 8.61e-04 8.61e-04 8.61e-04 8.61e-04 8.61e-O4
Pd 106 2..98e-04 6.05e-04 8.95e-04 9.14e-04 9..15e-04 9.,15e-04 9.15e-04 9.15e-04 9.15e-O4
Pd 107 5..08e-04 5..08e-04 5.08e-04 5.08e-04 5..08e-04 5.,08e-04 5.08e-04 5.07e-04 4.56e-04
Pd 108 3.41e-04 3..41e-04 3.41e-04 3.41e-04 3..41e-04 3.41e-04 3.41e-04 3.41e-04 3.41e-04
Pd 110 9.5Oe-O5 9.50e-05 9.5Oe-O5 9.50e-05 9.50e-05 9.5Oe-O5 9.50e-05 9.50e-05 9.50e-05
A.ft
U0 2 Fuel - Pission Products Mass: •ol/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Ag 107 1.33e-ll 6.74e-ll 2.84e-10 5.55e-10 1.10e-09 5.43e-09 5.42e-08 5.41e-07 5.14e-05
Ag 108 5.92e-17 8.88e-21 8.69e-21 8.46e-21 8.01e-21 5.17e-21 3.81e-23 O.OOe+00 O.OOe+OO
Ag 108m 2..83e-12 2.81e-12 2..75e-12 2.68e-12 2,54e-12 1.64e-12 1.21e-14 5.58e-36 O.OOe+OO
Ag 109 1..94e-04 1.95e-04 1..95e-04 1.95e-04 1.95e-04 1.95e-04 1.95e-04 1.95e-04 1.95e-04
Ag 110 1..10e-10 4.32e-15 7.,51e-17 4.73e-19 1.88e-23 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+OO
Ag 110m 7.85e-07 2.85e-07 4.95e-09 3.12e-ll 1.24e-15 O.OOe+00 0.0Oe+OO O.OOe+00 O.OOe+OO

Cd 108 3.09e-12 3.09e-12 10e-12 3.10e-12 3.12e-12 3.19e-12 3.33e-12 3.34e-12 3.34e-12
Cd 109 3.26e-15 1.89e-15 13e-16 1.39e-17 5.93e-20 6.52e-39 0.00e+00 O.OOe+00 O.OOe+OO
Cd 110 2.33e-05 38e-05 41e-05 2.41e-05 2.41e-05 2.41e-05 2.41e-O5 2.41e-05 ,41e-05
Cd 111 4.04e-05 35e-05 35e-05 4.35e-05 4.35e-05 4.35e-05 4.35e-O5 4.35e-05 35e-05
Cd 112 1.93e-O5 94e-05 94e-05 1.94e-05 .94e-05 1.94e-05 ,94e-05 1.94e-05 94e-05
Cd 113 2..79e-07 04e-07 04e-07 3.04e-07 .04e-07 3.04e-07 ,04e-07 3.04e-07 ,04e-07
Cd 113m 2..9Oe-07 76e-07 25e-07 1.74e-07 ,O5e-O7 1.78e-09 ,12e-29 O.OOe+00 O.OOe+OO
Cd 114 2..32e-05 2.32e-05 32e-05 2.32e-05 ,32e-05 2.32e-O5 ,32e-O5 2.32e-O5 2.32e-05
Cd 115m 2.,32e-07 7.95e-10 09e-19 5.14e-32 0.00e+00 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+OO
Cd 116 7.49e-06 7.49e-06 7.49e-06 7.49e-06 7.49e-06 7.49e-06 7.49e-06 7.49e-06 7.49e-06

In 113 3.67e-09 1.81e-08 6.89e-08 1.19e-07 1.89e-O7 2.92e-O7 2.94e-O7 2.94e-07 2.94e-07
In 114 6.29e-16 2.15e-18 2.81e-27 O.OOe+00 0.00e+00 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+OO
In 114m 2.23e-ll 1.34e-13 1..75e-22 1.37e-33 0.00e+00 0.00e+00 O.OOe+OO O.OOe+00 O.OOe+OO
In 115 5.31e-06 5.68e-06 5.,68e-06 5.68e-06 5.68e-06 5.68e-06 5.68e-06 5.68e-06 5.68e-06
In 115m 1.05e-08 3.21e-16 4.40e-26 0.00e+00 0.00e+00 0.00e+00 O.OOe+OO O.OOe+00 O.OOe+OO

Sn 114 3.14e-ll 5.24e-ll 5.25e-ll 25e-ll 25e-ll 5.25e-ll 5.25e-ll 25e-ll

Sn 115 2.55e-07 2.60e-07 2.60e-07 6Oe-O7 60e-07 2.6Oe-O7 2.60e-07 2.6Oe-O7 60e-07
Sn 116 2..09e-06 ,09e-06 2.09e-06 09e-06 09e-06 2.09e-06 2.09e-06 2.09e-06 09e-06
Sn 117 7..47e-06 ,48e-06 7.48e-06 48e-06 48e-06 7.48e-O6 7.48e-O6 7.48e-06 48e-06
Sn 117m 3..14e-10 A0e-18 0.,00e+00 0.00e+00 0.00e+00 0.00e+00 O.OOe+OO O.OOe+OO O.OOe+OO
Sn 118 7.,69e-06 ,69e-06 7.69e-06 69e-06 7.69e-06 7.69e-O6 7.69e-06 7.69e-06 69e-06
Sn 119 7..54e-06 ,60e-06 7.63e-06 63e-06 7.63e-06 7.63e-O6 7.63e-O6 7.63e-06 63e-06
Sn 119m 8.74e-08 lle-08 4.98e-10 84e-12 9.23e-17 0.00e+00 O.OOe+OO O.OOe+OO OOe+00
Sn 120 7.77e-O6 ,77e-06 7.,77e-06 77e-O6 7.77e-O6 7.77e-O6 7.77e-O6 7.77e-06 77e-06
Sn 121m 6.00e-09 ,93e-09 5.,64e-09 29e-09 4.67e-09 1.7Oe-O9 2.02e-14 O.OOe+OO O.OOe+OO
Sn 122 8.49e-06 8.49e-06 8.49e-06 8.49e-06 8.49e-06 8.49e-06 8.49e-06 8.49e-06 8.49e-06
Sn 123 1.44e-06 2.03e-07 7.98e-ll 4.43e-15 1.37e-23 0.00e+00 O.OOe+OO O.OOe+OO O.OOe+OO
Sn 124 1.26e-05 1.26e-05 1.26e-05 1.26e-05 1.26e-05 1.26e-05 1.26e-O5 1.26e-05 1.26e-0S
Sn 125 7.95e-07 3.12e-18 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+OO O.OOe+OO
Sn 126 3.92e-05 3.92e-05 3.92e-05 3.92e-05 3.92e-O5 3.92e-O5 3.9Oe-O5 3.66e-05 3.83e-08

Page A.9
UOj Fuel - Fission Products Mass: •ol/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 1O3 Year 10* Year 10 6 Year
Sb 121 8.'04e-06 8. lle-06 8. lle-06 8. lle-06 8. lle-06 8. lle-06 8. lle-06 8. lle-06 8. lle-06
Sb 123 8. 44e-06 9. 68e-06 9. 88e-06 9. 88e-06 9. 88e-06 9. 88e-O6 9. 88e-06 9. 88e-06 9. 88e-06
Sb 124 5. 13e-08 7.64e-10 3. 77e-17 2. 78e-26 0. 00e+00 0.OOe+CJ 0. OOe+00 0. OOe+00 0. OOe+00
Sb 125 2. 20e-05 1. 77e-O5 6. 52e-06 1.87e-06 1.53e-O7 3.09e-16 0. OOe+00 0. OOe+00 0. OOe+00
Sb 126 6. 91e-08 1. 87e-12 1. 87e-12 1.87e-12 1.86e-12 1.86e-12 1.85e-12 1. 74e-12 1.82e-15
Sb 126m 6. 29e-ll 1. 42e-14 1. 42e-14 1.42e-14 1.42e-14 1.42e-14 1. 41e-14 1. 32e-14 1. 38e-17
Te 122 1. 17e-07 1. 22e-07 1. 22e-07 1.22e-07 1. 22e-07 1.22e-O7 1. 22e-O7 1.22e-O7 1. 22e-O7
Te 123 2. 88e-10 4. 05e-10 4. 21e-10 4. 21e-10 4. 21e-10 4. 21e-10 4. 21e-10 4. 21e-10 4. 21e-10
Te 123m 1. 33e-10 1.60e-ll 3. 39e-15 8. 65e-20 5.63e-29 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00
Te 124 4. 96e-08 1.00e-07 1.01e-07 1.01e-O7 1.01e-07 1.Ole-07 1. Ole-07 1.Ole-07 1. Ole-07
Te 125 1. 29e-06 6. 26e-06 1.76e-05 2.24e-O5 2.41e-05 2.42e-O5 2.42e-O5 2.42e-05 2.42e-05
Te 125m 1. 75e-07 2. 46e-07 9. 12e-08 2.61e-08 2. 14e-09 4. 32e-18 0. OOe+00 0. OOe+00 0. OOe+00
Te 126 1.04e-06 1. lle-06 1. lle-06 1. lle-06 1. lle-06 1. 13e-06 1. 38e-06 3. 73e-06 4.03e-05
Te 127 2. 93e-07 2.73e-09 2.,52e-13 2. 28e-18 1.86e-28 0.OOe+00 0. OOe+00 0. OOe+00 0.,OOe+00
Te 127m 7.,52e-06 7.,81e-07 7.,20e-ll 6. 51e-16 5.,31e-26 0.. OOe+00 0..OOe+00 0.,OOe+00 0..OOe+00
Te 128 1.,94e-04 1.,95e-04 1.,95e-04 1,,95e-04 1.,95e-04 1.,95e-04 1.,95e-04 1.,95e-04 1.,95e-04
Te 129 1.,23e-07 6..16e-12 5..00e-25 0.,OOe+00 0.,00e+00 0..00e+00 0.. OOe+00 0..OOe+00 0,.OOe+00
Te 129m 1.,23e-05 6..58e-09 5..34e-22 2,,31e-38 0,.00e+00 0..OOe+00 0..OOe+00 0..OOe+00 0,.OOe+00
Te 130 6,.52e-04 6,.52e-04 6.,52e-04 6.,52e-04 6,.52e-04 6..52e-04 6..52e-04 6 .52e-04 6 ,52e-04
I 127 8 .61e-05 9 .63e-05 9 .70e-O5 9,.7Oe-O5 9 .7Oe-O5 9 .70e-05 9 .7Oe-O5 9 .7Oe-O5 9 .70e-05
I 129 3 .34e-04 3 .47e-04 3 .47e-04 3 .47e-04 3 .47e-04 3 .47e-04 3 .47e-04 3 .47e-04 3 .32e-04
I 131 5 .94e-05 1 .29e-18 0 .OOe+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Xe 128 1 .O7e-O6 1 .07e-06 1 .07e-06 1 .07e-06 1 .07e-06 1 .O7e-O6 1 .O7e-O6 1 .O7e-O6 1 .O7e-O6
Xe 129 2 .37e-09 2 .59e-09 2 .65e-09 2 .72e-O9 2 .88e-09 4 .10e-09 1.79e-O8 1 .56e-07 1 .5Oe-O5
Xe 130 5 .O6e-O7 9 .10e-07 9 .10e-07 9 .10e-07 9 .10e-07 9 .10e-07 9 .10e-07 9 .10e-07 9 .10e-07
Xe 131 9 .31e-04 9 .93e-04 9 .93e-04 9 .93e-04 9 .93e-O4 9 .93e-04 9 .93e-04 9 .93e-04 9 .93e-04
Xe 131m 9 ,81e-07 1 .77e-15 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Xe 132 1 .71e-O3 1.75e-03 1 .75e-03 1.75e-03 1 .75e-O3 1.75e-03 1.75e-03 1 .75e-O3 1 .75e-03
Xe 134 2 .62e-03 2 .62e-03 2 .62e-03 2 .62e-O3 2 .62e-O3 2 .62e-03 2 .62e-03 2 .62e-03 2 .62e-03
Xe 136 4 .42e-03 4 .42e-03 4 .42e-O3 4 .42e-O3 4 .42e-03 4 .42e-03 4 .42e-03 4 .42e-03 4 .42e-03

Cs 133 2 .18e-03 2 .27e-O3 2 .27e-03 2 .27e-O3 2 .27e-O3 2 .27e-O3 2 .27e-03 2 .27e-03 2 •27e-03
Cs 134 8 .73e-05 6 .24e-05 1 .63e-O5 3.03e-06 1.O5e-O7 2.19e-19 0 .OOe+00 0 .OOe+00 0 .OOe+00
Cs 135 1 .72e-04 1 .76e-O4 1.76e-04 1.76e-04 1.76e-04 1.76e-04 1.76e-04 1. 75e-O4 1. 30e-04
Cs 136 2 .25e-06 9 .10e-15 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Cs 137 2 .20e-03 2 .15e-03 1 .96e-03 1.75e-O3 1 .39e-03 2.21e-0A 2 •31e-13 0 .OOe+00 0 .OOe+00

Pase A. 10
uo 2 Fuel - Fission Products Mass: mol/kg inital U
3
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 Year 10 4 Year 106 Year
Ba 134 6. 03e-06 3. 09e-05 7. 71e-05 9. 03e-05 9. 32e-O5 9. 33e-05 9. 33e-05 9. 33e-05 9. 33e-05
Ba 135 1. 22e-08 1. 23e-08 1.25e-08 1.28e-08 1. 33e-08 1. 76e-08 6. 53e-08 5. 42e-07 4. 58e-05
Ba 136 1. 57e-05 1. 79e-05 1. 79e-05 1.79e-05 1. 79e-05 1. 79e-05 1. 79e-05 1. 79e-05 1. 79e-O5
Ba 137 1. 61e-05 6. 60e-05 2.55e-04 4. 67e-04 8. 26e-04 1. 99e-03 2. 21e-03 2. 21e-O3 2. 21e-O3
Ba 137m 3. 38e-10 3.27e-10 2.98e-10 2.66e-10 2. lle-10 3. 36e-ll 3. 51e-2O 0. OOe+00 0. OOe+00
Ba 138 2. 17e-03 2. I7e-O3 2. 17e-03 2. 17e-O3 2. 17e-03 2. 17e-03 2. 17e-O3 2. 17e-03 2. 17e-O3
Ba 140 1. 61e-04 4. 06e-13 0. 00e+00 0. 00e+00 0. 00e+00 0. 00e+00 0. OOe+00 0. OOe+00 0. OOe+00

La 138 1. 43e-08 1. A3e-08 1. 43e-08 1. 43e-08 1. 43e-08 1. 43e-08 1. 43e-08 1. 43e-08 1. Oe-08
La 139 2. 09e-03 2.09e-03 2.09e-03 2.O9e-O3 2. 09e-03 2. 09e-03 2. 09e-O3 2. 09e-03 2.09e-03
La 140 2. 25e-05 6. 13e-14 0. 00e+00 0. 00e+00 0. 00e+00 0. 00e+00 0. OOe+00 0. OOe+00 0. OOe+00
Ce 140 1. 99e-03 2. 18e-03 2.18e-03 2. 18e-03 2. 18e-03 2. 18e-03 2. 18e-03 2. 18e-03 2. 18e-03
Ce 141 3. 85e-04 1. 6Oe-O7 4. 74e-21 5. 81e-38 0. 00e+00 0. 00e+00 0. OOe+00 0. OOe+00 0. OOe+00
Cfe 142 1. 91e-03 1. 91e-O3 1.91e-03 1. 91e-03 1. 91e-03 1. 91e-03 1. 91e-03 1. 91e-03 1.91e-03
Ce 144 1. 24e-03 5. 09e-04 1.44e-05 1. 68e-07 2. 28e-ll 0. 00e+00 0. OOe+00 0. OOe+00 0. OOe+00
Pr 141 1,,52e-03 1.,91e-O3 1.,91e-03 1.,91e-03 1.,91e-03 1.,91e-03 1. 91e-03 1. 91e-03 1.,91e-03
Pr 143 1,,41e-04 1.,23e-12 0.. OOe+00 0..00e+00 0.,00e+00 0. 00e+00 0..OOe+00 0..OOe+00 0.,OOe+00
Pr 144 5,.44e-08 2,,15e-08 6..09e-10 7..09e-12 9.,62e-16 0.,00e+00 0..OOe+00 0..OOe+00 0..OOe+00
Pr 144m 2,.62e-10 1,.07e-10 3,.O5e-12 3,.55e-14 4,.81e-18 0..00e+00 0.,OOe+00 0..OOe+00 0..OOe+00
Nd 142 1 .52e-05 1 .54e-05 1,.54e-05 1 .54e-05 1 .54e-05 1,.54e-05 1,.54e-O5 1..54e-05 1 .54e-05
Nd 143 1 .28e-O3 1,.43e-O3 1,.43e-03 1 .43e-03 1 .43e-03 1..43e-03 1,.43e-O3 1,.43e-O3 1 .43e-03
Nd 144 8 .15e-04 1 .55e-03 2 ,04e-03 2 .05e-03 2 .05e-03 2 .05e-03 2 .05e-03 2 .O5e-O3 2 .05e-03
Nd 145 1 .17e-O3 1 .17e-O3 1 .17e-03 1 .17e-O3 1 .17e-O3 1 .17e-O3 1 .17e-O3 1 . 17e-O3 1 .17e-O3
Nd 146 1 .03e-O3 1.O3e-O3 1 .03e-03 1 •03e-03 1 .O3e-O3 1 .03e-03 1 .03e-03 1 .O3e-O3 1 .03e-03
Nd 147 5 .16e-05 5 .9Oe-15 0 .00e+00 0 .00e+00 0 •OOe+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Nd 148 5 •90e-04 5 .9Oe-O4 5.90e-04 5 .90e-04 5 .90e-04 5 .90e-04 5 .90e-04 5 .90e-04 5 .90e-04
Nd 150 2 .83e-04 2 •83e-04 2.83e-04 2 .83e-04 2 .83e-04 2 .83e-04 2 .83e-OA 2 •83e-04 2 .83e-04
Pm 147 5 .10e-04 4 .31e-04 1.50e-04 4 .00e-05 2 .85e-06 1 .88e-15 0 .OOe+00 0 .00e+0C 0 .OOe+00
Pm 148 3 .94e-06 3 .22e-ll 7.21e-22 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Pm 148m 2 .02e-06 4 .39e-09 9 .8Ae-20 4 .79e-33 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Sm 147 4 .12e-O5 1.72e-04 4 .53e-04 5 .63e-0A 6 .00e-0A 6 .03e-04 6 .03e-04 6 .03e-0A 6 ,03e-04
Sm 148 6 .39e-05 6 .98e-05 6 .98e-05 6 .98e-05 6 .98e-05 6 .98e-05 6 .98e-05 6 .98e-05 6 .98e-05
Sm 149 3 .80e-06 1.2Oe-O5 1.20e-05 1.2Oe-O5 1 .20e-05 1 •2Oe-O5 1.20e-05 1.20e-05 1.20e-05
Sm 150 4 .58e-0A 4 .58e-0A 4 .58e-04 4 .58e-0A 4 .58e-0A 4 .58e-04 4 .58e-0A 4 .58e-0A 4 .58e-04
Sm 151 1 .47e-05 1.64e-05 1.59e-05 1 .53e-05 1 .Ale-05 7 .63e-06 7 .45e-09 0 .OOe+00 0 .OOe+00
A.11
U0 2 Fuel - Fission Products Mass: aol/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 104 Year 10s Year

Sm 152 2.89e-04 2.90e-04 2.90e-04 2.90e-04 2.90e-04 2.90e-04 2.90e-04 2.90e-04 2.90e-04
Sm 154 5.68e-05 5.68e-05 5.68e-05 5.68e-05 5.68e-05 5.68e-05 5.68e-05 5.68e-05 5.68e-05
Eu 151 09e-09 ,32e-07 6.28e-07 23e-06 2.36e-06 8.86e-06 1.65e-05 1.65e-05 1.65e-05
Eu 152 23e-08 ,17e-08 9.55e-09 ,40e-09 4.45e-09 7.53e-ll 9.00e-31 0.00e+00 0.00e+00
Eu 153 3Oe-O4 ,34e-04 1.34e-04 .34e-04 1..34e-04 1.34e-04 1.34e-04 1.34e-04 1.34e-04
Eu 154 71e-O5 2.50e-05 1.81e-05 .21e-05 5..40e-06 8.54e-09 0.00e+00 0.00e+00 0.00e+00
Eu 155 2Oe-O5 1.04e-05 5.95e-06 .96e-06 7.,32e-07 1.02e-ll 0.00e+00 0.0Oe+00 0.00e+00
Eu 156 9.7Oe-O6 5.64e-13 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.0Oe+OO 0.00e+00 0.00e+00
Gd 152 35e-O8 37e-08 1.43e-08 1.49e-08 57e-08 1.69e-08 1.69e-08 1.69e-08 1.69e-08
Gd 153 67e-O9 84e-10 8.83e-12 4.68e-14 31e-18 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Gd 154 29e-O7 52e-06 9.40e-06 1.54e-05 21e-05 2.75e-O5 .75e-O5 2.75e-05 2.75e-O5
Gd 155 ,55e-08 58e-06 6.04e-06 9.03e-06 13e-05 1..20e-05 .20e-Q5 1.20e-05 1.2Oe-O5
Gd 156 ,84e-05 ,82e-05 5.82e-05 5.82e-O5 5.82e-05 5..82e-05 ,82e-05 5.82e-05 5.82e-O5
Gd 157 ,06e-08 .35e-07 1.35e-07 1.35e-07 1.35e-07 1..35e-07 .35e-O7 1.35e-07 1.35e-07
Gd 158 .96e-05 .96e-05 1.96e-05 1.96e-05 1.96e-05 1..96e-05 .96e-O5 1.96e-O5 1.96e-05
Gd 160 1.50e-06 1.50e-06 1.50e-06 1.5Oe-06 1.50e-06 1.50e-06 1.50e-06 1.50e-06 1.5Oe-O6
Tb 159 3.31e-06 3.34e-06 3.34e-06 3.34e-06 3.34e-06 3.3«e-06 3.34e-06 3.34e-06 3.34e-06
Tb 160 6.69e-08 2.02e-09 1.66e-15 4.14e-23 2.56e-38 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Dy 160 4.29e-08 1.08e-07 1.10e-07 1.10e-07 1.10e-07 10e-07 1.10e-07 1.10e-07 1.10e-07
Dy 161 4.75e-07 5.25e-07 5.25e-07 5.25e-07 5.25e-07 25e-O7 5.25e-O7 5.25e-O7 5.25e-07
Dy 162 4.78e-07 4.78e-07 4.78e-07 4.78e-07 4.78e-07 , 78e-O7 4.78e-07 4.78e-07 4.78e-0?
Dy 163 2.21e-O7 2.21e-07 2.21e-07 2.21e-07 2.21e-O7 ,21e-O7 2.21e-O7 2.21e-O7 2.2U-O7
Dy 164 2.97e-08 2.97e-08 2.97e-08 2.97e-08 2.97e-O8 2.97e-08 2.97e-08 2.97e-08 2.97e-08
Ho 165 6.95e-08 6.96e-08 6.96e-08 6.96e-08 6.96e-08 6.96e-08 6.96e-08 6.96e-08 6.96e-08
Ho 166m 1.24e-10 1.24e-10 1.24e-10 1.24e-10 1.23e-10 1.17e-10 6.98e-ll 3.86e-13 0.00e+00
Er 166 9.57e-09 9.86e-09 9.86e-09 9.86e-09 9.86e-09 9.87e-09 9.92e-09 9.98e-09 9.99e-09
Er 167 1.49e-10 1.49e-10 1.49e-10 1.49e-10 1.49e-10 1.49e-10 1.49e-10 1.49e-10 1.49e-lO
TOTAL 6.90e-02 6.90e-02 6.90e-02 6.90e-02 6.90e-02 6.90e-02 6.9Oe-O2 6.9Oe-O2 6.90e-02

Page A.12
U0 2 Fuel - Actinides Mass: g/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 1O3 Year 10 4 Year 10 6 Year

Cf 252 l.O7e-15 8.24e-16 2.88e-16 7.75e-17 5.60e-18 4.19e-27 O.OOe+00 C.OOe+00 O.OOe+00
Cf 251 2.38e-15 2.38e~15 2.37e-15 2.36e-15 2.34e-15 2.20e-15 1.10e-15 1.06e-18 O.OOe+00
Cf 250 9.62e-15 9.26e-15 7.49e-15 5.75e-15 3.38e-15 4.88e-17 2.59e-23 1.05e-23 O.OOe+00
Cf 249 1.70e-15 3.15e-14 5.49e-14 5.53e-14 5.43e-14 4.63e-14 7.82e-15 1.46e-22 O.OOe+00
Bk 249 5.44e-14 2.48e-14 1.05e-15 2.00e-17 7.33e-21 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Cm 250 08e-19 08e-19 1.08e-19 1 ,08e-19 1.08e-19 1.07e-19 9.76e-20 3.95e-20 O.OOe+00
Cm 248 1 LI 1. 1.58e-ll 2.08e-12
Cm 247 6.51e-10 6.51e-10 6.51e-10 6.51e-10 6.51e-10 6.51e-10 6.51e-10 6.51e-10 6.23e-10
Cm 246 88e-07 88e-07 1.88e-07 1.87e-07 87e-O7 1.85e-07 1.62e-07 4.34e-08 O.OOe+00
Cm 245 93e-06 93e-06 1.93e-06 1.93e-06 93e-06 1.91e-06 1.78e-06 8.54e-07 O.OOe+00
Cm 244 16e-04 lle-04 1.81e-04 1.49e-04 ,02e-04 4.76e-06 5.21e-21 O.OOe+00 O.OOe+00
Cm 243 49e-06 40e-06 3.09e-06 2.74e-O6 . 14e-06 3.06e-07 9.54e-17 O.OOe+00 O.OOe+00
Cm 242 3.89e-04 8.41e-05 2.25e-O7 5.43e-08 5.18e-O8 3.59e-08 5.93e-10 8.89e-28 O.OOe+00
Am 243 2.61e-03 2.63e-03 2.63e-O3 2.63e-O3 2.62e-03 2.6Oe-O3 2.39e-03 l.O3e-O3 2.90e-13
Am 242 9.04e-06 2.79e-10 2.74e-10 2.68e-10 2.56e-10 1.78e-10 2.93e-12 4.38e-30 O.OOe+00
Am 242m 2.34e-05 2.33e-05 2.29e-05 2.24e-O5 2.14e-05 1.49e-05 2.45e-07 3.66e-25 O.OOe+00
Am 241 1.69e-03 1.22e-02 4.97e-02 8.72e-02 1.39e-01 2.02e-01 4.81e-02 6.87e-08 O.OOe+00
Pu 244 8.57e-07 8.57e-07 8.57e-07 8.57e-O7 8.57e-07 8.57e-07 8.57e-07 8.57e-07 8.50e-07
Pu 243 1.47e-05 2.32e-2O 2.32e-2O 2.32e-2O 2.32e-2O 2.32e-20 2.32e-2O 2.32e-20 2.22e-20
Pu 242 6..06e-02 6.06e-02 6.06e-02 6.06e-02 6.06e-02 6.06e-02 6.05e-02 ,95e-02 9.58e-03
Pu 241 2..29e-01 2.19e-01 1.81e-01 1.43e-01 8.93e-02 2.05e-03 3.03e-09 ,46e-09 O.OOe+00
Pu 240 1..03e+00 1..03e+00 1.03e+00 1.03e+00 1.03e+00 1.02e+00 9.27e-01 ,57e-01 6.61e-ll
Pu 239 2..64e+00 2.. 76e+00 2.76e+00 2.76e+OO 2.76e+OO 2.75e+OO 2.68e+00 ,07e+00 1.78e-12
Pu 238 4..61e-03 5..07e-03 4.99e-03 4.80e-03 4.44e-03 2.36e-03 2.05e-06 4.09e-25 O.OOe+00
Pu 236 3.95e-08 3.15e-08 1.19e-08 3.53e-O9 3.11e-10 l.lle-18 O.OOe+00 O.OOe+00 O.OOe+00
Np 240 7.03e-06 1.39e-21 1.39e-21 1.39e-21 1.39e-21 1.39e-21 1.39e-21 1.39e-21 1.37e-21
Np 240m 1.43e-19 1.43e-19 1.43e-19 1.43e-19 1.43e-19 1.43e-19 l.«3e-19 1.43e-19 1.42e-19
Np 239 1.15e-01 2.26e-09 2.26e-09 2.26e-O9 2.25e-09 2.24e-09 2.06e-09 8.83e-10 2.49e-19
Np 238 1.91e-04 4.20e-12 4.12e-12 4.03e-12 3.85e-12 2.67e-12 4.41e-14 O.OOe+00 O.OOe+00
Np 237 3.55e-02 3.8Oe-O2 3.82e-02 3.88e-O2 4.06e-02 6.50e-02 2.18e-01 2.65e-01 1.92e-01

U 240 1.64e-17 1.64e-17 1.64e-17 1.64e-17 1.64e-17 1.64e-17 1.64e-17 I.64e-17 1.63e-17
U 238 9.85e+02 9.85e+O2 9.85-+02 9.85e+02 9.85e+02 9.85e+02 9.85e+02 9.85e+02 9.85e+02
U 237 2.51e-O3 6.77e-09 5.61e-09 4.43e-09 2.76e-O9 6.36e-ll 9.37e-17 4.50e-17 O.OOe+00
U 236 7.67e-01 7.67e-01 7.67e-01 7.68e-01 7.69e-01 7.78e-01 8.69e-01 1.43e+00 1.73e+OO
U 235 2.01e+00 2.01e+00 2.01e+00 2.02e+OO 2.02e+00 2.02e+00 2.09e+00 2.69e+00 4.73e+OO
Page A.13
U0 2 Fuel - Actinides Mass: g/kg inital D
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10 4 Year 10 6 Year

U 234 4.27e-02 4.27e-02 4.29e-02 4.31e-O2 4.35e-02 4.55e-02 4.78e-02 4.80e-02 5.27a-02
U 233 9.28e-08 1.06e-07 1.54e-07 2.16e-07 3.42e-07 1.67e-06 4.73e-05 7.90e-04 1.48e-02
U 232 4.96e-09 1.34e-08 3.18e-08 3.83e-08 3.77e-O8 1.76e-08 3.04e-12 0.00e+00 0.00e+00
Pa 234 4.20e-13 2.65e-13 2.65e-13 2.65e-13 2.65e-13 2.65e-13 2.65e-13 2.65e-13 2.65e-13
Pa 234m 4.83e-13 4.82e-13 4.82e-13 4.82e-13 4.82e-13 4.82e-13 4.82e-13 4.82e-13 4.82e-13
Pa 233 9.64e-10 1.29e-09 1.30e-09 1.32e-09 1.38e-09 2.21e-09 7.40e-09 8.98e-09 6.52e-09
Pa 231 l.lle-08 1.32e-08 2.10e-08 3.07e-08 5.02e-08 2.06e-07 1.98e-06 2.08e-05 2.16e-04

Th 234 1.43e-08 1.43e-08 1.43e-08 1.43e-08 1.43e-08 1.43e-08 1.43e-08 1.43e-08 1.43e-08
Th 232 8.31e-09 3.06e-08 1.2Oe-O7 2.32e-07 4.55e-07 2.26e-06 2.38e-05 3.36e-04 5.09e-02
Th 231 1.46e-10 8.19e-12 8.19e-12 8.19e-12 8.20e-12 8.22e-12 8.50e-12 1.92e-ll
Th 230 7.33e-08 1.92e-07 6.7Oe-O7 1.27e-06 2.47e-06 1.24e-05 1.32e-04 1.28e-03 1.67e-02
Th 229 7.20e-13 1.15e-12 3.40e-12 7.38e-12 1.94e-ll 3.47e-10 7.92e-08 1.24e-05 6.75e-04
Th 228 9.03e-12 8.29e-ll 5.44e-10 8.91e-10 9.97e-10 4.73e-10 8.47e-14 4.50e-14 6.81e-12
Th 227 1.04e-16 7.12e-16 3.74e-15 8.99e-15 2.35e-14 2.23e-13 3.0Oe-12 3.15e-ll 3.28e-10
Ac 228 1.10e-23 1.19e-22 1.55e-21 4.86e-21 1.40e-20 1.10e-19 1.17e-18 1.65e-17 2.49e-15
Ac 227 5.91e-14 3.07e-13 1.61e-12 3.87e-12 9.6U-11 1.29e-09 1.36e-08 1.41e-07
Ac 225 4.28e-17 4.21e-18 1.24e-17 2.71e-17 7.1Oe-17 1.27e-15 2.9Oe-13 4.53e-ll 2.47e-09
Ra 228 9.02e-20 9.80e-19 1.27e-17 4.00e-17 1.15e-16 9.07e-16 9.59e-15 1.35e-13 2.05e-ll
Ra 226 2.22e-13 1.40e-12 1.66e-ll 5.94e-ll 2.24e-10 5.39e-09 5.05e-C7 2.03e-05 3.4U-04
Ra 225 7.63e-17 6.23e-18 1.84e-17 4.0Oe-17 1.05e-16 1.88e-15 4.30e-13 6.71e-ll 3.66e-09
Ra 224 4.36e-14 4.27e-13 2.80e-12 4.59e-12 5.13e-12 2.43e-12 4.36e-16 2.32e-16 3.50e-14
Ra 223 5.27e-17 4.34e-16 2.27e-15 5.47e-15 1.43e-14 1.36e-13 1.82e-12 1.92e-ll 2.00e-10
Fr 223 1.52e-21 7.92e-21 4.15e-20 9.99e-20 2.61e-19 2.48e-18 3.33e-17 3.51e-16 3.65e-15
Fr 221 1.40e-20 1.38e-21 4.08e-21 8.86e-21 2.32e-20 4.16e-19 9.51e-17 1.48e-14 8.10e-13
Rn 222 1.36e-18 8.98e-18 l.O7e-16 3.82e-16 1.44e-15 3.46e-14 3.25e-12 1.30e-10 2.19e-09
Rn 220 7.53e-18 7.37e-17 4.84e-16 7.92e-16 8.86e-16 4.20e-16 7.53e-20 4.00e-20 6.05e-18
Rn 219 2.08e-22 1.71e-21 8.96e-21 2.15e-20 5.63e-20 5.34e-19 7.18e-18 7.55e-17 7.85e-16
At 217 1.54e-24 1.52e-25 4.49e-25 9.76e-25 2.56e-24 4.58e-23 1.05e~20 1.63e-18 8.92e-17
Po 218 7.41e-22 4.88e-21 5.81e-2O 2.08e-19 7.84e-19 ,88e-l7 1.77e-15 7.08e-14 1.19e-12
Po 216 1.99e-2O 1.95e-19 1.28e-18 2.1Oe-18 2.35e-18 .lle-18 1.99e-22 1.06e-22 1.60e-20
Po 215 9.16e-26 7.53e-25 3..95e-24 9.51e-24 2.48e-23 .36e-22 3.17e-21 3.33e-20 3.47e-19
Po 214 6.53e-28 4.30e-27 5..12e-26 1.83e-25 6.91e-25 .66e-23 1.56e 21 6.24e-20 1.05e-18
Po 213 l-93e-28 1.90e-29 5.60e-29 1.22e-28 3.19e-28 .73e-27 1.3le-24 2.04e-22 l.lle-20
Page A. 14
uo 2 Fuel - Actinides Mass: g/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 106 Year
Po 211 7. 30e-26 6. 00e-25 3. 15e-24 7.57e-24 1.98e-23 1.88e-22 2.53e-21 2.66e-20 2.76e-19
Po 210 6. 35e-20 2. 31e-18 2. 04e-16 1. 32e-15 9.03e-15 6. 58e-13 1. lle-10 4.46e-09 7.51e-08

Bi 214 4. 75e-21 3. 13e-20 3. 72e-19 1. 33e-18 5.02e-18 1. 21e-16 1. 13e-14 4. 54e-13 7. 64e-12
Bi 213 1. 28e-19 1. 26e-20 3. 74e-20 8. 12e-20 2. 13e-19 3.82e-18 8. 71e-16 1.36e-13 7.43e-12
Bi 212 4. 74e-16 4. 64e-15 3.04e-14 4. 99e-14 5.58e-14 2. 64e-14 4. 74e-18 2.52e-18 3.81e-16
Bi 211 6. 46e-21 5.,31e-20 2. 78e-19 6. 70e-19 1. 75e-18 1.,66e-17 2.23e-16 2. 35e-15 2. 44e-14
Bi 210 1. Ole-20 1.,86e-19 7. 38e-18 4. 80e-17 3. 27e-16 2.,38e-14 4. 02e-12 1.61e-10 2. 72e-09
Bi 209 1. 52e-16 3.,35e-16 1,,09e-15 3. 35e-15 1. 44e-14 1.,02e-12 1.,96e-09 3. 66e-06 5.,14e-02
Pb 214 6.,39e-21 4..21e-20 5.,01e-19 1. 79e-18 6. 76e-18 1.,62e-16 1.,52e-14 6. lle-13 1.,03e-ll
Pb 212 5,.00e-15 4,.89e-14 3,.21e-13 5.,26e-13 5. 88e-13 2,,79e-13 5.,00e-17 2.66e-17 4. 02e-15
Pb 211 1,,09e-19 8,.99e-19 4..72e-18 1.,14e-17 2. 97e-17 2.,82e-16 3..79e-15 3. 98e-14 4..14e-13
Pb 210 1,,81e-17 3,.Ole-16 1,.20e-14 7..79e-14 5. 32e-13 3,.87e-ll 6,,54e-09 2. 62e-07 4. 42e-06
Pb 209 5 ,39e-19 5 .30e-20 1 .57e-19 3,.41e-19 8. 93e-19 1 .60e-17 3 ,66e-15 5. 71e-13 3,>12e-ll
Pb 208 4 .90e-13 1.41e-ll 4 .29e-10 1,.66e-09 4. 90e-09 2 .37e-08 3 .99e-08 4. 00e-08 1,.17e-06
Pb 207 1 .72e-16 4 .94e-15 1 .10e-13 4 .97e-13 2.,47e-12 1 .19e-10 1 .82e-08 1. 93e-06 3 .89e-03
Pb 206 1 •42e-20 1 .48e-18 4 .50e-16 5 .93e-15 8.,31e-14 3 .31e-ll 6 .64e-08 3. 37e-05 1 .24e-01
Tl 209 1 .31e-22 1 .29e-23 3 .82e-23 8 .29e-23 2..18e-22 3 .90e-21 8 .90e-19 1. 39e-16 7 .58e-15
Tl 208 8 .47e-18 8 .3Oe-17 5 .44e-16 8 .92e-16 9.,97e-16 4.73e-16 8 .47e-20 4..50e-20 6 .81e-18
Tl 207 1 .41e-20 1 .16e-19 6 .10e-19 1 .47e-18 3,.84e-18 3 .64e-17 4 .89e-16 5,.15e-15 5 •35e-14
He 4 2.50e-06 1.18e-05 3.24e-05 6.12e-05 1.31e-04 8.31e-04 6.19e-03 2.69e-02 9.63e-02
TOTAL 9.92e+02 9.92e+02 9.92e+02 9.92e+02 9.92e+02 9.92e+02 9.92e+O2 9.92e+02 9.92e+02

Page A.15
U02 Fuel - Fission Products Mass: g/kg inital 0

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

H 3 1.45e-05 1.37e-05 1.10e-05 8.27e-06 4.72e-06 5.29e-08 0.00e+00 0.0Oe+00 0.00e+00

Ge 72 1.44e-06 1.47e-06 1.47e-06 1.47e-06 1.47e-06 1.47e-06 1.47e-06 1.47e-06 1.47e-06

Ge 73 3.88e-06 3.89e-06 3.89e-06 3.89e-06 3.89e-06 3.89e-06 3.89e-06 3.89e-06 3.89e-06
Ge 74 l.O9e-05 1.09e-05 1.09e-05 1.09e-05 1.09e-05 1.09e-05 1.09e-05 1.09e-05 1.09e-05
Ge 76 8.26e-05 8.26e-05 8.26e-05 8.26e-05 8.26e-05 8.26e-05 8.26e-05 8.26e-05 8.26e-05

As 75 2.99e-05 2.99e-05 2.99e-05 2.99e-05 2.99e-05 2.99e-05 2.99e-05 2.99e-05 2.99e-05

Se 76 59e-07 2.62e-07 2.62e-07 62e-07 2.62e-07 2.62e-07 2.62e-07 2.62e-07 2.62e-07

Se 77 ,93e-04 1.95e-04 1.95e-04 ,95e-O4 1.95e-04 1.95e-04 1.95e-04 1.95e-04 1.95e-04
Se 78 .04e-04 5.,04e-04 5.04e-04 ,04e-04 5.04e-04 5.04e-04 5.04e-04 5.04e-04 5.04e-04
Se 79 .29e-03 1..29e-03 1.29e-03 .29e-O3 1.29e-O3 1.29e-03 1.28e-03 1.16e-03 3.00e-08
Se 80 .20e-03 3.,20e-03 3.20e-03 ,20e-03 3.2Oe-O3 3.2Oe-O3 3.2Oe-O3 3.2Oe-03 3.2Oe-O3
Se 82 7.87e-03 7.87e-03 7.87e-03 7.87e-O3 7.87e-O3 7.87e-O3 7.87e-03 7.87e-03 7.87e-03

Br 79 7.96e-09 2.18e-08 7.7Oe-O8 1.46e-07 2.84e-07 1.39e-06 1.37e-05 1.31e-04 1.29e-03

Br 81 5.32e-03 5.32e-03 5.32e-03 5.32e-03 5.32e-O3 5.32e-03 5.32e-03 5.32e-03 5.32e-03

Kr 80 7.40e-08 41e-08 7..41e-08 7.41e-08 7.41e-08 7.41e-08 7.41e-08 7.41e-08 7.41e-08

Kr 81 5.45e-09 45e 09 5..45e-09 5.45e-09 5.45e-09 5.45e-09 5.43e-09 5.27e-09 2.01e-10
Kr 82 8.00e-05 13e-05 8.13e-05 8.13e-O5 8.13e-05 8.13e-C5 8 13e-05 8.13e-05 8.13e-05
Kr 83 9.91e-03 92e-03 9.92e-03 9.92e-O3 9.92e-03 9.92e-03 9.92e-03 9.92e-03 9.92e-03
Kr 84 2. 44e-02 44e-02 2.44e-02 2.44e-O2 2.44e-02 2.44e-02 2.44e-02 2.44e-02 2.44e-02
Kr 85 5.98e-03 5.6U-03 4.33e-03 3.13e-O3 1.64e-03 9.3Oe-O6 0.00e+00 O.OOe+00 O.OOe+00
Kr 86 4.20e-02 4.20e-02 4.20e-02 4.20e-02 4.20e-02 4.20e-02 4.20e-02 4.2Oe-02 4.20e-02

Rb 85 2.25e-02 2.29e-02 2.42e-02 2.54e-O2 2.69e-02 2.85e-02 2.85e-02 2.85e-02 2.85e-02

Rb 86 6.20e-06 7.94e-12 0.00e+00 O.OOe+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+00
Rb 87 5.49e-02 5.49e-02 5.49e-02 5.49e-O2 5.49e-O2 5.49e-02 5.49e-02 5.49e-02 5.49e-02

Sr 86 60e-05 ,22e-05 3.22e-05 3.22e-05 3.22e-05 3.22e-O5 3.22e-05 3.22e-05 22e-05

Sr 87 41e-07 ,41e-07 4.41e-07 4.41e-O7 4.41e-O7 4.41e-07 4.42e-07 4.49e-07 ,25e-06
Sr 88 93e-02 .94e-02 7.94e-02 7.94e-02 7.94e-O2 7.94e-02 7.94e-02 7.94e-02 ,94e-02
Sr 89 84e-02 .89e-04 3.69e-13 4.78e-24 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00 .00e+00
Sr 90 1.29e-01 1.26e-01 1.15e-01 1.02e-01 8.02e-02 1.19e-02 5.92e-12 O.OOe+00 O.OOe+00

Y 89 7.71e-02 1.05e-01 1.06e-01 1.06e-01 1.06e-01 1.06e-01 1.06e-01 l.O6e-01 1.06e-01

Y 90 3.54e-05 3.16e-05 2.87e-O5 2.55e-05 2.01e-05 2.99e-06 1.49e-15 O.OOe+00 O.OOe+00
Y 91 4.31e-02 5.73e-04 1.74e-ll 6.99e-21 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Page A.16
U02 Fuel - Fission Products Mass: g/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10 4 Year 10« Year

Zr 90 1.10e-03 4.15e-03 ,56e-02 85e-02 00e-02 1..18e-01 ,30e-01 30e-01 .30e-01

Zr 91 9.43e-02 1.37e-01 ,38e-01 38e-01 38e-01 1..38e-01 .38e-01 38e-01 .38e-01
Zr 92 1.47e-01 .48e-01 ,48e-01 48e-01 48e-01 1..48e-01 .48e-01 48e-01 .48e-01
Zr 93 1.68e-01 .68e-01 ,68e-01 68e~01 68e-01 1..68e-01 .68e-01 67e-01 .07e-01
Zr 94 1.79e-01 .79e-01 .79e-01 79e-01 79e-01 1..79e-01 .79e-01 79e-01 .79e-01
Zr 95 6.78e-02 ,30e-03 ,73e-10 4.41e-19 87e-36 0.00e+00 0.00e+00 0.00e+00 0. OOe+00
Zr 96 1.89e-01 1.89e-01 1.89e-01 1.89e-01 1.89e-01 1.89e-01 1.89e-01 1.89e-01 1.89e-01

Nb 93 4.82e-09 1.18e-08 7.22e-O8 2.1Oe-O7 6.37e-07 ,23e-06 7.47e-05 7.58e-04 6.12e-02

Nb 93m 2.66e-08 9.57e-08 3.40e-07 5.82e-07 9.16e-07 .41e-06 1.42e-06 1.41e-06 9.01e-07
Nb 94 2.34e-07 2.34e-07 2.34e-07 2.34e-07 2.34e-07 .34e-07 2.26e-07 1.67e-07 3.46e-22
Nb 95 3.43e-02 1.60e-03 2.11e-10 5.38e-19 0.00e+00 .00e+00 0.00e+00 0.OOe+00 0.00e+00
Nb 95m 2.71e-05 5.42e-07 7.24e-14 1.85e-22 0.00e+00 0.OOe+00 0.00e+00 0.00e+00 0.00e+00

Mo 95 8.49e-02 1.84e-01 1.87e-01 1.87e-01 1.87e-01 1.87e-01 1.87e-01 1.87e-01 1.87e-01

Mo 96 1.35e-03 1.35e-03 1.35e-03 1.35e-03 1.35e-03 1.35e-03 1.35e-03 1.35e-03 1.35e-03
Mo 97 1.92e-01 1.93e-01 1.93e-01 1.93e-01 1.93e-01 1.93e-01 1.93e-01 1.93e-01 1.93e-01
Mo 98 1.96e-01 1.96e-01 1.96e-01 1.96e-01 1.96e-01 1.96e-01 1.96e-01 1.96e-01 1.96e-01
Mo 100 2.26e-01 2.26e-01 2.26e-01 2.26e-01 2.26e-01 2.26e-01 2.26e-01 2.26e-01 2.26e-01
Tc 99 2.01e-01 2.05e-01 2.05e-01 2.05e-01 2.05e-01 2.05e-01 2.04e-01 1.98e-01 7.90e-03
Ru 99 00e-07 8.67e-07 3.53e-06 86e-06 1.35e-05 68e-05 65e-0« 6.55e-03 97e-01
Ru 100 22e-03 7.22e-O3 7.22e-03 22e-03 7.22e-03 ,22e-O3 22e-O3 7.22e-O3 22e-03
Ru 101 89e-01 .89e-01 1.89e-01 89e-01 1.89e-01 89e-01 89e-01 1..89e-01 89e-01
Ru 102 80e-01 ,80e-01 1.80e-01 80e-01 1.80e-01 .80e-01 80e-01 1.,80e-01 80e-01
Ru 103 73e-O2 .51e-05 4.77e-16 4.80e-30 0.OOe+00 •OOe+00 00e+00 0.OOe+00 0. OOe+00
Ru 104 33e-01 .33e-01 1.33e-01 1.33e~01 1.33e-01 .33e-01 33e-01 1.33e-01 1.33e-01
Ru 106 6.54e-02 3.29e-02 2.10e-03 6.74e-05 6.96e-08 0.00e+00 0.00e+00 0.OOe+00 0. OOe+00

Rh 103 1.08e-01 1.55e-01 1.55e-01 1.55e-01 1.55e-01 1.55a-01 1.55e-01 1.558-01 1.55«-01
Rh 103m 4.23e-05 6.72e-08 4.26e-19 4.29e-33 0.OOe+00 0.OOe+00 0.00e+00 0.OOe+00 0.OOe+00
Rh 106 1.00e-07 3.09e-08 1.97e-09 6.34e-ll 6.54e-14 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Pd 104 1.78e-O2 1.78e-02 1.78e-02 1.78e-O2 1.78e-02 1.78e-02 1.78e-O2 1.78e-02 1.78e-O2
Pd 105 8.91e-O2 9.04e-02 9.04e-02 9.04e-02 9.04e-02 9.04e-02 9.04e-02 9.04e-02 9.04e-02
Pd 106 3.16e-02 6.Ale-02 9.49e-02 9.69e-02 9.70e-02 9.70e-02 9.70e-02 9.70e-02 9.70e-02
Pd 107 5.43e-O2 5.43e-O2 5.43e-02 5.43e-02 5.43e-02 5..43e-02 5.43e-O2 5.43e-O2 4.88e-02
Pd 108 3.68e-02 3.68e-02 3.68e-02 3.68e-02 3.68e-02 3..68e-02 3.68e-02 3.68e-02 3.68e-O2
Pd 110 1.04e-02 1.04e-02 1.04e-02 1.04e-02 l.OAe-02 1.04e-02 1.04e-02 1.04e-02 1.04e-02

Page A. 17
uo 2 Fuel - Fission Products Mass: inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Ag 107 1.42e-09 7.22e-09 3.04e-08 5. 94e-08 1. 17e-O7 5. 81e-07 5. 79e-O6 5.79e-O5 5.49e-O3
Ag 108 6. 40e-15 9. 59e-19 9. 39e-19 9. 13e-19 8.65e-19 5. 59e-19 4. lle-21 0.OOe+00 0.OOe+00
Ag 108m 3.05e-10 3.04e-10 2. 97e-10 2.89e-10 2.74e-10 1. 77e-10 1.3Oe-12 6.02e-34 0.OOe+00
Ag 109 2. lle-02 2. 12e-02 2. 12e-02 2. 12e-02 2. 12e-02 2. 12e-02 2. 12e-02 2. 12e-O2 2. 12e-O2
Ag 109m 1.09e-07 2.03e-19 2. 29e-20 1. 50e-21 6. 39e-24 0. 00e+00 0.00e+00 0.OOe+00 0.OOe+00
Ag 110 1. 21e-08 4. 75e-13 8. 26e-15 5. 21e-17 2.O7e-21 0. 00e+00 0. 00e+00 0. OOe+00 0.OOe+00
Ag 110m 8. 64e-05 3. 14e-05 5. 45e-07 3.44e-09 1.37e-13 0. 00e+00 0.00e+00 0.OOe+00 0.OOe+00
Ag 111 3. 37e-04 5.88e-19 0. OOe+00 0. 00e+00 0. 00e+00 0. 00e+00 0.00e+00 0.OOe+00 0.OOe+00
Cd 108 3. 34e-10 3. 34e-10 3. 34e-10 3. 35e-10 3.36e-10 3.45e-10 3.60e-10 3.60e-10 3.60e-10
Cd 109 3. 55e-13 2.06e-13 2. 32e-14 1. 52e-15 6.47e-18 7. lle-37 0.00e+00 0. OOe+00 0. OOe+00
Cd 110 2.57e-03 2.62e-03 2. 65e-03 2.65e-03 2.65e-03 2.65e-03 2.65e-03 2.65e-03 2.65e-03
Cd 111 4. 49e-03 4.83e-03 4. 83e-03 4.83e-03 4.83e-O3 4.83e-03 4.83e-03 4.83e-03 4.83e-03
Cd 112 2. 16e-03 2.18e-03 2. 18e-03 2.18e-03 2.18e-03 2. 18e-03 2.18e-03 2.18e-03 2.18e-03
Cd 113 3..15e-05 3.,44e-05 3. 44e-05 3.44e-05 3.44e-05 3.44e-05 3.44e-05 3.44e-05 3.44e-05
Cd 113m 3.,28e-05 3.,12e-05 2. 54e-05 1.97e-05 1.18e-05 2.Ole-07 2.39e-27 0.OOe+00 0.,OOe+00
Cd 114 2.,64e-03 2.,64e-03 2. 64e-03 2.64e-03 2.64e-03 2.64e-03 2.64e-03 2.64e-03 2.,64e-03
Cd 115m 2.,67e-05 9..14e-08 1.,26e-17 5.91e-30 0. 00e+00 0. 00e+00 0. 00e+00 0. OOe+00 0..OOe+00
Cd 116 8..69e-04 8..69e-04 8.,69e-04 8. 69e-04 8. 69e-04 8. 69e-04 8. 69e-04 8. 69e-04 8.,69e-04
In 113 4 .14e-07 2 .04e-06 7,.79e-06 1..35e-05 2..14e-05 3., 3Oe-O5 3.,32e-O5 3.,32e-O5 3..32e-05
In 114 7 .17e-14 2,.46e-16 3..21e-25 0..00e+00 0..00e+00 0.,00e+00 0..00e+00 0.,OOe+00 0,.OOe+00
In 114m 2 .54e-09 1 .53e-ll 1,.99e-20 1..57e-31 0,.00e+00 0,.00e+00 0..00e+00 0,.OOe+00 0 .OOe+00
In 115 6 .lle-04 6 •54e-04 6 .54e-04 6..54e-04 6..54e-04 6.. 54e-04 6 .54e-04 6,.54e-04 6 .54e-04
In 115m 1 .21e-06 3 .69e-14 5 .06e-24 0,.00e+00 0,.00e+00 0,.00e+00 0 .OOe+00 0,.OOe+00 0 .OOe+00
Sn 114 3 .57e-09 5 .98e-09 5 .99e-09 5 .99e-09 5 .99e-09 5 .99e-09 5 •99e-09 5.99e-O9 5 .99e-09
Sn 115 2 .93e-05 2 .99e-05 2 .99e-05 2 .99e-05 2 .99e-05 2 .99e-05 2 .99e-05 2 .99e-O5 2 .99e-05
Sn 116 2 ,42e-04 2 .42e-04 2 .42e-04 2 .42e-04 2 .42e-04 2 .42e-04 2 .42e-04 2 .42e-04 2 .42e-04
Sn 117 8 .74e-04 8 •75e-04 8 .75e-04 8 •75e-04 8 .75e-04 8 . 75e-04 8 .75e-O4 8 .75e-04 8 .75e-04
Sn 117m 3 .68e-08 5 •15e-16 0 .00e+00 0 •OOe+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Sn 118 9 .08e-0A 9 .08e-04 9 .08e-04 9 .08e-04 9 .08e-04 9 .08e-04 9 .08e-O4 9 .08e-04 9 •08e-04
Sn 119 8 .97e-04 9 .04e-04 9 •08e-04 9 .08e-04 9 .08e-04 9 .08e-04 9 .08e-04 9 .08e-04 9 .08e-04
Sn 119m 1 .04e-05 3.70e-06 5 •93e-08 3 .38e-10 1.10e-14 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Sn 120 9 .32e-O4 9 .32e-04 9 .32e-04 9 .32e-04 9 .32e-O4 9 .32e-O4 9 .32e-04 9 .32e-04 9 .32e-04
Sn 121m 7 .26e-07 7.17e-07 6 .82e-07 6 .40e-07 5 .65e-07 2.O6e-O7 2.44e-12 0 .OOe+00 0 .OOe+00
Sn 122 1 .04e-03 1.04e-03 1 .OAe-03 1 .04e-03 1.OAe-03 1.04e-03 1•04e-03 1.04e-03 1 .04e-03
Sn 123 1 .77e-04 2 .49e-05 9 .82e-09 5 .45e-13 1.68e-21 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Sn 124 1 .56e-03 1.56e-03 1.56e-03 1.56e-03 1.56e-O3 1,56e-O3 1 .56e-03 1.56e-03 1.56e-03
Sn 125 9>.94e-05 3.90e-16 0 .00e+00 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0i. OOe+00
Sn 126 4 .94e-03 4 ,94e-03 4 .94e-03 4 .94e-03 4 .94e-03 4 .94e-03 4 ,91e-03 4 .61e-03 4 .83e~O6
Page A.18
U02 Fuel - Fission Products Mass: inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 10 6 Year

Sb 121 9.72e-04 9.81e-04 9.81e-04 9.81e-04 9.81e-04 9.82e-04 9.82e-04 9.82e-04 9.82e-04
Sb 123 1.04e-03 1.19e-03 1.22e-03 1.22e-03 1.22e-03 1.22e-03 1.22e-03 1.22e-03 1.22e-03
Sb 124 6.36e-06 9.47e-08 4. 68e-15 3.45e-24 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Sb 125 2. 75e-03 2. 22e-03 8.15e-04 2. 33e-04 1.91e-05 3.86e-14 0.OOe+00 0.OOe+00 0.OOe+00
Sb 126 8.71e-06 2. 35e-10 2. 35e-10 2. 35e-10 2.35e-10 2. 35e-10 2. 33e-10 2. 19e-10 2. 29e-13
Sb 126m 7.93e-09 1.79e-12 1.79e-12 1.79e-12 1.79e-12 1.78e-12 1.77e-12 1.67e-12 1.74e-15

Te 122 1.43e-05 1.49e-05 1.49e-05 1.49e-05 1.49e-05 1.49e-05 1.49e-05 1.49e-05 1.49e-05
Te 123 3.54e-08 4. 98e-08 5.18e-08 5.18e-08 5.18e-08 5.18e-08 5.18e-08 5.18e-08 5.18e-08
Te 123m 1.63e-08 1.97e-09 4. 17e-13 1.06e-17 6.93e-27 0.00e+00 0.OOe+00 0.OOe+00 0.OOe+00
Te 124 6.15e-06 1.24e-05 1.25e-05 1.25e-O5 1.25e-05 1.25e-05 1.25e-05 1.25e-05 1.25e-05
Te 125 1.61e-04 7.83e-04 2. 20e-03 2. 79e-O3 3.01e-03 3.O3e-O3 3.03e-03 3.O3e-O3 3.O3e-O3
Te 125m 2. 18e-05 3.08e-05 1.14e-05 3.26e-06 2.67e-07 5.39e-16 0.OOe+00 0.OOe+00 0.OOe+00
Te 126 1.31e-04 1.39e-04 1.39e-04 1.40e-04 1.40e-04 1.43e-04 1.73e-04 4. 70e-04 5.08e-03
Te 127 3.72e-05 3.47e-07 3.20e-ll 2.89e-16 2.36e-26 0.00e+00 0.OOe+00 0.OOe+00 0.OOe+00
Te 127m 9.56e-04 9.92e-05 9.15e-09 8.26e-14 6.75e-24 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Te 128 2..49e-02 2.,49e-02 2.,49e-02 2. 49e-02 2. 49e-02 2. 49e-02 2. 49e-02 2. 49e-02 2. 49e-02
Te 129 .58e-05 7..95e-10 6.,45e-23 0.. OOe+00 0.,OOe+00 0..OOe+00 0.. OOe+00 0..OOe+00 0.,OOe+00
Te 129m 1..58e-03 8.,49e-07 6.,89e-20 2. 98e-36 0.,00e+00 0.. OOe+00 0.,OOe+00 0..OOe+00 0.,OOe+00
Te 130 8..48e-02 8,.48e-02 8.,48e-02 8,,48e-02 8.,48e-02 8..48e-02 8..48e-02 8 .48e-02 8..48e-02
I 127 1,.09e-02 1,.22e-02 1,.23e-02 1,.23e-O2 1,.23e-02 1..23e-02 1,.23e-02 1,.23e-02 1..23e-02
I 129 4 .31e-O2 4 .48e-02 4 .48e-02 4 .48e-02 4 .48e-02 4 .48e-02 4 .48e-02 4 .48e-02 A .28e-02
I 131 7.79e-03 1.69e-16 0.00e+00 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0,.OOe+00

Xe 128 1.37e-04 1•37e-04 1.37e-04 1.37e-04 1.37e-04 1.37e-O4 1.37e-04 1.37e-04 1.37e-04
Xe 129 3.O5e-O7 3.34e-07 3.41e-07 3.51e-O7 3•71e-07 5.29e-07 2.31e-06 2.Ole-05 1.93e-03
Xe 130 1.18e-04 1.18e-04 1.18e-04 1.18e-04 1.18e-04 1.18e-04 1.18e-04 1.18e-04 1.18e-04
Xe 131 1.22e-01 1.30e-01 1.30e-01 1.30e-01 1.30e-01 1.30e-01 1.30e-01 1•30e-01 1.30e-01
Xe 131m 1.29e-04 2.32e-13 0 .00e+00 0 .00e+00 0.OOe+000.00e+00 0.OOe+00 0 .OOe+00 0.OOe+00
Xe 132 2.26e-01 2,31e-01 2.31e-01 2.31e-01 2.31e-01 2.31e-01 2.31e-01 2.31e-01 2.31e-01
Xe 134 3.51e-01 3.51e-01 3.51e-01 3.51e-01 3.51e-01 3.51e-01 3.51e-01 3.51e-01 3.51e-01
Xe 136 6.02e-01 6.02e-01 6.02e-0l 6.02e-01 6.02e-01 6,02e-01 6.02e-01 6.02e-01 6.02e-01
Cs 133 2.90e-01 3.01e-01 3.01e-01 3.01e-01 2.Qle-01 3.01e-01 3.Ole-01 3.Ole-01 3.Ole-01
Cs 134 1.Ve-Ci 8.36e-03 2.18e-03 4.06e-04 1.41e-05 2,94e-17 0.OOe+00 0.00«+00 0.OOe+00
Cs 135 2.32e-O2 2.37e-O2 2.37e-O2 2.37e-O2 2.37e-O2 2,37e-02 2.37e-02 2.37e-02 1.76e-02
Cs 136 3•07e-04 1.24e-12 0.00e+00 0.00e+00 0.OOe+00 3.00e+00 0.OOe+00 0.OOe+00 0.OOe+00
Cs 137 3.Ole-01 2.94e-01 2.68e-01 2.39e-01 1.90e-01 3.O3e-O2 3.16e-ll 0.OOe+00 0 .OOe+00

Page A.19
uo 2, Fuel - Fission Products Mass: g/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 10 6 Year

Ba 134 8.07e-04 4.15e-03 l.O3e-O2 1.21e-02 1.25e-02 1.,25e-02 1.25e-02 1.25e-O2 1.25e-02
Ba 135 1.65e-06 1.66e-06 1.69e-06 1.73e-06 1.80e-06 2.,37e-O6 8.81e-06 7.31e-05 6.18e-03
Ba 136 2.13e-03 2.44e-03 2.44e-03 2.44e-03 2.44e-03 2.,446-03 2.44e-03 2.44e-03 2.44e-03
Ba 136m 1.37e-ll 5.51e-20 0.00e+00 0.00e+00 0.00e+00 0.,00e+00 0.00e+00 0 .00e+00 0 .00e+00
Ba 137 2.21e-03 9.05e-03 3.49e-02 6.4Oe-O2 1.13e-01 2.73e-01 3.03e-01 3•03e-01 3.03e-01
Ba 137m 4.64e-08 4.48e-08 4.08e-08 3.64e-O8 2.89e-08 4.60e-09 4.81e-18 0.00e+00 0 .00e+00
Ba 138 3.00e-01 3.00e-01 3.00e-01 3.00e-01 3.00e-01 3..00e-01 3.00e-01 3.00e-01 3.00e-01
Ba 140 2.25e-02 5.69e-ll 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
La 138 1.97e-06 1.97e-06 1.97e-06 1.97e-06 1.97e-06 1.97e-O6 1.97e-06 1.97e-06 1.97e-06
La 139 2.90e-01 2.90e-01 2.90e-01 2.90e-01 2.90e-01 2.90e-01 2.90e-01 2.90e-01 2.90e-01
La 140 3.15e-03 8.58e-12 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0 .00e+00 0 .00e+00

Ce 140 2.79e-01 3.05e-01 3.05e-01 3.05e-01 3.05e-01 3.05e-01 3.05e-01 3 .05e-01 3.05e-01
Ce 141 5.42e-02 2.26e-05 6.68e-19 8.19e-36 0.00e+00 0.00e+00 0.00e+00 0 .00e+00 0.00e+00
Ce 142 2.71e-01 2.71e-01 2.71e-01 2.71e-01 2.71e-01 2.71e-01 2.71e-01 2,.71e-01 2.71e-01
Ce 144 1.78e-01 7.32e-02 2.08e-03 2.42e-O5 3.28e-09 0.00e+00 0,.00e+00 0,.00e+00 0 .00e+00

Pr 141 2.14e-01 2.69e-01 2.69e-01 2.69e-01 2.69e-01 2.69e-01 2,.69e-01 2,.69e-01 2 .69e-01
Pr 143 2.02e-02 1.75e-10 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0,.00e+00 0,.00e+00 0 .00e+00
Pr 144 7.83e-06 3.09e-06 8.77e-08 1.02e-09 1.39e-13 0.00e+00 0,.00e+00 0..00e+00 0,.00e+00
Pr 144m 3.78e-08 1.55e-O8 4.39e-10 5.11e-12 6.93e-16 0.00e+00 0,.00e+00 0..00e+00 0,.00e+00

Nd 142 2.17e-03 2.19e-03 2.19e-03 2.19e-03 2.19e-03 2.19e-03 2,.19e-03 2.,19e-03 2..19e-03
Nd 143 1.83e-01 2.05e-01 2.05e-01 2.05e-01 2.05e-01 2.05e-01 2.,05e-01 2.,05e-01 2.,05e-01
Nd 144 1.17e-01 2.23e-01 2.94e-01 2.96e-01 2.96e-01 2.96e-01 2.,96e-01 2..96e-01 2.,96e-01
Nd 145 1.70e-01 1.70e-01 1.70e-01 1.70e-01 1.70e-01 1.70e-01 1.,70e-01 1.,70e-01 1.,70e-01
Nd 146 1.51e-01 1.51e-01 1.51e-01 1.51e-01 1.51e-01 1.51e-01 1..51e-01 1.,51e-01 1.,51e-01
Nd 147 7.59e-03 8.67e-13 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Nd 148 8.73e-02 8.73e-02 8.73e-02 8.73e-02 8.73e-02 8.73e-02 8.73e-02 8.73e-02 8.73e-02
Nd 150 4.25e-02 4.25e-02 4.25e-02 4.25e-02 4.25e-02 4.25e-02 4.25e-02 4.25e-02 4.25e-02
Pm 147 7.49e-02 6.34e-02 2.20e-02 5.88e-03 4.19e-04 2.76e-13 0.00e+00 0.00e+00 0.00e+00
Pm 148 5.84e-04 4.76e-09 1.07e-19 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Pm 148m 2.99e-04 6-50e-07 1.46e-17 7.09e-31 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Sm 147 6.06e-03 2.52e-02 6.66e-02 8.28e-02 8.82e-02 8.86e-02 8.86e-02 8.86e-02 8.86e-02
Sm 148 9.45e-03 1.03e-02 1.03e-02 1.03e-02 l.O3e-02 1.03e-02 1.03e-02 1.03e-02 1.03e-02
Sm 149 5.65e-04 1.79e-O3 1.79e-03 1.79e-03 1.79e-03 1.79e-O3 1.79e-03 1.79e-03 1.79e-03
Sm 150 6.86e-02 6.86e-02 6.86e-02 6.86e-02 6.86e-02 6.86e-O2 6.86e-02 6.86e-02 6.86e-02
Sm 151 2.23e-O3 2.47e-O3 2.4Oe-O3 2.3Oe-O3 2.13e-O3 1.15e-03 1.12e-06 0.00e+00 0.00e+00
Page A.20
U0 2 Fuel - Fission Products Mass: g/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Sm 152 4.4Oe-02 4.40e-02 4.40e-02 4.40e-02 4.40e-02 4.40e-02 4.40e-02 4.40e-02 4.40e-02
Sm 154 8.74e-03 8.75e-03 8.75e-03 8.75e-03 8.75e-03 8.75e-O3 8.75e-03 8.75e-03 8.75e-03

Eu 151 7.68e-07 ,99e-05 48e-05 85e-04 3.56e-04 •34e-03

2.49e-03 2.49e-03 2.49e-03
Eu 152 1.87e-06 ,78e-06 ,45e-06 12e-06 6.76e-07 , 15e-O8
1.37e-28 0.00e+00 O.OOe+00
Eu 153 1.99e-02 ,05e-02 ,05e-02 05e-02 2.05e-02 ,05e-O2
2.05e-02 2.05e-02 2.05e-02
Eu 154 4.17e-03 .84e-03 ,78e-03 86e-O3 8.31e-04 .32e-O6
O.OOe+00 O.OOe+00 O.OOe+00
Eu 155 1.86e-03 .61e-03 ,23e-04 4.59e-04 1.13e-04 .58e-09
0.00e+00 O.OOe+00 O.OOe+00
Eu 156 1.51e-03 8.80e-ll 0.00e+00 0.00e+00 O.00e+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00

Gd 152 2.04e-06 2.08e-06 2.17e-06 26e-06 2.39e-06 2.57e-O6 2.57e-O6 2.57e-O6 2.57e-06
Gd 153 2.55e-O7 8.94e-08 1.35e-09 16e-12 2.01e-16 O.OOe+00 0.00e+00 O.OOe+00 O.OOe+00
Gd 154 6.61e-05 3.89e-04 1.45e-03 37e-03 3.40e-03 4.23e-03 4.23e-O3 4.23e-03 4.23e-03
Gd 155 2.39e-06 2.45e-04 9.36e-04 40e-03 1.75e-03 1.86e-03 1.86e-O3 1.86e-03 1.86e-03
Gd 156 7.55e-03 9.07e-03 9.07e-03 9.07e-03 9.07e-03 9.07e-03 9.07e-03 9.07e-03 9.07e-03
Gd 157 9.52e-06 2.13e-05 2.13e-O5 2.13e-O5 2.13e-05 2.13e-O5 2.13e-O5 2.13e-O5 2.13e-05
Gd 158 3.10e-03 3.10e-03 3.10e-03 3.10e-03 3.10e-03 3.1Oe-O3 3.10e-O3 3.1Oe-03 3.1Oe-O3
Gd 160 2.40e-04 2.4Oe-04 2.40e-04 2.40e-04 2.40e-04 2.40e-04 2.40e-04 2.40e-04 2.40e-04

Tb 159 5.26e-04 5.31e-04 5.31e-04 5.31e-04 5.31e-O4 5.31e-O4 5.31e-O4 5.31e-04 5.31e-04
Tb 160 1.07e-05 3.23e-07 2.66e-13 6.62e-21 4.09e-36 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+00

Dy 160 6.87e-06 1.73e-05 1.76e-05 1.76e-O5 1.76e-05 1.76e-05 1.76e-O5 1.76e-05 1.76e-05
Dy 161 7.64e-05 8.45e-05 8.45e-05 8.45e-O5 8.45e-05 8.45e-O5 8.45e-O5 8.45e-05 8.45e-05
Dy 162 7.74e-05 7.74e-05 7.74e-05 7.74e-O5 7.74e-O5 7.74e-O5 7.74e-05 7.74e-05 7.74e-05
Dy 163 3.60e-05 3.60e-05 3.60e-05 3.60e-O5 3.60e-05 3.6Oe-O5 3.6Oe-O5 3.60e-05 3.6Oe-O5
Dy 164 4.86e-06 4.87e-06 4.87e-06 4.87e-O6 4.87e-06 4.87e-06 4.87e-O6 4.87e-06 4.87e-06

Ho 165 1.15e-05 1.15e-O5 l.l5e-05 1.15e-O5 1.15e-O5 1.15e-05 1.15e-05 1.15e-05 1.15e-05
Ho 166m 2.07e-08 2.06e-08 2.06e-08 2.05e-08 2.04e-08 1.95e-08 1.16e-08 6.4Oe-ll O.OOe+00

Er 166 1.59e-06 1.64e-06 1.64e-06 1.64e-O6 1.64e-06 1.64e-O6 1.65e-06 1.66e-06 1.66e-06
Er 167 2.49e-08 2.49e-08 2.49e-08 2.49e-O8 2.49e-08 2.49e-O8 2.49e-O8 2.49e-08 2.49e-08

TOTAL 8.12e+00 8.12e+00 8.12e+0O 8.12e+OO 8.12e+00 8.12e+OO 8.12e+00 8.12e+00 8.12e+00

Page A.21
U02 Fuel - Actinides Activity: Bq/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Es 253 7.66e-04 5.70e-08 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Cf 254 8.95e-07 9.58e-09 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Cf 253 2.25e-03 1.50e-09 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Cf 252 2.13e-02 1.64e-02 5.74e-03 1.54e-03 l.lle-04 8.33e-14 O.OOe+00 O.OOe+00 O.OOe+00
Cf 251 1.40e-04 1.40e-04 1.39e-04 1.39e-04 1.38e-04 1.30e-04 6.48e-05 6.22e-08 O.OOe+00
Cf 250 3.89e-02 3.74e-02 3.03e-02 2.33e-O2 1.37e-O2 1.97e-04 1.05e-10 4.26e-ll O.OOe+00
Cf 249 2.57e-04 4.77e-03 8.33e-03 8.40e-03 8.21e-03 7.03e-03 1.18e-03 2.22e-ll O.OOe+00

Bk 250 2.04e+01 1.16e-10 1.16e-10 1.16e-10 1.16e-10 1.15e-10 1.05e-10 4.26e-ll O.OOe+00
Bk 249 3.30e+00 1.50e+00 6.33e-02 1.21e-03 4.44e-07 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Cm 250 8.29e-10 8.29e-10 8.29e-10 8.29e-10 8.25e-10 8.18e-10 7.47e-10 3.03e-10 O.OOe+00
Cm 248 2.53e-03 2.53e-03 2.53e-03 2.53e-O3 2.53e-03 2.53e-O3 2.53e-03 2.48e-03 3.28e-04
Cm 247 2..23e-03 2.23e-03 2..23e-03 2..23e-O3 2.23e-03 ,23e-03 2.23e-03 2.23e-03 2.14e-03
Cm 246 2.,13e+03 2.13e+03 2..13e+03 2..13e+O3 2.13e+03 lle+03 .84e+03 4.92e+02 O.OOe+00
Cm 245 1..22e+04 1.22e+04 1..22e+O4 1..22e+O4 1.22e+04 ,22e+O4 ,13e+04 5.44e+03 O.OOe+00
Cm 244 6..48e+08 6.33e+08 5.,40e+08 4..48e+08 3.05e+08 43e+07 .56e-08 O.OOe+00 O.OOe+00
Cm 243 6..66e+06 6.51e+06 5..92e+06 5..22e+06 4.11e+06 5.85e+05 ,82e-04 O.OOe+00 O.OOe+00
Cm 242 4.77e+10 1.03e+10 2.76e+07 6.66e+06 6.33e+06 4.40e+06 7.25e+04 1.09e-13 O.OOe+00

Am 245 3.29e+05 2.25e-05 9.51e-07 1.82e-08 6.66e-12 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Am 243 1.93e+07 1.94e+07 1.94e+07 1.94e+07 1.94e+07 1.92e+O7 1.76e+07 7.59e+06 2.14e-03
Am 242 2.70e+ll 8.36e+O6 8.21e+06 8.03e+06 7.66e+O6 5.33e+06 8.77e+04 1.31e-13 O.OOe+00
Am 242m 8.44e+06 8.40e+06 8.25e+06 8.07e+06 7.70e+06 5.33e+06 8.81e+04 1.32e-13 O.OOe+00
Am 241 2.15e+08 1.56e+09 6.33e+09 l.lle+10 1.77e+10 2.56e+10 6.11e+09 8.73e+03 O.OOe+00

Pu 244 62e-01 5.62e-01 5.62e-01 5.62e-01 5.62e-01 5.62e-01 5.62e-01 5.62e-01 5.59e-01
Pu 243 42e+12 2.23e-03 2.23e-O3 2.23e-O3 2.23e-03 2.23e-03 2.23e-03 2.23e-03 2.14e-03
Pu 242 ,81e+06 8.81e+06 8.81e+06 8.81e+O6 8.81e+06 8.81e+06 8.81e+06 8.66e+06 1.39e+O6
Pu 241 ,58e+ll 8.18e+ll 6.77e+ll 5.37e+ll 3.34e+ll 7.66e+09 1..13e+04 5.44e+03 O.OOe+00
Pu 240 ,70e+09 8.70e+09 8.70e+09 8.70e+09 8.66e+09 8.62e+09 7..81e+09 3.01e+09 5.59e-01
Pu 239 .O7e+O9 6.,36e+09 6.36e+09 6.36e+09 6.36e+09 6.33e+09 6..18e+09 4.77e+09 4..lle-03
Pu 238 ,92e+09 3.,21e+09 3.16e+09 3.04e+09 2.81e+09 1.50e+09 1.,30e+06 2.59e-13 0..OOe+00
Pu 236 7.77e+05 6.18e+05 2.34e+05 6.96e+04 6.lle+03 2.18e-05 O.OOe+00 O.OOe+00 O.OOe+00

Np 240 3.14e+12 6.18e-04 6.18e-04 6.18e-04 6.18e-04 6.18e-04 6.18e-04 6.18e-04 6.14e-04
Np 240m 5.62e-01 5.62e-01 5.62e-01 5.62e-01 5.62e-01 5.62e-01 5.62e-01 5.62e-01 5.59e-01
Np 239 9.92e+14 1.94e+07 1.94e+07 1.94e+O7 1.94e+07 1.92e+07 1.76e+07 7.59e+06 2.14e-03

Page A.22
U0 2 Fuel - Actinides Activity: Bq/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Np 238 1.83e+12 4.03e+04 3.96e+04 3.89e+04 3.70e+04 2.56e+04 4.22e+O2 O.OOe+00 O.OOe+00
Np 237 9.25e+05 9.92e+05 9.99e+05 l.Ole+06 1.06e+06 1.69e+06 5.70e+06 6.92e+06 5.00e+06

U 240 62e-01 5.62e-01 5.62e-01 62e-01 62e-01 62e~01 62e-01 62e-01 5.59e-01
U 238 22e+07 22e+07 22e+O7 22e+07 22e+07 22e+07 22e+O7 22e+07 1.22e+O7
U 237 59e+12 05e+07 69e+07 34e+07 8.36e+06 92e+05 83e-01 36e-01 O.OOe+00
U 236 84e+06 84e+06 84e+06 84e+06 .84e+06 86e+06 08e+06 42e+06 4.14e+06
U 235 61e+05 ,61e+05 61e+05 61e+05 .61e+05 62e+05 67e+O5 16e+05 3.77e+O5
U 234 9.88e+06 ,88e+06 92e+06 95e+06 .Ole+07 05e+07 lle+07 lle+07 1.22e+O7
U 233 3.32e+01 ,77e+01 55e+01 73e+01 .22e+02 99e+02 69e+O4 2.83e+05 5.33e+06
U 232 3.92e+03 1.07e+04 2.52e+04 3.03e+04 2.99e+04 1.39e+04 2.41e+00 O.OOe+00 O.OOe+00
Pa 234 3.11e+04 1.96e+04 1.96e+04 1.96e+04 1.96e+04 1.96e+04 1.96e+04 1.96e+04 1.96e+04
Pa 234m 1.23e+07 1.22e+O7 1.22e+07 1.22e+07 1.22e+07 1.22e+07 1.22e+O7 1.22e+07 1.22e+O7
Pa 233 7.4Oe+O5 9.92e+O5 9.99e+05 1.01e+06 1.06e+06 1.69e+06 5.70e+06 6.92e+06 5.00e+06
Pa 231 1.94e+01 2.3Oe+Ol 3.67e+01 5.37e+01 8.77e+01 3.61e+02 3.46e+03 3.64e+04 3.77e+05
Th 234 22e+07 22e+07 1.22e+07 1.22e+07 22e+07 1.22e+O7 22e+O7 1.22e+07 1.22e+07
Th 232 37e-O5 24e-04 4.88e-04 9.40e-04 85e-03 9.18e-03 69e-02 1.37e+OO 2.06e+02
Th 231 88e+06 61e+05 1.61e+05 1.61e+05 ,61e+05 1.62e+05 67e+05 2.16e+05 3.77e+O5
Th 230 A8e+01 44e+02 5..OOe+02 9.47e+02 ,85e+03 9.29e+03 84e+04 9.55e+05 1.25e+07
Th 229 66e-03 9.03e-03 2..68e-02 5.81e-02 ,52e-01 2.73e+OO 6.25e+O2 9.73e+04 5.33e+06
Th 228 74e+O2 2.52e+03 1..65e+04 2.70e+04 .03e+04 1.43e+04 2.57e+OO 1.37e+OO 2.06e+02
Th 227 1.18e-01 8.10e-01 4.26e+00 1.02e+01 2.68e+01 2.54e+O2 3.41e+03 3.59e+04 3.74e+05

Ac 228 9.1Oe-O7 9.88e-06 1.29e-04 4.03e-04 1.16e-03 9.18e-03 9.69e-02 1.37e+OO 2.06e+02
Ac 227 1.58e-01 8.21e-01 4.29e+00 1.04e+01 2.71e+01 2.58e+02 3.46e+03 3.64e+04 3.77e+05
Ac 225 9.18e-02 9.03e-03 2.68e-02 5.81e-02 1.52e-01 2.73e+OO 6.25e+02 9.73e+04 5.33e+06

Ra 228 9.1Oe-O7 9.88e-06 1.29e-04 4.03e-04 1.16e-03 9.18e-03 9.69e-02 1.37e+00 2.06e+02
Ra 226 8.10e-03 5.11e-02 6.lle-01 2.18e+00 8.21e+00 1.97e+02 1.85e+O4 7.40e+05 1.25e+07
Ra 225 1..lle-01 9.03e-03 2.68e-02 5.81e-02 1.52e-01 2.73e+OO 6.25e+O2 9.73e+04 5.33e+06
Ra 224 2..57e+O2 2.52e+03 1.65e+04 2.70e+04 3.03e+04 1.43e+04 2.57e+OO 1.37e*OO 2.06e+02
Ra 223 9.99e-02 8.21e-01 4.33e-f00 1.04e+01 2.71e+01 2.58e+02 3.46e+O3 3.64e+04 3.77e+05

Fr 223 2.18e-03 1.13e-02 5.96e-02 1.43e-01 3.74e-01 3.55e+00 4.77e+01 5.03e+02 5.22e+03
Fr 221 9.18e-O2 9.03e-03 2.68e-02 5.81e-02 1.52e-01 2.73e+00 6.25e+O2 9.73e+04 5.33e+06

Rn 222 7.77e-03 5.11e-02 6.lle-01 2.18e+0O 8.21e+OO 1.97e+02 1.85e+04 ?.40e+05 1.25e+07
Rn 220 2.57e+02 2.52e+03 1.65e+04 2.7Oe+O4 3.03e+04 1.43e+04 2.57e+OO 1.37e+OO 2.06e+02
Rn 219 9.99e-02 8.21e-01 4.33e+00 1.04e+01 2.71e+01 2.58e+02 3.46e+03 3.64e+04 3.77e+O5
Page A.23
 Fuel - Actinides Activity: Bq/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

At 217 9.18e-02 9.03e-03 2.68e-02 5.81e-02 1.52e-01 2.73e+OO 6.25e+O2 9.73e+04 5.33e+06

Po 218 77e-O3 5.11e-02 lle-01 18e+00 8.21e+00 ,97e+02 85e+04 40e+05 ,25e+07
Po 216 57e+02 2.52e+03 65e+04 70e+04 3.03e+04 43e+04 ,57e+OO 37e+OO 06e+02
Po 215 99e-02 8.21e-01 33e+00 04e+01 2.71e+01 ,58e+02 .46e+03 64e+04 .77e+O5
Po 214 77e-03 5.11e-O2 ,07e-01 17e+00 8.21e+00 ,97e+O2 .85e+04 40e+05 ,25e+07
Po 213 8.99e-02 8.84e-03 ,62e-02 .70e-02 1.49e-01 .67e+00 6.11e+02 9.51e+04 .22e+06
Po 212 .65e+02 .61e+03 .06e+04 .73e+04 1.94e+04 .18e+03 1.65e+00 8,73e-01 .32e+02
Po 211 .80e-04 .3Oe-O3 .21e-02 .90e-02 7.59e-02 ,22e-01 9.69e+00 l.O2e+O2 .06e+03
Po 210 1.06e-05 3.85e-04 3.39e-02 2.20e-01 1.50e+00 1.10e+02 1.85e+04 7.40e+05 1.25e+07

Bi 214 7.77e-03 5.11e-02 6.07e-01 2.18e+0O 8.21e+OO 1.97e+O2 1.85e+04 7.40e+05 1.25e+07
Bi 213 9.18e-02 9.03e-03 2.68e-02 5.81e-02 1.52e-01 2.73e+OO 6.25e+02 9.73e+04 5.33e+06
Bi 212 2.57e+02 2.52e+03 1.65e+04 2.70e+04 3.03e+04 1.43e+04 2.57e+00 1.37e+00 2.06e+02
Bi 211 9.99e-02 8.21e-01 4.33e+00 1.04e+01 2.71e+01 2.58e+02 3.46e+03 3.64e+04 3.77e+O5
Bi 210 4.66e-05 8.51e-04 3.39e-02 2.20e-01 1.50e+00 1.10e+02 1.85e+04 7.40e+05 1.25e+07

Pb 214 7.77e-03 5.11e-02 6.07e-01 2.18e+00 8.21e+00 1.97e+O2 1.85e+04 7.40e+05 1.25e+07
Pb 212 2.57e+02 2.52e+03 1.65e+04 2.70e+04 3.03e+04 1.43e+04 2.57e+00 1.37e+OO 2.06e+02
Pb 211 9.99e-02 8.21e-01 4.33e+00 1.04e+01 2.71e+01 2.58e+02 3.46e+03 3.64e+04 3.77e+O5
Pb 210 5.11e-05 8.51e-04 3.39e-02 2.20e-01 1.50e+00 1.10e+02 1.85e+04 7.40e+05 1.25e+07
Pb 209 9.18e-02 9.03e-03 2.68e-02 5.81e-02 1.52e-01 2.73e+OO 6.25e+02 9.73e+04 5.33e+06

Tl 209 1.99e-03 1.95e-04 5.77e-04 1.25e-03 3.29e-03 5.88e-02 1.35e+01 2.1Oe+03 1.15e+05
Tl 208 9.25e+01 9.03e+02 5.92e+03 9.73e+03 1.09e+04 5.14e+03 9.25e-01 4.92e-01 7.44e+01
Tl 207 9.95e-02 8.18e-01 4.29e+00 1.04e+01 2.7Oe+Ol 2.57e+O2 3.45e+03 3.63e+04 3.77e+O5

TOTAL 2.00e+15 8.47e+ll 7.03e+ll 5.66e+ll 3.7Oe+ll 5.00e+10 2.02e+10 7.88e+09 2.42e+08

Page A.2A
U0 2 Fuel - Fission Products Activity: Bq/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10 4 Year 106 Year

H 3 5.18e+09 4.88e+09 3.92e+09 2.96e+09 1.69e+09 1.89e+07 O.OOe+00 0.00e+00 0.00e+00

Se 79 3.33e+06 3.33e+06 3.33e+O6 3.33e+06 3.33e+06 3.33e+06 3.30e+06 3.00e+06 7.73e+01

Kr 81 4.26e+00 4.26e+00 4.26e+00 4.26e+00 4.26e+00 4.26e+00 4.22e+00 4.11e+00 1.56e-01

Kr 85 8.70e+10 8.14e+10 6.29e+10 4.55e+10 2.38e+10 1.35e+08 O.OOe+00 O.OOe+00 O.OOe+00
Rb 86 1.87e+10 2.39e+04 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Rb 87 1.78e+02 1.78e+02 1.78e+02 1.78e+O2 1.78e+02 1.78e+02 1.78e+02 1.78e+02 1.78e+02

Sr 89 3.06e+13 2.03e+ll 3.96e+02 5.14e-09 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Sr 90 6.51e+ll 6.36e+ll 5.77e+ll 5.14e+ll 4.03e+ll 6.03e+10 2.99e+01 O.OOe+00 O.OOe+00
Y 90 7.14e+ll 6.36e+ll 5.77e+ll 5.14e+ll 4.03e+ll 6.03e+10 2.99e+01 O.OOe+00 O.OOe+00
Y 91 3.92e+13 5.22e+ll 1.58e+04 6.3*e-06 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Zr 93 1.56e+07 1.56e+07 1.56e+07 1.56e+07 1.56e+07 1.56e+07 1.56e+07 1.55e+07 9.92e+06
Zr 95 5.40e+13 1.03e+12 1.38e+05 3.51e-04 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Nb 93m 2.78e+05 1.00e+06 3.55e+06 6.11e+06 9.58e+06 1.48e+07 1.48e+07 1.48e+07 9.44e+06
Nb 94 1.62e+03 1.62e+03 1.62e+03 1.62e+03 1.62e+03 1.62e+03 1.57e+03 1.15e+03 2.40e-12
Nb 95 4.96e+13 2.32e+12 3.05e+05 7.81e-04 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Nb 95m 3.81e+ll 7.66e+O9 1.02e+03 2.60e-06 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Tc 99 1.26e+08 1.28e+08 1.28e+08 1.28e+08 1.28e+08 1.28e+08 1.28e+08 1.24e+08 4.96e+06
Ru 103 5.66e+13 8.95e+10 5.7Oe-Ol 5.74e-15 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ru 106 8.10e+12 4.07e+12 2.60e+ll 8.36e+09 8.62e+06 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Rh 103m 5.11e+13 8.10e+10 5.14e-01 5.18e-15 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOa+00
Rh 106 1.32e+13 4.07e+12 2.60e+ll 8.36e+09 8.62e+06 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Pd 107 l.O3e+O6 1.03e+06 1.03e+06 1.03e+06 1.03e+06 1.03e+06 l.O3e+O6 1.03e+06 9.29e+05
Ag 108 74e+05 2.61e+01 2.55e+01 2.48e+01 2.3Se+01 1..52e+01 1.12e-01 O.OOe+00 O.OOe+00
Ag 108m 95e+O2 2.93e+02 2.87e+02 2.79e+02 2.64e+02 1..71e+02 1.25e+00 O.OOe+00 O.OOe+00
Ag 109m 05e+13 1..96e+01 2.22e+00 1.45e-01 6.18e-04 0..OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ag 110 87e+12 7..33e+07 1.27e+O6 8.03e+03 3.20e-01 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ag 110m 52e+10 5..51e+09 9.58e+O7 6.03e+05 2.41e+01 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ag 111 1.97e+12 3.44e-03 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Page A. 25
U0 2 Fuel - Fission Products Activity: Bq/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Cd 3.39e+01 1.96e+01 2.22e+00 1.45e-01 6.18e-04 0.OOe+00 0.OOe+00 0. OOe+00 0.OOe+00

Cd 113 3.96e-07 4.33e-07 4.33e-07 4.33e-07 4.33e-07 4.33e-07 4.33e-07 4.33e-07 4.33e-07
Cd 113m 2.82e+08 2.69e+08 2.19e+08 1.70e+08 1.02e+08 1.73e+06 2.06e-14 0. OOe+00 0.OOe+00
Cd 115m 2.52e+10 8.62e+07 1.18e-02 5.55e-15 0.OOe+00 0.OOe+00 0. OOe+00 0.OOe+00 0.OOe+00
In 114 3.66e+O6 1.25e+04 1.64e-05 0.OOe+00 0.OOe+00 0.OOe+00 0. OOe+00 0.OOe+00 0.OOe+00
In 114m 2.18e+06 1.31e+04 1.71e-05 0.00e+00 0.OOe+00 0.OOe+00 0. OOe+00 0.OOe+00 0. OOe+00
In 115 1.38e-04 1.48e-04 1.48e-04 1.48e-04 1.48e-04 1.48e-04 1.48e-04 1.48e-04 1.48e-04
In 115m 2.83e+ll 8.66e+O3 1.19e-06 0.OOe+00 0.OOe+00 0.OOe+00 0. OOe+00 0.OOe+00 0.OOe+00

Sn 117m 1.08e+08 1.52e+00 0.00e+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Sn 119m 1.72e+O9 6.14e+08 9.84e+06 5.59e+04 1.82e+00 0.OOe+00 0. OOe+00 0.OOe+00 0.OOe+00
Sn 121m 1.44e+06 1.42e+06 1.36e+06 1.27e+06 1.12e+06 4.11e+05 4.85e+00 0.OOe+00 0.OOe+00
Sn 123 5.37e+10 7.59e+09 2.,99e+06 1.66e+02 5.11e-07 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Sn 125 4.00e+ll 1.57e+00 0..OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Sn 126 5.18e+06 5.18e+06 5.18e+06 5.18e+06 5.18e+06 5.18e+O6 5.14e+O6 4.85e+O6 5.07e+03
Sb 124 4.11e+09 6.14e+07 3.03e+00 2.23e-09 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Sb 125 1.05e+ll 8.47e+10 3.12e+10 8.92e+O9 7.29e+08 1.47e+00 0. OOe+00 0.OOe+00 0.OOe+00
Sb 126 2.69e+10 7.29e+05 7.25e+05 7.25e+05 7.25e+05 7.25e+O5 7.22e+05 6.77e+O5 7.1Oe+O2
Sb 126m 2.31e+10 5.18e+06 5.18e+06 5.18e+06 5.18e+06 5.18e+O6 5.14e+06 4.85e+O6 5.07e+03
Te 123 81e-O7 5.37e-07 59e-07 5.59e-07 5.59e-07 5.59e-07 5.59e-07 5.59e-07 5.59e-07
Te 123m 37e+06 6.48e+05 37e+02 3.49e-03 2.28e-12 0.OOe+00 0. OOe+00 0.OOe+00 0.OOe+00
Te 125m 45e+10 .05e+10 59e+09 2..18e+O9 1.78e+08 3.60e-01 0.OOe+00 0.OOe+00 0.OOe+00
Te 127 63e+12 .39e+10 13e+06 2..83e+01 2.31e-09 0.OOe+00 0. OOe+00 0. OOe+00 0.OOe+00
Te 127m 34e+ll .46e+10 19e+06 2.•89e+01 2.36e-09 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Te 129 22e+13 . 18e+08 00e-05 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Te 129m 1.76e+12 9.47e+08 7.70e-05 0.OOe+00 0.00e+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
I 129 2.82e+05 2.93e+05 2.93e+05 2.93e+05 2.93e+05 2.93e+O5 2.93e+05 2.92e+O5 2.80e+05
I 131 3.57e+13 7.77e-01 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Xe 129m 1.23e+08 2.21e-06 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Xe 131m 4.00e+ll 7.18e+02 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Xe 133 6.81e+13 9.18e-08 0.OOe+00 0. OOe+00 0.OOe+00 0. OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Cs 134 5.59e+ll 4.00e+ll 1.04e+ll 1.94e+10 6.73e+O8 1.41e-O3 0.OOe+00 0.OOe+00 0. OOe+00
Cs 135 9.88e+05 1.01e+06 1.01e+06 1.01e+06 1.01e+06 1.01e+06 1.01e+06 1.01e+06 7.47e+05
Cs 136 8.33e+ll 3.36e+03 0.OOe+00 0. OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Cs 137 9.62e+ll 9.44e+ll 8.58e+ll 7.66e+U 6.lle+11 9.69e+10 1.01e+02 0.OOe+00 0.OOe+00
Page A.26
U0 2 Fuel - Fission Products Activity: Bq/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 10 6 Year

Ba 136m 1.37e+ll 5.55e+02 0.00e+00 O.OOe+00 O.OOe+00 0.00e+00 O.OOe+00 0.00e+00 0.00e+00
Ba 137m 9.21e+ll 8.92e+ll 8.14e+ll 7.25e+ll 5.77e+ll 9.18e+10 9.58e+01 0.00e+00 O.OOe+00
Ba 140 6.07e+13 1.54e+05 0.00e+00 O.OOe+00 O.OOe+00 0.00e+00 0.00e+00 0.00e+00 O.OOe+00

La 138 1.40e-03 1.40e-03 1.40e-03 1.40e-03 1.40e-03 1.40e-03 1.40e-03 1.40e-03 1.40e-03
La 140 6.48e+13 1.77e+05 O.OOe+OO O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+OO O.OOe+00
Ce 141 5.74e+13 2.38e+10 7.03e-04 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ce 142 2.41e+02 2.41e+02 2.41e+02 2.41e+O2 2.41e+02 2.41e+02 2.41e+02 2.41e+02 2.41e+02
Ce 144 2.11e+13 8.66e+12 2.45e+ll 2.86e+O9 3.89e+O5 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Pr 143 5.03e+13 4.37e+05 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Pr 144 2.19e+13 8.66e+12 2.45e+ll 2.86e+09 3.89e+O5 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Pr 144m 2.53e+ll 1.04e+ll 2.95e+09 3.43e+07 4.66e+O3 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00
Nd 144 5.14e-03 9.77e-03 1.29e-02 1.30e-O2 1.3Oe-O2 1.3Oe-O2 1.30e-02 1.30e-02 1.30e-02
Nd 147 2.25e+13 2.58e+03 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+OO O.OOe+00
Pm 147 2.57e+12 2.18e+12 7.55e+ll 2.02e+ll 1.44e+10 9.47e+OO O.OOe+OO O.OOe+OO O.OOe+00
Pm 148 3.55e+12 2.90e+07 6.48e-04 O.OOe+OO O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+00
Pm 148m 2.36e+ll 5.14e+08 1.15e-02 O.OOe+OO O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+00
Sm 147 5.22e+00 2.17e+01 5.74e+01 7.14e+01 7.59e+01 7.62e+01 7.62e+01 7.62e+01 7.62e+01
Sm 148 l.O7e-O4 1.17e-O4 1.17e-04 1.17e-O4 1.17e-O4 1.17e-04 1.17e-04 1.17e-04 1.17e-04
Sm 149 5.03e-06 1.59e-05 1.59e-05 1.59e-O5 1.59e-O5 1.59e-05 1.59e-05 1.59e-05 1.59e-05
Sm 151 2.17e+09 2.41e+09 2.33e+O9 2.25e+09 2.08e+09 1.12e+09 1.10e+06 O.OOe+00 O.OOe+00
Eu 152 1.2Oe+O7 1.14e+O7 9.29e+O6 7.22e+O6 4.33e+O6 7.33e+O4 O.OOe+00 O.OOe+OO O.OOfc+00
Eu 154 4.18e+10 3.85e+10 2.78e+10 1.86e+10 8.29e+O9 1.31e+O7 O.OOe+00 O.OOe+00 O.OOe+00
Eu 155 3.19e+10 2.78e+10 1.59e+10 7.88e+O9 1.95e+09 2.72e+04 O.OOe+00 O.OOe+00 O.OOe+OO
Eu 156 3.09e+12 1.79e+05 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Gd 152 1.65e-06 1.68e-06 1.75e-06 1.82e-06 1.92e-O6 2.07e-06 2.08e-06 2.08e-06 2.08e-06
Gd 153 3.33e+O7 1.17e+O7 1.76e+05 9.36e+02 2.63e-O2 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Tb 160 4.48e+09 1.35e+O8 l.lle+02 2.76e-06 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00
Tb 161
3.52e+10 4.03e-06 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ho 166m
1.37e+O3 1.37e+O3 1.37e+O3 i.37e+O3 1.36e+03 1.30e+03 7.7Oe+O2 4.26e+00 O.OOe+00
TOTAL
5.74e+15 3.58e+13 4.85e+12 2.85e+12 2.05e+12 3.10e+ll 1.76e+08 1.7Oe+O8 2.63e+O7 Page A. 27
U0 2 Fuel - Actinides Decay Heat: U/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 1O3 Year 1O4 Year 106 Year

Es 253 8.26e-16 6.14e-20 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00

Cf 254 2.86e-17 3.06e-19 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Cf 252 4.11e-14 3.16e-14 l.lle-14 2.98e-15 2.15e-16 1.61e-25 O.OOc+00 0.OOe+00 0.OOe+00
Cf 251 1.35e-16 1.35e-16 1.34e-16 1.34e-16 1.,33e-16 1.25e-16 6.24e-17 6.00e-20 0.OOe+00
Cf 250 3.92e-14 3.77e-14 3.05e-14 2.34e-14 1..38e-14 1.98e-16 1.05e-22 4.27e-23 0.OOe+00
Cf 249 3.21e-16 5.98e-15 1.04e-14 1.05e-14 1.03e-14 8.78e-15 1.48e-15 2.77e-23 0.OOe+00

Bk 249 6.61e-14 3.01e-14 1.27e-15 2.43e-17 8.90e-21 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Cm 250 1.63e-20 1.64e-20 1.63e-20 1.63e-20 1.63e-20 1.62e-20 1.48e-20 5.99e-21 0.OOe+00
Cm 248 8.53e-15 8.53e-15 8.53e-15 8.53e-15 8.53e-15 8.53e-15 8.51e-15 8.36e-15 1.10e-15
Cm 247 1..93e-15 1..93e-15 .93e-15 1.93e-15 1.,93e-15 1.93e-15 1.93e-15 1.93e-15 1.85e-15
Cm 246 1..89e-09 1.•89e-09 .89e-09 1.89e-09 1..88e-09 1..86e-09 1.63e-09 4.36e-10 0.OOe+00
Cm 245 1.•10e-08 1..10e-08 ,10e-08 1.10e-08 1.,10e-08 1.,09e-08 1.01e-08 4.87e-09 0.OOe+00
Cm 244 6..lle-04 5..97e-04 ,12e-04 4.23e-04 2..88e-04 1..35e-05 1.47e-20 0.OOe+00 0.OOe+00
Cm 243 6.61e-06 6.45e-06 .85e-06 5.18e-06 4..06e-06 5..81e-07 1.81e-16 0.OOe+00 0.OOe+00
Cm 242 4.74e-02 1.03e-02 2.74e-05 6.62e-06 6.31e-06 4.38e-06 7.23e-08 1.08e-25 0. OOe+00
Am 245 1.68e-08 1.15e-18 4.85e-20 9.28e-22 3.40e-25 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Am 243 1.68e-05 1.68e-05 1.68e-05 1.68e-05 1.68e-05 1.67e-05 1.53e-05 6.59e-06 1.86e-15
Am 242 8.30e-03 2.56e-07 2.52e-07 2.46e-07 2.35e-07 1.63e-07 2.69e-09 4.02e-27 0.OOe+00
Am 242m 9.00e-08 8.96e-08 8.79e-08 8.60e-08 8.21e-08 5.70e-08 9.41e-10 1.41e-27 0.OOe+00
Am 241 1.93e-04 1.40e-03 5.66e-03 9.94e-03 1.59e-02 2.3Oe-O2 5.49e-03 7.83e-09 0.OOe+00
Pu 244 4.41e-13 4.41e-13 4.41e-13 4.41e-13 4.41e-13 4.41e-13 4.41e-13 4.41e-13 4.37e-13
Pu 243 4.43e-02 6.98e-17 6.98e-17 6.98e-17 6.98e-17 6.98e-17 6.98e-17 6.97e-17 6.67e-17
Pu 242 7..04e-06 7..04e-06 .04e-06 7.,04e-06 7.04e-06 7.03e-06 7.02e-O6 6.91e-06 l.lle-06
Pu 241 7..41e-04 7..07e-04 .86e-04 4.,63e-04 2.89e-04 6.64e-06 9.80e-12 4.,7Oe-12 0. OOe+00
Pu 240 7..32e-03 7..32e-03 .31e-03 7..31e-O3 7.30e-03 24e-03 6.58e-03 2..53e-O3 4.69e-13
Pu 239 5.,O7e-O3 5..29e-03 .29e-O3 5.,29e-03 5.29e-03 28e-03 5..14e-03 3..97e-03 3,42e-15
Pu 238 2.62a-03 2..88e-03 .83e-O3 2.72e-03 2.52e-03 34e-03 1..16e-06 2..32e-25 0.OOe+00
Pu 236 7.31e-07 5.83e-07 2.2Oe-O7 6.53e-08 5.74e-09 2.05e-17 0.OOe+00 O.OOe+00 0.OOe+00

Np 240 8.99e-01 1.77e-16 1.77e-16 1.77e-16 1.77e-16 l.77e-16 1.77e-16 1.77e-16 1.76e-16
Np 240m 8.80e-14 8.80e-14 8.80e-14 8.80e-14 8.80e-14 8.80e-14 8.80e-14 8,80e-14 8.73e-14
Np 239 6.48e+01 1.27e-06 1.27e-06 1.27e-06 1.26e-06 1.26e-06 1.15e-06 4.95e-07 1.40e-16
Np 238 2.37e-01 5.22e-O9 5.12e-09 5.01e-09 4.78e-09 3.32e-09 5.48e-ll 0.OOe+00 0.OOe+00
Np 237 7.65e-O7 8.2Oe-O7 8.24e-07 8.36e-O7 8.75e-07 1.40e-06 4.70e-O6 5.70e-06 4.14e-06

Page A.28
U02 Fuel - Actinides Decay Heat: V/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

U 240 1.25e-14 1.25e-14 1.25e-14 1.25e-14 1.25e-14 1.25e-14 1.25e-14 1.25e-14 1.24e-14
U 238 8.40e-06 8.40e-06 8.40e-06 8.40e-06 8.40e-06 8.40e-06 8.40e-06 8.40e-06 8.40e-06
U 237 3,.88e-01 1.05e-06 8.66e-07 6.,84e-07 4.27e-O7 9.82e-09 1.45e-14 6.95e-15 O.OOe+00
U 236 1,.34e-06 1.34e-06 1..35e-06 1..35e-06 1.35e-06 1.36e-06 1.52e-06 2.51e-06 3.03e-06
U 235 1,.14e-07 1.14e-07 1..14e-07 1..14e-07 1.14e-07 1.15e-O7 1.18e-07 1.53e-07 2.68e-07
U 234 7..69e-06 7Oe-O6 7.,73e-06 7..76e-06 7.82e-06 8.19e-06 8.62e-06 8.64e-06 9.49e-06
U 233 2, 98e-ll 4..35e-ll 6.07e-ll 9.62e-ll 4.71e-10 1.33e-08 2.22e-O7 4.18e-06
U 232 3.41e-09 9.24e-09 2.18e-08 2.63e-08 2.59e-08 1.21e-08 2.09e-12 O.OOe+00 O.OOe+00

Pa 234 1.21e-08 7.61e-09 7.61e-09 7.61e-09 7.61e-09 7.61e-O9 7.61e-09 7.61e-09 7.61e-09
Pa 234m 1.64e-06 1.64e-06 1.64e-06 1.64e-06 1.64e-06 1.64e-06 1.64e-06 1.64e-06 1.64e-06
Pa 233 4.54e-08 6.09e-08 6.12e-08 6.21e-08 6.50e-08 1.04e-07 3.49e-07 4.23e-07 3.07e-07
Pa 231 1.58e-ll 1.87e-ll 2.99e-ll 4.38e-ll 7.16e-ll 2.94e-10 2.82e-09 2.96e-08 3.08e-07

Th 234 1..34e-07 1.34e-07 1.34e-07 1.34e-07 1 34e-O7 34e-07 1.34e-07 1.34e-07 34e-07
Th 232 2..21e-17 8.14e-17 3.19e-16 6.15e-16 1.21e-15 ,99e-15 6.33e-14 8.93e-13 35e-10
Th 231 4..37e-08 2.45e-09 2.45e-09 2.45e-09 2.45e-09 2.45e-09 2.•54e-09 3.27e-09 74e-09
Th 230 4. 1.10e-10 3.83e-10 7.25e-10 1.41e-09 7.09e-09 7..53e-08 7.29e-07 56e-06
Th 229 4.69e-15 7.48e-15 2.21e-14 4.81e-14 1.26e-13 2.26e-12 5..16e-10 8.05e-08 .39e-06
Th 228 2.42e-10 2.22e-09 1.46e-08 2.39e-08 2.67e-08 1.27e-08 2.27e-12 1.21e-12 1.83e-10
Th 227 1.17e-13 7.99e-13 4.19e-12 l.Ole-11 2.64e-ll 2.50e-10 3.37e-O9 3.54e-08 3.68e-07

Ac 228 2.13e-19 2.31e-18 3.00e-17 9.43e-17 2.71e-16 2.14e-15 2.26e-14 3.19e-13 4.83e-ll
Ac 227 2.07e-15 1.08e-14 5.64e-14 1.36e-13 3.55e-13 3.37e-12 4.53e-ll 4.76e-10 4.95e-09
Ac 225 8.68e-14 8.54e-15 2.52e-14 5.49e-14 1.44e-13 2.58e-12 5.89e-10 9.19e-08 5.02e-06

Ra 228 1.69e-21 1.84e-20 2.39e-19 7.50e-19 2.16e-18 1.7Oe-17 1.80e-16 2.54e-15 3.84e-13
Ra 226 6.33e-15 3.99e-14 4.75e-13 1.70e-12 6.41e-12 1.54e-10 1.44e-08 5.79e-07 9.75e-06
Ra 225 2.10e-15 1.71e-16 5.07e-16 1.10e-15 2.89e-15 5.18e-14 1.85e-09 l.Ole-07
Ra 224 2.38e-10 2.33e-09 1.53e-08 2.51e-08 2.81e-08 1.33e-O8 2.38e-12 1.27e-12 1.92e-10
Ra 223 9.62e-14 7.91e-13 4.15e-12 9.98e-12 2.61e-ll 2.48e-10 3.33e-09 3.50e-08 3.64e-07

Fr 223 1.53e-16 7.96e-16 4.17e-15 1.00e-14 2.62e-14 2.49e-13 3.35e-12 3.52e-ll 3.66e-10
Fr 221 9.59e-14 9.43e-15 2.79e-H 6.06e-14 1.59e-13 2.85e-12 6.51e-10 l.O2e-O7 5.54e-06

Rn 222 6.95e-15 4.58e-14 5.45e-13 1.95e-12 7.35e-12 1.77e-10 1.66e-08 6.64e-07 1.12e-05
Rn 220 2.64e-10 2.58e-09 1.69e-08 2.78e-08 3.10e-08 1.47e-08 2.64e-12 1.40e-12 2.12e-10
Rn 219 1.12e-13 9.22e-13 4.84e-12 3.04e-ll 2.89e-10 3.88e-09 4.08e-08 4.24e-07

At 217 1.06e-13 1.04e-14 3.08e-14 6.70e-14 1.76e-13 3.15e-12 7.19e-10 1.12e-O7 6.13e-06

Page A.29
 Fuel - Actinides Decay Heat: V/kg inital U
uo 2
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Po 218 7.60e-15 5.Ole-14 5.96e-13 2.13e-12 8.0^e-12 1.93e-10 1.81e-08 7.26e-07 1.22e-05
Po 216 2.84e-10 2.78e-09 1.83e-08 2.99e-08 3.35e-08 1.59e-08 2.84e-12 1.51e-12 2.29e-10
Po 215 1.21e-13 9.92e-13 5.20e-12 1.25e-ll 3.27e-ll 3.lle-10 4.17e-09 4.39e-08 4.56e-07
Po 214 9.73e-15 6.41e-14 7.64e-13 2.73e-12 1.03e-ll 2.47e-10 2.32e-O8 9.30e-07 1.57e-05
Po 213 1.23e-13 1.21e-14 3.58e-14 7.78e-14 2.O4e-13 3.66e-12 8.35e-10 1.3Oe-O7 7.lle-06
Po 212 2.36e-10 2.31e-09 1.52e-08 2.49e-08 2.78e-08 1.32e-08 2.36e-12 1.25e-12 1.90e-10
Po 211 3.40e-16 2.,80e-15 1.,47e-14 3.53e-14 9.23e-14 8.77e-13 1.18e-ll 1.24e-10 1.29e-09
Po 210 9.,15e-18 3.,32e-!6 2.,93e-14 1.91e-13 1.30e-12 9.48e-ll 1.60e-08 6.42e-07 1.08e-05

Bi 214 2..69e-15 1.,77e-14 2..lls-13 7.53e-13 2.84e-12 6.83e-ll 6.40e-09 2.57e-07 4.,33e-06
Bi 213 1..04e-14 1,.03e-15 3.,04e-15 6.60e-15 1.,73e-14 3.10e-13 7.09e-ll 1.lle-08 6.,04e-07
Bi 212 1..18e-10 1,,16e-09 7..59e-09 1.,24e-08 1.39e-08 6.,59e-09 1..18e-12 6.28e-13 9.,50e-ll
Bi 211 1..08e-13 8,.86e-13 4,.65e-12 1.,12e-ll 2,,92e-ll 2.,77e-10 3..73e-09 3.-92e-08 4..O8e-O7
Bi 210 2 .90e-18 5 .31e-17 2 .lle-15 1,.37e-14 9,,36e-14 6,.82e-12 1..15e-09 4..62e-08 7..78e-07

Pb 214 6 .69e-16 4 .40e-15 5 .25e-14 1,.87e-13 7,.08e-13 1,,70e-ll 1,.59e-09 6 .39e-08 1,.08e-06
Pb 212 1.32e-ll 1.30e-10 8 .50e-10 1..39e-09 1..56e-09 7,•38e-10 1.32e-13 7.03e-14 1.06e-ll
Pb 211 8 .10e-15 6 .66e-14 3•49e-13 8 .40e-13 2.20e-12 2.08e-ll 2 .80e-10 2 .95e-09 3 ,06e-08
Pb 210 3.20e-19 5.34e-18 2•12e-16 1,38e-l5 9.41e-15 6.85e-13 1.16e-10 4 .64e-09 7,82e-08
Pb 209 2.91e-15 2.86e-16 8 .46e-16 1,84e-15 4.83e-15 8.65e-14 1.97e-ll 3,08e-09 1.68e-07

Tl 209 8 .92e-16 8.77e-17 2•59e-16 5.64e-16 1.48e-15 2.65e-14 6.05e-12 9.44e-10 5.16e-08
Tl 208 5.87e-ll 5.75e-10 3•77e-O9 6.18e-09 6.91e-09 3.28e-09 5.87e-13 3.12e-13 4.72e-ll
Tl 207 7 •91e-15 6 •50e-14 3.41e-13 8.21e-13 2.15e-12 2•04e-ll 2•74e-10 2.88e-09 2 .99e-08

TOTAL 1.39e+02 2.85e-O2 2.23e-O2 2.62e-02 3.16e-O2 3.69e-02 1.73e-02 6.55e-03 1.40e-04

Page A.30
U0 2 Fuel - Fission Products Decay Heat: tf/kg ioital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

H 3 4.73e-06 4.47e-06 3.57e-06 2.7Oe-O6 1.54e-06 1.73e-08 0.00e+00 0.00e+00 0.00e+00

Se 79 1.72e-08 1.72e-08 1.72e-08 1.72e-08 1.71e-08 1.71e-08 1.70e-08 1.54e-08 3.98e-13

Kr 81 1.41e-14 1.41e-14 1.41e-14 1.41e-14 l-41e-14 1.41e-14 1.41e-14 1.37e-14 5.20e-16

Kr 85 3.51e-03 3.30e-03 2.55e-03 1.84e-03 9.65e-04 5.47e-06 0.00e+00 O.OOe+00 0.00e+00

Rb 86 2.28e-03 2.92e-09 O.OOe+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00

Rb 87 2.24e-12 2.24e-12 2.24e-12 2.24e-12 2.24e-12 2.24e-12 2.24e-12 2.24e-12 2.24e-12

Sr 89 2.86e+OO 1.9Oe-O2 3.7Oe-ll 4.8Oe-22 O.OOe+00 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+00

Sr 90 2.04e-02 2.00e-02 1.82e-02 1.61e-02 1.27e-02 1.89e-03 9.38e-13 O.OOe+00 O.OOe+00

Y 90 1.07e-01 9.54e-02 8.67e-02 7.7Oe-O2 6.07e-02 9.03e-03 4.48e-12 O.OOe+00 O.OOe+00

Y 91 3.80e+00 5.05e-02 1.54e-09 6.16e-19 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00

Zr 93 4.89e-08 4.90e-08 4.9Oe-O8 4.90e-08 4.90e-08 4.90e-08 4.90e-08 4.88e-08 3.12e-08

Zr 95 7.38e+00 1.41e-01 1.88e-08 4.8Oe-17 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00

Nb 93m 1.33e-09 4.80e-09 1.7Oe-O8 2.92e-O8 4.59e-08 7.06e-08 7.10e-08 7.08e-08 4.52e-08
Nb 94 4.48e-10 4.48e-10 4.47e-10 4.47e-10 4.47e-10 4.46e-10 4.33e-10 3.18e-10 6.62e-25
Nb 95 6.45e+00 3.00e-01 3.96e-08 1.01e-16 O.OOe+00 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Nb 95m 1.43e-02 2.87e-O4 3.83e-ll 9.77e-20 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+OC

Tc 99 1.71e-06 1.74e-06 1.74e-06 1.74e-06 1.74e-06 1.74e-06 1.74e-O6 1.69e-O6 6.72e-O8

Ru 103 5.11e+00 8.11e-03 5.15e-14 5.18e-28 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+OO O.OOe+00
Ru 106 1.3Oe-O2 6.52e-03 4.16e-04 1.34e-05 1.38e-08 O.OOe+00 O.OOe+OO O.OOe+OO O.OOe+OO

Rh 103m 3.17e-01 5.03e-04 3.19e-15 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Rh 106 3.42e+00 1.05e+00 6.74e-02 2.16e-03 2.23e-06 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Pd 107 1.52e-09 1.52e-09 1.52e-09 1.52e-09 1.52e-09 1.52e-09 1.52e-O9 1.52e-09 1.37e-09

Ag 108 1..75e-O8 2.63e-12 2.57e-12 50e-12 2.37e-12 1.53e-12 1.13e-14 O.OOe+00 O.OOe+00
Ag 108m 7..75e-ll 7.71e-ll 7.54e-ll 34e-ll 6.95e-ll 4.49e-ll 3.30e-13 O.OOe+00 O.OOe+00
Ag 109m 1..47e-01 2.74e-13 3.09e-14 2.02e-15 8.61e-18 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ag 110 3.•63e-01 1.42e-05 2.47e-07 56e-09 6.21e-14 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ag 110m 6.85e-03 2.49e-03 4.32e-05 73e-O7 1.09e-ll O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ag 111 1.19e-01 2.08e-16 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Page A.31
U0 2 Fuel - Fission Products Decay Heat: V/kg inital D

Nuclide Discharge 1 Year i

5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 106 Year

Cd :109 l.lD7e-13 6. 21e-14 7 J 00e-15 4. 57e-16 1. 95e-18 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00
Cd :113 5.'94e-21 6. 47e-21 6. 47e-21 6. 47e-21 6. 47e-21 6. 48e-21 6. 48e-21 6. 48e-21 6. 48e-21
Cd 113m 9.1B6e-06 9. 38e-06 7. 65e-06 5. 93e-06 3. 56e-06 6. 03e-08 7. 20e-28 0. OOe+00 0. OOe+00
Cd 115m 2. 54e-03 8. 68e-06 1. 19e-15 5. 61e-28 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00

In 114 4. 53e-07 1. 55e-09 2. 03e-18 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00
In 114m 8. 29e-08 4. 98e-10 6. 51e-19 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00
In 115 3. 36e-18 3. 59e-18 3. 59e-18 3. 59e-18 3. 59e-18 3. 59e-18 3. 59e-18 3. 59e-18 3. 59e-18
In 115m 1. 53e-02 4. 66e-10 6. 40e-20 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00

Sn 117m 5. 44e-06 7. 61e-14 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00
Sn 119m 2. 41e-05 8. 57e-06 1. 37e-O7 7. 83e-10 2.54e-14 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00
Sn 121m 3. 63e-08 3. 58e-08 3. 40e-08 3. 20e-08 2.82e-08 1. 03e-08 1. 22e-13 0. OOe+00 0. OOe+00
Sn 123 4. 54e-03 6. 40e-04 2. 52e-07 1. 40e-ll 4. 32e-20 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00
Sn 125 7. 14e-02 2. 80e-13 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0.,OOe+00
Sn 126 1. 75e-07 1.,75e-07 1. 75e-07 1. 75e-O7 1. 75e-O7 1. 75e-O7 1. 74e-07 1. 63e-07 1. 71e-10

Sb 124 1. 48e-03 2.,20e-05 1. 09e-12 8. Ole-22 0., OOe+00 0.,OOe+00 0.,OOe+00 0.,OOe+00 0..OOe+00
Sb 125 8. 87e-03 7..16e-03 2. 63e-O3 7. 53e-04 6.,17e-O5 1.,25e-13 0.,OOe+00 0. OOe+00 0..OOe+00
Sb 126 1. 35e-02 3..63e-07 3.,63e-07 3.,63e-07 3..63e-07 3.,63e-07 3.,61e-O7 3..39e-07 3 .54e-10
Sb 126m 7.,94e-03 1 .79e-06 1,.79e-06 1,.79e-06 1,.79e-O6 1,.79e-06 1..77e-O6 1..67e-06 1 .74e-09

Te 123 1.,04e-21 1 .47e-21 1,.53e-21 1,.53e-21 1..53e-21 1,.53e-21 1,.53e-21 1,.53e-21 1 .53e-21
Te 123m 2..lle-07 2 .55e-08 5,.39e-12 1 .37e-16 8 .95e-26 0 .OOe+00 0 .OOe+00 0..OOe+00 0 .OOe+00
Te 125m 3,.31e-04 4 .66e-04 1..73e-04 4 .94e-05 4 .04e-06 8 .17e-15 0 .OOe+00 0 .OOe+00 0 .OOe+00
Te 127 1,.33e-01 1 .24e-03 1 .14e-07 1 .03e-12 8 .42e-23 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Te 127m 4 .85e-03 5 •03e-04 4 .64e-08 4 .19e-13 3 .42e-23 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Te 129 1 .18e+00 5 .95e-05 4 .83e-18 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Te 129m 8 .36e-02 4 •49e-05 3 .64e-18 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00

I 129 3 .52e-09 3 •66e-09 3 .66e-09 3 .66e-09 3 .66e-09 3 .66e-09 3 .66e-09 3 .65e-09 3 .50e-09
I 131 3 .28e+00 7 .14e-14 0 .OOe+00 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Xe 129m 4 .55e-06 8 .19e-20 0 .OOe+00 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Xe 131m 1 .04e-02 1 .87e-ll 0 .OOe+00 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00

Cs 134 1 .54e-01 1 .10e-01 2 .87e-02 5 •34e-03 1 .85e-04 3 .87e-16 0 .OOe+00 0 .OOe+00 0i. OOe+00
Cs 135 8 •91e-09 9 .13e-09 9 .13e-09 9 .13e-09 9 •13e-09 9 .13e-09 9 •13e-09 9 .10e-09 6 .75e-09
Cs 136 3 •07e-01 1 .24e-09 0 .OOe+00 0 .00e+00 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0i. OOe+00
Cs 137 2 .88e-02 2 .82e-02 2 .57e-O2 2 .29e-02 1 .82e-02 2 .9Oe-O3 3.O3e-12 0 .OOe+00 cI. OOe+00
Page A.32
002 Fuel - Fission Products Decay Heat: V/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Ba 136m 4.46e-02 1.80e-10 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ba 137m 9.80e-02 9.46e-02 8.63e-02 7.69e-02 6.11e-02 9.72e-03 1.02e-ll 0.00e+00 0.00e+00
Ba 140 4.59e+00 1.16e-08 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

La 138 2.86e-16 2.86e-16 2.86e-16 2.86e-16 2.86e-16 2.86e-16 2.86e-16 2.86e-16 2.86e-16
La 140 2.94e+01 8.01e-08 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Ce 141 2.26e+00 9.43e-04 2.79e-17 0.00e+00 0.00e+00 0.00e+00 0.0Oe+00 0.00e+00 0.00e+00
Ce 142 5.56e-ll 5.56e-ll 5.56e-ll 5.56e-ll 5.56e-ll 5.56e-ll 5.56e-ll 5.56e-ll 5.56e-ll
Ce 144 3.78e-01 1.55e-01 4.40e-03 5.12e-05 6.95e-09 0.00e+00 0.0Oe+00 0.00e+00 0.00e+00

Pr 143 2.53e+00 2.20e-08 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Pr 144 4.35e+00 1.72e+OO 4.87e-02 5.68e-04 7.70e-08 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Pr 144m 2.34e-03 9.59e-04 2.72e-O5 3.17e-07 4.30e-ll 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Nd 144 1.58e-15 2.99e-15 3.95e-15 3.96e-15 3.98e-15 3.98e-15 3.98e-15 3.98e-15 3.98e-15
Nd 147 1.47e+00 1.68e-10 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Pm 147 2.49e-02 2.11e-02 7.33e-03 1.96e-03 1.39e-04 9.18e-14 0.00e+00 0.00e+00 0.00e+00
Pm 148 7.39e-01 6.03e-06 1.35e-16 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Pm 148m 8.10e-02 1.76e-04 3.95e-15 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Sm 147 1.93e-12 8.04e-12 2.12e-ll 2.6Ae-ll 2.81e-ll 2.83e-ll 2.83e-ll 2 . 8 3 e - l l 2.83e-ll

Sm 148 3.39e-17 3.71e-17 3.71e-17 3.71e-17 3.71e-17 3.71e-17 3.71e-17 3.71e-17 3.71e-17
Sm 149 1.54e-18 4.86e-18 4.86e-18 4.86e-18 4.86e-18 4.86e-18 4.86e-18 4.86e-18 4.86e-18
Sm 151 6.88e-06 7.63e-06 7.40e-06 7.12e-06 6.59e-06 3.56e-06 3.47e-09 0.00e+00 0.00e+00

Eu 152 2.46e-06 2.33e-06 1.90e-06 1.48e-06 8.86e-07 1.50e-08 0.00e+00 0.00e+00 O.OOe+00
Eu 154 l.Ol-i-02 9.28e-03 6.73e-03 4.49e-03 2.01e-03 3.18e-06 0.00e+00 0.00e+00 0.00e+00
Eu 155 6.28e-04 5.46e-04 3.12e-04 1.55e-04 3.84e-05 5.35e-10 0.00e+00 0.00e+00 0.00e+00
Eu 156 8.61e-01 5.00e-08 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Gd 152 5.80e-19 5.90e-19 6.16e-19 6.42e-19 6.77e-19 7.30e-19 7.31e-19 7.31e-19 7.31e-19
Gd 153 8.14e-07 2.85e-07 4.31e-09 2.29e-ll 6.42e-16 0.00e + 00 0.00e + 00 0.00e+00 0.00e+00

Tb 160 9.85e-04 2.97e-05 2.45e-ll 6.09e-19 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.0Oe+00
Tb 161
1.29e-03 1.48e-19 0.00e+00 0.00e + 00 0.00e+00 0.00e + 00 0.00e + 00 0.00e + 00 O.OOe^OO
Ho 166m
4.11e-10 4.11e-10 4.10e-10 4.08e-10 4.06e-10 3.88e-10 2.31e-10 1.27e-12 0.00e+00
TOTAL
1.82e+O3 3.85e+OO 3.86e-01 2.10e-01 1.56e-01 2.36e-O2 4.20e-06 4.00e-06 1.58e-O7 Page A.33
U0 2 Fuel - Actinides Activity: Ci/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10* Year 106 Year
Es 253 2.07e-14 1.54e-18 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Cf 254 2.42e-17 2.59e-lc- 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00 0.OOe+00 0. OOe+00
Cf 253 6.07e-14 4.06e-20 0. OOe+00 0. OOe+00 0.OOe+00 0. OOe+00 0. OOe+00 o. OOe+00 0. OOe+00
Cf 252 5.76e-13 4.43e-13 1.55e-13 4. 17e-14 3.Ole-15 2. 25e-24 0. OOe+00 0. OOe+00 0. OOe+00
Cf 251 3.78e-15 3. 78e-15 3. 76e-15 3. 75e-15 3.72e-15 3.50e-15 1. 75e-15 1.68e-18 0. OOe+00
Cf 250 1.05e-12 1.Ole-12 8. 20e-13 6. 29e-13 3.70e-13 5. 33e-15 2.83e-21 1. 15e-21 0. OOe+00
Cf 249 6. 94e-15 1. 29e-13 2.25e-13 2.27e-13 2.22e-13 1. 90e-13 3. 20e-14 5. 99e-22 0. OOe+00
Bk 250 5.52e-10 3. 13e-21 3. 13e-21 3. 13e-21 3. i3e-21 3. 10e-21 2.83e-21 1. 15e-21 0. OOe+00
Bk 249 8. 92e-ll 4.06e-ll 1. 71e-12 3. 28e-14 1.20e-17 0. OOe+00 0. OOe+00 0. OOe+00 0. OOe+00
Cm 250 2. 24e-20 2.24e-20 2. 24e-20 2. 24e-20 2.23e-20 2. 21e-20 2.02e-20 8. 20e-21 0. OOe+00
Cm 248 6. 85e-14 6.85e-14 6. 85e-14 6. 85e-14 6.85e-14 6. 85e-14 6. 84e-14 6. 71e-14 8. 87e-15
Cm 247 6. 04e-14 6.04e-14 6. 04e-14 6. 04e-14 6.04e-14 6. 04e-14 6. 04e-14 6. 04e-14 5.78e-14
Cm 246 5.,77e-08 5.,77e-O8 5. 77e-O8 5. 76e-08 5.75e-08 5. 69e-08 4. 98e-08 1.33e-08 0. OOe+00
Cm 245 3. 31e-07 3.,31e-O7 3. 31e-O7 3.,31e-07 3.,31e-07 3. 29e-O7 3.,06e-07 1.47e-07 0. OOe+00
Cm 244 1.,75e-02 1.,71e-O2 X •,46e-02 1. 21e-02 8.,24e-03 3. 86e-04 4.,22e-19 0. OOe+00 0., OOe+00
Cm 243 1..80e-04 1.,76e-O4 1.,60e-04 1,,41e-04 1.,lle-04 1.,58e-05 4.,92e-15 0. OOe+00 0..OOe+00
Cm 242 1,.29e+00 2,.78e-01 7..45e-04 1,.80e-04 1.,71e-04 1., 19e-04 1..96e-06 2.,94e-24 0..OOe+00
Am 245 8 .90e-06 6 .09e-16 2,.57e-17 4,.92e-19 1,.8Oe-22 0,.OOe+00 0,.OOe+00 0,.OOe+00 0,.OOe+00
Am 243 5 .21e-04 5 .24e-04 5,.24e-04 5 .24e-04 5 .23e-04 5,.19e-04 4 . 77e-04 2,.05e-04 5,.78e-14
Am 242 7 .31e+00 2 .26e-04 2,.22e-04 2 .17e-04 2,.07e-04 1,.44e-04 2 .37e-06 3..55e-24 0,.OOe+00
Am 242m 2 .28e-04 2 .27e-04 2 .23e-04 2 .18e-04 2 .08e-04 1..44e-04 2 .38e-06 3,.56e-24 0 .OOe+00
Am 241 5 .82e-03 4 .21e-O2 1 .71e-01 2 .99e-01 4 .78e-01 6 .92e-01 1 .65e-01 2,.36e-07 0 .OOe+00
Pu 244 1.52e-ll 1 .52e-ll 1.52e-ll 1.52e-ll 1.52e-ll 1 .52e-ll 1 .52e-ll 1 .52e-ll 1.51e-ll
Pu 243 3 .84e+01 6 .04e-14 6 .04e-14 6 .04e-14 6 .04e-14 6 .04e-14 6 .04e-14 6 .04e-14 5 .78e-14
Pu 242 2 .38e-04 2 .38e-04 2 .38e-04 2.38e-04 2.38e-04 2 .38e-04 2 .38e-04 2 .34e-04 3.77e-O5
Pu 241 2.32e+01 2 •21e+01 1 .83e+01 1.45e+01 9 .02e+00 2 .07e-01 3 .06e-O7 1.47e-07 0 .OOe+00
Pu 240 2.35e-01 2 .35e-01 2 .35e-01 2.35e-01 2 .34e-01 2 .33e-01 2 .lle-01 8 .14e-02 1.51e-ll
Pu 239 1.64e-01 1 .72e 01 1 .72e-01 1.72e-01 1 .72e-01 1 •71e-01 1.67e-01 1.29e-01 1.lle-13
Pu 238 7•90e-02 8 .68e-02 8 .55e-02 8 .22e-02 7 •60e-02 4 .05e-02 3 .50e-05 7.00e-24 0 .OOe+00
Pu 236 2.10e-05 1 .67e-05 6 .33e-06 1.88e-06 1.65e-07 5 .89e-16 0 .OOe+00 0 .OOe+00 0 .OOe+00
Np 240 8 .48e+01 1 .67e-14 1.67e-14 1.67e-14 1.67e-14 1 .67e-14 1•67e-14 1.67e-14 1.66e-14
Np 240m 1 •52e-ll 1 .52e-ll 1.52e-ll 1.52e-ll 1.52e-ll 1.52e-ll 1.52e-li 1.52e-U 1.51e-ll
Np 239 2 .68e+04 5 .24e-04 5 .24e-04 5 .24e-04 5.23e-04 5 .19e-04 4 .77e-O4 2.05e-04 5.78e-14
Np 238 4 .95e+01 1 .09e-06 1 ,07e-06 1•05e-06 9 .99e-07 6 .93e-07 1.14e-08 0 .OOe+00 0 .OOe+00
Np 237 2 .50e-05 2 .68e-05 2 .7Oe-O5 2.74e-05 2 .86e-05 4 .58e-05 1.S4e-04 1.87e-04 1.35e-04
Page A.34
uo 2 Fuel - Actinides Activity: Ci/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 10* Year

U 240 1. 52e-ll 1. 52e-ll 1.52e-ll 1. 52e-ll 1.52e-ll 1. 52e-ll 1. 52e-ll 1. 52e-ll 1. 51e-ll
U 238 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04
U 237 2. 05e+02 5. 53e-04 4. 58e-04 3. 62e-04 2.26e-04 5. 19e-06 7. 65e-12 3. 67e-12 0. 00e+00
U 236 4. 96e-05 4. 96e-05 4. 97e-05 4. 97e-O5 4. 98e-05 5.03e-05 5. 62e-05 9. 25e-05 1. 12e-04
U 235 4. 36e-06 4. 36e-06 4. 36e-06 4. 36e-06 4. 36e-06 4. 37e-O6 4. 52e-O6 5. 83e-06 1.02e-05
U 234 2. 67e-04 2. 67e-04 2.68e-04 2.69e-04 2. 72e-04 2.84e-04 2. 99e-04 3. 00e-04 3. 29e-04
U 2.43 8. 98e-10 1. 02e-09 1. 50e-09 2.09e-09 3.31e-09 1. 62e-O8 4. 58e-07 7. 65e-06 1. 44e-04
U 232 1. O6e-O7 2. 88e-07 6. 80e-07 8. 20e-07 8.08e-07 3. 77e-O7 6. 51e-ll 0. 00e+00 0. 00e+00

Pa 234 8. 40e-07 5. 30e-07 5.30e-07 5. 3Oe-O7 5. 30e-07 5. 3Oe-O7 5. 3Oe-O7 5. 3Oe-O7 5. 3Oe-O7
Pa 234m 3. 32e-04 j . 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04
Pa 233 2.00e-05 2. 68e-05 2. 70e-O3 2. 74e-05 2.86e-05 4. 58e-05 1. 54e-04 1.87e-04 1. 35e-04
Pa 231 5. 23e-10 6. 22e-10 9. 91e-10 1.45e-O9 2. 37e-09 9. 76e-O9 9. 35e-08 9. 83e-07 1. O2e-O5
Th 234 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04 3. 31e-04
Th 232 9. 12e-16 3. 36e-15 1. 32e-14 2.54e-14 5.00e-14 2.48e-13 2. 62e-12 3. 69e-ll 5. 58e-09
Th 231 7.,79e-05 4.,36e-06 4.,36e-06 4. 36e-06 4. 36e-06 4. 37e-06 4. 52e-06 5. 83e-06 1.,O2e-O5
Th 230 1.,48e-09 3.,89e-09 1.,35e-08 2. 56e-08 5. 00e-08 2. 51e-07 2. 66e-06 2. 58e-05 3.,38e-04
Th 229 1..53e-13 2.,44e-13 7.,23e-13 1.,57e-12 4.,12e-12 7.,38e-ll 1.,69e-08 2. 63e-06 1.,44e-04
Th 228 7..41e-09 6..80e-08 4.,46e-07 7. 31e-O7 8. 18e-O7 3. 87e-O7 6.,94e-ll 3. 69e-ll 5.,58e-09
Th in 3.20e-12 2..19e-ll 1,.15*-10 2.,76e-10 7.,23e-10 6.,86e-09 9..22e-O8 9. 69e-07 1,.01e-05

Ac 228 2..46e-17 2 .67e-16 3,.48e-15 1,,09e-14 3,.14e-14 2,,48e-13 2,.62e-12 3.,69e-ll 5..58e-09
Ac 227 4 .28e-12 2 ,22e-ll 1 .16e-10 2..80e-10 7,.32e-10 6..96e-09 9 .35e-08 9.,83e-07 1..02e-05
Ac 225 2 .48e-12 2 .44e-13 7 .23e-13 1,.57e-12 4,.12e-12 7,.38e-ll 1 .69e-08 2..63e-06 1..44e-04
Ra 228 2 .46e-17 2 •67e-16 3 .48e-15 1 .09e-14 3 .14e-14 2 •48e-13 2 .62e-12 3..69e-ll 5 .58e-09
Ra 226 2 .19e-13 1 •38e-12 1 .65e-ll 5 .88e-ll 2 .22e-10 5 .33e-09 5 .00e-07 2 .00e-05 3 .38e-04
Ra 225 2 .99e-12 2 .44e-13 7 .23e-13 1 .57e-12 4 .12e-12 7 .38e-U 1 .69e-08 2 .63e-06 1 .44e-04
Ra 224 6 .95e-09 6 .80e-08 4 .46e-07 7 .31e-O7 8 .18e-07 3 .87e-07 6 .95e-ll 3 .69e-ll 5 .58e-09
Ra 223 2 .70e-12 2 .22e-ll 1 .17e-10 2 .80e-10 7 .33e-10 6 .96e-09 9 .35e-08 9 .83e-07 1 .02e-05

Fr 223 5 .90e-14 3 .06e-13 1 .61e-12 3 •87e-12 1 •Ole-11 9 .60e-ll 1 .29e-09 1.36e-08 1 .41e-07
Fr 221 2 .48e-12 2 .44e-13 7 .23e-13 1 .57e-12 4 .12e-12 7 .38e-ll 1 •69e-08 2 .63e-06 1 .44e-04

Rn 222 2 .10e-13 1 .38e-12 1 .65e-ll 5 .88e-ll 2 .22e-10 5 .33e-09 5 .0Oe-07 2 .00e-05 3 .38e-04
Rn 220 6 .95e-09 6 .80e-08 4 .46e-07 7.31e-O7 8 .18e-07 3 .87e-07 6 .95e-ll 3 .69e-ll 5 .58e-09
Rn 219 2 .70e-12 2 .22e-ll 1 .17e-10 2 .80e-10 7•33e-10 6 .96e-09 9 .35e-08 9 .83e-07 1 .02e-05

At 217 2 •48e-12 2 .44e-13 7 .23e-13 1 .57e-12 4 •12e-12 7 .38e-ll 1 .69e-08 2 •63e-06 1.44e-04

Page A.35
U02 Fuel - Actinides Activity: Ci/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Po 218 2.10e-13 1.38e-12 1.65e-ll 5.88e-ll 2.22e-10 5.33e-O9 5.00e-07 2.00e-05 3.38e-04
Po 216 6.95e-09 6.80e-08 4.46e-07 7.31e-O7 8.18e-07 3.87e-07 6.95e-ll 3.69e-ll 5.58e-09
Po 215 2.70e-12 2.22e-ll 1.17e-10 2.80e-10 7.33e-10 6.96e-09 9.35e-08 9.83e-07 1.02e-05
Po 214 2.10e-13 1.38e-12 1.64e-ll 5.87e-ll 2.22e-10 5.33e-09 4.99e-07 2.00e-05 3.38e-04
Po 213 2.43e-12 2.39e-13 7.07e-13 1.54e-12 4.03e-12 7.22e-ll 1.65e-08 2.57e-06 1.41e-04
Po 212 4.45e-09 4.36e-08 2.86e-07 4.68e-07 5.24e-07 2.48e-07 4.45e-ll 2.36e-ll 3.58e-09
Po 211 7.57e-15 6.22e-14 3.26e-13 7.85e-13 2.05e-12 1.,95e-ll 2.62e-10 2.75e-09 2.86e-08
Po 210 2.86e-16 1.04e-14 9.15e-13 5.,95e-12 4.,06e-ll 2.,96e-09 4.,99e-07 2.00e-05 3.38e-04
Bi 214 2.10e-13 1.38e-12 1.,64e-ll 5.88e-ll 2.22e-10 5.,33e-09 4.,99e-07 2.00e-05 3.,38e-04
Bi 213 2.,48e-12 2.,44e-13 7.,23e-13 1.,57e-12 4.,12e-12 7,.38e-ll 1.,69e-08 2..63e-06 1,.44e-04
Bi 212 6.,95e-09 6.,80e-08 4.,46e-07 7.,31e-07 8..18e-07 3,.87e-07 6..95e-ll 3.69e-ll 5.,58e-09
Bi 211 2.,70e-12 2,.22e-ll 1,,17e-10 2,.80e-10 7..33e-10 6 .96e-09 9..35e-08 9.,83e-07 1..02e-05
Bi 210 1,.26e-15 2,.30e~14 9.,15e-13 5,.95e-12 4 .06e-ll 2 .96e-09 4,.99e-07 2..00e-05 3,.38e-04
Pb 214 2.10e-13 1.38e-12 1,64e-ll 5,.88e-ll 2.22e-10 5.33e-09 4 .99e-07 2 .00e-05 3.38e-04
Pb 212 6.95e-09 6 .80e-08 4.46e-07 7.31e-O7 8.18e-07 3.87e-07 6 .95e-ll 3 .69e-ll 5 .58e-09
Pb 211 2.70e-12 2.22e-ll 1.17e-10 2.80e-10 7.33e-10 6•96e-09 9.35e-08 9 .83e-07 1.02e-05
Pb 210 1.38e-15 2.30e-14 9.15e-13 5.95e-12 4•06e-ll 2.96e-09 4 .99e~07 2 .00e-05 3,38e-04
Pb 209 2.48e-12 2.44e-13 7.23e-13 1•57e-12 4.12e-12 7•38e-ll 1.69e-08 2.63e-06 1.44e-04
Tl 209 5.37e-14 5 .28e-15 1.56e-14 3.39e-14 8.90e-14 1.59e-12 3•64e-10 5.68e-08 3.10e-06
Tl 208 2.50e-09 2.44e-08 1.60e-07 2.63e-O7 2.94e-07 1.39e-07 2•5Oe-ll 1.33e-ll 2.Ole-09
Tl 207 2.69e-12 2.21e-ll 1.16e-10 2.80e-10 7.31e-10 6.94e-09 9.32e-08 9.80e-07 1.02e-05
TOTAL 5.41e+04 2.29e+01 1.90e+01 1.53e+01 9•99e+00 1.35e+00 5•46e-01 2.13e-01 6.53e-03
U0 2 Fuel - Fission Products Activity: Ci/kg inital U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year
H 3 l.A0e-01 1.32e-01 1.06e-01 7.99e-02 4.56e-02 5.11e-04 0.00e+00 O.OOe+00 O.OOe+00

Se 79 9.01e-05 9.01e-05 9.01e-05 9.01e-05 9.01e-05 9.00e-05 8.92e-O5 8.10e-05 2.09e-09

Kr 81 1.15e-10 1.15e-10 1.15e-10 1.15e-10 1.15e-10 1.15e-10 1.14e-10 l.lle-10 4.22e-12
Kr 85 2.35e+00 2.20e+00 1.70e+00 1.23e+00 6.44e-01 3.65e-03 O.OOe+00 0.00e+00 O.OOe+00
Rb 86 5.05e-01 6.46e-07 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00
Rb 87 4.80e-09 4.80e-09 4.80e-09 4.80e-09 4.80e-09 4.80e-09 4.80e-09 4.80e-09 4.80e-09
Sr 89 8.26e+02 5.49e+00 1.07e-08 1.39e-19 0.00e+00 0.00e+00 0.00e+00 0.00e+00 O.OOe+00
Sr 90 1.76e+01 1.72e+01 1.56e+01 1.39e+01 1.09e+01 1.63e+OO 8.08e-10 O.OOe+00 O.OOe+00
Y 90 1.93e+01 1.72e+01 1.56e+01 1.39e+01 1.09e+01 1.63e+OO 8.09e-10 0.0Oe+0O O.OOe+00
Y 91 1.06e+03 1.41e+01 4.28e-07 1.72e-16 0.00e+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00
Zr 93 4.21e-04 4.22e-04 4.22e-04 4.22e-04 4.22e-04 4.22e-04 4.22e-04 4.20e-04 2.68e-04
Zr 95 1.46e+03 2.79e+01 3.72e-06 9.48e-15 O.OC'j+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00
Nb 93m 7.52e-06 2.71e-05 9.60e-05 1.65e-04 2.59e-04 3.99e-04 4.01e-04 3.99e-04 2.55e-04
Nb 94 4.39e-08 4.39e-08 4.39e-08 4.39e-08 4.39e-08 4.38e-08 4.24e-08 3.12e-08 6.49e-23
Nb 95 1.34e+03 6.26e+01 8.25e-06 2.11e-14 O.OOe+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00
Nb 95m 1.03e+01 2.07e-01 2.76e-08 7.03e-17 0.00e+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00
Tc 99 3.41e-03 3.47e-03 3.47e-03 3.47e-03 3.47e-03 3.47e-03 3.46e-03 3.36e-03 1.34e-04
Ru 103 1.53e+03 2.42e+00 1.54e-ll 1.55e-25 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ru 106 2.19e+02 1.10e+02 7.03e+00 2.26e-01 2.33e-04 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Rh 103m 1.38e+03 2.19e+00 1.39e-ll 1.40e-25 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+00
Rh 106 3.57e+02 1.10e+02 7.03e+00 2.26e-01 2.33e-04 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Pd 107 2.79e-05 2.79e-05 2.79e-05 2.79e-05 2.79e-05 2.79e-O5 2.79e-05 2.79e-O5 2.51e-05
Ag 108 4.70e-06 7.05e-10 90e-10 71e-10 36e-10 lie-10 3.02e-12 O.OOe+00 O.OOe+00
Ag 108m 7..97e-09 7.92e-09 75e-09 ,54e-09 lAe-09 62e-09 3.39e-ll O.OOe+00 O.OOe+00
Ag 109m 2..85e+02 5.31e-10 99e-ll ,9le-12 67e-14 iOOe+00 00e+0O O.OOe+00 O.OOe+00
Ag 110 5..05e+01 1.98e-03 44e-05 .17e-O7 64e-12 , OOe+00 00e+OO O.OOe+00 O.OOe+00
Ag 110m 4.11e-01 1.49e-01 59e-03 63e-05 50e-10 , 00e+00 00e+OO O.OOe+00 O.OOe+00
Ag 111 5.33e+01 9.29e-14 00e+00 .00e+00 O.OOe+00 O.OOe+00 00e+00 O.OOe+00 0,OOe+00
Page A.37
U02 Fuel - Fission Products Activity: Ci/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 10« Year

Cd 109 9.17e-10 5.31e-10 5.99e-ll 3.91e-12 1.67e-14 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Cd 113 1.07e-17 1.17e-17 1.17e-17 1.17e-17 1.17e-17 1.17e-17 1.17e-17 1.17e-17 1.17e-17
Cd 113m 7.63e-03 7.26e-03 5.92e-03 4.59e-03 2.75e-03 4.67e-05 5.57e-25 O.OOe+OO O.OOe+OO
Cd 115m 6.80e-01 2.33e-03 3.20e-13 1.50e-25 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO

In 114 9.88e-05 3.38e-07 4.42e-16 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
In 114m 5.88e-05 3.53e-07 4.62e-16 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
In 115 3.73e-15 3.99e-15 3.99e-15 3.99e-15 3.99e-15 3.99e-15 3.99e-15 3.99e-15 3.99e-15
In 115m 7.66e+00 2.34e-07 3.21e-17 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO

Sn 117m 2.93e-03 4.10e-ll O.OOe+00 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Sn 119m 4.66e-02 1.66e-02 2.66e-04 1.51e-06 4.92e-ll O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Sn 121m 3.90e-05 3.85e-05 3.67e-05 3.44e-05 3.03e-05 l.lle-05 1.31e-10 O.OOe+OO O.OOe+OO
Sn 123 1.45e+00 2.05e-01 8.07e-05 4.48e-09 1.38e-17 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Sn 125 1.08e+01 4.23e-ll 0.00e+00 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Sn 126 1.40e-04 1.40e-04 1.40e-04 l.A0e-04 1.40e-04 1.40e-04 1.39e-04 1.31e-04 1.37e-07

Sb 124 l.lle-01 1.66e-03 8.19e-ll 6.03e-20 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Sb 125 2.84e+00 2.29e+00 8.42e-01 2.41e-01 1.97e-O2 3.98e-ll O.OOe+OO O.OOe+OO O.OOe+OO
Sb 126 7.28e-01 1.97e-05 1.96e-05 1.96e-05 1.96e-05 1.96e-05 1.95e-05 1.83e-05 1.92e-08
Sb 126m 6.23e-01 1.40e-04 1.40e-04 l.AOe-OA 1.40e-04 1.40e-04 1.39e-04 1.31e-04 1.37e-O7

Te 123 l.O3e-17 1.45e-17 1..51e-17 1.51e-17 1.51e-17 1.51e-17 1.51e-17 1.51e-17 1.51e-17
Te 123m 1.45e-04 1.75e-05 3..70e-09 9.44e-14 6.15e-23 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Te 125m 3.93e-01 5..55e-01 2..05e-01 5..88e-02 4.81e-03 9.72e-12 O.OOe+OO O.OOe+OO O.OOe+OO
Te 127 9.81e+01 9..17e-01 8.45e-05 7..64e-10 6.24e-20 0.,OOe+00 O.OOe+OO O.OOe+OO O.OOe+OO
Te 127m 9.02e+00 9..36e-01 8.63e-05 7..80e-10 6.37e-20 0.,OOe+00 O.OOe+OO O.OOe+OO O.OOe+OO
Te 129 3.31e+02 1..67e-02 1.35e-15 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Te 129m 4.77e+01 2.56e-02 2.08e-15 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO

I 129 7.61e-06 7.91e-06 7.91e-06 7.91e-06 7.91e-O6 7.91e-06 7.91e-06 7.90e-06 7.56e-06
I 131 9.66e+02 2.10e-ll O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO

Xe 129m 3.32e-03 5.98e-17 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Xe 131m 1.08e+01 1.94e-08 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Xe 133 1.84e+03 2.48e-18 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO

C? 134 ,51e+01 1.08e+01 2.82e+00 5.25e-01 1.82e-02 3.80e-14 O.OOe+OO O.OOe+OO O.OOe+OO
Cs 135 ,67e-05 2.74e-05 2.74e-05 2.74e-05 2.74e-05 2.74e-O5 2.73e-05 2.73e-05 2.02e-05
Cs 136 ,25e+01 9.07e-08 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Cs 137 ,60e+01 2.55e+01 2.32e+01 2.07e+01 1.65e+01 2.62e+OO 2.74e-09 O.OOe+OO O.OOe+OO
Page A.38
U0 2 Fuel - Fission Products Activity: Ci/kg inital U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 10* Year

Ba 136m 3.71e+OO 1.50e-08 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ba 137m 2.49e+01 2.41e+01 2.2Oe+Ol 1.96e+01 1.56e+01 2.48e+00 2.59e-O9 0.00e+00 0.00e+00
Ba 140 1.64e+03 4.15e-06 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

La 138 3.79e-14 3.79e-14 3.79e-14 3.79e-14 3.79e-14 3.79e-14 3.79e-14 3.79e-U 3.79e-l4
La 140 1.75e+O3 4.78e-06 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Ce 141 1.55e+03 6.44e-01 1.90e-14 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ce 142 6.50e-09 6.50e-09 6.50e-09 6.50e-09 6.50e-09 6.50e-09 6.50e-09 6.50e-09 6.50e-09
Ce 144 5.69e+02 2.34e+02 6.63e+00 7.72e-02 1.05e-05 0.00e+00 0.00e+0O 0.00e+00 0.00e+00

Pr 143 1.36e+03 1.18e-05 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Pr 144 5.92e+02 2.34e+02 6.63e+00 7.72e-02 1.05e-05 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Pr 144m 6.85e+00 2.80e+00 7.96e-02 9.27e-04 1.26e-07 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Nd 144 1.39e-13 2.64e-13 3.49e-13 3.51e-13 3.51e-13 3.51e-13 3.51e-13 3.51e-13 3.51e-13
Nd 147 6.09e+02 6.97e-08 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Pm 147 6.95e+01 5.88e+01 2.04e+01 5.45e+00 3.88e-01 2.56e-10 0.00e+00 0.00e+00 0.00e+00
Pm 148 9.59e+01 7.83e-04 1.75e-14 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Pm 148m 6.39e+0O 1.39e-02 3.11e-13 0.00e+00 0.00e+00 0.00e+00 0.00e+0O 0.00e+00 0.00e+00

Sm 147 1.41e-10 5.87e-10 1.55e-09 1.93e-09 2.05e-09 2.06e-09 2.06e-09 2.06e-09 2.06e-09
Sm 148 2.88e-15 3.15e-15 3.15e-15 3.15e-15 3.15e-15 3.15e-15 3.15e-15 3.15e-15 3.15e-15
Sm 149 1.36e-16 4.30e-16 4.30e-16 4.30e-16 4.30e-16 4.30e-16 4.30e-16 4.30e-16 4.30e-16
Sm 151 5.86e-02 6.50e-02 6.30e-02 6.07e-02 5.62e-02 3.03e-02 2.96e-05 0.00e+00 0.00e+00

Eu 152 3.24e-O4 3.08e-04 2.51e-04 1.95e-04 1.17e-04 1.98e-06 0.00e+00 0.00e+00 0.00e+0O
Eu 154 1.13e+00 1.04e+00 7.52e-01 5.03e-01 2.24e-01 3.55e-04 0.00e+00 0.00e+00 0.00e+00
Eu 155 8.63e-01 7.51e-01 4.29e-01 2.13e-01 5.28e-02 7.36e-O7 0.00e+00 0.00e+00 0.00e+00
Eu 156 8.3Ae+01 4.35e-06 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 O.00e+00 0.00e+00

Gd 152 4.45e-17 4.53e-17 4.73e-17 4.92e-17 5.20e-17 5.60e-17 5.61e-17 5.61e-17 5.61e-17
Gd 153 9.01e-04 3.16e-04 4.77e-06 2.53e-08 7.11e-13 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Tb 160 1.21e-01 3.64e-03 3.01e-09 7.47e-17 0.00e+00 0.00e+00 0.00e+00 0.00e+OO 0.00e+00
Tb 161
9.51e-01 1.09e-16 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ho 166m
3.71e-O8 3.71e-O8 3.7Oe-O8 3.69e-08 3.67e-08 3.50e-08 2.08e-08 1.15e-10 0.00e+00
TOTAL
1.55e+05 9.68e+02 1.31e+O2 7.7Oe+Ol 5.54e+01 8.39e+00 4.76e-O3 4.60e-03 7.10e-O4 Page A.39
 APPENDIX B

U P , FUEL - IMPURITY ACTIVATION PRODUCTS

Fuel Bruce "A" Reactor

Burnup 685 GJ/kg initial U
Neutron Flux 1.67 z 1014 n-cnr^s- 1
Power 0.034664 MW/kg initial U
Irradiation Time 228.72 d

Burnup-Dependent Library
ORIGEN-S Code
 - B.3 -

CONTENTS

Page
UO2 Fuel - Impurity Activation Products Mass : (mol/kg initial U) B.4
U0 2 Fuel - Impurity Activation Products Mass : (g/kg initial U) B.ll
U0 2 Fuel - Impurity Activation Products Activity : (Bq/kg initial U) B.18
U0 2 Fuel - Impurity Activation Products Activity : (Ci/kg initial U) B.21
UO, Fuel - Iapurity Activation Products Mass: uol/kg initial U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10* Year 10 4 Year 10* Year

H 1 1.73e-05 1. 73e-05 1.73e-O5 1.73e-O5 1.73e-O5 1.73e-05 1.73e-05 1.73e-05 1.73e-05

H 2 7. 32e-09 7. 32e-09 7.32e-09 7.32e-09 7.32e-09 7.32e-09 7.32e-09 7.32e-09 7.32e-O9
H 3 2. 62e-10 2. 48e-10 1.98e-10 1.50e-10 8.54e-ll 9.58e-13 0.00e+00 0.00e+00 0.00e+00
He 3 6. 15e-13 1.49e-ll 6.48e-ll 1.13e-10 1.78e-10 2.62e-10 2.63e-10 2. 63e-10 2. 63e-10
He 4 1.42e-04 1.42e-04 1.42e-04 1.42e-04 1.42e-04 1.42e-04 1.42e-04 1.42e-04 1.42e-04
Li 6 3.49e-13 3.49e-13 3.49e-13 3.49e-13 3.49e-13 3.49e-13 3.49e-13 3.49e-13 3.49e-13
Li 7 5.55e-06 5.55e-06 5.55e-O6 5.55e-O6 5.55e-06 5.55e-06 5.55e-06 5.55e-06 5.55e-06
Be 9 2. Ole-08 2.Ole-08 2.Ole-08 2.Ole-08 2.Ole-08 2.Ole-08 2.Ole-08 2.Ole-08 2.Ole-08
Be 10 8.54e-10 8.54e-10 8.54e-10 8.54e-10 8.54e-10 8.54e-10 8.53e-10 8.50e-10 5.53e-10
B 10 3.67e-10 3.67e-10 3.,67e-10 3.67e-10 3.67e-10 3.67e-10 3.67e-10 3. 71e-10 6. 67e-10
B 11 2. 28e-05 2. 28e-05 2.,28e-05 2. 28e-05 2. 28e-05 2. 28e-05 2. 28e-05 2. 28e-05 2. 28e-O5
C 12 8.,23e-03 8. 23e-O3 8.,23e-O3 8.23e-O3 8.,23e-03 8.,23e-03 8. 23e-03 8. 23e-03 8..23e-O3
C 13 2..26e-04 2..26e-04 2,,26e-04 2.,26e-04 2.,26e-04 2.,26e-04 2.,26e-04 2..26e-04 2..26e-04
C 14 1..84e-05 1,,84e-05 1,.84e-05 1,,84e-05 1.,84e-05 1,.82e-O5 1.,63e-05 5..50e-06 0,.O0e+O0
N 14 3,.54e-O3 3,.54e-O3 3,.54e-03 3,,54e-03 3..54e-03 3,.54e-03 3..54e-03 3 .55e-03 3.,56e-U?>
N 15 1,,38e-05 1,.38e-05 1,,38e-05 1..38e-O5 1,.38e-05 1,.38e-05 1,.38e-05 1,.38e-05 1,,38e-05
0 16 8 .38e+00 8 .38e+OO 8 .38e+00 8 .38e+00 8 .38e+00 8 .38e+00 8 .38e+00 8 .38e+00 8 .38e+OO
0 17 3 .19e-03 3 .19e-03 3 .19e-03 3 .19e-O3 3 .19e-03 3 .19e-03 3 .19e-03 3 .19e-03 3 .19e-03
0 18 1 •71e-02 1 .71e-O2 1 .71e-O2 1 .71e-O2 1 .71e-02 1 •71e-02 1 .71e-02 1 .71e-02 1 .71e-O2
F 19 1 .08e-08 1 .08e-08 1 .08e-08 1 .O8e-O8 1 .08e-08 1•08e-08 1 .08e-08 1 .08e-08 1 .08e-08
20 1 .48e-13 1 .48e-13 1.48e-13 1 .48e-13 1.48e-13 1 .48e-13 1 .48e-13 1 .48e-13 1 .48e-13
21 4 .97e-09 4 .97e-09 4 .97e-09 4 .97e-09 4 .97e-09 4 .97e-09 4 .97e-09 4 •97e-09 4 .97e-09
22 7 .15e-09 7 .15e-09 7 .15e-09 7 .15e-09 7 .15e-09 7 .15e-09 7 .15e-09 7 .15e-09 7 .15e-09
Na 23 1 .39e-09 1 .39e-09 1 •39e-09 1 .39e-09 1•39e-09 1 .39e-09 1 .39e-09 1 .39e-09 1 ,39e-09
Mg 24 1 •62e-03 1 .62e-O3 1 .62e-O3 1 .62e-03 1 .62e-03 1 .62e-O3 1 .62e-O3 1 •62e-03 1 .62e-03
Mg 25 2 .06e-04 2 .06e-04 2 .06e-04 2 .06e-04 2 .06e-04 2 .06e-04 2 .06e-04 2 .06e-04 2 .06e-04
Mg 26 2 .26e-O4 2 .26e-04 2 .26e-04 2 .26e-04 2 .26e-04 2 .26e-04 2 .26e-04 2 .26e-04 2 .26e-04
AI 27 1 .85e-03 1 .85e-03 1•85e-03 1 .85e-03 I.85e-03 1.85e-03 1.85e-O3 1.85e-03 1,85e-03
Page B.4
U0 2 Fuel - Impurity Activation Products Mass: aol/kg initial U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 10* Year

Si 28 1.97e-03 1.97e-03 1.97e-03 1.97e-03 1.97e-03 1.97e-03 1.97e-03 1.97e-03 1.97e-03

Si 29 1.00e-04 1.00e-04 1.00e-04 1.00e-04 1.00e-04 1.00e-04 l.OOe-04 1.00e-04 l.OOe-04
Si 30 6.62e-05 6.62e-05 6.62e-05 6.62e-05 6.62e-05 6.62e-05 6.62e-05 6.62e-05 6.62e-05
Si 32 1.55e-14 1.55e-14 1.53e-14 1.52e-14 1.49e-14 1.26e-14 1.9Oe-15 1.17e-23 0.00e+00

P 31 1.93e-08 1.93e-08 1.93e-08 1.93e-08 1.93e-08 1.93e-08 1.93e-O8 1.93e-08 1.93e-08

P 32 8.41e-13 1.85e-18 1.82e-18 1.8Oe-18 1.76e-18 1.49e-18 2.25e-19 1.38e-27 0.00e+00
S 32 4.25e-12 5.09e-12 5.09e-12 5.09e-12 5.09e-12 5.09e-12 5.10e-12 5.11e-12 5.11e-12
S 33 1.73e-15 1.76e-15 1.76e-15 1.76e-15 1.76e-15 1.76e-15 1.76e-15 1.76e-15
S 34 9.41e-14 9.41e-14 9.41e-14 9.41e-14 9.41e-14 9.41e-14 9.41e-14 9.41e-14 9.41e-14
S 35 l.lle-17 6.13e-19 5.72e-24 2.95e-30 0.00e+00 O.OOe+00 0.00e+00 0.00e+00 O.OOe+00
Cl 35 4.58e-18 1.51e-17 1.57e-17 1.57e-17 1.57e-17 1.57e-17 1.57e-17 1.57e-17 1.57e-17
Cl 36 3.89e-18 3.89e-18 3.89e-18 3.89e-18 3.89e-18 3.89e-18 3.88e-18 3.80e-18 3.89e-19
Cl 37 9.14e-08 1.17e-O7 1.17e-07 1.17e-O7 1.17e-O7 1.17e-07 1.17e-07 1.17e-07 l,17e-07
Ar 37 2.6Oe-O8 1.88e-ll 5.19e-24 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ar 38 4.02e-ll 4.02e-ll 4.02e-ll 4.02e-ll 4.02e-ll 4.02e-ll 4.02e-ll 4.02e-ll 4.02e-ll
Ar 39 2.08e-10 2.08e-10 2.05e-10 2.03e-10 1.98e-10 1.61e-10 1.58e-ll 1.34e-21 O.OOe+00
Ar 40 1.41e-09 1.41e-09 1.41e-09 1.41e-09 1.41e-09 1.41e-09 1.41e-O9 1.41e-09 1.42e-09
Ar 42 1.56e-18 1.53e-18 1.41e-18 1.27e-18 1.03e-18 1.91e-19 1.18e-27 O.OOe+00 O.OOe+00
K 39 2.05e-13 7.41e-13 2.87e-12 5.50e-12 1.07e-ll 4.75e-ll 1.92e-10 2.08e-10 2.08e-10
K 40 2.?le-07 2.21e-07 2.21e-07 2.21e-07 2.21e-07 2.21e-O7 2.21e-O7 2.21e-07 2.21e-07
K 41 8.13e-09 8.14e-09 8.17e-09 8.22e-09 8.30e-09 9.01e-09 1.69e-O8 9.37e-08 1.32e-06
Ca 40 1.21e-03 1.21e-03 1.21e-03 1.21e-03 1.21e-03 1.21e-O3 1.21e-O3 1.21e-03 1.21e-03
Ca 41 1.32e-06 1.32e-06 1.32e-06 1.31e-06 1.31e-06 1.31e-06 1.31e-06 1.23e-06 1.57e-09
Ca 42 8.04e-06 8.04e-06 8.04e-06 8.04e-06 8.04e-06 8.04e-06 8.04e-O6 8.04e-06 8.04e-06
Ca 43 1..61e-06 1.61e-06 1.61e-06 1.61e-06 1.61e-O6 1.61e-06 1.61e-O6 1.61e-06 1.61e-06
Ca 44 2.•60e-05 2.60e-05 2.60e-05 2.60e-05 2.60e-05 2.60e-05 2.6Oe-O5 2.60e-05 2.60e-05
Ca 45 4.•34e-08 9.27e-09 1.93e-ll 8.57e-15 1.69e-21 O.OOe+00 0.00e+00 O.OOe+00 O.OOe+00
Ca 46 4.•35e-08 4.35e-08 4.35e-08 4.35e-08 4.35e-08 4.35e-08 A.35e-O8 4.35e-08 4.35e-08
Ca 48 2.36e-06 2.36e-06 2.36e-06 2.36e-06 2.36e-06 2.36e-O6 2.36e-O6 2.36e-06 2.36e-06

Sc 45 2.36e-08 5.78e-08 6.70e-08 6.70e-08 6.70e-08 6.70e-08 6.7Oe-O8 6.70e-08 6.7Oe-O8

Sc 46 3.75e-10 1.83e-ll 1.03e-16 2.83e-23 2.14e-36 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ti 46 2.02e-10 5.59e-10 5.77e-10 5.77e-10 5.77e-10 5.77e-10 5.77e-10 5.77e-10 5.77e-10
Ti 47 1.03e-10 1.07e-10 1.07e-10 1.07e-10 1.07e-10 1.07e-10 1.07e-10 1.07e-10 1.07e-10
Page B.5
U02 Fuel - Iapucity Activation Products Mass: aol/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Ti 48 2.43e-13 2.43e-13 2.43e-13 2.43e-13 2.43e-13 2.43e-13 2.43e-13 2.43e-13 2.43e-13

Ti 49 6.37e-09 6.37e-09 6.37e-09 6.37e-09 6.37e-O9 6.37e-09 6.37e-09 6.37e-09 6.37e-09
Ti 50 2.94e-10 2.94e-10 2.94e-10 2.94e-10 2.94e-10 2.94e-10 2.94e-10 2.94e-10 2.94e-10
V 50 9.66e-10 9.66e-10 9.66e-10 9.66e-10 9.66e-10 9.66e-10 9.66e-10 9.66e-10 9.66e-10
V 51 6.89e-07 8.34e-07 8.34e-07 8.34e-07 8.34e-07 8.34e-07 8.34e-07 8.34e-07 8.34e-07
Cr 50 2.Ole-05 2.Ole-05 2.Ole-05 2.Ole-05 2.Ole-05 2.Ole-05 2.Ole-05 2.Ole-05 2.Ole-05
Cr 51 1.45e-07 1.56e-ll 2.O7e-27 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Cr 52 4.02e-04 4.02e-04 4.02e-04 4.02e-04 4.02e-04 4.O2e-O4 4.02e-04 4.02e-04 4.02e-04
Cr 53 4.43e-05 4.43e-05 4.43e-05 4.43e-05 4.43e-05 4.43e-05 4.43e-05 4.43e-05 4.43e-05
Cr 54 1.34e-05 1.34e-05 1.34e-05 1.34e-05 1.34e-05 1.34e-05 1.34e-05 1.34e-05 1.34e-05

Mn 54 1.09e-08 4.84e-09 1.89e-10 3.29e-12 9.98e-16 0.00e+00 0.00e+0O 0.00e+00 0.O0e+00

Mn 55 1.76e-04 1.76e-04 1.76e-04 1.76e-04 1.76e-04 1.76e-04 1.76e-04 1.76e-04 1.76e-04
Fe 54 1.03e-04 1.03e-04 1.,03e-04 1.03e-04 1.03e-04 1.03e-04 1.03e-O4 1.03e-04 1.03e-04
Fe 55 5.,58e-07 4.32e-07 1.,55e-07 4.29e-08 3.29e-09 3.95e-18 0.,00e+00 0.00e+00 0.,00e+00
Fe 56 1.,64e-03 1.,64e-03 1,.64e-03 1.64e-03 1..64e-03 1.,64e-03 1.,64e-03 1.64e-03 1,.64e-03
Fe 57 4.,93e-05 4.,93e-05 4.,93e-05 4.93e-O5 4.,93e-05 4.,93e-O5 4.,93e-05 4.93e-05 4.,93e-05
Fe 58 5,,47e-06 5..48e-06 5,.48e-06 5.,48e-06 5..48e-06 5..48e-06 5,,48e-06 5.,48e-06 5,,48e-06
Fe 59 4,.67e-09 1,.60e-ll 2.19e-21 1.,03e-33 0.,00e+00 0,.00e+00 0,•00e+00 0..00e+00 0,.00e+00
Co 58 8 .98e-09 2,.51e-10 1.53e-16 2,.62e-24 0 .00e+00 0 .00e+00 0 .00e+00 0,.00e+00 0 .00e+00
Co 59 6 .17e-08 6 .63e-08 6.65e-08 6.,66e-08 6.70e-08 6.96e-08 9 .90e-08 3,.8Oe-O7 3.62e-06
Co 60 3.63e-09 3.18e-09 1.88e-09 9,,74e-10 2.62e-10 7.05e-15 0 .00e+00 0,.00e+00 0 .00e+00
Ni 58 3.44e-04 3.44e-04 3.44e-04 3.44e-04
3.44e-04 3.44e-04 3.44e-04
3,44e-04 3.44e-04
Ni 59 3.55e-06 3.55e-06 3.55e-O6 3.55e-06
3.55e-06 3.55e-06 3.52e-06
3.24e-06 3.44e-10
Ni 60 1.33e-04 1.33e-O4 1.33e-04 1•33e-04
1.33e-04 1.33e-04 1.33e-04
1.33e-04 1.33e-04
Ni 61 6.69e-06 6.69e-06 6.69e-06 6•69e-06
6.69e-06 6.69e-06 6,69e-06
6.69e-06 6.69e-06
Ni 62 1•77e-05 1.77e-05
1.77e-05 1.77e-O5 1.77e-O5 1.77e-O5 1•77e-05 1.77e-05 1.77e-05
Ni 63 6•43e-07 6.2Oe-O7 5.98e-07 5.56e-07
6.38e-07 3.12e-O7 4.70e-10 0.00e+00 0.00e+00
Ni 64 6.32e-06 6.33e-06 6•33e-06 6.33e-06 6.33e-06 6.33e-O6 6.33e-06 6.33e-06 6.33e-06
Cu 63 2.15e-04 2.15e-04 2.15e-04 2.15e-04 2•15e-04 2.15e-04 2.16e-04 2.16e-04 2.16e-04
Cu 65 9.63e-05 9.63e-05 9•63e-05 9.63e-05 9.63e-05 9.63e-05 9.63e-05 9.63e-05 9.63e-05
Zn 64 9•92e-07 9•96e-07 9•96e-O7 9.96e-07 9.96e-O7 9,96e-07 9.96e-07 9.96e-07 9.96e-07
Zn 65 9'.37e-10 3.32e-10 5i.22e-12 2.91e-14 9•02e-19 0 .00e+00 0.00e+00 0.00e+00 0 .00e+00
Zn 66 5>.77e-07 5.77e-07 5i.77e-O7 5.77e-O7 5•77e-O7 5.77e-O7 5.77e-O7 5.77e-07 5.77e-O7
Page B.6
UO, Fuel - Impurity Activation Products Mass: aol/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 10* Year

Zn 67 6.65e-10 6.65e-10 6.65e-10 6.65e-10 6.65e-10 6.65e-10 6.65e-10 6.65e-10 6.65e-10

Zn 68 5.06e-12 5.06e-12 5.06e-12 5.06e-12 5.06e-12 5.06e-12 5.06e-12 5.06e-12 5.06e-12

Ga 69 4.54e-15 4.55e-15 4.55e-15 4.55e-15 4.55e-15 4.55e-15 4.55e-15 4.55e-15 4.55e-15

Ga 71 8.13e-21 1.20e-20 1.2Oe-2O 1.20e-20 1.2Oe-20 1.2Oe-2O 1.2Oe-2O 1.20e-20 1.20e-20

Ge 70 7.94e-18 7.94e-18 7.94e-18 7.94e-18 7.94e-18 7.94e-18 7.94e-18 7.94e-18 7.94e-18

Sr 88 8.01e-18 8.01e-18 8.01e-18 8.01e-18 8.01e-18 8.01e-18 8.01e-18 8.01e-18 8.01e-18

Sr 89 4.06e-18 2.70e-20 5.26e-29 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Sr 90 2.22e-19 2.17e-19 1.97e-19 1.75e-19 1.38e-19 2.06e~20 1.02e-29 0.00e+00 0.00e+00

Y 89 3.84e-13 3.92e-13 3.92e-13 3.92e-13 3.92e-13 3.92e-13 3.92e-13 3.92e-13 3.92e-13

Y 91 8.47e-19 1.12e-20 3.40e-28 1.36e-37 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Zr 90 5.91e-16 6.12e-16 6.12e-16 6.12e-16 6.12e-16 6.12e-16 6.12e-16 6.12e-16 6.12e-16

Zr 91 5.22e-12 5.22e-12 5.22e-12 5.22e-12 5.22e-12 5.22e-12 5.22e-12 5.22e-12 5.22e-12
Zr 92 1.22e-10 1.27e-10 1.27e-10 1.27e-10 1.27e-10 1.27e-10 1.27e-10 1.27e-10 1.27e-10
Zr 93 4.38e-12 4.38e-12 4.38e-12 4.38e-12 4.38e-12 4.38e-12 4.38e-12 4.36e-12 2.78e-12
Zr 94 1.07e-ll 1.07e-ll 1.07e-ll 1.07e-ll 1.07e-ll 1.07e-ll 1.07e-ll 1.07e-ll 1.07e-ll
Zr 95 5.06e-13 9.67e-15 1.29e-21 3.29e-30 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Nb 93 1.05e-15 1.40e-14 2.12e-13 7.36e-13 2.46e-12 2.58e-ll 2.87e-10 1.40e-09 1.62e-09

Nb 93m 9.91e-14 4.08e-13 1.49e-12 2.58e-12 4.06e-12 6.17e-12 5.19e-12 8.74e-13 2.35e-17
Nb 94 6.41e-12 6.41e-12 6.41e-12 6.40e-12 6.40e-12 6.38e-12 6.19e-12 4.55e-12 9.47e-27
Nb 95 6.81e-13 1.23e-14 1.57e-21 4.02e-30 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Nb 95m 1.99e-16 4.05e-18 5.40e-25 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

No 92 6.16e-O6 6.16e-06 6.16e-06 16e-06 6.16e-06 6.16e-06 6.16e-06 6.16e~06 6.16e-06

Mo 93 1.62e-09 1.62e-09 1.62e-09 62e-09 1.62e-09 1.59e-09 1.33e-09 2.24e-10 0.00e+00
Mo 94 3.87e-06 3.87e-06 3.87e-06 87e-06 3.87e-06 3.87e-06 3.87e-06 3.87e-06 3.87e-06
Mo 95 6.29e-06 6.29e-06 6.29e-06 29e-06 6.29e-06 6.29e-06 6.29e-06 6.29e-06 6.29e-06
Mo 96 7.25e-06 7.25e-06 7.25e-06 25e-06 7.25e-06 7.25e-06 7.25e-06 7.25e-06 7.25e-06
Mo 97 4.01e-06 4.01e-06 4.01e-06 01e-06 4.01e-06 4.01e-06 A.01e-06 4.01e-06 4.01e-06
Mo 98 1.01e-05 1.01e-05 1.01e-05 01e-05 1.01e-05 1.01e-05 1.01e-05 1.01e-05 1.01e-05
Mo 100 3.99e-O6 3.99e-06 3.99e-06 3.99e-06 3.99e-06 3.99e-06 3.99e-06 3.99e-06 3.99e-06

Tc 99 1.66e-08 1.69e-08 1.69e-08 1.69e-08 1.69e-08 1.69e-08 1.69e-08 1.64e-08 6.54e-10

Ru 99 1.66e-14 7.17e-14 2.92e-13 5.68e-13 1.12e-12 5.53e-12 5.50e-ll 5.42e-10 1.63e-08

Ru 100 7.70e-10 7.70e-10 7.70e-10 7.70e-10 7.70e-10 7.70e-10 7.70e-10 7,70e-10 7.70e-10
Page B.7
U0 2 Fuel - Iapurity Activation Products Mass: aol/kg initial 0
Nuclide Discharge 1 Year 5 Year 10 Yyar 20 Year 100 Year 103 Year 104 Year 106 Year

Ru 101 5.26e-09 5.26e-09 5.26e-09 5.26e-09 5.26e-09 5.26e-09 5.26e-09 5.26e-09 5.26e-09
Ru 102 6.13e-ll 6.13e-ll 6.13e-ll 6.13e-ll 6.13e-ll 6.13e-ll 6.13e-ll 6.13e-ll 6.13e-ll
Ru 103 3.99e-14 6.33e-17 4.02e-28 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Ru 104 2.16e-18 2.16e-18 2.16e-18 2.16e-18 2.16e-18 2.16e-18 2.16e-18 2.16e-18 2.16e-18
Rh 103 4.04e-15 8.00e-15 8.Ole-15 8.Ole-15 8.Ole-15 8.Ole-15 8.Ole-15 8.Ole-15 8.Ole-15
Pd 104 4.79e-16 4.79e-16 4.79e-16 4.79e-16 4.79e-16 4.79e-16 4.79e-16 4.79e-16 4.79e-16
Pd 108 1.05e-08 1.07e-08 1.15e-08 1.24e-08 1.43e-08 2.59e-08 4.70e-08 4.7le-08 4.71e-08
Pd 110 4.26e-09 4.26e-09 4.27e-09 4.27e-09 4.27e-09 4.27e-09 4.27e-09 4.27e-09 4.27e-09
Ag 107 4.30e-06 3Oe-O6 4.30e-06 4.30e-06 4.30e-06 4.30e-06 4.30e-06 4.30e-06 4.30e-06
Ag 108 4.54e-12 26e-16 1.23e-16 1.20e-16 1.14e-16 7.34e-17 5.40e-19 0.OOe+00 0.OOe+00
Ag 108m 4..Ole-08 ,99e-08 3.90e-08 3.80e-08 3.60e-08 2.32e-O8 1.7le-10 7.91e-32 0.OOe+00
Ag 109 2..95e-06 ,95e-06 2.95e-06 2.95e-06 2.95e-06 2.95e-06 2.95e-O6 2.95e-06 2.95e-06
Ag 109m 2.47e-15 ,03e-16 3.42e-17 2.23e-18 9.53e-21 0. OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Ag 110 2.09e-12 ,26e-16 5.66e-18 3.57e-20 1.42e-24 0. OOe+00 0. OOe+00 0.OOe+00 0.OOe+00
Ag 110m 5.92e-08 2.15e-08 3.74e-10 2.36e-12 9.38e-17 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00

Cd 106 31e-08 31e-08 31e-08 31e-08 31e-08 31e-08 2.31e-08 31e-08 31e-O8
Cd 108 63e-O7 63e-07 63e-07 63e-07 63e-07 64e-07 4.66e-07 66e-07 66e-07
Cd 109 30e-10 07e-10 3.46e-ll 2.26e-12 65e-15 06e-33 0.OOe+00 0.OOe+00 0.OOe+00
Cd 110 63e-06 67e-06 1.69e-06 1.69e-06 69e-06 69e-O6 1.69e-06 1.69e-06 1.69e-06
Cd 111 51e-07 2.52e-07 2.52e-07 2.52e-07 52e-07 52e-07 52e-07 2.52e-07 2.52e-07
Cd 112 4.41e-07 4.41e-07 4.41e-07 4.41e-07 4.41e-07 41e-07 41e-07 4.41e-07 4.41e-07
Cd 113 4.lle-11 4.lle-11 4.,lle-11 4.lle-11 4.lle-11 lle-11 lle-11 4.lle-11 4.lle-11
Cd 114 7.27e-O7 7.27e-O7 7.,27e-07 7.27e-O7 7.27e-O7 27e-O7 27e-O7 7.27e-O7 7.27e-07
Cd 115m 1.04e-10 3.57e-13 4.•90e-23 2.31e-35 0.OOe+00 0. OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Cd 116 1.33e-07 1.33e-07 1.33e-O7 1.33e-O7 1.33e-07 1.33e-O7 1.33e-O7 1.33e-O7 1.33e-07

In 115 1.85e-10 2.89e-10 2.89e-10 2.89e-10 2.89e-10 2.89e-10 2.89e-10 2.89e-10 2.89e-10
Sn 116 9.02e-ll 9.02e-ll 9.02e-ll 9.02e-ll 9.02e-ll 9.02e-ll 9.02e-ll 9.02e-ll 9.02e-ll
Sn 117 1.16e-10 1.16e-10 1.16e-10 1.16e-10 1.16e-10 1.16e-10 1.16e-10 1.16e-10 1.16e-10
Sn 118 5.63e-13 5.63e-13 5.63e-13 5.63e-13 5.63e-13 5.63e-13 5.63e-13 5.63e-13 5.63e-13
Sn 119 4.20e-17 2.06e-16 2.96e-16 2.97e-16 2.97e-16 2.97e-16 2.97e-16 2.97e-16 2.97e-16
Sn 119m 2.55e-16 9.07e-17 1.45e-18 8.29e-21 2.69e-25 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Sn 120 5.36e-20 5.36e-20 5.36e-20 5.36e-2O 5.36e-2O 5.36e-2O 5.36e-20 5.36e-20 5.36e-20
Sm 149 3.28e-18 3.28e-18 3.28e-18 3.28e-18 3.28e-18 3.28e-18 3.28e-18 3.28e-18 3.28e-18
Sm 150 4.79e-15 4.79e-15 4.79e-15 4.79e-15 4.79e-15 4.79e-15 4.79e-15 4.79e-15 4.79e-15
Page B.8
U0 2 Fuel - Inpurity Activation Products Mass: aol/kg initial I)

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10 4 Year 10 s Year

Sm 151 5.O8e-17 5.04e-17 4.89e-17 4.70e-17 4.35e-17 2.35e-17 2.29e-20 0. 00e+00 0. OOe+00
Sm 152 9. 73e-14 9. 73e-14 9.73e-14 9.73e-14 9. 73e-14 9.73e-14 9. 73e-14 9. 73e-14 9. 73e-14
Sm 154 3.47e-16 3.47e-16 3.47e-16 3.47e-16 3.47e-16 3.47e-16 3.47e-16 3. 47e-16 3.47e-16
Eu 151 1.27e-20 4.O2e-19 1.93e-18 3.78e-18 7.26e-18 2. 73e-17 5.O8e-17 5.O8e-17 5.O8e-17
Eu 152 3. 13e-20 2.98e-20 2.43e-20 1.88e-20 1. 13e-20 1.92e-22 0. 00e+00 0. OOe+00 0. OOe+00
Eu 153 2.67e-10 7.64e-10 1.03e-09 1.03e-O9 1.03e-09 1.03e-09 1.03e-09 1. 03e-09 1.O3e-09
Eu 154 9. 08e-ll 8. 37e-ll 6. 07e-ll 4.05e-ll 1.81e-ll 2.87e-14 0. 00e+00 0. OOe+00 0. OOe+00
Eu 155 2. 47e-ll 2.15e-ll 1.23e-ll 6. 10e-12 1.51e-12 2. 10e-17 0. OOe+00 0. OOe+00 0. OOe+00
Eu 156 1.83e-ll 1.06e-18 0.00e+00 0.00e+00 0. 00e+00 0.00e+00 0. 00e+00 0. OOe+00 0. OOe+00

Gd 152 3. 61e-ll 3. 61e-ll 3.61e-ll 3.61e-ll 3.61e-ll 3. 61e-ll 3. 61e-ll 3. 61e-ll 3. 61e-ll
Gd 153 7.65e-10 2.68e-10 4.06e-12 2.15e-14 6. 04e-19 0. 00e+00 0. 00e+00 0. OOe+00 0. OOe+00
Gd 154 1.04e-08 1.O5e-O8 1.05e-08 1.05e-08 1.05e-08 1.05e-08 1.05e-08 1.05e-08 1.05e-08
Gd 155 2,.67e-ll 2.,99e-ll 3.91e-ll 4.53e-ll 4.,99e-ll 5. 14e-ll 5. 14e-ll 5. 14e-ll 5. 14e-ll
Gd 156 2,.22e-O7 2.,22e-O7 2.22e-07 2.22e-07 2.,22e-07 ,22e-07 2.22e-07 2. 22e-07 2.,22e-07
Gd 157 1,.38e-ll 1.,45e-ll 1.75e-ll 2.10e-ll 2.,79e-ll 7.,31e-ll 1.,73e-10 1. 74e-10 1..74e-10
Gd 158 2,.59e-07 2..59e-07 2.,59e-07 2.,59e-O7 2.,59e-O7 2.,59e-07 2.,59e-07 2..59e-O7 2..59e-07
Gd 160 1,.38e-07 1,,38e-07 1.,38e-O7 1.,38e-O7 1..38e-O7 1..38e-07 1.,38e-07 1..38e-07 1,.38e-07
Tb 157 1 .60e-10 1 .60e-10 1,.57e-10 1,.53e~10 1 .46e-10 1,.Ole-10 1,.58e-12 1..36e-30 0,.OOe+00
Tb 159 4 .05e-09 4 .13e-09 4,. 14e-09 4,. 14e-09 4,.14e-09 4,.14e-09 4..I4e-O9 4..14e-09 4 .14e-09
Tb 160 1 .13e-10 3 .39e-12 2,.80e-18 6,.96e-26 0 .00e+00 0,.00e+00 0,.00e+00 0 .OOe+00 0 .OOe+00
Dy 156 3 .65e-10 3.65e-10 3.65e-10 3 .65e-10 3 .65e-10 3 .65e-10 3 .65e-10 3 .65e-10 3.65e-10
Dy 158 8 .26e-10 8 •26e-10 8 •26e-10 8 .26e-10 8 .26e-10 8 .26e-10 8 .26e-10 8 .26e-10 8 .26e-10
Dy 159 7.46e-ll 1.29e-ll 1.16e-14 1.81e-18 4 .39e-26 0 .00e+00 0 .00e+00 0 .OOe+00 0 .OOe+00
Dy 160 1 .438-08 1.44e-08 1.44e-08 1.44e-08 1.44e-08 1.44e-08 1 .44e-08 1.44e-08 1.44e-08
Dy 161 4 . 10e-08 4 .lle-08 4 .lle-08 4 .lle-08 4 .lle-08 4 .lle-08 4 .lle-08 4 .lle-08 4 .lle-08
Dy 162 1.89e-07 1.89e-07 1.89e-07 1.89e-07 1 .89e-07 1.89e-07 1 .89e-07 1.89e-07 I.89e-07
Dy 163 2 .72e-O7 2.72e-O7 2.72e-O7 2.72e-O7 2.72e-O7 2.72e-07 2 .72e-07 2 .72e-O7 2 .72e-O7
Dy 164 2 .61e-08 2 .61e-08 2 .61e-08 2 .61e-08 2 .61e-08 2 .61e-08 2 .6le-08 2 .61e-08 2 .61e-08
Ho 165 2 .92e-07 2•92e-07 2.92e-O7 2.92e-07 2.92e-O7 2.92e-07 2 .92e-07 2 .92e-07 2 •92e-07
Ho 166m 2 .91e-09 2 .91e-09 2.90e-09 2 .89e-09 2.88e-09 2 . 75e-09 1 .63e-09 9 .O2e-12 0 .OOe+00
Er 166 7 .21e-08 7.28e-08 7.28e-08 7.28e-08 7.29e-08 7.30e-08 7 .41e-08 7 .57e-08 7•57e-08
Er 167 1 .79e-09 1.79e-09 1.79e-09 1.79e-09 1•79e-09 1.79e-09 1.79e-09 1 .79e-09 1•79e-09
Er 168 1 .62e-09 1.62e-09 1.62e-09 1.62e-09 1.62e-O9 1.62e-09 1 .62e-09 1.62e-09 1 .62e-09
Er 170 1 ,52e-16 8 .05e-16 9 .lle-16 9 .lle-16 9 .lle-16 9 .lle-16 9 .lle-16 9 .lle-16 9 .lle-16
Page B.9
U0 2 Fuel - Iapurity Activation Products Mass: aol/kg initial U

Muclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Tm 169 4 .36e-12 5.63e-12 5.63e-12 5.63e-12 5.63e-12 5.63e-12 5.63e-12 5.63e-12 5.63e-12
Tm 170 5 •06e-13 7.07e-14 2.69e-17 1.43e-21 4.01e-30 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Tm 171 2 .87e-14 2.00e-14 4.72e-15 7.77e-lf> 2.1Oe-17 6.00e-30 O.OOe+00 O.OOe+00 O.OOe+00

Yb 170 9 .96e-14 5.35e-13 6.05e-13 6.05e-13 6.05e-13 6.05e-13 6.05e-13 6.05e-13 6.05e-13
Yb 171 2 .39e-15 l.lle-14 2.64e-14 3.03e-14 3.11e-14 3.11e-14 3.11e-14 3.11e-14 3.11e-14
Yb 172 2 •26e-16 2.46e-16 2.46e-16 2.46e-16 2.46e-16 2.46e-16 2.46e-16 2.46e-16 2.46e-16
Yb 173 2 .71e-19 2.71e-19 2.71e-19 2.71e-19 2.71e-19 2.71e-19 2.71e-19 2.71e-19 2.71e-19

TOTAL 8 .42e+00 8.42e+0O 8.42e+00 8.42e+00 8.42e+00 8.42e+00 8.42e+00 8.42e+00 8.42e+00

Page B.10
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 106 Year

H 1 1.73e-05 1.73e-05 1.73e-O5 1.73e-05 1.73e-05 1.73e-05 1.73e-05 1.73e-05 1.73e-O5

H 2 1.46e-08 1.46e-08 1.46e-08 1.46e-08 1.46e-08 1.46e-08 1.46e-08 1.46e-08 1.46e-08
H 3 7.87e-10 7.44e-10 5.94e-10 4.49e-10 2.56e-10 2.87e-12 0.OOe+00 0.OOe+00 0.OOe+00

He 3 1.84e-12 4.48e-ll 1.94e-10 3.40e-10 5.33e-10 7.86e-10 7.89e-10 7.89e-10 7.89e-10

He 4 5.67e-04 5.67e-04 5.67e-04 5.67e-04 5.67e-O4 5.67e-04 5.67e-04 5.67e-04 5.67e-04
Li 6 2.09e-12 2.09e-12 2.09e-12 2.09e-12 2.09e-12 2.09e-12 2.09e-12 2.09e-12 2.09e-12
Li 7 3.89e-05 3.89e-05 3.89e-05 3.89e-05 3.89e-05 3.89e~05 3.89e-05 3.89e-05 3.89e-05

Be 9 1.81e-07 1.81e-07 1.81e-07 1.81e-07 1.81e-07 1.81e-07 1.81e-07 1.81e-07 1.81e-07

Be 10 8.54e-09 8.54e-09 8.54e-09 8.54e-09 8.54e-09 8.54e-09 8.53e-09 8.50e-09 5.53e-09

B 10 3.67e-09 3.67e-09 3.67e-O9 3.67e-09 3.67e-09 3.67e-09 3.67e-09 3.71e-09 6.67e-09

B 11 2. 50e-04 2.50e-04 2.50e-04 2.50e-04 2.50e-04 2.50e-04 2. 50e-04 2.50e-04 2. 50e-04
C 12 9.88e-02 9.88e-02 9.88e-02 9.88e-02 9.88e-02 9.88e-02 9.88e-02 9.88e-02 9.88e-02
C 13 2.,94e-03 2.94e-03 2.,94e-03 2.94e-03 2.94e-03 2.94e-03 2. 94e-03 2.,94e-03 2.,94e-03
C 14 2.,58e-04 2.58e-04 2.,58e-04 2.58e-04 2.57e-04 2.55e-04 2. 29e-04 7.,70e-05 0.,OOe+00
N 14 4,.96e-02 4,,96e-02 4..96e-02 4.,96e-02 4..96e-02 4.,96e-02 4,.96e-02 4,.97e-O2 4,.98e-02
N 15 2,.07e-04 2.,07e-04 2,.07e-04 2,,07e-04 2..07e-04 2.,07e-04 2..07e-04 2.,07e-0' 2,,07e-04
0 16 1 .34e+02 1,,34e+02 1,.34e+02 1,.34e+02 1 .34e+02 1..34e+02 1,.34e+02 1,.34e+02 1,.34e+02
0 17 5 .43e-02 5 .43t>-02 5 .43e-02 5,.43e-02 5 .43e-02 5,.43e-02 5 .43e-02 5 .43e-02 5 ,43e-02
0 18 3 .08e-01 3 ,08e-01 3 .08e-01 3,.08e-01 3.08e-01 3,.08e-01 3 .08e-01 3 .08e-01 3 .08e-01
F 19 2 .05e-07 2.05e-07 2 .05e-07 2 .05e-07 2.05e-07 2 .05e-07 2 .05e-07 2.O5e-O7 2 .05e-07
Ne 20 2 .95e-1.2 2 .95e-12 2 .95e-12 2 .95e-12 2 .95e-12 2 .95e-12 2 .95e-12 2 .95e-12 2 •95e-12
Ne 21 1 .04e-07 1.04e-07 1.04e-O7 1.04e-07 1.O4e-O7 1.04e-07 1.04e-07 1.04e-07 1 .04e-07
Ne 22 1•57e-07 1.57e-07 1•57e-O7 1-57e-O7 1.57e-07 1.57e-07 1.57e-07 1 .57e-07 1 •57e-07

Na 23 3 .19e-08 3.19e-08 3.19e-08 3.19e-08 3.19e-08 3.19e-08 3.19e-08 3.19e-08 3.19e-08

Mg 24 3 .9Oe-O2 3•90e-02 3.9Oe-O2 3.9Oe-O2 3.9Oe-O2 3.9Oe-02 3.9Oe-O2 3 .90e-02 3.90e-02
Mg 25 5 .14e-03 5 .14e-03 5 .14e-03 5 .14e-03 5 .14e-03 5 .14e-03 5 .14e-03 5 .14e-03 5 .14e-03
Mg 26 5 .89e-03 5.89e-03 5.89e-03 5 .89e-03 5.89e-03 5 .89e-03 5 .89e-03 5 .89e-03 5.89e-03
Al 27 5.OOe-02 5.OOe-02 5 .OOe-02 5.OOe-02 5.OOe-02 5.OOe-02 5 .OOe-02 5.OOe-02 5.OOe-02
Page B.ll
U0 2 Fuel - Impurity Activation Products Mass: g/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10 4 Year 10 6 Year

Si 28 5.51e-02 5.51e-02 5.51e-02 5.51e-O2 5.51e-02 5.51e-02 5.5U-02 5.51e-02 5.51e-02

Si 29 2.91e-03 2.91e-03 2.91e-03 2.91e-C3 2.91e-03 2.91e-03 2.91e-03 2.91e-03 2.91e-03
Si 30 1.99e-03 1.99e-03 1.99e-O3 1.99e-03 1.99e-03 1.99e-03 1.99e-03 1.99e-O3 1.99e-03
Si 32 4.96e-13 4.95e-13 4.91e-13 4.86e-13 4.76e-13 4.02e-13 6.07e-14 3.74e-22 O.OOe+00

P 31 5.98e-07 5.98e-07 5.98e-07 5.98e-07 5.98e-07 5.98e-07 5.98e-07 5.98e-07 5.98e-07

P 32 2.69e-ll 5.92e-17 5.82e-17 5.76e-17 5.64e-l7 4.77e-17 7.20e-18 4.43e-26 0.00e+00
P 33 7.80e-16 3.65e-20 1.76e-37 O.OOe+OO O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

S 32 1.36e-10 1.63e-10 1.63e-10 1.63e-10 1.63e-10 1.63e-10 1.63e-10 1.63e-10 1.63e-10

S 33 5.72e-14 5.80e-14 5.8Oe-14 5.8Oe-U 5.80e-14 5.80e-14 5.80e-14 5.80e-14 5.80e-14
S 34 3.20e-12 3.20e-12 3.20e-12 3.2Oe-12 3.2Oe-12 3.2Oe-12 3.20e-12 3.20e-12 3.20e-12
S 35 3.88e-16 2.14e-17 2.00e-22 1.03e-28 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+OO
Cl 35 1.60e-16 5.27e-16 5.48e-16 5.48e-16 5.48e-16 5.48e-16 5.48e-16 5.48e-16 5.48e-16
Cl 36 1.40e-16 1.40e-16 1.40e-16 1.40e-16 1.40e-16 1.40e-16 1.40e-16 1.37e-16 1.40e-17
Cl 37 3.38e-06 4.34e-06 4.34e-O6 4.34e-06 4.34e-06 4.34e-06 4.34e-06 4.34e-06 4.34e-06
Ar 37 9.62e-07 6.97e-10 1.92e-22 O.OOe+OO O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+OO O.OOe+00
Ar 38 1.53e-09 1.53e-09 1.53e-09 1.53e-O9 1.53e-09 1.53e-09 1.53e-09 1.53e-09 1.53e-O9
Ar 39 8.12e-09 8.10e-09 8.01e-09 7.91e-O9 7.71e-09 6.27e-09 6.17e-10 5.22e-20 O.OOe+00
Ar 40 5.63e-08 5.63e-08 5.63e-08 5.63e-O8 5.63e-08 5.63e-08 5.63e-O8 5.63e-08 5.68e-08
Ar 42 6.57e-17 6.43e-17 5.92e-17 5.33e-17 4.32e-17 8.04e-18 4.95e-26 O.OOe+00 O.OOe+OO
K 39 8.00e-12 2.89e-ll 1.12e-10 2.14e-10 4.16e-10 1.85e-09 7.51e-O9 8.12e-09 8.12e-09
K 40 8.86e-06 8.86e-06 8.86e-06 8.86e-06 8.86e-06 8.86e-06 8.86e-06 8.86e-06 8.85e-O6
K 41 3.33e-O7 3.34e-O7 3.35e-O7 3.37e-O7 3.40e-07 3.69e-07 6.95e-07 3.84e-06 5.42e-O5
Ca 40 4.83e-02 4..83e-02 4.83e-02 4.83e-02 4.83e-02 4.83e-02 4.83e-02 4.83e-02
Ca 41 5.39e-O5 5.39e-O5 5..39e-O5 5.39e-05 5.39e-05 5.39e-05 5.36e-05 5.04e-05 6.44e-08
Ca 42 3.38e-04 3..38e-04 3..38e-04 3.38e-O4 3.38e-04 3.38e-04 3.38e-04 3.,38e-0A 3.38e-04
Ca 43 6.91e-05 6.91e-05 6.91e-05 6.91e-O5 6.91e-05 6.91e-05 6.91e-05 6..91e-05 6.91e-05
Ca 44 1.14e-03 1.14e-O3 1.14e-03 1.14e-O3 1.14e-03 1.14e-03 1.14e-03 1..14e-03 1.14e-O3
Ca 43 1.95e-06 4.17e-O7 8.68e-10 3.86e-13 7.61e-20 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ca 46 2. 00e-06 2.00e-06 2.00e-06 2.00e-06 2.00e-06 2.00e-06 2.00e-06 2.00e-06 2.00e-06
Ca 48 1.13e-O4 1.13e-O4 1.13e-04 1.13e-04 1.13e-04 1.13e-04 1.13e-04 1.13e-04 1.13e-04

Sc 45 1.06e-06 2.60e-06 3.02e-06 3.02e-06 3.02e-06 3.02e-06 3.02e-06 3.02e-06 3.02e-O6

Sc 46 1.73e-O8 8.41e-10 4.74e-15 1.30e-21 9.85e-35 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Pares B.12
U0 2 Fuel - Iapurity Activation Products Mass: g/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Ti 46 9.30e-09 57e-08 2.66e-08 2.66e-08 66e-08 2.66e-08 2.66e-08 2.66e-08 2.66e-08

Ti 47 4.86e-09 05e-09 5.05e-09 5.05e-09 05e-09 5.05e-09 5.05e-09 5.05e-09 5.05e-09
Ti 48
Ti 49 3.12e-O7 12e-07 3.12e-07 3.12e-07 12e-07 3.12e-07 3.12e-07 3.12e-07 3.12e-07
Ti 50 1.47e-08 1.47e-08 1.47e-08 1.47e-08 1.47e-08 1.47e-08 1.47e-08 1.47e-08 1.47e-08

V 50 4.83e-08 4.83e-08 4.83e-08 4.83e-08 4.83e-08 4.83e-08 4.83e-08 4.83e-08 4.83e-08

V 51 3.52e-05 4.25e-05 4.25e-05 4.25e-05 4.25e-05 4.25e-05 4.25e-05 4.25e-05 4.25e-05

Cr 50 1.00e-03 1.00e-03 1.00e-03 1.00e-03 1.00e-03 1.00e-03 1.00e-03 1.00e-03 1.00e-03

Cr 51 7.39e-06 7.93e-10 1.05e-25 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Cr 52 2.09e-02 2.09e-02 2.09e-02 2.09e-02 2.09e-02 2.09e-02 2.09e-02 2.09e-02 2.09e-02
Cr 53 2.35e-03 2.35e-03 2.35e-03 2.35e-03 2.35e-03 2.35e-03 2.35e-03 2.35e-O3 2.35e-O3
Cr 54 7.25e-04 7.26e-04 7.26e-04 7.26e-04 7.26e-04 7.26e-04 7.26e-04 7.26e-04 7.26e-04

Mn 54 5.87e-07 2.61e-07 1.02e-08 1.78e-10 5.39e-14 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Mn 55 9.66e-03 9.66e-03 9.68e-03 9.69e-03 9.69e-03 9.69e-O3 9.69e-03 9.69e-03 9.69e-03

Fe 54 5.58e-03 58e-03 5.58e-03 5.58e-03 58e-03 58e-03 58e-03 5.58e-03 5.58e-03

Fe 55 3.07e-05 ,38e-05 8.51e-06 2.36e-06 81e-07 17e-16 00e+00 0.00e+00 0.00e+00
Fe 56 9.16e-02 .16e-02 9.16e-02 9.16e-02 16e-02 .16e-02 16e-02 9.16e-02 9.16e-02
Fe 57 2.81e-03 .81e-03 2.81e-03 2.81e-03 81e-03 ,81e-03 81e-03 2.81e-03 2.81e-03
Fe 58 3.17e-04 .18e-04 3.18e-04 3.18e-04 18e-04 .18e-04 18e-04 3.18e-04 3.18e-04
Fe 59 2.75e-07 9.42e-10 1.29e-19 6.09e-32 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Co 58 5.21e-07 1.46e-08 8.89e-15 1.52e-22 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Co 59 3.64e-06 3.91e-06 3.92e-06 3.93e-06 3.95e-06 4.11e-06 5.84e-06 2.24e-05 2.14e-04
Co 60 2.18e-07 1.91e-07 1.13e-07 5.85e-08 1.57e-08 4.23e-13 0.00e+00 0.00e+00 0.00e+00

Ni 58 00e-02 2.00e-02 2.00e-02 00e-02 ,00e-02 2.00e-02 2.00e-02 2.00e-02 2.OOe-O2

Ni 59 10e-04 2.10a-04 2.10e-04 10e-04 10e-04 2.09e-04 2.08e-04 1.91e-04 2.03e-08
Ni 60 97e-03 7.97e-03 7.97e-03 97e-O3 ,97e-O3 7.97e-03 7.97e-03 7.97e-03 7.97e-O3
Ni 61 08e-04 4.08e-04 4.08e-04 08e-04 ,08e-04 4.08e-04 4.08e-04 4.08e-04 4.08e-04
Ni 62 10e-03 1.10e-03 1.10e-03 10e-03 .10e-03 1.10e-03 10e-03 1.10e-03 1.10e-03
Ni 63 05e-05 4.02e-05 3.91e-05 3.77e-O5 ,50e-05 1.97e-05 96e-08 0.00e+00 0.00e+00
Ni 64 4.05e-04 4.05e-04 4.05e-04 4.05e-04 4.05e-04 4.05e-04 4.05e-04 4.05e-04 4.05e-04

Cu 63 1.3Se-02 1.35e-02 1.35e-02 1.35e-02 1.35e-02 1.36e-02 1.36e-O2 1.36e-O2 1.36e-02

Cu 65 6.26e-03 6.26e-03 6.26e-03 6.26e-03 6.26e-03 6.26e-03 6.26e-O3 6.26e-03 6.26e-03

Page B.13
U0 2 Fuel - Iapurity Activation Products Mass: g/kg initial U
Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 104 Year 106 Year

Zn 64 6.35e-05 .37e-05 37e-05 37e-05 37e-05 6.37e-05 6.37e-05 6.37e-05 6.37e-05

Zn 65 6.09e-08 ,16e-08 39e-10 89e-12 86e-l/ 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Zn 66 3..81e-05 .81e-05 81e-05 81e-05 81e-05 3.81e-05 3.81e-05 3.81e-O5 3.81e-05
Zn 67 4..46e-08 .46e-08 46e-08 46e-08 46e-08 4.46e-08 4.46e-08 4.46e-08 4.46e-08
Zn 68 3..44e-10 ,44e-10 3.44e-10 44e-10 ,44e-10 3.44e-10 3.44e-10 3.44e-10 3.44e-10
Ga 69 3.13e-13 3.14e-13 3.14e-13 3.14e-13 3.14e-13 3.14e~13 3.14e-13 3.14e-13 3.14e-13
Ga 71 5.77e-19 8.51e-19 8.51e-19 8.51e-19 8.51e-19 8.51e-19 8.51e-19 8.51e-19 8.51e-19
Ge 70 5.56e-16 5.56e-16 5.56e-16 5.56e-16 5.56e-16 5.56e-16 5.56e-16 5.56e-16 5.56e-16

Sr 88 7.04e-16 7.04e-16 7.04e-16 7.04e-16 7.04e-16 7.04e-16 7.04e-16 7.04e-16 7.04e-16

Sr 89 3.61e-16 2.40e-18 4.68e-27 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Sr 90 2.00e-l7 1.95e-17 1.78e-17 1.58e-17 1.24e-17 1.85e-18 9.18e-28 0.00e+00 0.00e+00

Y 89 3.41e-ll 3.49e-ll 3.49e-ll 3.49e-ll 3.49e-ll 3.49e-ll 3.49e-ll 3.49e-ll 3.49e-ll

Y 91 7.71e-17 1.02e-18 3.10e-26 1.24e-35 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Zr 90 5.32e-14 5.5U-14 5.51e-14 5.51e-14 5.51e-14 5.51e-14 5.51e-14 5.51e-14 5.51e-14
Zr 91 4.75e-10 4.75e-10 4.75e-10 4.75e-10 4.75e-10 4.75e-10 4.75e-10 4,75e-10 4.75e-10
Zr 92 1.12e-08 1.17e-08 1.17e-O8 1.17e-08 1.17e-08 1.17e-O8 1.17e-O8 1.17e-08 l.l7e-08
Zr 93 4.07e-10 4.07e-10 4.07e-10 4.07e-10 4.07e-10 4.07e-10 4.07e-10 4.05e-10 2.59e-10
Zr 94 1.00e-09 1.00e-09 1.00e-09 1.00e-09 1.00e-09 1.00e-09 1.00e-09 l.OOe-09 1.00e-09
Zr 95 4.81e-ll 9.19e-13 1.23e-19 3.13e-28 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Nb 93 9.80e-14 1.31e-12 1.97e-ll 6.85e-ll 2.29e-10 2.40e-09 2.66e-08 1.3Oe-O7 1.51e-07
Nb 93m 9.22e-12 3.79e-ll 1.39e-10 2.39e-10 3.77e-10 5.74e-10 4.83e-10 8.12e-ll 2.19e-15
Nb 94 6.02e-10 6.02e-10 6.02e-10 6.02e-10 6.02e-10 6.00e-10 5.82e-10 4.28e-10 8.90e-25
Nb 95 6.47e-ll 1.16e-12 1.50e-19 3.81e-28 0.00e+00 0.00e+00 0.00e+00 0.0Oe+00 0.00e+00
Nb 95m 1.89e-14 3.84e-16 5.13e-23 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.0Oe+00 0.00e+00

Mo 92 67e-04 5.67e-04 67e-04 67e-04 67e-04 67e-O4 5.67e-04 5.67e-04 5.67e-04

Mo 93 51e-O7 1.51e-O7 51e-07 51e-07 5Oe-O7 48e-07 1.24e-07 2.08e-08 0.00e+00
Mo 94 64e-04 3.64e-04 3.64e-04 64e-04 64e-04 64e-04 3.64e-04 3.64e-04 3..64e-04
Mo 95 ,97e-04 5.97e-04 5.97e-04 97e-04 97e-04 97e-04 5.97e-04 5.97e-04 5..97e-04
Mo 96 .96e-04 6. 96e-04 6.96e-04 96e-O4 6.96e-04 6.96e-04 6..96e-04 6.96e-04 6..96e-04
Mo 97 .89e-04 3.89e-04 3.89e-04 89e-04 3.89e-04 3.89e-04 3..89e-04 3.89e-04 3..89e-04
Mo 98 .85e-04 9.85e-04 9.85e-04 9.85e-04 9.85e-04 9.85e-04 9.85e-04 9.85e-04 9..85e-04
Mo 100 3.99e-04 3.99e-04 3.99e-04 3.99e-04 3.99e-04 3.99e-04 3.99e-04 3.99e-04 3.99e-04

Tc 99 1.64e-06 1.68e-06 1.68e-06 1.68e-06 1.68e-06 l.68e-06 1.67e-06 1.62e-06 6.47e-08

Page B.14
UO, Fuel - Impurity Activation Products Mass: g/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10* Year 10« Year

Ru 99 1.64e-12 7.10e-12 2.89e-ll 5.62e-ll l.lle-10 5.47e-10 5.45e-09 5.37e-08 1.61e-06

Ru 100 7.70e-08 7.70e-08 7.7Oe-O8 7.70e-08 7.7Oe-O8 7.70e-08 7.70e-08 7.70e-08 7.70e-08
Ru 101 5.31e-07 5.31e-07 5.31e-07 5.31e-O7 5.31e-07 5.31e-07 5.31e-O7 5.31e-07 5.31e-07
Ru 102 6.26e-09 6.26e-09 6.26e-09 5.26e-O9 6.26e-09 6.26e-09 6.26e-09 6.26e-09 6.26e-09
Ru 103 4.11e-12 6.52e-15 4.14e-26 0.00e+00 0.00e+00 0.00e+00 0.00e+00 O.00e+00 0.00e+00
Ru 104 2.25e-16 2.25e-16 2.25e-16 2.25e-16 2.25e-16 2.25e-16 2.25e-16 2.25e-16 2.25e-16
Rh 1.03 4.17e-13 8.24e-13 8.25e-13 8.25e-13 8.25e-13 8.25e-13 8.25e-13 8.25e-13 8.25e-13

Pd 104 4.98e-14 ,98e-14 4.98e-14 98e-14 4.98e-14 4.98e-14 4.98e-14 4.98e-14 4.98e-14
Pd 105 1.87e-19 ,97e-19 1.97e-19 97e-19 1.97e-19 1.97e-19 1.97e-19 1.97e-19 1.97e-19
Pd 106 5.19e-20 ,19e-20 5.19e-20 . 19e-20 5.19e-20 5.19e-20 5.19e-2O 5.19e-20 5.19e-2O
Pd 108 1.13e-06 .16e-06 1.24e-06 .34e-06 1.54e-06 2.80e-06 5.07e-06 5.09e-06 5.09e-06
Pd 110 4.69e-07 4.69e-07 4.69e-O7 4.69e-07 4.69e-07 4.69e-07 4.69e-07 4.69e-07 4.69e-07

Ag 107 60e-04 4.60e-04 4.60e-04 60e-04 4.60e-04 4.60e-04 4.60e-04 4.60e-04 4.60e-04
Ag 108 ,90e-10 1.36e-14 1.33e-14 3Oe-14 1.23e-14 7.93e-15 5.83e-17 0.00e+00 0.00e+00
Ag 108m ,33e-O6 4..31e-O6 4..22e-06 10e-06 3.89e-06 2.51e-06 1.85e-O8 8.54e-30 0.0Oe+0O
Ag 109 .22e-O4 3..22e-04 3..22e-04 22e-04 3.22e-04 3.22e-04 3.22e-04 3.22e-04 3.22e-04
Ag 109m .69e-13 3..31e-14 3..73e-15 2.43e-16 l.O4e-18 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ag 110 .29e-10 3..58e-14 6.23e-16 3.93e-18 1.56e-22 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ag 110m 6.51e-06 2.37e-O6 4.11e-08 2.59e-10 l.O3e-14 0.00e+00 O.00e+OO 0.00e+00 0.00e+00

Cd 106 2.44e-06 2.44e-06 44e-06 44e-06 44e-06 2.44e-06 44e-06 2.44e-06 2.44e-06
Cd 108 ,00e-05 5.00e-05 00e-05 00e-05 00e-05 5.01e-05 03e-05 5.03e-05 5.03e-05
Cd 109 . 77e-08 35e-08 77e-09 46e-10 05e-12 1..16e-31 00e+00 0.00e+00 O.OOe+OO
Cd 110 .79e-04 84e~04 86e-04 86e-04 86e-04 1..86e-04 86e-O4 1.86e-04 1.86e-04
Cd 111 •79e-O5 80e-05 80e-05 80e-05 2.80e-05 2..80e-05 2,8Oe-O5 2.80e-05 2.80e-05
Cd 112 .94e-05 94e-05 4.94e-05 94e-05 4.94e-05 4.94e-05 4.94e-05 4.94e-05 4.94e-05
Cd 113 •65e-09 4.65e-09 4.65e-09 65e-09 4.65e-09 4.65e-09 4.65e-09 4.65e-09 4.65e-09
Cd 114 8.29e-05 8.29e-05 8.29e-05 8.29e-05 8.29e-05 8.29e-05 8.29e-O5 8.29e-05 8.29e-05
Cd 115m 1.2Oe-O8 A.10e-ll 5.64e-21 2.65e-33 O.OOe+00 0.00e+00 0.00e+OO 0.00e+00 0.00e+0O
Cd 116 1.55e-05 1.55e-05 1.55e-05 1.55e-05 1.55e-05 1.55e-05 1.55e-O5 1.55e-05 1.55e-05

In 115 2.13e-08 3.32e-08 3.33e-08 3.33e-08 3.33e-08 3.33e-O8 3.33e-O8 3.33e-O8 3-33e-O8

Sn 116 1.05e-08 1.05e-08 1.05e-08 1.05e-08 1.05e-08 1.05e-08 i.05e-O8 1.05e-O8 1.05e-08
Sn 117 1.36e-08 1.36e-08 1.36e-08 1.36e-08 1.36e-08 1.36e-08 1.36e-O8 1.36e-08 1.36e-08
Sn 117m 2.02e-12 2.83e-2O 0.0Oe+00 0.00e+00 0.00e+00 0.00e+00 0.00e+OO 0.00e+00 O.GOe+00
Sn 118 6.64e-ll 6.64e-ll 6.64e-U 6.64e-ll 6.64e-ll 6.64e-ll 6.64e-ll 6.64e-ll 6.64e-ll
Sn 119 5.00e-15 2.45e-14 3.52e-14 3.53e-14 3.53e-14 3.53e-14 3.53e-U 3.53e-14 3.53e-14
Page B.15
UOj Fuel - Impurity Activation Products Mass: g/kg initial (I

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Sn 119m 3.03e-14 1.08e-14 1.73e-16 9.86e-19 3.20e-23 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 120 6.43e-18 6.43e-18 6.43e-18 6.43e-18 6.43e-18 6.43e-18 6.43e-18 6.43e-18 6.43e-18

Sm 149 4.89e-16 4.89e-16 4.89e-16 4.89e-16 4.89e-16 4.89e-16 4.89e-16 4.89e-16 4.89e-16
Sm 150 7.19e-13 7.19e-13 7.19e-13 7.19e-13 7.19e-13 7.19e-13 7.19e-13 7.19e-13 7.19e-13
Sm 151 7.67e-15 7.61e-15 7.38e-15 7.1Oe-15 6.57e-15 3.55e-15 3.46e-18 O.OOe+00 O.OOe+00
Sm 152 1.48e-ll 1.48e-ll 1.48e-ll 1.48e-ll 1.48e-ll 1.48e-ll 1.48e-ll 1.48e-ll 1.48e-ll
Sm 154 5.34e-14 5.34e-14 5.34e-14 5.34e-14 5.34e-14 5.34e-14 5.34e-14 5.34e-14 5.34e-14

Eu 151 1.92e-18 6.07e-17 2.92e-16 5.7Oe-16 1.10e-15 4.12e-15 7.67e-15 7.67e-15 7.67e-15
Eu 152 4.77e-18 4.53e-18 3.69e-18 2.86e-18 1.72e-18 2.91e-2O 0.00e+00 0.00e+00 0.00e+00
Eu 153 4.09e-08 1.17e-O7 1.57e-O7 1.58e-07 1.58e-07 1.58e-07 1.58e-O7 1.58e-07 1.58e-O7
Eu 154 1.40e-08 1.29e-08 9.34e-09 6.24e-09 2.79e-09 4.41e-12 0.00e+00 O.OOe+00 0.00e+00
Eu 155 3.83e-09 3.33e-09 1.90e-09 9.46e-10 2.34e-10 3.26e-15 0.00e+O0 O.OOe+00 0.00e+00
Eu 156 2.85e-09 1.65e-16 0.00e+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+OO 0.00e+00 0.00e+00

Gd 152 5.48e-09 48e-09 5.48e-09 48e-09 5.48e-09 5.48e-09 5.48e-09 5.48e-09 5.48e-09
Gd 153 1.17e-O7 10e-08 6.20e-10 29e-12 9.24e-17 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Gd 154 1.61e-06 61e-06 1.61e-06 62e-06 1.62e-06 1.62e-06 1.62e-06 1.62e-06 1.62e-06
Gd 155 4.14e-09 64e-09 6.06e-09 02e-09 7.73e-09 7.97e-09 7.97e-09 7.97e-09 7.97e-09
Gd 156 3.47e-05 47e-05 3.47e-05 47e-05 3.47e-05 3.47e-05 3.47e-05 3.47e-05 3.47e-05
Gd 157 2.17e-09 28e-09 2.74e-09 30e-09 4.39e-09 1.15e-08 2.71e-08 2.,73e-08 2.73e-08
Gd 158 4.09e-05 4.09e-05 4.09e-05 09e-05 4.09e-05 4.09e-05 4.09e-05 4..09e-05 4.09e-05
Gd 160 2.21e-05 2.21e-05 2.21e-05 2.21e-05 2.21e-05 2.21e-O5 2.21e-O5 2.21e-05 2.21e-05

Tb 157 2.51e-08 2.51e-08 2.46e-08 2.40e-08 2.30e-08 1.59e-08 2.48e-10 2.14e-28 O.OOe+00
Tb 159 6.43e-07 6.57e-07 6.59e-07 6.59e-07 6.59e-07 6.59e-O7 6.59e-07 6.59e-07 6.59e-07
Tb 160 1.8Oe-O8 5.43e-10 4.48e-16 l.lle-23 0.00e+00 O.OOe+00 O.OOe+OO 0.00e+00 0. 00e+00

Dy 156 70e-08 5.70e-08 70e-08 70e-08 5.70e-08 5.70e-O8 5.70e-08 5.70e-08 5.7Oe-O8
Dy 158 31e-O7 1.31e-O7 31e-O7 31e-O7 1.31e-O7 1.31e-O7 1.31e-O7 1.3U-O7 1.31e-O7
Dy 159 19e-08 2.05e-09 85e-12 88e-16 6.99e-24 O.OOe+00 O.QOe+00 O.OOe+00 O.OOe+00
Dy 160 28e-06 2.3Oe-O6 30e-06 30e-06 2.30e-06 2.30e-06 2.30e-06 2.30e-06 2.30e-06
Dy 161 6.61e-06 6.61e-06 61e-06 6.61e-06 6.61e-06 6.61e-06 6.61e-06 6.61e-06 6.61e-06
Dy 162 3.06e-05 3.06e-05 06e-05 3.06e-05 3.06e-05 3.06e-05 3.06e-05 3.06e-05 3.06e-05
Dy 163 4.43e-05 4.43e-05 43e-05 4.43e-05 4.43e-05 4.43e-05 4.43e-05 4.43e-05 4.43e-05
Dy 164 4 28e-06 4.28e-06 4.28e-06 4.28e-06 4.28e-06 4.28e-06 4.28e-06 4.28e-06 4.28e-06

Ho 165 4.81e-05 4.81e-05 4.81e-05 4.81e-05 4.81e-05 4.81e-05 4.81e-05 4.81e-05 4.81e-05
Ho 166m 4.83e-07 4.83e-07 4.82e-07 4.80e-07 4.78e-07 4.56e-07 2.71e-O7 1.50e-09 O.OOe+00

Page B.16
U02 Fuel - Iapurity Activation Products Mass: g/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Er 166 1.20e-05 1.21e-05 1.21e-05 1.21e-O5 1.21e-05 1.21e-05 1.23e-05 1.26e-05 1.26e-05
Er 167 3.00e-07 3.00e-07 3.00e-07 3.00e-07 3.OOe-O7 3.OOe-O7 3.OOe-07 3.OOe-07 3.OOe-07
Er 168 2.71e-07 2.71e-07 2.71e-07 2.71e-O7 2.71e-O7 2.71e-07 2.71e-07 2.71e-07 2.71e-07
Er 170 2.58e-14 1.37e-13 1.55e-13 1.55e-13 1.55e-13 1.55e-13 1.55e-13 1.55e-13 1.55e-13

Tm 169 7.37e-10 9.51e-10 9.51e-10 9.51e-10 9.51e-10 9.51e-10 9.51e-10 9.51e-10 9.51e-10
Tm 170 8.61e-ll 1.20e-ll 4.57e-15 2.42e-19 6.82e-28 0.OOe+00 0.O0e+00 0.OOe+00 0.OOe+00
Tm 171 4.91e-12 3.42e-12 8.08e-13 1.33e-13 3.59e-15 1.03e-27 0.OOe+00 0.OOe+00 0.OOe+00

Yb 170 1.69e-ll 9.09e-ll 1.03e-10 1.03e-10 1.03e-10 1.03e-10 1.03e-10 1.03e-10 1.03e-10
Yb 171 4.09e-13 1.90e-12 4.51e-12 5.19e-12 5.32e-12 5.32e-12 5.32e-12 5.32e-12 5.32e-12
Yb 172 3.89e-14 4.24e-14 4.24e-14 4.24e-14 4.24e-14 4.24e-14 4.24e-14 4.24e-14 4.24e-14
Yb 173 4.69e-17 4.69e-17 4.69e-17 4.69e-17 4.69e-17 4.69e-17 4.69e-17 4.69e-17 4.69e-17
Yb 174 7.7Oe-19 7.7Oe-19 7.70e-19 7.70e-19 7.7Oe-19 7.7Oe-19 7.7Oe-19 7.70e-19 7.7Oe-19

Lu 175 9.1Oe-21 1.18e-20 1.18e-20 1.18e-20 1.18e-20 1.18e-20 1.18e-20 1.18e-20 1.18e-20

TOTAL 1.35e+02 1.35e+02 1.35e+02 1.35e+O2 1.35e+02 1.35e+02 1.35e+02 1.35e+02 1.35e+02

Page B.17
U0 2 Fuel - Iapurity Activation Products Activity: Bq/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year \04 Year 10* Year

H 3 2.81e+05 2.66e+05 2.12e+05 1.60e+05 9.14e+04 l.O2e+O3 0.00e+00 0.00e+00 0.00e+00

Be 10 7.O7e+OO 7.O7e+OO 7.07e+OO 7.07e+00 7.O7e+OO 7.07e+00 7.07e+00 7.03e+00 4.59e+00

C 14 4.26e+07 4.26e+07 4.26e+07 4.26e+O7 4.26e+07 4.22e+07 3.77e+O7 1.27e+O7 0.00e+00

Si 32 6.22e-01 6.22e-01 6.14e-01 6.11e-01 5.96e-01 5.03e-01 7.62e-02 4.70e-10 0.00e+00

P 32 2.84e+05 6.25e-01 6.14e-01 6.11e-01 5.96e-01 5.03e-01 7.62e-02 4.70e-10 0.00e+00

P 33
4.48e+00 2.11e-04 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
S 35
6.14e-01 3.39e-02 3.16e-O7 1.63e-13 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Cl 36
1.71e-07 1.71e-07 1.71e-O7 1.71e-07 1.71e-07 1.71e-07 1.71e-07 1.67e-07 1.71e-08
Ar 37
Ar 39 3.59e+09 2.6Oe+O6 7.18e-O7 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ar 42 1.02e+04 1.02e+04 1.01e+04 9.99e+03 9.73e+O3 7.92e+03 7.77e+02 6.59e-08 0.00e+00
6.29e-04 6.14e-04 5.66e-04 5.07e-04 4.11e-04 7.66e-05 4.74e-13 0.00e+00 0.00e+00
K 40
2.29e+00 2.29e+00 2.29e+00 2.29e+00 2.29e+00 2.29e+00 2.29e+00 2.29e+00 2.29e+OO
K 42
1.17e+O7 6.14e-04 5.66e-04 5.07e-04 4.11e-04 7.66e-05 4.74e-13 0.00e+00 0.00e+00
Ca 41 1.69e+05 1.69e+05 1.69e+05 1.69e+05 1.69e+05 1.69e+05 1.68e+05 1.58e+O5 2.02e+02
Ca 45
l.28e+09 2.73e+O8 5.7Oe+O5 2.52e+O2 5.00e-05 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Sc 46
2.16e+O7 1.05e+06 5.96e+00 1.64e-06 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Cr 51
2.53e+10 2.72e+O6 3.61e-10 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Mn 54
1.68e-rO8 7.47e+O7 2.93e+06 5.11e+04 1.54e+01 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Fe 55
Fe 59 2.74e+09 2.12e+09 7.59e+O8 2.1Oe+O8 1.61e+07 1.94e-02 0.00e+00 0.00e+00 0.00e+00
5.07e+08 1.73e+06 2.38e-04 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Co 58 1.71e+O7 1.05e+01 1.79e-07 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Co 60 9.10e+06 7.99e+06 4.74e+06 2.45e+06 6.55e+05 1.77e+01 0.00e+00 0.00e+00 0.00e+00

Ni 59 6.25e+05 6.25e+05 6.25e + 05 6.25e + 05 6.25e+05 6.25e + 05 6.22e + 05 5.70e + 05 6.07e + 01

Ni 63 8.84e+07 8.8U+O7 8.55e+07 8.25e+07 7.66e+07 4.29e+07 6.48e+04 0.00e+00 0.00e+00

Zn 65 1.86e+07 6.59e+C6 1.04e+05 5.77e+O2 1.79e-02 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Page B.18
U0 2 Fuel - Impurity Activation Products Activity: Bq/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10* Year 10* Year

Sr 89 3.89e-01 2.58e-03 5.03e-12 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.0Oe+00 0.00e+00

Sr 90 1.01e-04 9.88e-05 8.95e-05 7.96e-05 6.29e-05 9.36e-O6 4.63e-15 0.00e+00 0.00e+00

Y 90 3.77e+01 9.88e-05 8.95e-05 7.96e-O5 6.29e-05 9.36e-O6 4.63e-15 0.00e+00 0.00e+00

Y 91 6.99e-02 9.25e-04 2.81e-ll O.OOe+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Zr 93 3.77e-02 3.77e-02 3.77e-O2 3.77e-O2 3.77e-O2 3.77e-O2 3.77e-02 3.77e-O2 2.41e-02

Zr 95 3.81e+04 7.29e+02 9.73e-05 2.49e-13 O.OOe+00 0.00e+00 0.00e+00 0.00e+00 0.0Oe+00

Nb 92 2.42e+06 3.55e-05 0.00e+00 O.OOe+00 0.00e+00 0.00e+00 0.00e+00 0.0Oe+00 0.00e+00

Nb 93m 9.66e+01 3.96e+02 1.45e+03 2.50e+03 3.96e+03 5.99e+03 5.07e+03 8.51e+02 2.29e-02
Kb 94 4.18e+00 4.18e+00 4.18e+00 4.18e+00 4.18e+00 4.14e+00 4.03e+00 2.97e+OO 6.18e-15
Nb 95 9.36e+04 1.68e+03 2.16e-04 5.51e-13 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
2.66e+02 5.40e+00 7.22e-07 0.00e+00 O.OOe+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Nb 95m
6.14e+03 6.14e+03 6.14e+03 6.14e+03 6.11e+03 6.03e+03 5.O3e-fO3 8.47e+02 0.00e+00
Mo 93
1.03e+03 1.05e+03 1.05e+03 1.05e+03 1.05e+03 1.05e+03 1.05e+03 1.02e+03 4.07e+01
Tc 99
4,92e+03 7.81e+00 4.96e-ll 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ru 103
Ag 108 1.33e+10 3.70e+05 3.62e+05 3.52e+05 3.34e+05 2.16e+05 1.58e+03 0.00e+00 0.00e+00
Ag 108m 4.18e+06 4.14e+06 4.07e+06 3.96e+06 3.74e+06 2.42e+06 1.78e+04 0.00e+00 0.00e+00
Ag 109m 2.60e+07 3.20e+06 3.60e+05 2.36e+04 1.01e+02 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ag 110 3.54e+10 5.51e+06 9.62e+04 6.07e+02 2.41e-02 O.OOe+00 0.00e+00 0.00e+00 0.00e+00
Ag 110m 1.15e+09 4.14e+08 7.22e+06 4.55e+04 1.81e+00 O.OOe+00 0.00e+00 0.00e+00 0.00e+00
Ag 111 3.55e+08 6.18e-07 0.00e+00 O.OOe+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.0Oe+00

Cd 109 5.51e+06 3.20e+06 3.60e+05 2.36e+04 1.01e+02 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Cd 115m 1.13e+07 3.89e+04 5.33e-06 O.OOe+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00

In U S 4.81e-09 7.51e-09 7.51e-09 7.51e-09 7.51e-09 7.51e-09 7.5le-09 7.51e-09 7.51e-09

Sn 117m 5,96e+03 8.33e-05 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00
Sn 119m 5.03e+00 1.79e+00 2.87e-02 1.64e-04 5.33e-O9 0.00e+00 0.00e+00 0.00e+00 O.OOe+00

Sm 151 7.47e-03 7.40e-03 7.18e-03 6.92e-03 6.40e-03 3.46e-03 3.37e-06 O.OOe+00 O.UOe+00

Eu 152 3.05e-05 2.9Oe-O5 2.36e-05 1.83e-O5 1.10e-05 1.86e-O7 O.OOe+00 O.OOe+00 O.OOe+00
Eu 154 1.39e+05 1.29e+05 9.32e+04 6.25e+04 2.79e+04 4.40e+01 O.OOe+00 O.OOe+00 O.OOe+00

Page B.19
U0 2 Fuel - Impurity Activation Products Activity: Bq/k« initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 104 Year 10* Year

Eu 155 6.59e+04 5.74e+04 3.27e+04 1.63e+04 4.03e+03 5.62e-02 0.OOe+00 0.00e+00 0.00e+00
Eu 156 5.81e+06 3.36e-01 0.OOe+00 0.OOe+00 0., OOe+00 0.OOe+00 0.OOe+00 0.00e+00 0.00e+00
Gd 152 4.40e-09 4.40e-09 4. 40e-09 4.40e-09 4.,40e-09 4.,40e-09 4.40e-09 4.40e-09 4.40e-09
Gd 153 1.53e+07 5.37e+06 8.,10e+04 4.29e+02 1.,21e-02 0., OOe+00 0.OOe+00 0.00e+00 0.00e+00
1.41e+04 1.41e+04 1,,38e+04 1.,35e+04 1.,29e+O4

00 O
Tb 157 ,92e+O3 1.39e+02 0.00e+00 0.00e+00
Tb 160 7.51e+06 2.27e+05 1,,87e-01 4.66e-09 0.. OOe+00 .00e+00 0.. OOe+00 0.00e+00 0.00e+00
Tb 161 2.08e+07 2.39e-09 0,.00e+00 0..00e+00 0..00e+00 ,OOe+00 0..00e+00 0.00e+00 0.00e+00

O
Dy 159 2.50e+06 4.33e+05 3 .89e+02 6..O7e-O2 1.47e-09 0,.00e+00 0..00e+00 0.00e+00 0.OOe+00
Ho 166m 3.21e+04 3.21e+04 3 .20e+04 3 .19e+04 3 .17e+O4 3 .03e+04 1,.80e+04 9.95e+01 0.OOe+00
Er 169 6.51e+05 1.31e-06 0 .OOe+00 0 .00e+00 0 .00e+00 0 .00e+00 0 .00e+00 0.OOe+00 0.OOe+00
Tm 170 1.90e+04 2.66e+03 1 .01e+00 5 .37e-O5 1 .51e-13 0 .OOe+00 0 .00e+00 0.OOe+00 0.OOe+00
Tm 171 1.98e+02 1.38e+02 3 .26e+01 5 .37e+OO 1.45e-01 4 •14e-14 0 .00e+00 0.OOe+00 0.OOe+00
TOTAL 4.40e+ll 3.07e+09 9 .07e+08 3 .43e+08 1 .41e+08 8 .84e+07 3 •85e+07 1.34e+07 3.1Oe+O2

Page B.20
U0 2 Fuel - Impurity Activation Products Activity: Ci/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

H 3 60e-06 7.18e-06 74e-06 33e-06 2 .47e-06 77e-O8 0.00e+00 0.00e+00 0.00e+00

Be 10 91e-10 1.91e-10 91e-10 91e-10 1 .91e-10 91e-10 1.91e-10 90e-10 1.24e-10
C 14 15e-03 1.15e-03 15e-03 15e-03 1,.15e-03 14e-03 1.02e-03 43e-04 0.00e+00
Si 32 68e-ll 1.68e-ll 66e-ll 65e-ll 1 36e-ll 2.06e-12 27e-20 0.00e+00
P 32 68e-06 1.69e-ll 66e-ll 65e-ll 1 36e-ll 2.06e-12 27e-2O 0.00e+00
P 33 21e-10 5.69e-15 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
S 35 ,66e-ll 9.15e-13 8.54e-18 4.40e-24 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Cl 36 ,62e-18 4.62e-18 4.62e-18 4.62e-18 4.62e-18 4.62e-18 4.61e-18 4.52e-18 4.62e-19
Ar 37 .7Oe-O2 7.03e-05 0.00e+00 0.,00e+00 0.00e+00 0.00e+0O 0.00e+00 0.00e+00
Ar 39 2.77e-O7 2./6e-07 2.73e-07 7Oe-O7 2.63e-07 2.14e-07 10e-08 1.78e-18 0.00e+00
Ar A2 1.70e-14 1.66e-14 1.53e-14 37e-14 1.lle-14 2.07e-15 28e-23 0.00e+00 0.00e+00
K 40 6.20e-ll 6.20e-ll 6.20e-ll 20e-ll 6.20e-ll 6.20e-ll 20e-ll 6.20e-ll 6.2Oe-ll
K 42 3.16e-04 1.66e-14 53e-14 37e-14 1.lle-14 2.07e-15 28e-23 0.00e+00 0.00e+00
Ca 41 4.57e-06 4.57e-06 57e-06 57e-06 4.57e-06 4.56e-06 54e-06 4.27e-06 5.45e-09
Ca 45 3.46e-02 7.38e-03 54e-05 82e-09 1.35e-15 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Sc 46 5.85e-04 2.85e-05 61e-10 42e-17 0.00e+00 0.00e+00 0.00e+0O 0.00e+0O 0.00e+00
Cr 51 6.83e-01 7.34e-05 9.75e-21 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Mn 54 4.55e-03 2.02e-03 7.91e-05 1.38e-06 4.17e-10 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Fe 55 7.4Oe-O2 5.72e-O2 2.05e-02 5.68e-03 4.36e-04 5.23e-13 0.00e+00 0.00e+00 0.00e+00
Fe 59 1.37e-O2 4.68e-05 6.43e-15 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Co 58 1.66e-02 4.63e-04 2.83e-10 4.83e-18 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Co 60 2.46e-04 2.16e-04 1.28e-04 6.61e-05 1.77e-05 4.79e-10 0.00e+00 0.00e+00 0.00e+00
Ni 59 1.69e-05 1.69e-05 1.69e-05 1.69e-05 1.69e-05 1.69e-05 1.68e-05 1.54e-05 1.64e-09
Ni 63 2.39e-03 2.38e-03 2.31e-03 2.23e-03 2.07e-03 1.16e-03 1.75e-06 0.00e+00 0.00e+00
Zn 65 5.02e-04 1.78e-04 2.80e-06 1.56e-08 4.83e-13 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Sr 89 1.05e-ll 6.98e-U 1.36e-22 0.00e+00 0.00e+00 0.00e+00 0.00e+0O 0.00e+00 0.00e+00
Sr 90 2.73e-15 2.67e-15 2.42e-15 2. 15e-15 1.70e-15 2.53e-16 1.25e-25 0.00e+00 0.00e+00
Y 90 1.02e-09 2.67e-15 2.42e-15 2. 15e-15 1.70e-15 2.53e-16 1.25e-25 0.00e+00 0.00e+00
Y 91 1.89e-12 2.5Oe-14 7.59e-22 0.00e+00 O.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Zr 93 1.02e-12 l.O2e-12 1.02e-12 l.O2e-12 l.O2e-12 1.02e-12 1.02e-12 1.02e-12 6.51e-13
Zr 95 1.03e-06 1.97e-08 2.63e-15 6.72e-24 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Nb 92 6.53e-O5 9.59e-16 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+OO
Nb 93m 2.61e-O9 1.07e-08 3.93e-08 6.77e-08 1.O7e-O7 1.62e-07 1.37e-O7 2.30e-08 6.18e-13
Nb 94 1.13e-10 1.13e-10 1.13e-10 1.13e-10 1.13e-10 1.12e-10 1.09e-10 8.02e-ll 1.67e-25
Nb 95 2.53e-06 4.55e-C8 5.85e-15 1.49e-23 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Nb 95m 7.19e-09 1.46e-10 1.95e-17 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Mo 93 1.66e-O7 1.66e-07 1.66e-07 1.66e-07 1.65e-07 1.63e-07 1.36e-07 2.29e-08 0.00e+00
Tc 99 2.79e-O8 2.84e-08 2.84e-08 2.84e-08 2.84e-08 2.84e-08 2.83e-08 2.75e-08 1.10e-09
Ru 103 1.33e-O7 2.11e-10 1.34e-21 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ag 108 3.60e-01 1.00e-05 9.79e-06 9.52e-06 9.02e-06 5.83e-06 4.28e-08 0.00e+00 0.00e+00
Ag 103m 1.13e-04 1.12e-04 1.10e-04 1.07e-04 1.01e-04 6.55e-05 4.81e-07 0.00e+00 0.00e*00
Page B.21
U0 2 Fuel - Impurity Activation Products Activity: Ci/kg initial U

Nuclide Discharge 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10* Year 106 Year

Ag 109m 7.04e-04 8.64e-05 9.74e-06 6.37e-07 2.72e-09 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ag 110 9.57e-01 1.49e-04 2.60e-06 1.64e-08 6.52e-13 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ag 110m 3.10e-02 1.12e-O2 1.95e-04 1.23e-06 4.90e-ll 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ag 111 9..59e-O3 1.67e-17 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Cd 109 1..49e-04 8.64e-05 9.74e-06 6.37e-07 2.72e-09 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Cd 115m 3..05e-04 05e-06 1.44e-16 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
In 115 1..30e-19 03e-19 2.03e-19 2.03e-19 2.03e-19 2.03e-19 2.03e-19 2.03e-19 2.03e-19
Sn 117m 1..61e-07 25e-15 0.00a+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Sn 119m 1..36e-10 84e-ll 7.75e-13 4.42e-15 1.44e-19 0.00e+00 0.00e+00 O.OOe+00 O.OOe-i-00
Sm 151 2..02e-13 00e-13 1.94e-13 1.87e-13 1.73e-13 9.34e-14 9.12e-17 0.00e+00 0.00e+00
Eu 152 8..24e-16 83e-16 6.39e-16 4.95e-16 2.97e-16 5.04e-18 0.00e+00 0.00e+00 0.00e+00
Eu 154 3..77e-06 48e-06 2.52e-06 1.69e-06 7.53e-07 1.19e-09 0.00e+00 0.00e+00 0.00e+00
Eu 155 1..78e-O6 55e-06 8.85e-07 4.40e-07 l.O9e-O7 1.52e-12 0.00e+00 0.00e+00 0.00e+00
Eu 156 1..57e-04 ,08e-12 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Gd 152 1..19e-19 ,19e-19 1.19e-19 1..19e-19 1.19e-19 1.19e-19 1.19e-19 1.19e-19 1.19e-19
Gd 153 4..14e-04 ,45e-04 2.19e-06 1.. 16e-08 3.27e-13 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Tb 157 3..82e-07 ,81e-07 3.74e-07 3.65e-07 3.49e-07 2.41e-07 3.76e-O9 0.00e+00 0.0Oe+00
Tb 160 2..03e-04 .13e-06 5.06e-12 1.26e-19 0.00e+00 0.00e+00 0.00e+OO 0.00e+00 0.00e+00
Tb 161 5.•62e-04 6.45e-20 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Dy 159 6..75e-05 1.17e-05 1.05e-08 1.64e-12 3.97e-2O 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ho 166m 8.67e-O7 8.67e-07 8.65e-07 8.62e-07 8.58e-07 8.19e-07 4.87e-07 2.69e-09 0.00e+00
Er 169 1.76e-05 3.53e-17 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Tm 170 S.14e-07 7.18e-08 2.73e-ll 1.45e-15 4.08e-24 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Tin 171 5.35e-09 3.73e-09 8.80e-10 1.45e-10 3.91e-12 1.12e-24 0.00e+00 0.00e+00 0.00e+00

TOTAL 1.19e+01 8.31e-02 2.45e-02 9.27e-03 3.81e-03 2.39e-O3 1.04e-03 3.63e-04 8.38e-09

Page B.22
 -/ci
- C.I -

APPENDIX C

ACTIVATION PRODUCTS FOR ZIRCALOY-4 CLADDING AND IMPURITIES IN ZIRCALOY-4

Fuel Bruce "A" Reactor

Burnup 685 GJ/kg initial U
Neutron Flux 1.72 x 1014 n* cm-^S"1
Power 0.034664 MW/kg initial U
Irradiation Time 228.72 d

Burnup-Dependent Library
ORIGEN-S Code
 - C.3 -

CONTENTS

Zircaloy-4 Activation Products Mass : (aol/kg initial Zirc-4) C.4

Zircaloy-4 Activation Products Mass : (g/kg initial Zirc-4) C.12
Zircaloy-4 Activation Products Activity : (Bq/kg initial Zirc-4) C.20
Zircaloy-4 Activation Products Activity : (Ci/kg initial Zirc-4) C.24
Zircaloy-4 Activation Products
Nuolide Initial 1 Tear 5 Ye
Zircaloy-4 Activation Products Mass: m l / k g i n i t i a l Zirc-4
Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10* Year 10 6 Year

Si 28 3.94e-03 3.94e-03 3.94e-03 3.94e-03 3.94e-03 3.94e-03 3.94e-03 3.94e-03 3.94e-03

Si 29 2.01e-04 2.01e-04 2.01e-04 2.01e-04 2.01e-04 2.01e-04 2.01e-04 2.0U-04 2.01e-04
Si 30 1.32e-04 1.32e-04 1.32e-04 1.32e-04 1.32e-04 1.32e-04 1.32e-04 1.32e-04 1.32e-04
Si 32 3.31e-14 3.30e-14 3.27e-14 3.24e-14 3.17e-14 2.68e-14 4.04e-15 2.49e-23 O.OOe+00
P 31 3.98e-08 3.98e-08 3.98e-08 3.98e-08 3.98e-08 3.98e-08 3.98e-08 3.98e-08 3.98e-08
P 32 1.79e-12 3.95e-18 3.88e-18 3.84e-18 3.76e-18 3.18e-18 4.80e-19 2.95e-27 O.OOe+OO
S 32 9.06e-12 1.09e-ll 1.09e-ll 1.09e-ll 1.09e-ll 1.09e-ll 1.09e-ll 1.09e-ll 1.09e-ll
S 33 3.81e-15 3.86e-15 3.86e-15 3.86e-15 3.86e-15 3.86e-15 3.86e-15 3.86e-lS 3.86e-15
Ar 40 1.06e-15 1.06e-15 1.06e-15 1.06e-15 1.06e-15 1.06e-15 1.06e-15 1.06e-15 1.06e-15

R 41 3.38e-17 3.38e-17 3.38e-17 3.38e-17 3.38e-17 3.38e-17 3.38e-17 3.38e-17 3.38e-17

Ca 42 2.28e-19 2.30e-19 2.30e-19 2.3Oe-19 2.30e-19 2.3Oe-19 2.30e-19 2.30e-19 2.30e-19
Ca 43 1.19e-10 1.19e-10 1.19e-10 1.19e-10 1.19e-10 1.19e-10 1.19e-10 1.19e-10 1.19e-10
Ca 44 9.01e-10 9.01e-10 9.01e-10 9.01e-10 9.01e-10 9.01e-10 9.01e-10 9.01e-10 9.01e-10
Ca 45 1.23e-ll 2.63e-12 5.46e-15 2.43e-18 4.79e-25 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ca 46 1.09e-10 1.09e-10 1.09e-10 1.09e-10 1.09e-10 1.09e-10 1.09e-10 1.09e-10 1.09e-10
Sc 45 6.50e-12 1.62e-ll 1.88e-ll 1.88e-ll 1.88e-ll 1.88e-ll 1.88e-ll 1.88e-ll 1.88e-ll
Sc 46 1.05e-09 5.10e-ll 2.87e-16 7.90e-23 5.97e-36 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ti 46 8.59e-05 8.59e-05 8.59e-05 8.59C-05 8.59e-05 8.59«-05 8.59e-05 8.59e-05 8.59e-05
Ti 47 7.75e-05 7.75e-05 7.75e-05 7.75e-O5 7.75e-05 7.75e-05 7.75e-05 7.75e-05 7.75e-05
Ti 48 7.54e-04 7.54e-04 7.54e-04 7.54e-04 7.54e-04 7.54e-04 7.54e-04 7.54e-04 7.54e-04
Ti 49 7.17e-05 7.17e-05 7.17e-05 7.17e-05 7.17e-05 7.17e-05 7.17e-05 7.17e-05 7.17e-05
Ti 50 5.46C-05 5.46e-05 5.46e-05 5.46e-05 5.46e-05 5.46e-05 5.46e-05 5.46e-05 5.46e-05
V 50 2.07«-06 2.07e-06 2.07e-06 2.07e-06 2.07e-06 2.07e-06 2.07e-06 2.07e-06 2.07«-06
V 51 1.00e-03 1.01e-03 1.01e-03 1.01e-03 l.Ole-03 1.01e-03 1.01e-03 1.01e-03 1.01e-03
Cr 50 04«-03 1.04e-03 1.04«-03 1.04«-03 1.04e-03 1.04.-03 1.04e-03 1.04e-03 1.04e-03
Cr 51 77e-06 8.34t-10 l.lle-25 O.OOe+00 O.OOe+00 O.OOe+00 0.00t+00 O.OOe+00 O.OOe+00
Cr 52 09t-02 2.09e-02 2.09C-02 2.09e-02 2.09c-02 2.09e-02 2.09e-02 2.09«-02 2.09e-02
Cr 53 3Oe-O3 2.30e-03 2.3O«-O3 2.3O«-O3 2.3Oe-03 2.3Oe-O3 2.3Oe-O3 2.30e-03 2.30c-03
Cr 54 7.02«-04 7.02«.04 7.02t-04 7.02e-04 7.02«-04 7.02t-04 7.02e-04 7.02.-O4 7.02e-O4
Mn 54 2.69C-07 1.20e-07 4.69t-09 8.16t-ll 2.47e-14 O.OOe+00 O.OOc+00 O.OOe+00 O.OOe+00
Mn 55 8.78t-04 8.8U-04 8.88e-04 8.9U-04 8.92c-04 8.92e-04 8.92e-04 8.92«-04 8.92c-04
Page C.5
Zircaloy-4 Activation Products Mass: aol/kg initial Zirc-4

Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10* Year 10s Year

Fe 54 2.48e-03 2.48e-03 2.48e-03 2.48e-03 2.48e-03 2.48e-03 2. 48e-03 2.48e-03 2.48e-03

Fe 55 1.38e-05 1.07e-05 3.83e-06 1.06e-06 8. lAe-08 9. 78e-17 0.00e+00 0.00e+00 0. OOe+00
Fe 56 3.91e-02 3. 91e-02 3.91e-02 3.91e-02 3. 91e-02 3.91e-02 3. 91e-02 3.91e-02 3.91e-02
Fe 57 1.19e-03 1. 19e-03 1.19e-O3 1.19e-03 1. 19e-03 1.19e-03 1. 19e-03 1. 19e-03 1. 19e-03
Fe 58 1. 31e-04 1. 31e-04 1.31e-04 1.31e-04 1. 31e-04 1.31e-04 1. 31e-04 1. 31e-04 1.31e-04
Fe 59 1. 15e-07 3. 95e-10 5.43e-20 2.56e-32 0. OOe+00 0.OOe+00 0. 00e+00 0.00e+00 0.OOe+00
Co 58 2. lle-08 5. 90e-10 3.61e-16 6. 16e-24 0. 00e+00 0.00e+00 0.OOe+00 0.00e+00 0.OOe+00
Co 59 3.05e-04 3.05e-04 3.05e-04 3.05e-04 3.05e-04 3. 05e-04 3. 05e-04 3.06e-04 3. 13e-04
Co 60 3.31e-05 2.91e-05 1.72e-05 8. 89e-06 2.39e-O6 6. 44e-ll 0. OOei-00 0. 00e+00 0.OOe+00
Ni 58 8.03e-04 8. 03e-04 8.03e-04 8. 03e-04 8.03e-04 8. 03e-04 8. 03e-04 8.03e-04 8.03e-04
Ni 59 8.52e-06 8.52e-06 8.52e-06 8. 52e-06 8. 52e-06 8. 51e-06 8. 44e-06 7.77e-06 8. 25e-10
Ni 60 3. lle-04 3. 15e-04 3.27e-04 3. 36e-04 3. 42e-04 3. 44e-04 3.,44e-04 3.44e-04 3. 44e-04
Ni 61 1.,58e-05 1.,58e-05 1.58e-05 1. 58e-05 1. 58e-05 1.58e-05 1. 58e-05 1.,58e-05 1.,58e-05
Ni 62 4. 13e-05 4.,13e-05 4. 13e-05 4.. 13e-05 4. 13e-05 4. 13e-05 4.,13e-05 4. 13e-05 4.,13e-05
Ni 63 1,.55e-06 1,.54e-06 1.,49e-06 1. 44e-06 1. 34e-06 7.51e-O7 1. 13e-09 0.,00e+00 0..00e+00
Ni 64 1..52e-05 1..52e-05 1.,52e-05 1..52e-05 1.,52e-05 1.,52e-05 1.,52e-05 1.,52e-05 1,,52e-05
Cu 63 5,.37e-04 5,,37e-04 5..37e-04 5,.37e-04 5,.37e-04 5-.38e-04 5,.39e-04 5,.39e-04 5,.39e-04
Cu 65 2,.41e-04 2 .41e-04 2.,41e-04 2,.41e-04 2..41e-04 2..41e-04 2 .41e-04 2,.41e-04 2 .41e-04
Zn 64 2 .56e-06 2 .57e-06 2 .57e-06 2 .57e-06 2,.57e-06 2,.57e-06 2 .57e-O6 2,.57e-O6 2,.57e-06
Zn 65 2 .50e-09 8 .84e-10 1 .39e-ll 7 .75e-14 2 .A0e-18 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .00e+00
Zn 66 1.49e-06 1.49e-06 1 .49e-06 1 .49e-06 1 .49e-06 1 .A9e-06 1 .49e-06 1.49e-06 1 .49e-06
Zn 67 1•77e-O9 1.77e-O9 1.77e-09 1 .77e-09 1 .77e-09 1 .77e-O9 1 .77e-09 1.77e-O9 1 .77e-09
Zn 68 1•39e-ll 1 .39e-ll 1.39e-ll 1 .39e-ll 1 .39e-ll 1 .39e-ll 1 .39e-ll 1•39e-ll 1 .39e-ll
Ga 69 1 .29e-14 1 .29e-14 1.29e-14 1 •29e-14 1 .29e-14 1.29e-14 1.29e-14 1.29e-14 1 •29e-14
6a 71 2 .46e-20 3.63e-20 3 .63e-20 3 .63e-20 3 .63e-20 3 .63e-20 3.63e-2O 3.63e-2O 3.63e-20
Ge 70 2 .33e-17 2.33e-17 2 .33e-17 2 .33e-17 2 •33e-17 2 .33e-17 2 .33e-17 2 .33e-17 2.33e-17
Sr 87 4 .09e-084 .09e-08 4 .09e-08 4 .09e-08 4 .09e-08 4 .09e-08 4 .09e-08 4 .09e-08 4 .09e-08
Sr 88 3.79e-06 3.79e-06 3. 79e-06 3 .79e-06 3 .79e-06 3.79e-06 3 .79e-06 3•79e-06 3.79e-06
Sr 89 8 .80e-085 .85e-10 1 .14e-18 1 .48e-29 0 .OOe+00 0 .OOe+00 0 .00e+00 0 .OOe+00 0 •OOe+00
Sr 90 1.59e-10 1.55e-10 1.41e-10 1 .25e-10 9 .88e-ll 1.47e-ll 7 .3Oe-21 0.OOe+00 0 .OOe+00
Y 89 1.98e-07 2.85e-07 2 .86e-07 2 .86e-07 2 .86e-07 2 .86e-07 2 .86e-07 2•86e-07 2.86e-O7
Y 90 1.79«-07 3 .90e-14 3.54e-14 3 .14e-14 2 .48e-14 3 .69e-15 1.83e-24 0 .00e+00 0 .OOe+00
Y 91 2.65e-07 3.50e-09 1 .06e-16 4 .27e-26 0 .00e+00 0 .OOe+00 0 .00e+00 0 .OOe+00 0 .OOe+00
Page C.6
Zircaloy-4 Activation Products Mass: aol/kg initial Zirc-4

Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10< Year 10 6 Year

Zr 90 5.51e+00 5. 51e+00 5. 51e+00 5. 51e+00 5.51e+00 5.51e+00 5. 51e+00 5.51e+00 5.51e+00

Zr 91 1.20e+00 1. 20e+00 1. 20e+00 1. 20e+00 1.20e+00 1.20e+G0 1. 20e+00 1.20e+00 1.20e+00
Zr 92 1.83e+00 1. 83e+00 1. 83e+00 1. 83e+00 1.83e+OO 1.83e+00 1. 83e+OO 1.83e+00 1.83e+00
Zr 93 1.62e-03 1. 62e-03 1. 62e-03 1. 62e-03 1.62e-03 1.62e-03 1. 62e-03 1.61e-03 1.03e-03
Zr 94 1.86e+00 1. 86e+00 1. 86e+OO 1. 86e+00 1.86e+00 1.86e+00 1.86e-rC0 1.86e+00 1.86e+00
Zr 95 1.73e-04 3. 32e-06 4. 43e-13 1. 13e-21 7.35e-39 0.00e+00 0.00e+00 0.OOe+00 0. OOe+00
Zr 96 2.99e-01 2. 99e-01 2.99e-01 2.99e-01 2.99e-01 2.99e-01 2.99e-01 2.99e-01 2.99e-01
Nb 93 1.07e-03 1. 07e-03 1.O7e-O3 1.O7e-O3 1.O7e-O3 1.07e-03 1.07e-03 1.08e-03 1. 66e-03
Nb 93m 2. 17e-10 8. 90e-10 3.27e-09 5. 63e-09 8. 88e-09 1.37e-08 1. 37e-08 1. 36e-08 8. 70e-09
Nb 94 5. 30e-06 5. 30e-06 5.30e-06 5. 30e-06 5.3Oe-O6 5.28e-06 5. 12e-06 3. 77e-06 7. 84e-21
Nb 95 8. 57e-05 4. 09e-06 5.40e-13 1. 38e-21 0. 00e+00 0.00e+00 0. 00e+00 0. OOe+00 0.OOe+00
Nb 95m 6. 8U-08 1. 39e-09 1.85e-16 4. 72e-25 0.OOe+00 0.00e+00 0. 00e+00 0.OOe+00 0. OOe+00
No 92 7..70e-05 7.,70e-05 7.70e-05 7.,70e-05 7.70e-05 7.,70e-05 7. 70e-05 7. 70e-05 7. 70e-05
No 93 2..09e-08 2.,09e-08 2. 09e-08 2. 09e-08 2.09e-08 2.05e-08 1. 72e-08 2.89e-09 0.OOe+00
No 94 4,.84e-05 4..84e-05 4.,84e-05 4.,84e-05 4.,84e-05 4.,84e-05 4.,86e-05 4,.99e-05 5..37e-05
No 95 2..82e-04 5.,34e-04 5.,42e-04 5..42e-04 5.,42e-04 5.,42e-04 5.,42e-04 5..42e-04 5.,42e-04
No 96 9 .48e-05 9.,A8e-05 9,,A8e-05 9,,48e-05 o,,48e-05 9,.48e-05 9.,48e-05 9,.48e-05 9..48e-05
Ho 97 3 .85e-04 3,.87e-04 3..87e-04 3..87e-04 3,,87e-04 3..87e-04 3..87e-04 3 .87e-04 3,.87e-04
No 98 1 .27e-04 1,,27e-04 1,.27e-04 1..27e-O4 1,.27e-04 1,.27e-04 1,.27e-04 1 .27e-04 1..27e-04
Mo 100 4 .99e-05 4 .99e-05 4,.99e-05 4 ,99e-05 4,.99e-05 4,.99e-05 4,.99e-05 4 .99e-05 4.,99e-05
Tc 99 2 .15e-07 2 .19e-07 2 .19e-O7 2 .19e-07 2 .19e-07 2 .19e-O7 2..18e-07 2 .12e-07 8 ,46e-09
Ru 99 2 .lAe-13 9 •27e-13 3 .78e-12 7 .34e-12 1 .45e-ll 7.15e-ll 7.12e-10 7 .Ole-09 2 .lle-07
Ru 100 1 .03e-08 1.03e-08 1.03e-08 1 .03e-08 1 .03e-08 1.03e-08 1.03e-08 1 .03e-08 1 .03e-08
Ru 101 6 .78e-08 6 .78e-08 6 .78e-08 6 .78e-08 6 .78e-08 6 .78e-08 6 .78e-08 6 .78e-08 6 .78e-08
Ru 102 8 .17e-10 8 .17e-10 8 •17e-10 8 .17e-10 8 .17e-10 8 .17e-10 8 .17e-10 8 .17e-10 8 .17e-10
Ru 103 5 .49e-13 8 .71e-16 5 .52e-27 0 .OOe+00 0 .OOe+00 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .00e+00
Ru 104 3 .06e-17 3 .06e-17 3 .06e-17 3 .06e-17 3 •06e-17 3.06e-17 3 .06e-17 3 .06e-17 3 .06e-17
Rh 103 5.54e-14 1.10e-13 1.10e-13 1.10e-13 1.10e-13 1.10e-13 1.10e-13 1.10e-13 1.10e-13
Pd 104 6 .78«-15 6 .78c-15 6 .78.-15 6 .78e-15 6.78e-15 6.78e-15 6 .78e-15 6 •78e-15 6 .78e-15
Pd 105 2 .59e-2O 2 .73e-2O 2 .73e-20 2.73e-2O 2.73e-20 2.73e-20 2 .73e-2O 2 .73«-2O 2 .73e-2O
Pd 108 1 .68c-13 1.71t-13 1.83e-13 1.98e-13 2 .28e-13 4.12e-13 7 .45e-13 7.48e-13 7.48«-13
Pd 110 6 .27t-15 6 .27e-15 6 .27t-15 6 .27t-15 6 .27e-15 6 .27e-15 6 .27e-15 6 .27e-15 6 .27«-15

P«g« C.7
Zircaloy-4 Activation Products Mass: aol/kg initial Zirc-4
Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 106 Year

Ag 107 1.37e-10 1.37e-10 1.37e-10 1.37e-10 1.37e-10 1.37e-10 1.37e-10 1.37e-lO 1.37e-10
Ag 108m 6.36e-13 6.32e-13 6.19e-13 6.02e-13 5-7Oe-13 3.68e-13 2.71e-15 1.25e-36 O.OOe+00
Ag 109 1.30e-ll 4.17e-ll 7.68e-ll 8.09e-ll 8.12e-ll 8.12e-ll 8.12e-ll 8.12e-ll 8.12e-ll
Ag 109m 6.74e-17 3.91e-17 4.40e-18 2.88e-19 1.23e-21 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00
Ag 110m 1.06e-13 3.85e-I4 6.68e-16 L.68e-22 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Cd 106 5.76e-08 76e-O8 5.76e-08 5.7Se-08 5.76e-08 5.76e-08 5.76e-08 5.76e-08 5.76e-08
Cd 108 3.94e-08 94e-08 3.94e-08 3.94e-08 3.94e-08 3.94e-08 3.94e-08 3.94e-08 3.94e-08
Cd 109 6.82e-ll 95e-ll 4.46e-12 2.91e-13 ,24e-15 1.37e-34 O.OOe+00 O.OOe+00 O.OOe+00
Cd 110 5..37e-O7 37e-O7 5.37e-O7 ,37e-07 37e-07 5.37e-O7 5.37e-07 5.37e-O7 5.37e-07
Cd 111 5..49e-07 49e-07 49e-07 .49e-07 ,49e-07 5.49e-07 .49e-07 .49e-07 5.49e-07
Cd 112 1..10e-06 10e-06 10e-06 10e-06 10e-06 1.10e-06 .10e-06 .10e-06 1.10e-06
Cd 113 1..04e-10 04e-10 04e-10 ,04e-10 .04e-10 1.04e-10 .04e-10 .04e-10 1.04e-10
Cd 114 1..82e-06 83e-06 83e-06 .83e-O6 .83e-06 1.83e-06 .83e-06 .83e-06 1.83e-06
Cd 115m 2.69e-10 9.22e-13 1.27e-22 5.96e-35 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Cd 116 3.33e-O7 3.33e-O7 3.33e-07 3.33e-07 3.33e-07 3.33e-O7 3.33e-07 3.33e-07 3.33e-O7
In 113 9.57e-06 1.49e-05 1.56e-05 1.56e-05 1.56e-05 1.56e-05 1.56e-05 1.56e-05 1.56e-05
In 113m 3.60e-09 3.99e-10 6.02e-14 1.01e-18 2.82e-28 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
In 114 2.57e-12 8.42e-15 1.10e-23 8.64e-35 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+00
In 114m 8.70e-08 5.23e-10 6.84e-19 5.37e-30 0.00e+00 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+00
In 115 6.66e-10 9.35e-10 9.36e-10 9.36e-10 9.36e-10 9.36e-10 9.36e-10 9.36e-10 9.36e-10
Sn 112 1.42e-03 1.42e-03 1.42e-03 42e-03 1.42e-03 1.42e-03 1.42e-03 1.42e-03 1.42e-03
Sn 113 6.00e-06 6.65e-07 1.00e-10 68e-15 4.69e-25 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 114 59e-04 9.59e-04 9.59e-04 59e-04 59e-04 9. 59e-04 9.59e-04 9.59e-04 9.59e-04
Sn 115 79e-04 4.79e-04 4.79e-04 79e-04 79e-04 4.79e-04 4.79e-04 4..79e-04 4.,79e-04
Sn 116 10e-02 2.10e-02 2.1Oe-O2 10e-02 10e-02 2. 10e-02 2.1Oe-O2 2..10e-02 2.. 10e-02
Sn 117 10e-02 1.10e-02 1.10e-02 10e-02 10e-02 1.10e-02 1.10e-02 1..10e-02 1., 10e-02
Sn 117m 05e-06 7.07e-14 0.00e+00 O.OOe+00 O.OOe+00 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 118 48e-02 3.48e-02 3.48e-02 3.48e-02 3.48e-02 3.48e-02 3.48e-02 3..48e-O2 3.48e-02
Sn 119 22e-O2 1.23e-O2 1.,23e-02 23e-02 1.23e-02 1.23e-O2 1.23e-02 1..23e-O2 1.23e-O2
Sn 119m 4.18e-05 1.49e-05 2. 38e-07 36e-09 4.42e-14 0.OOe-t-00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 120 4.64e-02 4.64e-02 4.,64e-02 64e-02 4.64e-02 4.64e-02 4.64e-02 4.64e-02 4.64e-02
Sn 121m 2.29e-07 2.26e-07 2. 15e-07 O2e-O7 1.78e-07 6.,49e-08 7.69e-13 O.OOe+00 O.OOe+00
Sn 122 6.58e-03 6.58e-03 6.58e-03 6.58e-03 6.58e-03 6. 58e-03 6.58e-03 6.58e-03 6.58e-O3
Sn 123 2.44e-06 3.43e-07 1.35e-10 7.51e-15 2.32e-23 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 124 8.00e-03 8.00e-03 8.00e-03 8.00e-03 8.00e-03 8.00e-03 8.00e-03 8.00e-03 8.00e-03
Sn 125 2.27e-08 8.90e-20 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Page C.8
Zircaloy-4 Activation Products
Zircaloy-4 Activation Products Mass: sol/kg initial ?irc-4

Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 10* Year

Hf 180 2.26e-04 2.26e-04 2.26e-04 2.26e-O4 2. 26e-04 2.26e-04 2.26e-04 2.26e-04 2.26e-04
Hf 181 2.49e-06 6. 35e-09 2,69e-19 2.90e-32 0. OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Hf 182 1.80e-07 1. 80e-07 1.80e-07 1.80e-07 1.80e-07 1.8Oe-O7 1.80e-07 1.8Oe-O7 1.67e-07
Ta 180 1.90e-08 1. 90e-08 1.90e-08 1.90e-08 1.90e-08 1.90e-08 1.90e-08 1.90e-08 1.90e-08
Ta 181 9. 48e-04 9. 50e-04 9- 50e-04 9. 50e-04 9. 50e-04 9. 50e-04 9.50e-04 9. 50e-04 9. 50e-04
Ta 182 6. 91e-06 7. 64e-07 1. 14e-10 8. 20e-15 6. 3Oe-15 6. 30e-15 6. 30e-15 6. 3Oe-15 5.83e-15
tf 180 6. 59e-07 6. 59e-07 6. 59e-07 6. 59e-07 6. 59e-07 6. 59e-07 6. 59e-07 6. 59e-07 6.59e-07
V 181 2.65e-08 3. 26e-09 7.54e-13 2.15e-17 1.74e-26 0. OOe+00 0. OOe+00 0. OOe+00 0.OOe+00
tf 182 1.34e-04 1. 40e-04 1.41e-04 1.41e-04 1.41e-04 1.41e-04 1. 41e-04 1. 41e-04 1.41e-04
tf 183 2.27e-04 2. 32e-04 2.32e-04 2.32e-04 2.32e-04 2.32e-04 2.32e-04 2. 32e-04 2. 32e-04
V 184 1.78e-04 1. 78e-04 1.,78e-04 1.78e-04 1.78e-04 1.78e-04 1.78e-04 1. 78e-04 1. 78e-04
W 185 5. 77e-07 1. 98e-08 2. 75e-14 1.32e-21 3.OOe-36 0.OOe+00 0.OOe+00 0. OOe+00 0. OOe+00
V 186 1.,30e-04 1. 30e-04 1.,30e-04 1.,30e-04 1. 30e-04 1.3Oe-O4 1.30e-04 1. 30e-04 1. 30e-04
tf 188 6.,07e-08 1. 58e-09 7.,26e-16 8.,68e-24 0..OOe+00 0.OOe+00 0., OOe+00 0.OOe+00 0. OOe+00
Re 185 6.,34e-07 1.,19e-06 1.,21e-06 1.21e-06 1. 21e-06 1.,21e-06 1.,21e-06 1.21e-06 1. 21e-06
Re 187 2,.23e-05 2..24e-05 2,.24e-05 2,.24e-05 2..24e-05 2.,24e-05 2,.24e-05 2. 24e-05 2. 24e-05
Re 188 2,.36e-08 1,,63e-ll 7,,48e-18 8.,94e-26 0,.OOe+00 0.,OOe+00 0..OOe+00 0..OOe+00 0..OOe+00
Os 186 1 .34e-07 1 ,42e-07 1 .42e-07 1,.42e-O7 1.,42e-07 1,,42e-07 1 .42e-07 1.,42e-07 1,.42e-O7
Os 187 7 ,25e-17 3 .83e-16 1.63e-15 3 •18e-15 6 .29e-15 3,,12e-14 3 .lle-13 3..lle-12 3..lle-10
Os 188 2 .77e-06 2 .85e-06 2 .86e-06 2 .86e-06 2 .86e-06 2 ,86e-06 2 .86e-06 2,.86e-06 2 .86e-06
Os 189 4 .68e-08 4 .68e-08 4 .68e-08 4 .68e-08 4 .68e-08 4 .68e-08 4 .68e-08 4,,68e-08 4 ,68e-08
Os 190 3 .46e-09 3 .46e-09 3 .46e-09 3 .46e-09 3 .46e-09 3 ,46e-09 3.46e-09 3..46e-09 3 ,46e-09
Os 191 9 .84e-12 7 .39e-19 0 .00e+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0..OOe+00 0 .OOe+00
Os 192 6 .20e-14 2 .49e-13 2.55e-J3 2.55e-13 2 .55e-13 2•55e-13 2•55e-13 2 .55e-13 2 .55e-13
Os 194 1 .54e-18 1 .37e-18 8 .64e-19 4 .85e-19 1 .53e-19 1.48e-23 0 .OOe+00 0 .OOe+00 0 .OOe+00
Ir 191 1 .23e-ll 2 .24e-ll 2 .24e-ll 2 .24e-ll 2 .24e-ll 2 .24e-ll 2 .24e-ll 2 .24e-ll 2 .24e-ll
Ir 192 4 .lle-12 1 .34e-13 2 .59e-18 2.40e-18 2.33e-18 1.85e-18 1.39e-19 7.95e-31 0 .OOe+00
Ir 192a 2 .93e-15 2 .92e-15 2.89e-15 2.85e-15 2.77e-15 2.20e-15 1.65e-16 9 .44e-28 0 .OOe+00
Ir 193 1 .57e-12 1.57e-12 1.57e-12 1.58e-12 1.58e-12 1.58e-12 1.58e-12 1.58e-12 1 .58e-12
Ir 194a 6 .69e-15 1•52e-15 4.08e-18 2.48e-21 9 .22e-28 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Pt 192 1.25e-12 5 .04e-12 5.17e-12 5.17e-12 5.17e-12 5 .17e-12 5 .17e-12
5 .17e-12 5 ,17e-12
Pt 193 9 .54e-15 9 .69e-15 9 .16e-15 8 .55e-15 7 .44e-15 2 .45e-15 9 .35e-21
0 .OOe+00 0 .OOe+00
Pt 194 1.35e-13 1.45e-13 1.47e-13 1.47e-13 1.47e-13 1.47e-13 1.47e-13
1.47e-13 1.47e-13
Pt 195 6 .42e-17 6.50.-17 6.50e-17 6.5Oe-17 6 .5Oe-17 6 .5Oe-17
6 .5Oe-17 6 .5Oe-17 6 .5Oe-17
Pt 196 1.16e-18 1.16e-18 1.16e-18 1.16e-18 1.16e-18 1.16e-18 1.16e-18 1 .16e-18 1. 16e-18
Page C I O
Zircaloy-4 Activation Products Mass: mol/kg initial Zirc-4

Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Tl 205 2.74e-16 1.15e-15 4.66e-15 9.05e-15 1.78e-14 8.80e-14 8.78e-13 8.77e-12 8.58e-10

Pb 204 8.76e-06 8.76e-06 8.76e-06 8.76e-06 8.76e-06 8.76e-06 8.76e-06 8.76e-06 8.76e-06
Pb 205 1.91e-08 1.91e-08 1.91e-08 1.91e-08 1.91e-08 1.91e-08 1.91e-08 1.91e-08 1.83e-08
Pb 206 1.40e-04 1.40e-04 1.40e-04 1.40e-04 1.40e-04 1.40e-04 1.40e-04 1.40e-04 1.40e-04
Pb 207 1.50e-04 1.50e-04 1.50e-04 1.50e-04 1.50e-04 1.50e-04 1.50e-04 1.50e-04 1.50e-04
Pb 208 3.29e-04 3.29e-04 3.29e-04 3.29e-04 3.29e-04 3.29e-04 3.29e-O4 3.29e-04 3.29e-04

Bi 208 8.06e-13 8.06e-13 8.06e-13 8.06e-13 8.06e-13 8.06e-13 8.04e-13 7.91e-13 1.23e-13
Bi 209 4.01e-07 4.02e-07 4.02e-07 4.02e-07 4.02e-07 4.02e-07 4.02e-07 4.02e-07 4.02e-07
Bi 210m 1.20e-ll 1.20e-ll 1.20e-ll 1.20e-ll 1.20e-ll 1.20e-ll 1.20e-ll 1.20e-ll 9.53e-12

Po 210 1.09e-ll 1.92e-12 1.27e-15 1.42e-19 6.07e-21 6.07e-21 6.06e-21 6.05e-21 4.81e-21

TOTAL l.lle+01 l.lle+01 l.lle+01 l.lle+01 l.lle+01 l.lle+01 l.lle+01 l.lle+01 l.lle+01

Page C.ll
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Zircaloy-4 Activation Products Mass: g/kg initial Zirc-4

Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10* Year 106 Year

Si 28 1.10e-01 1.10e-01 1.10e-01 1.10e-01 1.10e-01 1.10e-01 1.10e-01 1.10e-01 1.10e-01

Si 29 5.83e-03 5.83e-O3 5.83e-03 5.83e-O3 5.83e-03 5.83e-03 5.83e-03 5.83e-O3
Si 30 3.97e-03 3.97e-O3 3.97e-03 3.97e-03 3.97e-03 3.97e-03 3.97e-03 3.97e-03 3.97e-03
Si 32 1.06e-12 1.06e-12 1.05e-12 1.04e-12 1.01e-12 8.57e-13 1.29e-13 7.97e-22 0.00e+00
P 31 1.23e-06 1.24e-06 1.24e-O6 1.24e-06 1.24e-06 1.24e-06 1.24e-06 1.24e-06 1.24e-06
P 32 5.73e-ll 1.26e-16 1.24e-16 1.23e-16 1.20e-16 1.02e-16 1.53e-17 9.45e-26 O.OOe+00
P 33 1.77e-15 8.29e-20 4.00e-37 O.OOe+00 0.00e+00 0.00e+00 O.OOe+00 O.OOe+OO O.OOe+OO

S 32 2.90e-10 3.47e-10 3.47e-10 3.47e-10 3.47e-10 3.47e-10 3.48e-10 3.48e-10 3.48e-10

S 33
1.26e-13 1.27e-13 1.27e-13 1.27e-13 1.27e-13 1.27e-13 1.27e-13 1.27e-13 1.27e-13
Ar 40
4.23e-14 4.23e-14 4.23e-14 4.23e-14 4.23e-14 4.23e-14 4.23e-14 4.23e-14 4.23e-14
K 41
1.39e-15 1.39e-15 1.39e-15 1.39e-15 1.39e-15 1.39e-15 1.39e-15 1.39e-15 1.39e-15
Ca 42 9.57e-18 9.66e-18 9.66e-18 9.66e-18 9.66e-18 9.66e-18 9.66e-18 9.66e-18 9.66e-18
Ca 43 5.12e-09 5.12e-09 5.12e-09 5.12e-09 12e-09 5.12e-09 5.12e-O9 5.12e-09 5.12e-O9
Ca 44 3.96e-08 3.96e-08 3.96e-08 3.96e-08 96e-08 3.96e-08 3.96e-08 3.96e-08 3.96e-08
Ca 45 5.53e-10 1.18e-10 2.46e-13 1.09e-16 16e-23 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+OO
Ca 46 5.03e-09 5.03e-09 5.03e-09 5.03e-09 5.03e~09 5.03e-09 5.03e-09 5.03e-09 5.03e-O9
Sc 45 2.92e-10 7.28e-10 8.45e-10 8.46e-10 8.46e-10 8.46e-10 3.46e-10 8.46e-10 8.46e-10
Sc 46 4.81e-08 2.34e-09 1.32e-14 3.63e-21 2.75e-34 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+OC
Ti 46 3.95e-03 3.95e-03 3.95e-03 3.95e-03 3.95e-03 3.95e-03 3.95e-03 3.95e-03 3.95e-03
Ti 47 3.64e-03 3.64e-03 3.64e-03 3.64e-03 3.64e-03 3.64e-03 3.64e-03 3.64e-03 3.64e-03
Ti 48 3.62e-O2 3.62e-O2 3.62e-O2 3.62e-02 3.626-02 3.62e-02 3.62e-02 3.62e-02 3.62e-02
Ti 49 3.51e-0S 3.51e-03 3.51e-03 3.51e-03 3.51e-03 3.51e-03 3.51e-03 3.51e-03 3.51e-O3
Ti 50 2.73e-03 2.73e-O3 2.73e-O3 2.73e-03 2.73e-03 2.73e-03 2.73e-O3 2.73e-O3 2.73e-O3
V 50 1.03e-04 1.03e-04 1.03e-04 1.03e-04 1.03e-04 1.03e-04 1.03e-04 1.03e-04 1.036-04
V 51 5.11e-02 5.15e-02 5.15e-02 5.156-02 5.15e-02 5.15e-02 5.15e-02 5.15e-O2 5.15e-O2

Cr 50 5.21e-02 5.21e-02 5.21e-O2 5.21e-02 5.21e-02 5.21e-02 5.21e-02 5.21e-02 5.216-02

Cr 51 3.96e-04 4.25e-08 5.65e-24 0.006+00 0.006+00 O.OOe+00 0.006+00 O.OOe+00 O.OOe+00
Cr 52 1.09e+00 1.09e-i-00 1.096+00 1.096+00 1.09e+00 1.09e+00 1.09e+00 1.09e+00 1.09e+OO
Cr 53 1.22e-01 1.226-01 1.226-01 1.226-01 1.22e-01 1.22e-01 1.22e-01 1.22e-01 1.22e-01
Cr 54 3.79e-02 3.79e-O2 3.796-02 3.796-02 3.796-02 3.79e-O2 3.79e-02 3.79e-O2 3.79e-02

Page C.13
Zircaloy-4 Activation Products Mass: g/kg initial Zirc-4

Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 106 Year

Mn 54 1.45e-05 6.47e-06 2.53e-07 4.41e-09 1.33e-12 0.00e+00 0.00e+00 0.00e+00 0.00e+00

Mn 55 4.83e-02 4.85e-02 4.89e-02 4.90e-02 4.91e-02 4.91e-02 4.91e-02 4.91e-02 4.9le-02

Fe 54 34e-01 1.34e-01 1.34e-01 1.34e-01 1.34e-01 1.34e-01 1.34e-01 1.34e-01 1.34e-01

Fe 55 60e-04 5.88e-04 2.11e-04 5.83e-05 4.48e-06 5.38e-15 0.00e+00 0.00e+00 0.00e+O0
Fe 56 ,19e+00 2.19e+00 2.19e+00 2.19e+00 2.19e+00 2.19e+OO 2.19e+OO 2.19e+OO 2.19e+OO
Fe 57 79e-02 6.79e-02 6.79e-02 6.79e-02 6.79e-02 6.79e-02 6.79e-02 6.79e-02 6.79e-O2
Fe 58 ,60e-03 7.61e-03 7.61e-03 7.61e-03 7.6U-03 7.61e-03 7.61e-03 7.61e-03 7.61e-O3
Fe 59 6.81e-06 2.33e-08 3.21e-18 1.51e-30 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Co 58 1.22e-06 3.42e-08 2.09e-14 3.57e-22 0.00e+00 0.00e+00 0.00e+00 0.0Oe+O0 0.00e+00
Co 59 1.3Oe-O2 1.80e-02 1.80e-02 1.80e-02 1.80e-02 1.80e-02 1.80e-02 1.80e-02 l.B5e-O2
Co 60 1.99e-C3 1.74e-03 1.03e-03 5.34e-04 1.43e-04 3.86e-09 0.0Oe+OO 0.00e+00 0.00e+00
Ni 58 4.66e-02 66e-02 4.66e-02 4.66e-02 4.66e-02 66e-02 4.66e-02 4.66e-02 4.66e-02
Ni 59 5.03e-04 03e-04 5.03e-04 5.03e-04 5.03e-04 02e-04 4.98e-04 4.58e-04 4.87e-08
Ni 60 1.87e-02 89e-02 1.96e-02 2.01e-02 2.05e-02 07e-02 2.07e-02 2.07e-02 2.07e-02
Ni 61 9.64e-04 64e-04 9.64e-04 9.64e-04 9.64e-04 64e-04 9.64e-O4 9.64e-04 9.64e-04
Ni 62 2.56e-O3 56e-03 2.56e-03 2.56e-03 2.56e-03 56e-03 2.56e-O3 2.56e-O3 2.56e-O3
Ni 63 9.74e-05 9.67e-05 9.40e-05 9.07e-Q5 3.43e-05 4.73e-05 7.12e-O8 0.00e+00 0.00e+00
Ni 64 9.70e-04 9.71e-04 9.71e-04 9.71e-04 9.71e-04 9.71e-04 9.71e-04 9.71e-O4 9.71e-04

Cu 63 3.38e-02 3.38<»-02 3.38e-02 3.38e-02 3.38e-02 3.39e-02 3.39e-02 3.39e-O2 3.39e-O2

Cu 65 1.56e-02 1.5f- J2 1.56e-02 1.56e-02 1.56e-02 1.56e-02 1.56e-02 1.56e-02 1.56e-02
Zn 64 1.64e-04 1.64e-04 1.64e-04 1.64e-04 1.64e-04 1.64e-04 1.64e-04 1.64e-04 1.64e-04
Zn 65 1.62e-07 5.75e-08 9.04e-10 5.04e-12 1.56e-16 0.00e+00 0.00e+O0 0.00e+00 0.00e+00
Zn 66 9.83e-05 9.83e-05 9.83e-05 9.83e-05 9.83e-05 9.83e-05 9.83e-05 9.83e-05 9.83e-05
Zn 67 1.19e-O7 1.19e-07 1.19e-07 1.19e-O7 1.19e-07 1.19e-07 1.19e-O7 1.19e-O7 1.19e-07
Zn 68 9.46e-10 9.46e-10 9.46e-10 9.46e-10 9.46e-10 9.46e 10 9.46e-10 9.46e-10 9.46e-10
Ga 69 8.9Oe-13 8.91e~i3 8.91e-13 8.91e-13 8.91e-13 8.91e-13 8.91e-13 8.91e-13 8.9le-13
Ga 71 1.75e-18 2.58e-18 2.58e-18 2.58e-18 2.58e-18 2.58e-18 2.58e-18 2.58e-18 2.58e-18
Ge 70 1.63e-15 1.63e-15 1.63e-15 1.63e-15 1.63e-15 1.63e-15 1.63e-15 1.63e-15 1.63e-15
Sr 87 3.56e-06 3.56e-06 3.56e-06 3.56e-06 3.56e-06 3.56e-06 3.56e-06 3.56e-06 3.56e-06
Sr 88 3.34e-04 3.34e-04 3.34e-04 3.34e-04 3.34e-04 3.34e-04 3.34e-04 3.34e-04 3.34e~04
Sr 89 7.84e-06 5.21e-08 1.02e-16 1.32e-27 O.OOe+00 0.00e+00 0.00e+00 0.00e+00 O.OOe^OO
Sr 90 1.43e-08 1.40e-08 1.27e-O8 1.13e-O8 8.89e-09 1.32e-09 6.57e-19 O.OOe^OO O.00e+'X>
Page C.14
Ziccaloy-4 Activation Products Mass: g/kg initial Zirc-4

Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 10s Year 10* Year 10s Year

Y 89 1.76e-05 2.54e-05 2.54e-05 2.54e-05 2.54e-05 2.54e-05 2.54e-05 2.54e-05 2.54e-05

Y 90 1.61e-05 3.51e-12 3.19e-12 2.83e-12 2.23e-12 3.32e-13 1.65e-22 0.OOe+00 0.OOe+00
Y 91 2.41e-05 3.18e-07 9.67e-15 3.88e-24 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00

Zr 90 96e+02 4.96e+O2 4.96e+02 96e+02 4.96e+02 96e+02 96e+02 4.96e+02 96e+02

Zr 91 09e+02 09e+02 .09e+02 09e+02 09e+02 09e+02 09e+O2 1.09e+02 .09e+02
Zr 92 69e+02 69e+02 .69e+02 69e+02 69e+02 69e+02 69e+02 .69e+02
Zr 93 51e-01 51e-01 .51e-01 51e-01 51e-01 51e-01 51e-01 l!5Oe-6l 9.58e-02
Zr 94 75e+02 75e+O2 .75e+02 75e+02 75e+O2 75e+02 75e+02 1.75e+02 1.75e+02
Zr 95 1.65e-02 3.15e-04 4.20e-ll 1.07e-19 6.98e-37 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Zr 96 2.87e+01 2.87e+01 2.87e+01 2.87e+01 2.87e+01 2.87e+01 2.87e+01 2.87e+01 2.87e+01

Nb 92 6.03e-09 8.84e-20 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00

Nb 93 9.95e-02 9.95e-02 9.95e-02 9.95e-02 9.95e-02 9.95e-02 9.96e-02 1.00e-01 1.54e-01
Nb 93m 2.02e-08 8.28e-08 3.04e-07 5..23e-07 8.26e-07 1.27e-06 1.28e-06 1.27e-06 8.09e-07
Nb 94 4.98e-04 4.98e-04 4.98e-04 4..98e-04 4.98e-04 4.97e-04 4.82e-04 3.54e-04 7.37e-19
Nb 95 8.14e-03 3.89e-04 1.31e-19 0.OOe+00 0.OOe+00 0.OOe+00 0. OOe+00 0.OOe+00
Nb 95m 6.47e-06 1.32e-07 l!76e-14 4.49e-23 0.OOe+00 0.00e+00 0.OOe+00 0.OOe+00 0.OOe+00

Mo 92 7..09e-03 .09e-03 7.09e-03 7.09e-03 7.09e-03 7.09e-03 09e-03 7.09e-03 7.09e-03

Mo 93 1..95e-06 .95e-06 1.95e-06 1.94e-06 1.94e-06 1.91e-06 60e-06 2.69e-07 0.OOe+00
Mo 94 4.55e~03 4.55e-03 4.55e-03 4.55e-03 4.55e-03 4.55e-03 57e-03 4.69e-03 05e-03
Mo 95 2.68e-02 5.07e-02 5.15e-02 5.15e-02 5.15e-02 5.15e-02 15e-02 5.l5e-02 15e-02
Mo 96 9.10e-03 9.1Oe-O3 9..10e-03 9.10e-03 9.10e-03 9.1Oe-O3 9.10e-03 9.10e-03 10e-03
Mo 97 3.74e-02 3.75e-02 3..75e-02 3.75e-02 3.75e-O2 3.75e-O2 3.75e-02 3.,75e-02 75e-02
Mo 93 1.25e-02 1.25e-02 1..25e-02 1.25e-02 1.25e-O2 1.25e-O2 1.25e-02 1.25e-02 25e-02
Mo 100 4.99e-03 4.99e-03 4..99e-03 4.99e-03 4.99e-03 4.99e-03 4.99e-03 4.99e-03 4.99e-03
Tc 99 2.13e-05 2.17e-05 2.17e-05 2.17e-05 2.17e-05 2.17e-05 2.16e-O5 2.1Oe-O5 8.37e-07

Ru 99 2.] 9 3.74e-10 7.27e-10 1.43e-09 7.08e-09 7.05e-08 6.94e-07 2.08e-05

Ru 100 1.03e-06 l.O3e-06 1.03e-06 1.03e-06 1.03e-06 1.03e-06 1.03e-06 1.03e-06 1.03e-06
Ru 101 6.85e-06 6.85e-06 6.85e-06 6.85e-06 6.85e-06 6.85e-06 6.85e-06 6.85e-06 6.85e-06
Ru 102 8.33e-08 8.33e-08 8.33e-08 8.33e-08 8.33e-08 8.33e-08 8.33e-08 8.33e-08 8.33e-08
Ru 103 5.65e-ll 8.97e-14 5.69e-25 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Ru 104 3.19e-15 3.19e-15 3.19e-15 3.19e-15 3.19e-15 3.19e-15 3.19e-15 3.19e-15 3.19e-15

Rh 103 5.71e-12 1. 1. 1. 1. 1. 1. 1. 1.

Pd 104 7.05e-13 7.05e-13 7.05e-13 7.05e-13 7.05e-13 7.05e-13 7.05e-13 7.05e-13 7.05e-13
Pd 105 2.72e-18 2.87e-18 2.87e-18 2.87e-18 2.87e-18 2.87e-18 2.87«-18 2.87e-18 2.87e-18
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Zircaloy-4 Activation Products Mass: g/kg initial Zirc-4

Muclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10« Year 106 Year

Sn 122 8.03e-01 8.03e-01 8. 03e-01 8. 03e-01 8. 03e-01 8. 03e-01 8.03e-01 8.03e-01 8.03e-01
Sn 123 3. 00e-04 4.22e-05 1. 66e-08 9. 24e-13 2.85e-21 0.OOe+00 0.OOe+00 0.OOe+OO 0.OOe+00
Sn 124 9. 92e-01 9. 92e-01 9. 92e-01 9. 92e-01 9. 92e-01 9. 92e-01 9. 92e-01 9. 92e-01 9. 92e-01
Sn 125 2.84e-06 1.lle-17 0. 00e+00 0. 00e+00 0.OOe+00 0. OOe+00 0.OOe+00 0. OOe+00 0.OOe+00
Sb 121 3.77e-03 3.80e-03 3.8Oe-O3 3.81e-03 3.81e-03 3. 82e-03 3.83e-03 3.83e-03 3.83e-03
Sb 123 2. 19e-04 4.77e-04 5. 19e-04 5. 19e-04 5. 19e-04 5. 19e-O4 5. 19e-04 5. 19e-04 5.19e-04
Sb 124 1.46e-06 2.18e-08 1.08e-15 7.92e-25 0. 00e+00 0. OOe+00 0. OOe+00 0.OOe+00 0.OOe+00
Sb 125 1.42e-03 1.lle-03 4.07e-04 1. 16e-04 9. 53e-06 1. 93e-14 0. OOe+00 0.OOe+00 0.OOe+00
Sb 126 3.88e-07 5.26e-16 0. OOe+00 0. 0Oe+0O 0. 00e+00 0. OOe+00 0. OOe+00 0.OOe+00 0.OOe+00
Te 122 8. 34e-05 8. 63e-05 8. 63e-05 8. 63e-05 8. 63e-05 8. 63e-05 8. 63e-05 8. 63e-05 8. 63e-O5
Te 123 2.54e-07 3.95e-07 4. 14e-07 4. 14e-07 4. 14e-07 4. 14e-07 4. 14e-07 4.,14e-07 4. 14e-07
Te 123m 1.6Oe-O7 1.93e-08 4. 08e-12 1.04e-16 6. 78e-26 0.,OOe+00 0. OOe+00 0. OOe+00 0.OOe+00
Te 124 1.26e-O6 2.,70e-06 2. 73e-O6 2. 73e-06 2. 73e-06 2.,73e-O6 2. 73e-06 2.,73e-06 2.,73e-O6
Te 125 1.00e-04 4,,12e-04 1.,12e-03 1. 42e-03 1. 53e-03 1.,53e-03 1.,53e-03 1..53e-O3 1..53e-03
Te 125m 1. 25e-05 1.,54e-O5 5.,69e-06 1. 63e-06 1. 33e-07 2.,69e-16 0..OOe+00 0..OOe+00 0..OOe+00
Te 126 4. 66e-06 5,.05e-06 5..05e-06 5.,05e-06 5.05e-06 5.,05e-06 5..05e-06 5..05e-06 5..05e-06
Te 127 5.,02e-ll 2,.30e-13 2,.12e-17 1,.92e-22 0. OOe+00 0,.OOe+00 0..OOe+00 0,.OOe+00 0..OOe+00
Te 127m 6.,72e-10 6,.58e-ll 6..07e-15 5,.48e-20 4.,48e-30 0,.OOe+00 0,.OOe+00 0 .OOe+00 0 .OOe+00
Te 128 3.,85e-12 3,.85e-12 3.,85e-12 3..85e-12 3.,85e-12 3,,85e-12 3,.85e-12 3,.85e-12 3,.85e-12
Te 129m 3.,47e-17 1,,85e-20 1,.51e- 33 0 .OOe+OO 0..OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
I 127 6,.33e-09 6 .98e-09 7 •05e-09 7 •05e-09 7.,05e-09 7 .05e-09 7 .05e-09 7 .05e-09 7 .05e-09
I 129 8 .55e-16 8 .91e-16 8 .91e-16 8 .91e-16 8.,91e-16 8 .91e-16 8 .91e-16 8 .90e-16 8 .52e-16
Xe 128 6 .02e-ll 6 .02e-ll 6 .02e-ll 6 .02e-ll 6 .02e-ll 6 .02e-ll 6 •02e-ll 6 .Q2e-ll 6 .02e-ll
Xe 129 1 .26e-13 1 .28e-13 1 .28e-13 1 .28e-13 1 .28e-13 1 .28e-13 1 .28e-13 1 .28e-13 1.28e-13
Xe 130 1 .66e-15 1 .66e-15 1.66e-15 1 .66e-15 1 .66e-15 1 .66e-15 1 .t»6e-15 1 .66e-15 1 .66e-15
Xe 131 3 .50e-18 3 .59e-18 3 .59e-18 3 .59e-18 3 .59e-18 3 .59e-18 3 .59e-18 3.59e-18 3 .59e-18
Xe 132 1.56e-19 1 .56e-19 1 .56e-19 1 .56e-19 1 .56e-19 1.56e-19 1.56e-19 1.56e-19 1 .56e-19
Yb 172 1 .906-14 1 .97e-14 1 .97e-14 1 .97e-14 1 .97e-14 1•97e-14 1.97e-14 1.97e-14 1 •97e-14
Yb 173 1 .24e-16 1.24e-16 1 .24e-16 1 .24e-16 1 .24e-16 1 .24e-16 1 .24e-16 1.24e-16 1.24e-16
Yb 174 4 .95e-18 4 .95e-18 4 .95«-18 4 .95e-18 4 .95e-18 4 .95e-18 4 .95e-18 4 .95e-18 4 .95e-18
Lu 175 6 .66e-05 9.99e-05 1 .Ole-04 1 .Ole-04 1.Ole-04 1.Ole-04 1.Ole-04 1.Ole-04 1 .Ole-04
Lu 176 2 .56t-07 2.56e-07 2 .56e-07 2 .S6e-07 2 .56e-07 2.56e-07 2.56e-07 2.56e-07 2.56e-07
Lu 177 1 .22t-07 6 ,03e-12 1.08e-14 3 .97e-18 5 .37e-25 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Lu 1 7 7 B 3 .lle-09 6.41e-10 1.15c-12 4 .22«-16 5 .71e-23 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Page C.17
Zircaloy-4 Activation Products Mass: g/kg initial Zirc-4

Nuclide Initial 1 Tear 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 10* Year

Hf 174 5.108e-05 5.08e-05 5.08e-05 5.08e-05 5.08e-05 5.08e-05 5.08e-05 5.08e-05 5.08e-05
Hf 175 3.43e-05 9.21e-07 4.79e-13 6. 70e-21 1.31e-36 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Hf 176 3.77e-03 3.77e-03 3.77e-03 3. 77e-O3 3.77e-O3 3.77e-03 3.77e-03 3.77e-O3 3.77e-03
Hf 177 1.19e-03 1.19e-03 1.19e-03 1. 19e-03 1.19e-03 1.19e-03 1.19e-03 1.19e-03 1.19e-03
Hf 178 2.27e-O2 2.27e-02 2.27e-O2 2.27e-02 2.27e-02 2.27e-02 2.27e-O2 2.27e-02 2.27e-02
Hf 179 3.Ole-02 3.Ole-02 3.Ole-02 3.Ole-02 3.Ole-02 3.Ole-02 3.Ole-02 3.Ole-02 3.Ole-02
Hf 180 4.06e-02 4.06e-02 4.06e-02 4.06e-02 4.06e-02 4.06e-02 4.06e-02 4.06e-02 4.06e-02
Hf 181 4.51e-04 1.15e-06 4.87e-17 5.25e-30 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00 0.OOe+00
Hf 182 3.28e-05 3.28e-05 3.28e-05 3. 28e-05 3.28e-05 3.28e-05 3.28e-05 3.28e-05 3.03e-05
Ta 180 3.43e-06 3.43e-06 3.43e-06 3.43e-06 3.43e-06 3.43e-06 3.43e-06 3.43e-06 3.43e-06
Ta 181 1.72e-01 1.72e-01 1.72e-01 1.72e-01 1.72e-01 1.72e-01 1.72e-01 1.72e-01 1. 72e-01
Ta 182 1.26e-03 1.39e-04 2.08e-08 1.49e-12 1.15e-12 1.15e-12 1.15e-12 1.15e-12 1.06e-12
V 180 1.19e-04 1.19e-04 1.19e-04 1. 19e-04 1.19e-04 1,19e-04 1.19e-04 1.19e-04 1. 19e-04
V 181 4.79e-06 5.91e-07 1.36e-10 3. 88e-15 3.,15e-24 0.OOe+00 0.OOe+00 0.OOe+00 0. OOe+00
V 182 2.43e-02 2.55e-02 2, 56e-02 2.,56e-02 2.,56e-02 2.56e-02 2.56e-02 2.56e-02 2. 56e-02
V 183 4. 16e-02 4.,24e-02 4.,24e-02 4.,24e-02 4..24e-02 4.,24e-02 4.24e-02 4.24e-02 4.,24e-02
V 184 3.,27e-O2 3..27e-02 3. 27e-02 3..27e-O2 3..27e-02 3.27e-O2 3.,27e-02 3.27e-02 3..27e-02
V 185 1.,07e-04 3..66e-06 5..09e-12 2,.43e-19 5..55e-34 0.OOe+00 0., OOe+00 0..OOe+00 0..OOe+00
V 186 2.,42e-02 2,.42e-02 2,.42e-02 2..42e-02 2..42e-02 2,,42e-02 2..42e-02 2,•42e-02 2,.42e-02
V 188 1,.14e-05 2..97e-07 1,.36e-13 1..63e-21 0,.OOe+00 0., OOe+00 0..OOe+00 0..OOe+00 0 .OOe+00
Re 185 1,.17e~04 2 .20e-04 2 .24e-04 2 .24e-04 2 .24e-04 2 .24e-04 2 .24e-04 2 .24e-04 2 .24e-04
Re 187 4 .17e-03 4 .19e-03 4 .19e-03 4 .19e-03 4 .19e-03 4 .19e-O3 4,.19e-03 4 .19e-03 4 .19e-03
Re 188 4 .45e-06 3 .06e-09 1 •41e-15 1 .68e-23 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Os 186 2 .49e-05 2 .64e-05 2 .64e-05 2 •64e-05 2 .64e-05 2.64e-05 2 .64e-05 2 .64e-05 2 .64e-05
Os 187 1.36e-14 7 .17e-14 3 •04e-13 5 .95e-13 1.18e-12 5.83e-12 5 .81e-ll 5 .81e-10 5 .81e-08
Os 188 5 .21e-04 5 .36e-04 5 .37e-04 5 .37e~04 5 .37e-04 5.37e-04 5.37e-04 5 .37e-04 5 .37e-04
Os 189 8 .84e-06 8 .84e-06 8 .84e-06 8 .84e-06 8 .84e-06 8.84e-06 8 .84e-06 8 .84e-06 8 .84e-06
Os 190 6 .57e-07 6 .57e-07 6 .57e-07 6 .57e-O7 6 .57e-07 6 .57e-07 6 ;57e-07 6.57e-07 6•57e-07
Os 191 1.88e-09 1.41e-16 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00 0 .OOe+00
Os 192 1 .19e-ll 4 .77e-ll 4 .89e-ll 4 .89e-ll 4 .89e-ll 4 .89e-ll 4 .90e-ll 4 .90e-ll 4 .90e-ll
Os 194 2 .99.2-16 2.66e-16 1 .68e-16 9 .40e-17 2 .96e-17 2.87e-21 0 .OOe+00 0 .OOe+00 0 .OOe+00
Ir 191 2 .34«-09 4 .29e-09 4 .29e-09 4 .29e-O9 4 .29e-09 4.29e-09 4 .29e-09 4 .29e-09 4 .29e-09
Ir 192 7 .89e-10 2 •58e-ll 4 .97e-16 4 •60e-16 4 .47e-16 3.55«-16 2.67e-17 1.53e-28 0 .OOe+00
Ir 192a 5 .63«-13 5 •61e-13 5 .55e-13 5 .47e-13 S.32e-13 4.22e-13 3.17e-14 1.81e-25 0 .OOe+00
Ir 193 3.04t-10 3 .04e-10 3 .04e-10 3 .04e-10 3i.04e-10 3.05e-10 3.06t-10 3.06e-10 3.06«-10
Page C.18
Zircaloy-4 Activation Products Mass: g/kg initial Zirc-4
Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10* Year 10 s Year
Ir 194 1.02e-12 9.69e-2O 6.10e-20 3.42e-20 1.08e-20 1.04e-24 0.00e+00 0.00e+00 0.00e+0O
Ir 194m 1.30e-12 2.95e-13 7.91e-16 4.82e-19 1.79e-25 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Pt 192 2.40e-10 9.68e-10 9.93e-10 9.93e-10 9.93e-10 9.93e-10 9.93e-10 9.93e-10 9.93e-10
Pt 193 1.84e-12 1.87e-12 1.77e-12 1.65e-12 1.44e-12 4.74e-13 1.81e-18 0.0Oe+0O COOe+00
Pt 194 2.61e-ll 2.81e-ll 2.84e-ll 2.84e-ll 2.84e-ll 2.84e-ll 2.84e-ll 2.84e-ll 2.84e-ll
Pt 195 1.25e-14 1.27e-14 1.27e-14 1.27e-14 1.27e-14 1.27e-14 1.27e-14 1.27e-14 1.27e-14
Pt 196 2.27e-16 2.27e-16 2.27e-16 2.27e-16 2.27e-16 2.27e-16 2.27e-16 2.27e-16 2.27e-16
Au 197 8.47e-20 8.95e-20 8.95e-20 8.95e-20 8.95e-20 8.95e-2O 8.95e-20 8.95e-20 8.95e-20
Hg 200 5.47e-21 1.41e-20 4.89e-20 9.22e-20 1.79e-19 8.73e-19 8.68e-18 8.68e-17 8.68e-15
Tl 205 5.61e-14 2.36e-13 9.56e-13 1.86e-12 3.65e-12 1.80e-ll 1.80e-10 1.80e-09 1.76e-07
Pb 204 1.79e-03 1.79e-03 1.79e-03 1.79e-03 1.79e-03 1.79e-03 1.79e-03 1.79e-03 1.79e-03
Pb 205 3.92e-06 3.92e-06 3.92e-06 3.92e-06 3.92e-06 3.92e-06 3.92e-06 3.92e-06 3.74e-06
Pb 206 2.88e-02 2.88e-02 2.88e-02 2.88e-O2 2.88e-02 2.88e-02 2.88e-02 2.88e-02 2.88e-02
Pb 207 3.09e-02 3.09e-02 3.09e-02 3.09e-02 3.09e-02 3.09e-02 3.09e-02 3.09e-02 3.09e-02
Pb 208 6.83e-02 6.83e-02 6.83e-02 6.83e-02 6.83e-02 6.83e-02 6.83e-02 6.83e-O2 6.83e-O2
Bi 208 ,68e-10 1.68e-10 1.68e-10 1.68e-10 1.68e-10 1.68e-10 1.67e-10 1.65e-10 2.55e-ll
Bi 209 ,39e-05 8.40e-05 8.40e-05 8.40e-05 8.40e-05 8.40e-05 8.40e-05 8.40e-05 8.40e-05
Bi 210m 2.52e-09 2.52e-09 2.52e-09 2.52e-09 2.52e-09 2.52e-09 2.52e-09 2.52e-09 2.00e-09
Po 210 2.30e-09 4.03e-10 2.68e-13 2.97e-17 1.27e-18 1.27e-18 1.27e-18 1.27e-18 1.01e-18
TOTAL 1.00e+03 1.00e+03 1.00e+03 1.00e+03 1.00e+03 l.OOe+03 1.00e+03 1.00e+03 1.00e+03

Pag* C 1 9
Zircaloy-4 Activation Products Activity: Bq/kg initial Zirc-4
Nuclide Initial 1 Year 5 Tear 10 Tear 20 Year 100 Year 10 3 Year 10* Year 10 6 Year
H 3 5.07e+05 4.81e+05 3.85e+O5 2.89e+05 1.65e+05 1.85e+03 0.00e+00 O.OOe+00 <\00e+00
Be 10 1.15e+01 1.15e+01 1.15e+01 1.15e+01 1.15e+01 1.15e+01 1.15e+01 1.1- 01 7.44e+OO
C 14 6.29e+07 6.29e+07 6.29e+O7 6.29e+O7 6.29e+07 6.22e+07 5.59e+07 1.88e+07 O.OOe+00
Si 32 1.32e+OO 1.32e+OO 1.31e+O0 1.30e+00 1.27e+OO 1.07e-i-00 1.62e-01 9.99e-10 0.00e+0O
P 32 6.07e+05 1.34e+00 1.31e+00 1.30e+00 1.27e+00 1.07e+00 1.62e-01 9.99e-10 O.OOe+00
P 33 1.02e+01 4.77e-04 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00 0.00e+00
Ar 42 8.18e-09 7.99e-O9 7.33e-09 6.59e-09 5.37e-09 9.92e-10 O.OOe+00 O.OOe+00 O.OOe+00
K 42 2.01e-02 7.99e-09 7.36e-09 6.59e-09 5.37e-09 9.99e-10 O.OOe+00 O.OOe+00 O.OOe+00
Ca 45 3.63e+05 7.73e+04 1.61e+02 7.14e-02 1.41e-08 0.00e+00 0.00e+00 0.00e+00 O.OOe+OO
Sc 46 6.03e+07 2.94e+06 1.66e+01 4.55e-06 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+OO
V 50 6.85e-07 6.85e-07 6.85e-07 6.85e-07 6.85e-07 6.85e-07 6.85e-07 6.85e-07 6.85e-07
Cr 51 1.35e+12 1.45e+08 1.94e-08 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Mn 54 4.18e+09 1.85e+09 7.25e+07 1.26e+06 3.81e+02 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Fe 55 6.77e+10 5.25e+10 1.88e+10 5.18e+09 4.00e+08 A.81e-01 O.OOe+OO O.OOe+OO O.OOe+OO
Fe 59 1.25e+10 4.29e+O7 5.88e-03 2.77e-15 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Co 58 1.44e+09 4.03e+07 2.46e+01 4.22e-07 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Co 60 8.33e+10 7.29e+10 4.29e+10 2.23e+10 5.99e+09 1.62e+05 O.OOe+OO O.OOe+OO O.OOe+OO
Ni 59 1.5Oe+O6 1.50e+06 1.50e+06 1.50e+06 1.50e+06 1.50e+06 1.49e+06 1.37e+06 1.45e+02
Ni 63 2.13e+08 2.12e+08 2.06e+08 1.98e+08 1.85e+08 1.04e+08 1.56e+05 O.OOe+OO O.OOe+OO
Zn 65 4.96e+07 1.75e+O7 2.76e+05 1.54e+03 4.77e-02 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Sr 89 8.44«+09 5.59e+07 1.09e-01 1.42e-12 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Sr 90 7.22«+04 7.07«+04 6.40e+04 5./Oe+O4 4.48e+04 6.70e+03 3.32e-06 O.OOe+OO O.OOe+OO
Y 90 3.24«+ll 7.07«+04 6.44e+04 5.70e+04 4.48e+04 6.7Ot+O3 3.32e-06 O.OOe+OO O.OOe+OO
Y 91 2.19e+10 2.89t+08 8.77e+OO 3.52e-09 O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO O.OOe+OO
Page C 2 0
Zircaloy-4 Activation Products Activity: Bq/kg initial Zirc-4

Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10* Year 10« Year

Zr 93 1.40e+07 1.40e+07 1.40e+07 1.40e+07 1.40e+07 1.40e+07 1.40e+07 1.39e+07 8.92e+06

Zr 95 1.31e+13 2.50e+ll 3.34e+04 8.55e-05 O.OOe+00 0.00e+00 0.00e+00 O.OOe+00 0.00e+00

Nb 92 3.12e+07 4.59e-04 0.00e+00 0.00e+00 O.OOe+00 0.00e+00 O.OOe+00 0.00e+00 0.00e+00

Nb 93m 2.11e+05 8.66e+05 3.18e+06 5.48e+06 8.62e+O6 1.33e+07 1.34e+07 1.33e+07 8.47e+06
Nb 94 3.46e+06 3..46e+06 3..46e+06 3.46e+06 3.45e+06 3.44e+06 3.34e+06 2.46e+06 5.11e-09
Nb 95 1.18e+13 5..62e+ll 7.,44e+04 1.89e-04 0.00e+00 0.00e+00 0.00e+00 0.00e+00 O.OOe+00
9.14e+10 1..86e+09 2.,48e+02 6.33e-07 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Nb 95m
7.92e+04 7.92e+04 7.92e+04 7.92e+04 7.88e+04 7.77e+04 6.51e+04 1.09e+04 O.OOe+00
Mo 93
1.34e+04 1.36e+04 1.36e+04 1.36e+04 1.36e+04 1.36e+04 1.36e+04 1.32e+04 5.25e+02
Tc 99
6.73e+04 l.O7e+O2 6.81e-10 O.OOe+OC O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ru 103
Ag 108 4.37e+05 5.85e+00 5.74e+00 59e+00 5.29e+00 3.42e+00 2.51e-02 O.OOe+00 O.OOe+00
Ag 108m 6.62e+01 6.59e+01 6.44e+01 29e+01 5.92e+01 3.85e+01 2.82e-01 O.OOe+00 O.OOe+00
Ag 109m 7.10e+05 4.11e+05 4.63e+04 O3e+O3 1.30e+01 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ag 110 1.61e+05 9.88e+00 1.72e-01 08e-03 4.33e-08 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Ag 110m 2.05e+03 7.44e+02 1.29e+01 8.14e-02 3.24e-06 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Cd 109 7.10e+05 4.11e+05 4.63e+04 3.03e+03 1.30e+01 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Cd 115m 2.92e+07 9.99e+04 1.37e-05 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
In 113m 2.52e+U 2.79e+10 4.22e+06 7.03e+01 1.97e-C8 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
In 114 1.49e+10 4.88e+07 6.40e-02 5.03e-13 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
In 114m 8.51e+09 5.11e+07 6.66e-02 5.25e-l3 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
In 115 1.73e-08 2.43e-08 2.43e-08 2.43e-O8 2.43e-08 2.43e-08 2.43e-08 2.43e-08 2.43e-08
Sn 113 2.52e+ll 79e+10 4.22e+06 7.03e+01 1.97e-08 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 117m 1.74e+12 44e+04 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 119m 8.25e+ll ,94e+ll 4.70e+09 2.68e+O7 8.73e+02 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 121m 5.51c+07 5.44C+07 5.18.+07 '••85e+07 4.29e+07 1.56e+07 1.85e+02 O.OOe+00 O.OOe+00
Sn 123 9.10e+10 1.28e+10 5.07e+06 2.81e+O2 8.66e-07 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 125 1.14e+10 4.48e-02 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Sb 124 9.47t+08 1.41C+07 6.96«-01 5.14t-10 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sb 125 5.44t+10 4.22e+10 1.55.+10 4.44t^09 3,64e+08 7.36C-01 O.OOe+00 O.OOe+00 O.OOc+00
Sb 126 1.20t+09 1.63«+00 O.OOe+00 0.00«+00 O.OOc-t-00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Page C.21
Zircaloy-4 Activation Products Activity: Bq/kg initial Zirc-4

Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 10 4 Year 106 Year

Te 123 2.73e-06 4.26e-06 4.44e-06 4.44e-06 4.44e-06 4.44e-06 4.44e-06 4.44e-06 4.44e-06
Te 123m 5.25e+07 6.33e+06 1.34e+03 3.42e-02 2.22e-ll 0.00e+00 O.OOe+OO O.OOe+OO O.OOe+OO
Te 125m 8.29e+09 1.02e+10 3.81e+09 1.08e+09 8.88e+07 1.79e-01 O.OOe+00 O.OOe+00 O.OOe+00
Te 127 4.92e+06 2.25e+04 2.08e+0O 1.88e-05 O.OOe+00 0.00e+00 O.OOe+OO O.OOe+OO O.OOe+00
Te 127m 2.35e+05 2.30e+04 2.12e+OO 1.91e-05 0.00e+00 0.00e+00 O.OOe+00 O.OOe+OO 0..00e+00
Te 129 1.06e+00 1.35e-05 0.00e+00 0.00e+00 O.OOe+00 0.00e+00 O.OOe+OO O.OOe+OO 0.OOe+OO
Te 129m 3.89e-02 2.07e-05 0.00e+00 0.00e+0O 0.00e+00 0.00e+00 O.OOe+OO O.OOe+OO O.OOe+00

I 129 5.59e-09 5.81e-09 5.81e-09 5.8U-09 5.81e-09 5.81e-09 5.81e-09 5.81e-09 5.59e-09

Lu 176 5.33e-04 5.33e-04 5.33e-04 5.33e-04 5.33e-04 5.33e-04 5.33e-04 5.33e-04 5.33e-04
Lu 177 4.96e+08 2.45e+04 4.40e+01 1.61e-02 2.19e-09 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Lu 177m 5.33e+05 1.09e+05 1.95e+02 7.18e-02 9.73e-09 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Hf 175 1.35e+10 3.63e+08 1.89e+O2 2.65e-06 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Hf 181 2.84e+ll 7.25e+08 3.06e-02 3.31e-15 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Hf 182 2.65e+02 2.65e+O2 2,65e+02 2.65e+02 2.65e+02 2.65e+02 2.6Se+02 2.6Se+02 2.4Se+02

Ta 180 2.52e-05 2.52e-05 2.52e-05 2.52e-O5 2.52e-05 2.52e-05 2.52e-O5 2.52e-05 2.52e-05
Ta 182 2.90e+ll 3.21e+10 4.81e+06 3.44e+02 2.65e+02 2.65e+02 2.65e+02 2.65e+02 2.45e+O2
Ta 183 4.44e+12 1.22e-09 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

V 181 1.06e+O9 1.31e+08 3.01e+O4 8.58e-01 6.96e-10 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
V 185 3.70e+10 1.27e+09 1.77e+O3 8.47e-05 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
W 188 4.22e+09 1.10e+08 5.07e+01 6.03e-07 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Re 187 5.88e+00 5.92e+00 5.92e+OO 5.92e+00 5.92e+00 5.92e+00 5.92e+00 5.92e+00 5.92e+OO
Re 188 1.62e+ll l.lle+08 5.11e+01 6.11e-O7 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
0s 191 3.09e+06 2.32e-01 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
0s 194 3.39e-03 3.02e-03 1.91e-03 l.O7e-O3 3.37e-04 3.26e-08 O.OOe+00 O.OOe+00 O.OOe+00
Ir 192 2.69e+0S 8.77e+O3 1.69e-01 1.57e-01 1.52e-01 1.21e-01 9.07e-03 5.18e-14 O.OOe+00
Ir 192m 1.61e-01 1.61e-01 1.59e-01 1.57e-01 1.52e-01 1.21e-01 9.07e-03 S.18e-14 O.OOe+00
Ir 194 3.20e+04 3.03e-03 1.91e-03 l.O7e-O3 3.37e-04 3.26e-08 O.OOe+00 O.OOe+00 O.OOe+00
Ir 1940 1.89e+02 4.29e+01 1.15e-01 7.03e-05 2.6Oe-ll O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00

Pt 193 2.53e+00 2.56e+00 2.42e+00 2.26e+00 1.97e+OO 6.51e-01 2.48e-06 O.OOe+00 O.OOe+00

Tl 206 5.66e-02 5.29e-02 5.29e-02 5.29e-02 5.29e-02 5.29e-02 5.29e-02 5.2Se-O2 4.18e-02

Page C.22
Zircaloy-4 Activation Products Activity: Bq/kg initial Zirc-4
Nuclide Initial 1 Tear 5 Year 10 Tear 20 Tear 100 Tear 10 3 Tear 10 4 Year 10 6 Tear
Pb 204 8.29e-07 8.29e-07 8.29e-07 8.29e-07 8.29e-07 8.29e-07 8.29e-07 8.29e-07 8.29e-07
Pb 205 1.68e+01 1.68e+01 1.68e+01 1.68e+01 1.68e+01 1.68e+01 1.68e+01 1.68e+01 1.60e+01
Bi 208 2.90e-02 2.90e-02 2.90e-02 2.90e-02 2.90e-02 2.90e-02 2.89e-02 2.85e-02 4.40e-03
Bi 210m 5.29e-02 5.29e-02 5.29e-02 S.29e-02 5.29e-02 5.29e-02 5.29e-02 5.29e-02 4.22e-02
Po 210 3.81e+05 6.70e+04 4.44e+01 4.96e-03 2.12e-04 2.12e-04 2.12e-04 2.11e-04 1.68e-04
TOTAL 7.29e+13 1.39e+12 8.62e + 10 3.34e+10 7.18e+09 2.Ue+08 8.8Ae+07 5.00e + 07 1.74e+07

Pag« C.23
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Zircaloy-4 Activation Products Activity: Ci/kg initial Zirc-4
Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 103 Year 104 Year 10s Year
In 113m 6.81e+00 7.55e-01 1.14e-04 90e-09 5.32e-19 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
In 114 4.04e-01 1.32e-03 1.73e-12 36e-23 O.OOe+OO O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
In 114m 2.30e-0l 1.38e-03 1.80e-12 42e-23 O.OOe+00 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+00
In 115 4.67e-19 6.56e-19 6.56e-19 6.56e-19 6.56e-19 6.56e-19 6.56e-19 6.56e-19 6.56e-19
Sn 113 6.81e+OO 7.54e-01 1.14e-04 1.90e-09 5.32e-19 O.OOe+OO O.OOe+00 O.OOe+00 O.OOe+00
Sn 117m 4.71e+01 6.59e-07 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 119m 2.23e+01 7.94e+00 1.27e-01 7.25e-04 2.36e-08 O.OOe+00 O.OOe+OO O.OOe+00 O.OOe+00
Sn 121m 1..49e-03 1.47e-03 1.40e-03 1.31e-03 1.16e-03 4.22e-04 5.00e-09 O.OOe+00 O.OOe+00
Sn 123 2..46e+00 3.47e-01 1.37e-04 7.6Oe-O9 2.34e-17 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sn 125 3.08e-01 1.21e-12 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sb 124 2.56e-02 3.81e-04 1.88e-ll 1.39e-20 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Sb 125 1..47e+00 l.Ue+00 4.20e-01 1.20e-01 9.85e-03 1.99e-ll O.OOe+00 O.OOe+00 O.OOe+00
Sb 126 3..24e-O2 4.40e-ll 0.00e+0O O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Te 123 7.•39e-17 1.15e-16 1.20e-16 1.20e-16 1.20e-16 1.20e-16 1.20e-16 1.20e-16 1.20e-16
Te 123m 1..42e-O3 1.71e-04 3.62e-08 9.24e-13 6.01e-22 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Te 125m 2..24e-01 2.77e-01 1.03e-01 2.93e-02 2.40e-03 4.85e-12 O.OOe+00 O.OOe+00 O.OOe+00
Te 127 1..33e-04 6.08e-07 5.61e-ll 5.07e-16 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Te 127m 6.34e-06 6.21e-07 5.73e-ll 5.17e-16 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Te 129 2.87e-ll 3.64e-16 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Te 129n 1.05e-12 5.59e-16 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
I 129 1..51e-19 1.57e-19 1.57e-19 1.57e-19 1.57e-19 1.57e-19 1.57e-19 1.57e-19 1.51e-19
Lu 176 1..44e-14 1.44e-14 1.44e-14 1. 44e-14 1.44e-14 1.44e-14 1.44e-14 1.44e-14 1.44e-14
Lu 177 1.,34e-O2 6. 63e-07 1.19e-09 4.36e-13 5.91e-20 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Lu 177m 1..44e-05 2.95e-06 5.28e-09 1.94e-12 2.63G-19 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Bf 175 3.66e-01 9.82e-03 5.11e-09 7.15e-17 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Hf 181 67e+OO 1.96e-02 8.28e-13 8.94e-26 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Hf 182 16e-09 7.16e-09 7.16e-09 7.16e-09 7.16e-09 7.16e-09 7.16e-09 7.15e-09 6.63e-09
Ta 180 6.81e-16 6.81e-16 6.81e-16 6.81e-16 6.81e-16 6.81e-16 6.81e-16 6.81e-16 6.81e-16
Ta 182 85e+00 8.68e-01 1.30e-04 9.31e-09 7.16e-09 7.16e-09 7.16e-09 7.15e-09 6.63e-09
Ta 183 20«+02 3.31e-20 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
V 181 86e-02 3.53e-03 8.14e-07 2.32e-ll 1.88e-20 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
V 185 l.OOe+00 3.44e-02 4..79e-08 2. 29e-15 0.00«+00 O.OOe+00 o:ooe-<oo O.OOe+00 O.OOe+00
V 188 2.97e-03 1..37e-09 1.,63e-17 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOc+00
Rt 187 1.59e-10 1.60e-10 1..60e-10 1..60e-10 1.60e-10 1.60e-10 1.60e-10 1.60e-10 1.60e-10
R* 188 4.37e+OO 3.00e-03 1..38e-09 1.,65e-17 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Os 191 8.35e-05 6.27e-12 0.00e+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
0* 194 9.17t-14 8.17e-14 5.15e-14 2.89e-14 9.10e-15 8.81e-19 O.OOe+00 O.OOc+00 O.OOe+00
Ir 192 7.26t-06 2.37t-07 4..56e-12 4.23C-12 4.11e-12 3.27e-12 2.45e-13 1.40C-24 O.OOc+00
Zr 192a 4.35t-12 4.34e-12 4.>29c-12 4.23«-12 4.lit-12 3.26«-12 2.45e-13 1.40e-24 O.OOe+00
Ir 194 8.64t-07 8.18«-14 5.15e-14 2.89e-14 9.10e-15 8.81e-19 O.OOe+00 O.OOe+00 O.OOe+00
Ir 194m 5.11c-09 1.16t-09 3.11e-12 1.90e-15 7.04e-22 O.OOe+00 O.OOe+00 O.OOe+00 O.OOe+00
Page C.25
Zircaloy-4 Activation Products Activity: Ci/kg initial Zirc-A
Nuclide Initial 1 Year 5 Year 10 Year 20 Year 100 Year 10 3 Year 10 4 Year 10 6 Year

Pt 193 6.83e-ll 6.93e-ll 6.55e-ll 6.12e-ll 5.32e-ll 1.76e-ll 6.69e-17 O.OOe+00 O.OOe+00
Tl 206 1.53e-12 1.43e-12 1.43e-12 1.43e-12 1.43e-12 1.43e-12 1.43e-12 1.42e-12 1.13e-12
Pb 204 2.24e-17 2.24e-17 2.24e-17 2.24e-17 2.24e-17 2.24e-17 2.24e-17 2.24e-17 2.24e-17
Pb 205 4.53e-10 4.53e-10 4.53e-10 4.53e-10 4.53e-10 4.53e-10 4.53e-10 4.53e-10 4.32e-10
Bi 208 7.83e-13 7.83e-13 7.83e-13 7.83e-13 7.83e-13 7.83e-13 7.82e-13 7.69e-13 1.19e-13
Bi 210m 1.43e-12 1.43e-12 1.43e-12 1.43e-12 1.43e-12 1.43e-12 1.43e-12 1.43e-12 1.14e-12
Po 210 1.03e-05 1.81e-06 1.20e-09 1.34e-13 5.73e-15 5.73e-15 5.73e-15 5.71e-15 4.54e-15
TOTAL 1.97e+03 3.77e+01 2.33e+00 9.03e-01 1.94e-01 5.78e-03 2.39e-03 1.35e-03 4.70e-04

Page C.26
 APPENDIX D

PROGRAM INPUT DATA AND OUTPUT VERIFICATION DATA

Fuel Bruce *A" Reactor

Burnup 685 GJ/kg initial U
Power 0.034664 MW/kg initial U
Irradiation Time 228.72 d

Burnup-Dependent Library
ORIGEN-S Code
 - D.3 -

CONTENTS

Page

UO 2 Fuel - Actinides and Fission Products D.4

U0 2 Fuel - Impurity Activation Products D.9
Zircaloy Activation Products D.14
 UP, Fuel - Actinides and F i s s i o n Products

FROGRAH INPUT DATA

1$$ 1 IT
FIRST BtfRNUP STEP USING 25% BUBNUP COMPOSITION LIBRARY
3$$ 21 A3 1 0 A6 1 A16 2 C 2T
35$$ 0 4T
54$$ PO
5$$$ 5 5 A4 0 0 3 A13 4 4 0 A17 1 0 0 E 5T
58** FO.034664
60** 22.8 45.7 68.6 91.5 114.4
73$$ 922380 922350 922340 80160
74** 992.836 7.110 0.054 134.43
75$$ 2 2 2 1 6T
SECOND BURHUP STEP USING 75% BURNUP COMPOSITION LIBRARY
3$$ 22 A3 1 0 A6 1 E 2T
35$$ 0 4T
54$$ F0
56$$ 5 5 A4 0 0 1 A10 5 A14 4 0 A17 1 0 0 E
57** 114.4 E 5T
58** F0.034664
«0»* 137.2 160.1 182.9 205.8 228.72 6T
54$$ FO
56$$ 0 8 A4 0 1 0 A10 5 A14 5 3 A17 4 0 0 E ST
BRUCE FUEL - FISSION (BURNUP-DBPENDENT LIB)
1 KG URANIUM
60** 1 5 10 20 14-2 1+3 1+4 1+6
61** Fl-20
65$$ A22 1 A2S 1 A28 1 A31 1 A43 1 A46 1 A49 1 A52 1 S ST
1$$ 0 IT

PROGRAM OUTPUT VERIFICATION DATA

PROGRAM VEK LOAD DATE USERHAME ACCOUNT NODE RUN XD NUMBER
ORIGINS 1.1 88-09-08 WXLKXN WFORM WC5 88-11-16 15.44.09
PROGRAM VERIFICATION INFORMATION

PROGRAM: OR1GENS
CREATION DATE: 88-09-08
LIBRARY: AICL$3AB1:[SAB CODES .SCALECODElORIOEN.EJtl
JOBNAMB: FW
DATE OF EXECUTION: 88-11-16
TINE OF EXECUTION: IS.44.09
1$ ARRAY 1 EHT1IXCS M A D
IT
3$ ARRAY 33 EllTHIIS HEAD
2T

Page D.A
 UP, Fuel - Actinides and Fission Products

DATA LIBRARY VERIFICATION INFORMATION

DEFAULT DIRECTOR? : AECL$SAB:(HILXIN.FWF]

UNIT
NUMBER DATA SET NAME UNIT FUNCTION

5 ORSINPFISS CARD INPUT

6 ORSOUTFISS OUTPUT PRINT
13 (undefined) FIDO EDIT OUTPUT
0 (undefined) MASTER PHOTON D/B
0 (undefined) NEUTRON ENERGY GROUPS
105 AECL$ SAB1:[SAB_CODES.SCALELIB]CPUrAC.DAT CPU NORMALIZATION
0 (undefined) ~ CARD PUNCH
11 SCR$SAB:IWILKIN1FOR011.DAT SCRATCR
0 (undefined) BINARY GAMMA SOURCE
21 AECL$SAB1:[SAB_SHIELD.LIBRARYJBRUCECY1WLIB.BIN LIBRARY DATA SET NUMBER

LIBRARY INFORMATION...

COUPLE PROCESSED CROSS SECTIONS WITH

ORIGEN-S DATA LIBRARIES FOR CANDU REACTOR
BRUCE rUEL ASSEMBLY BURNUP CALCULATIONS
UPDATE LIBRARY WITH PU243 CAPTURE DATA
UPDATE LIBRARY WITH CORRECTED NP236 DECAY DATA

ORIGEN-S INPUT DATA

3$ LIBRARY CONSTANTS
1. NDSET LIBRARY KNIT NUMBER 21 IS. IVMAI NUMBER OF LIBRARY NUCLIDE 1610
2. NOLIB NO. OF LIBRARIES IN NDSET 4 19. ILMAX NO. OF LIBRARY 1 NUCLIDES 6SS
3. NTYPE 0/1/>I LIBRARY TYPE 1 20. IAHAX BO. OF LIBRARY 2 NUCLIDES 102
4. NGRP -N/0/N »TR» ORP STRUCTURE 1 21. IFMAX NO OF LIBRARY 3 NUCLIDES 822
5. ROUT PUNT OUTPUT UNIT NUMBER 6 22. UMAX NO. OF OFF DIAG ELEMENTS 6585
6. MPCTAB 0/1 YES/NO AIR,HATER HXRDS 1 23. NREACT MAS. MO. OF REACS/NUCLIDE 0
7. 1NPT 0/1 PHTN LIB FROM NDSET 0 24. NFISO NO. OF FISSILE ISOTOPES S
8. IX 1/0 PRNT TRANS.MATRIX Y/N 0 25. HELEN MAX. ATOMIC HO. IN CALC. 99
9. LPU 0/N ACTINIDE CARDS/NDSET N « 26. NMO NORTH IN DATE OF LIBRARY 24
10. NN1 1/0 PRNT 1ST LIB. TBLE Y/N 0 27. NOAY DAY IN DATE . I
11. NN2 1/0 PRNT 2ND LIB. TBLE Y/« t 21. NYR YEAR IN DATE II
12. NN3 1/0 PRNT 3RD LIB. TILE Y/N 0 29. NENAC HO. ACTINIDE PHTH E ORPS II
13. HN4 1/0 PRNT 4TH LIB. TBLE Y/N 0 30. NENLE HO. OF LIGHT EL. PHTH GRP 12
14. HNS 1/0 PRNT STH LIB. TBLE Y/N 0 31. NENFP HO. FISSION PRO PHTR GRPS 12
15. NN6 1/0 PRNT 6TH LXB. TBLE Y/N 0 32. NVERT 0/-N/H INTEGRAL OPTXOH 0
1«. NN7 0/1/2/3 CONC. UNIT* 2 33. NO NUMBER OF ENtROY GROUPS 1
17. HNI -1/0 PRINT LIB. PROLOG N/Y -1

9$ LIBRARY POSITION NUMBER

1. NLIBE REACTOR LIB. POS. IN NDSET

1/2/3/4 HTGR/LWft/LMrBR/MSHR
Page D.5
 UP, Fuel - Actinides and Fission Products

54$ SPECIAL OPTIONS - OPTION I REQUESTED IF JOPT(I) <> 0

1. JOPT(l) PP F7.6.25 SCALE BOOK 2 0 7. JOPT(7) PP F7.S.25 SCALE BOOK 2 0

2. JOPT (2) PUNCH STRT CON. OF SUBCAS 0 «. JOPT(I) NOT USED 0
3. JOPT<3) PP F7.6.25 SCALE BOOK 2 0 9. JOPTI9) PP F7.6.25 SCALE BOOK 2 0
4. JOPT<4) PP F7.6.2S SCALE BOOK 2 0 ID. JOPT(IO) DO ADJOINT CALCULATIONS 0
5. JOPT(5) PP F7.6.25 IN SCALE BOOK 0 11. JOPT(11) NOT USED 0
6. JOPT(S) PP F7.6.25 SCALE BOOK 2 0 12. JOPT(12) MODEL REMOVABLE HEAT/FIS 0

56$ - SUBCASE INTEGER CONTROL CONSTANTS

1. MMN NO. OF IRRADIATION INTERVA 5 11. NTERM <NO. OF EXP EXPANSION TER 21
2. HOUT TINE INTERVALS IN SUBCASE S 12. NSHRT 100
3. INDEX 0/1 0 13. NXCMP NO. OF NUCLIDE OR EL.CORC 4
4. NTABLE 0/1 OUTPUT/SUMMARY TABLES 0 14. NURIT 1/2/3/4/5/6 TIME 4
5. MS TAR TINE FOR CUTOFF PHOT SOURC 0 15. NT I 0/1/2/3 0/TITLE/BASIS/BOT 0
«. nao -1/0/1/2/3 NEXT PROBLEM 3 16. NPUN 0/N NO PUNCHES/PUNCH OR N 0
7. HPROS PP F7.6.11 SCALE BOOK 2 0 17. JTO PP F7.6.11 IN SCALE BOOK 1
8. NPXOS 0 IF MPROS»0/N«MAX ORP. # 0 IS. NUC PP F7.6.12 SCALE BOOK 2 0
9. MFEED RUCLIDES FED TO S7STEM 0 19. NEL SAME AS NUC FOR ELE TABLE 0
10. HSUB PP F7.6.11 IN SCALE BOOK 2 0 20. KBLEND PP F7.6.11 IN SCALE BOOK 0

57* - SUBCASE FLOATING POINT CONSTANTS

1. TMO TIME(I)-TMO FIRST INTERVAL.0OO0OE+00 4. FRACPW TIME OF ALL IRXAD SUBCASE.10000E+01

2. RHO TOTAL MATERIAL DENSITY .O000OE+0O 5. TCORST SECS IN SPECIAL TIME UNIT.S6400E+05
3. CUT FRACTION CUTOFF IN DECAY .OOOOOE+00

3$ ARRAY 33 ENTRIES READ

2T
DATA LIBRARY VERIFICATION INFORMATION

DEFAULT DIRECTORY : AECL$SAB:(WILKXN.FWF)

UNIT
NUMBER DATA SET HAM! UNIT FUNCTION

5 OXfXNPFKi CARD INPUT

6 ORSOUTFIII OUTPUT PRIRT
13 (undefined) FIDO EDIT OUTPUT
60 AECL$SAS1:[SAB CODES.3CALELIBIPHOMASM0.DAT MASTER MOTOR D/B
0 (und«fin»d) •IUTROR ERSRGY GROUPS
10S AICL»IAB1:[SAB CODES.SCALELIBICPUFAC.DAT C»U NORKALItATIOR
0 (undaflnad) CARD PURC1
11 •C>$*AB:tWXI.RJIf JFOR011.DAT SCRATCH
SI (und*(in«d) BINARY OAHHA SOURCE
22 AECL*SAB1:(SAB SHIELD. LIBRARY 1BRUCBCT2WI.XB. BIN LIBRARY DATA SET MUNBCR

Page D.6
 DO, Fuel - Artinides and Fission Products

LIBRARY INFORMATION...

COUPLE PROCESSED CROSS SECTIONS WITH

ORIGEN-S DATA LIBRARIES FOR CANDU REACTOR
BRUCE FUEL ASSEMBLY BURHUP CALCULATIONS
UPDATE LIBRARY WITH PU243 CAPTURE DATA
UPDATE LIBRARY WITH CORRECTED NP236 DECAY DATA

ORIGEN-S INPUT DATA

3$ LIBRARY CONSTANTS
1. NDSET LIBRARY UNIT NUMBER 22 IS. ITMAX NUMBER OF LIBRARY NUCLIDE 1610
2. NOLIB NO. OF LIBRARIES IN NDSET 4 19. ILMAX NO. OF LIBRARY 1 NUCLIDES 688
3. NTYPE O/1/>1 LIBRARY TYPE 1 20. IAMAX NO. OF LIBRARY 2 NUCLIDES 102
4. NGRP -N/O/N NTRN GRP STRUCTURE 1 21. IFMAX NO OF LIBRARY 3 NUCLIDES 822
5. KOUT PRNT OUTPUT UNIT NUMBER 6 22. IZMAX NO. OF OFF DIAG ELEMENTS 6585
6. MPCTAB 0/1 YCS/NO AIR,WATER HZRDS 1 23. NREACT MAX. NO. OP REACS/RUCLIDE 0
7. INPT 0/1 PHTN LIB FROM NDSET 0 24. NFISO NO. OF FISSILE ISOTOPES 5
8. IR 1/0 PRNT TRANS.MATRIX Y/N 0 25. NELSM MAX. ATOMIC NO. IN CALC. 99
9. LPU 0/N ACTINIDE CARDS/NDSET N 0 26. MHO MONTH IN DATE OF LIBRARY 25
10. NN1 1/0 PRNT 1ST LIB. TBLE Y/N 0 ^7. RDAY DAY IN DATE 8
11. NN2 1/0 PRNT 2ND LIB. TBLE Y/N 0 28. NYR TEAR IN DATE 88
12. NN3 1/0 PRNT 3RD LIB. TBLE Y/N 0 29. •ENAC NO. ACTINIDE PHTN E GRPS 18
13. HN4 1/0 PRNT 4TH LIB. TBLE Y/N 0 30. NENLE NO. OF LIGHT EL. PHTN GRP 12
14. NNS 1/0 PRNT STH LIB. TBLE Y/N 0 31. NENFP NO. FISSION PRD PHTN GRPS 12
15. NN6 1/0 PRNT 6TH LIB. TBLI Y/N 0 32. NVERT 0/-I/N INTEGRAL OPTION 0
16. NN7 0/1/2/3 CONC. UNITS 2 33. NO NUMBER OF ENERGY GROUPS 1
17. NNI -1/0 PRINT LIB. PROLOG N/Y -1

5$ LIBRARY POSITION NUMBER

1. NLIBS REACTOR LIB. POS. IN NDSET

1/2/3/4 HTOR/LWR/LMFBR/MSBR

S4$ SPECIAL OPTIONS - OPTION I REQUESTED IF JOPT(I| <> 0

1. JOPT(l) PP F7.6.25 SCALE BOOK 2 0 7. JOPT<7) PP F7.6.25 SCALE BOOK 2 0
2. JOPTI2) PUNCH STRT CON. OF SUBCAS 0 «. JOPTI8) NOT USED , 0
3. JOPTI3) PP F7.6.25 SCALE BOOK 2 0 9. JOPT(9) PP F7.6.2S SCALE BOOK 2 0
4. JOPT(4) PP F7.6.25 SCALE BOOK 2 0 10. JOPT(IO) DO ADJOINT CALCULATIONS 0
5. JOPT(S) PP F7.6.2S IH SCALE BOOK 0 11. JOPT(ll) NOT USED 0
6. JOPTI6) PP F7.6.25 SCALE BOOK 2 0 12. JOPTI12) NODSL REMOVABLE HEAT/FIS 0

Page D.7
 UP, Fuel - Actinides and Fission Products

56$ - SUBCASE INTEGER CONTROL CONSTANTS

1. HMN NO. OF IRRADIATION INTERVA 5 11. NTERM <NO. OF EXP EXPANSION TER 21
2. MOUT TINE INTERVALS IN SUBCASE S 12. RSHRT 100
3. INDEX 0/1 0 13. NXCMP NO. OP NUCLIDE OR EL.CONC 0
4. HTABIE 0/1 OUTPUT/SUMMARY TABLES 0 14. NUNIT 1/2/3/4/5/6 TIME 4
5. MSTAR TIME FOR CUTOFF PHOT SOURC 0 IS. NT I 0/1/2/3 0/TITLE/BASIS/BOT 0
6. N60 -1/0/1/2/3 NEXT PROBLEM 1 16. NPUN 0/N NO PUNCHES/PUNCH OH N 0
7. MPROS PP F 7 . 6 . U SCALE BOOK 2 0 17. JTO PP F7.6.11 IN SCALE BOOK 1
a. HPROS 0 IF MPROS-0/N-MAX 6RP. * 0 ia. NUC PP F7.6.12 SCALE BOOK 2 0
9. HPEEO NUCLIDES FED TO SYSTEM 0 19. NEL SAME AS NUC FOR ELE TABLE 0
10. MSUB PP F7.6.11 IN SCALE BOOK 2 5 20. KBLERD PP F7.6.11 IN SCALE BOOK 0

57* - SUBCASE FLOATING POINT CONSTANTS

1. TMO T I M E I D - T M O FIRST INTERVAL. OOOOOE+00 4. FRACPW TIME OF ALL IRRAD SUBCASE.10000E+01

2. RHO TOTAL MATERIAL DENSITY .O00O0E+O0 5. TCONST SECS IN SPECIAL TIME UNIT.36400E+05
3. CUT FRACTION CUTOFF IN DECAY .00000E+OO

S6$ - SUBCASE INTEGER CONTROL CONSTANTS

1. MMN NO. OF IRRADIATION INTERVA 0 11. NTERM <NO. OF EXP EXPANSION TER 0
2. MOUT TIME INTERVALS III SUBCASE 8 12. NSHRT 0
3. INDEX 0/1 0 13. NXCMP NO. OF NUCLIDE OR EL.CONC 0
4. NTABLE 0/1 OUTPUT/SUMMARY TABLES 0 14. NUNIT 1/2/3/4/5/6 TIME S
S. MSTAR TIME FOR CUTOFF PHOT SOURC 0 15. NTI 0/1/2/3 0/TITLE/BASIS/BOT 3
6. NGO -1/0/1/2/3 NEXT PROBLEM 0 16. NPUN 0/N NO PUNCHES/PUNCH ON N 0
7. MPXOS PP F7.6.11 SCALE BOOK 2 0 17. JTO PP F7.6.11 IN SCALE BOOK 4
8. NPROS 0 IF MPROS-0/N-MAX ORP. * 0 It. NUC PP F7.6.12 SCALE BOOK 2 0
9. MFEED NUCLIDES TIB TO SYSTEM 0 19. NEL SAME AS NUC FOR ELE TABLE 0
10. MSUB PP F7.fi.11 IN SCALC BOOK 2 5 20. KBLERD PP F7.6.11 IN SCALE BOOK 0

57• - SUBCASE FLOATING POINT CONSTANTS

1. TMO TIMEUI-TMO FIRST INTERVAL. 000O0E + 0O 4. FRACPW TIME OF ALL IRRAD SUBCASE.10000E+01
2. RHO TOTAL MATERIAL OENIITY .000001+00 5. TCONST SECS IN SPECIAL TIME UNIT.«6400E+05
3. CUT FRACTION CUTOFF lit DECAY .000001+00

Page D.8
 UP, Fuel - Iapurity Activation Products

PROGRAM INPUT DATA

1$$ 1 IT
FIRST BURNUP STEP USING 25* BURNUP COMPOSITION LIBRARY
3$$ 21 A3 1 0 A6 1 A16 2 E 2T
35$$ 0 4T
54$$ 11R0 1
56$$ 5 5 1 0 0 3 A13 IS 4 0 A17 1 0 11 I Si
59** Fl.665+14
60** 22.8 45.7 68.6 91.5 114.4
73$$ 130000 50000 480000 200000 60000 240000 290000 660000 80000
640000 260000 120000 250000 420000 280000 140000 470000 70000
74** 50-3 .3-3 .2-3 50-3 100-3 25-3 20-3 .15-3 134.454
.1-3 100-3 50-3 10-3 4-3 30-3 60-3 1-3 5C-?
75$$ 4 4 4 4 4 4 4 4 4
4 4 4 4 4 4 4 4 4 6T
SECOND BURNUP STEP USING 75% BURNUP COMPOSITION LIBRARY
3$$ 22 A3 1 0 A6 1 E 2T
3 5 $ $ 0 4T
5 4 $ $ 11R0 1
5 6 $ $ 5 5 1 0 0 1 A10 5 A14 4 0 A17 1 0 0 E
5 7 * * 1 1 4 . 4 E 5T
59** Fl.665+14
6 0 * * 1 3 7 . 2 1 6 0 . 1 1 8 2 . 9 2 0 5 . 8 2 2 8 . 7 2 6T
5 4 $ $ F0
56$$ 0 8 A4 0 1 0 A10 5 A14 5 3 A17 4 0 0 E ST
BRUCE FUEL - FUEL ACTIVATION (BURNUP-DEPENDENT LIB)
1 KQ URANIUM
60** 1 5 10 20 1+2 1+3 1+4 1+6
61** Fl-20
65$$ Al 1 A4 1 A7 1 E 6T
1$$ 0 IT

PROGRAM OUTPUT VKRIFICATIOll DATA

PROGRAM VER LOAD DAT! USERNAME ACCOUNT NODE RUN ID NUMBER

ORIOENS 1.1 88-09-08 WILRIH WFORM MC4 88-10-27 23.46.57

PROGRAM VERIFICATION INFORMATION

PROGRAM: ORIOENS
CREATION D*-'*:•. 88-09-08
LIBRARY: AECLtSABl:(SAB CODEB.SCALECODEIORXOER.EXE
JOBRAME: FWF-FUEL
DATE OF EXECUTION: 88-10-27
TIME OF EXECUTION: 21.46.S7
1$ ARRAY 1 ENTRIES READ
IT
3$ ARRAY 33 ENTRIES READ
2T

Page D.9
 00, Fuel - Iapurity Activation Products

DATA LIBRARY VERIFICATION INFORMATION

DEFAULT DIRECTORY : AECL$SAB:(WILKIN.FWF]

UNIT
NUMBER DATA SET NAME URIT FUNCTION

5 ORSIRPFUEL CARD INPUT

6 ORSOUTFUEL OUTPUT PRIRT
13 ORSFIDFUEL FIDO EDIT OUTPUT
0 (und«fin«d) MASTER PHOTOR D/B
0 (undvfinad) REUTROR ENERGY GROUPS
105 AECL$SAB1:(SAB_CODES.SCALELIB]CPUFAC.DAT CPU NORMALIZATION
0 (undafin«d) ~ CARD PUNCH
11 SCRSSAB:(WILKIH1FOROU.DAT SCRATCH
0 (undefined) BINARY GAMMA SOURCE
21 AECLSSAB1:[SAB SHIELD.LIBRARY1BRUCECY1WLIB.BIN LIBRARY DATA SET NUMBER

LIBRARY INFORMATION...

COUPLE PROCESSED CROSS SECTIONS WITH

ORIGEN-S DATA LIBRARIES FOR CAHDU REACTOR
BRUCE rUEL ASSEMBLY BURRUP CALCULATIONS
UPDATE LIBRARY WITH PU243 CAPTURE DATA
UPDATE LIBRARY WITH CORRECTED NP236 DECAY DATA

ORIGEN-S INPUT DATA

3$ LIBRARY CONSTANTS

1. RDSET LIBRASS UHIT RUMBER 21 11. ITMAX RUMBER OF LIBRARY RUCLIDE 1610
2. ROLIB R O . OF LIBRARIES IR NDSET 4 19. ILMAX RO. OF LIBRARY 1 RUCLIDES <••
3. RTYPE 0/1/>1 LIBRARY TYPE 1 20. IAMAX RO. OF LIBRARY 2 HUCLZDES 102
4. HORP -R/O/R RTRR GRP STRUCTURE 1 21. IFMAJC HO OF LIBRARY 3 RUCLZDES *22
5. JCOUT PRRT OUTPUT URIT NUMBER 6 22. U M A X RO. OF OFF DIAG ELEMENTS «5»S
6. MPCTAB 0/1 YES/NO AIR .WATER HERDS 1 23. RREACT MAX. RO. OF REACS/NUCLZDE 0
7. IKPT 0/1 PHTN LIB FROM RDSST 0 24. RFISO RO. OF FISSILE ISOTOPES S
I. IR 1/0 PRRT TRANS.MATRIX Y/N 0 25. RELEM MAX. ATOMIC RO. ZR CALC. 99
9. LPU 0/R ACTIRIDE CARDS/RD9ST N 0 2(. RMO NORTH ZR DATE OF LIBRARY 24
10. RR1 1/0 PRUT 1ST LIB. TBLE «/" 0 27. HDAY DAY IR DATE •
II. Ml 2 1/0 PRRT 2ND LIB. TILS Y/R 0 21. NYR YEAR ZR DATS ••
12. UN3 1/0 PRRT 1RD LIB. TBLE Y/R 0 29. RERAC RO. ACTZRZDS PHTR S ORPS II
13. RR4 1/0 PRRT 4T« LIB. TBLE Y/R 0 30. RERLE RO. OF LIGHT EL. PNTN ORP 12
14 RRS 1/0 PRNT STB LIB. TBLE Y/N 0 31. RERFP RO. FISSION PRD PNTR ORPS 12
15. RR6 1/0 PRNT ITM LIB. TBLS Y/N 0 32. RVkAT 0/-R/R INTEGRAL OPTIOR 0
16. RH7 0/1/2/3 CONC. UNITS 2 33. RG NUMBER OF INElviY GROUPS 1
17. HNI -1/0 M I N T LIB. PROLOG H/Y -1

9$ LIBRARY POSITION NUMBER

1. RLIBE REACTOR LIB. POS. IN NDSET

1/2/3/4 MTOR/LWR/LMFBR/MSBR
PageD -l°
 UP, Fuel - I»purity Activation Products

54$ SPECIAL OPTIONS - OPTION I REQUESTED IF JOPT(I) <> 0

1. JOPT(l) PP F7.6.2 5 SCALE BOOK 2 0 7. JOPT(7) PP F7.6.25 SCALE BOOK 2
2. JOPT(2) PUNCH STRT CON. OF SUBCAS 0 8. JOPT(B) NOT USED
3. JOPTI3) PP F7.6.25 SCALE BOOK 2 0 9. JOPT(9) PP F7.6.25 SCALE BOOK 2
4. JOPT14) PP F7.6.25 SCALE BOOK 2 0 10. JOPT(IO) DO ADJOINT CALCULATIONS
5. JOPT(5) PP F7.6.25 IN SCALE BOOK 0 11. JOPT(ll) NOT USED
6. JOPT<6) PP F7.6.25 SCALE BOOK 2 0 12. JOPTU2) MODEL REMOVABLE HEAT/FIS

56$ - SUBCASE INTEGER CONTROL CONSTANTS

1. MMN NO. OF IRRADIATION INTERVA S 11. NTERM <NO. OF EXP EXPANSION TER 21
2. MOUT TIME INTERVALS IN SUBCASE 5 12. NSHRT 100
3. INDEX 0/1 1 13. NX CMP NO. OF NUCLIDE OR EL.CONC 18
4. NTABLE 0/1 OUTPUT/SUMMARY TABLES 0 14. NUNIT 1/2/3/4/5/6 TIME 4
5. MSTAR TIME FOR CUTOFF PHOT SOURC 0 15. NT I 0/1/2/3 0/TITLE/8ASIS/BOT 0
6. NGO -1/0/1/2/3 NEXT PROBLEM 3 16. NPUN 0/N NO PUNCHES/PUNCH ON N 0
7. MPROS PP F7.6.11 SCALE BOOK 2 0 17. JTO PP F7.6.11 IN SCALE BOOK 1
8. NPROS 0 IF MPROS>0/R'MAX GRP. * 0 IS. NUC PP F7.6.12 SCALE BOOK 2 0
9. MFEED NUCLIDCS FED TO SYSTEM 0 19. NEL SAME AS NUC FOR ELE TABLE 0
10. MSUB PP F7.6.11 IN SCALE BOOK 2 0 20. KBLEND PP F7.6.11 IN SCALE BOOK 0

57* - SUBCASE FLOATING POINT CONSTANTS

1. TMO TIMC(I)-TMO FIRST INTERVAL.OOOOOE+00 4. FRACPW TIME OF ALL IRRAD SUBCASE.10000E+01

2. RHO TOTAL MATERIAL DENSITY .OOOOOE+00 5. TCONST SECS IN SPECIAL TIME UNIT.86400E+05
3. CUT FRACTION CUTOFF IN DECAY .vJ0O0E+O0

3$ ARRAY 33 ENTRIES READ

2T
DATA LIBRARY VERIFICATION INFORMATION

DEFAULT DIRECTORY : AECL$SAB:IWILKIN.FWF]

UNIT
NUMBER DATA SIT NAME UNIT FUNCTION

i OR1IMPFUEL CARD INPUT

6 ORSOUTFUEL OUTPUT PXI1R
13 ORSFIDFUEL FIDO EDIT OUTPUT
60 AECL$IAB1:[SAB CODES.SCALELIBlPHOHAST60.DAT MASTER FHOTOR D/»
0 (und*fin«d) NEUTRON ENERGY GROUPS
10S AECLlSABl:[SAB CODES.SCALELIBICPUFAC.DAT CPU NORMALISATION
0 (undefined) CARD PUNCH
11 1CR$SAB:[VILKINIFOR011.DAT SCRATCH
SI (undefined) BINARY GAMMA SOURCE
22 AECL$SAB1:(SAB SHIELD.LIBRARY|BRUCECY2WLIB.BIN LIBRARY DATA SST NUMBER

P*ff« D.ll
 UP, Fuel - Impurity Activation Products

LIBRARY INFORMATION...

COUPLE PROCESSED CROSS SECTIONS WITH

0RI6EN-S DATA LIBRARZES FOR CAMDU REACTOR
BRUCE FUEL ASSEMBLY BURNUP CALCULATIONS
UPDATE LIBRARY WITH PU243 CAPTURE DATA
UPDATE LIBRARY WITH CORRECTED NP236 DECAY DATA
ORIGEN-S INPUT DATA

3$ LIBRARY CONSTANTS

1. NDSET LIBRARY UNIT NUMBER 22 18. ITMAX NUMBER OF LIBRARY NUCLIDE 1610
2. NOLIB N O . OF LIBRARIES IN NDSET 4 19. ILMAX NO. OF LIBRARY 1 NUCLIDES 688
3. NTYPE 0/l/>l LIBRARY TYPE 1 20. IAMAX NO. OF LIBRARY 2 NUCLIDES 102
4. NGRP -N/0/N NTRN 6RP STRUCTURE 1 21. IFMAX NO OF LIBRARY 3 NUCLIDES 822
5. KOUT PRNT OUTPUT UNIT NUMBER 6 22. IZMAX NO. OF OFF DIAG ELEMERTS 6585
6. MPCTAB 0/1 YES/NO AIR,WATER HZRDS 1 23. NREACT MAX. NO. OF REACS/RUCLIDE 0
7. INPT 0/1 PHTN LIB FROM NDSET 0 24. NFISO N O . OF FISSILE ISOTOPES 5
S. IR 1/0 PRNT TRANS.MATRIX Y/N 0 25. NELEM MAX. ATOMIC NO. IN CALC. 99
9. bPU 0/N ACTIHIDE CARDS/RDSET N 0 26. HMO MONTH IN DATE OF LIBRARY 25
10. NN1 1/0 PRNT 1ST LIB. TBLE Y/N 0 27. NDAY DA? IN DATE 3
11. NN2 1/5 PRNT 2ND LIB. TBLE Y/N 0 26. NYR YEAR IN DATE 88
12. NN3 1/0 PRNT 3 R D LIB. TBLE Y/N 0 29. NENAC NO. ACTINIDE PHTN E GRPS 18
13. NR4 1/0 PRRT 4TH LIB. TBLE Y/N 0 30. NENLE NO. OF LIGHT EL. PHTN GRP 12
14. HNS 1/0 PRNT 5TH LIB. TBLE Y/N 0 31. NENFP NO. FISSION PRD PHTN GRPS 12
IS. RICC 1/0 PRNT STH LIB. TBLE Y/N 0 32. NVERT 0/-R/N INTEGRAL OPTION 0
16. NR7 0/1/2/3 CONC. UNITS 2 33. RG NUMBER OF ERERGY GROUPS 1
17. NR8 >l/0 PRINT LIB. PROLOG N/Y -1

S$ LIBRARY POSITION NUMBER

1. NLIBC REACTOR LIB. POS. IR RD3ET

1/2/3/4 HTGR/LWR/LMFBR/MSBR

54$ SPECIAL OPTIORS - OPTIOR I REQUESTED IF JOPT(I) <> 0

1. JOPT(l) PP F7.6.25 SCALE BOOK 2 0 7. JOPT(7) PP F7.6.25 SCALE BOOK 2 0
2. J0PTI2) PUNCH STXT COR. OP SUBCAS 0 8. JOPT(3) ROT USED . 0
3. JOPT<3> PP F7.6.25 SCALE BOOR 2 0 9. JOPT(9) PP F7.6.23 SCALE BOOK 2 0
4. JOPTI4) PP F7.6.2S SCALE BOOR 2 0 10. JOPTU0I DO ADJOINT CALCULATIONS 0
i. JOPT(S) Pf F7.6.2S IR SCALE BOOK 0 11. JOPTU1I ROT USED 0
6. J0PTI6) PP F7.6.25 SCALE BOOK 2 0 12. JOPTU2) MODEL REMOVABLE RSAT/MS 1

Page 0.12
 00, Fuel - Impurity Activation Products

56$ - SUBCASE INTEGER CONTROL CONSTANTS

1. MMN NO. OF IRRADIATION INTERVA 5 11. NTERM <NO. OF EXP EXPANSION TER 21
2. MOUT TINE INTERVALS IN SUBCASE 5 12. HSHRT 100
3. INDEX 0/1 1 13. NXCMF NO. OF NUCLIDE OR EL.CONC 0
4. NTABLE 0/1 OUTPUT/SUMMARY TABLES 0 14. RUNIT 1/2/3/4/5/6 TIME 4
5. MSTAR TIME TOR CUTOFF PHOT SOURC 0 15. HTI 0/1/2/3 0/TITLE/BASIS/BOT 0
6. NGO -1/0/1/2/3 NEXT PROBLEM 1 16. HPUN 0/N NO PUNCHES/PUNCH ON N 0
7. MPROS PP F7.6.11 SCALE BOOK 2 0 17. JTO PP F7.6.11 IN SCALE BOOK 1
8. NPROS 0 IF MPROS-0/N-MAX GRP. # 0 IS. HUC PP F7.6.12 SCALE BOOK 2 0
9. HFEED NUCLIDES FED TO SYSTEM 0 19. REL SAME AS NUC FOR ELE TABLE 0
10. NSUB PP F7.6.11 IN SCALE BOOK 2 5 20. XBLEHD PP F7.6.11 IN SCALE BOOK 0

57* - SUBCASE FLOATING POINT CONSTANTS

1. TMO TIME(I)-TMO FIRST INTERVAL.00000E+00 4. FRACPW TIME OF ALL IRRAD SUBCASE.10000E+01

2. RHO TOTAL MATERIAL DENSITY . 0000OE+OO 5. TCONST SECS IN SPECIAL TIME UNIT.«6400E+05
3. CUT FRACTION CUTOFF IN DECAY .OOOOOE+00

56$ - SUBCASE INTEGER CONTROL CONSTANTS

1. MMN NO. OF IRRADIATION INTERVA 0 11. NTERM <NO. OF EXP EXPANSION TER 0
2. MOUT TIME INTERVALS IN SUBCASE 8 12. HSHRT 0
3. INDEX 0/1 0 13. NX CMP NO. OF NUCLIDE OR EL.CONC 0
4. NTABLE 0/1 OUTPUT/SUMMARY TABLES 0 14. NUNIT 1/2/3/4/5/6 TIME 5
5. MSTAR TIME FOR CUTOFF PHOT SOURC 1 IS. HTI 0/1/2/3 0/TITLE/BASIS/BOT 3
6. NGO -1/0/1/2/3 NEXT PROBLEM 0 16. HPUR 0/N NO PUNCHES/PUNCH OR H 0
7. MPROS PP F7.6.11 SCALE BOOK 2 0 17. JTO PP F7.6.11 IN SCALE BOOK 4
8. NPROS 0 IP MPRO3-0/N-MAX GRP. t 0 18. NUC PP F7.6.12 SCALE BOOK 2 0
9. MFEED NUCLIDES FED TO STSTCM 0 19. NEL SAME AS NUC FOR ELE TABLE 0
10. MSUB PP F7.6.11 IN SCALE BOOK 2 5 20. KBLERD PP F7.6.11 IH SCALE BOOK 0

57* - SUBCASE FLOATING POINT CONSTANTS

1. TMO TIMB(I)-TMO FIRST INTERVAL.OOOOOE+00 4. FRACPW TIME OF ALL IRRAD SUBCASE.10000E+01

2. RHO TOTAL MATERIAL DENSITY .00000E+00 5. TCONST SECS IN SPECIAL TIME URIT.86400E+05
3. CUT FRACTION CUTOFF IN DECAY .OOOOOE+00

Page D.13
 Zircaloy Activation Products

PROGRAM INPUT DATA

1$$ 1 IT.
FIRST BURHUF STEP USING 25* BURNUP COMPOSITION LIBRARY
3$$ 21 A3 1 0 A6 1 A16 2 E 2T
35$$ 0 4T
54$$ llRO 1
56$$ 5 5 1 0 0 3 A13 25 4 0 A17 1 0 0 E 5T
59*» Fl.719+14
S0»* 22.1 45.7 68.6 91.5 114.4
73$$ 500000 130000 50000 480000 60000 270000 290000 720000 10000
820000 120000 80000 400000 260000 250000 420000 280000 410000
70000 140000 730000 220000 740000 230000 240000
74«» 17 75-3 .5-3 .5-3 270-3 20-3 50-3 100-3 25-3
130-3 20-3 1.5 977.74 2.4 50-3 50-3 70-3 100-3
80-3 120-3 200-3 50-3 100-3 50-3 1.3
75$$ 4 4 4 4 4 4 4 4 4
4 4 4 4 4 4 4 4 4
4 4 4 4 4 4 4 6T
SSCOND BUKNUF STEP USINO 75% BURNUP COMPOSITION LIBRARY
3$$ 22 A3 1 0 A6 1 E 2T
35$$ 0 4T
54$$ 11R0 1
56$$ 5 5 1 0 0 1 A10 5 A14 4 0 A17 1 0 0 E
57*« 114.4 E 5T
59** Fl.719+14
60** 137.2 160.1 182.9 205.8 228.72 6T
54$$ P0
56$$ 0 8 A4 0 1 0 A10 5 A14 5 3 A17 4 0 0 E 5T
BRUCE FUEL - CLADDING ACTIVATION (BURNUP-DEPENDENT LIB)
1 KG 2IRCALOY
60** 1 5 10 20 1+2 1+3 1+4 1+6
6 1 " Fl-20
65$$ Al 1 A4 1 A7 1 E 6T
1$$ 0 IT

PEOCJtAH OUTPUT VERIFICATION DATA

PROGRAM VEX LOAD DATE USERNAME ACCOUNT NODE RUN ID NUMBER

ORIGENS 1.1 88-09-08 WILKIH WORM WC4 88-10-27 23.57.50

PROGRAM VERIFICATION INFORMATION

PROGRAM: ORIGENS
CREATION BATE: 88-01-08
LIBRARY: AECL$SAB1:tSAB CODE8.JCALECODEIORIGEN.EXE
JOBNAME: POT-CLAD
DATE OF EXECUTION: 88-10-27
T M I OP EXECUTION: 21.S7.S0
1$ ARRAY 1 ENTRIEI READ
IT
}$ ARRAY 33 ENTRIES READ
2T
Page D.K
 Zircaloy Activation Products

DATA LIBRARY VERIFICATION INFORMATION

DEFAULT DIRECTORY : AECL$SAB:[WILKIN.FWF ]

UNIT
NUMBER DATA SET NAME UNIT FUNCTION

5 ORSINFCLAD CARD INPUT

6 OSSOUTCLAD OUTPUT PRINT
13 ORSFIDCLAD FIDO EDIT OUTPUT
0 (undefined) MASTER PHOTON D/B
0 (undefined) HEUTSOR ENERGY CROUPS
105 AECL$SAB1:[SAB_CODES.SCALELIBICPUFAC.DAT CPU NORMALIZATION
0 (undefined) ~ CARD PUNCH
11 SCR$SAB:[WILKIN]FOR011.DAT SCRATCH
0 (undefined) BINARY GAMMA SOURCE
21 AECL$SAB1:[SAB SHIELD.LIBRARY1BRUCECY1WLIB.BIN LIBRARY DATA SET NUMBER

LIBRARY INFORMATION...

COUPLE PROCESSED CROSS SECTIONS WITH

ORIGEN-S DATA LIBRARIES FOR CANDU REACTOR
BRUCE FUEL ASSEMBLY BURNUP CALCULATIONS
UPDATE LIBRARY WITH PU243 CAPTURE DATA
UPDATE LIBRARY WITH CORRECTED NP236 DECAY DATA

ORIGEN-S INPUT DATA

3$ LIBRARY CONSTANTS

I. NDSET LIBRARY UNIT NUMBER 21 11. ITMAZ NUMBER OF LIBRARY RUCLIDE 1(10
HOLIB NO. OF LIBRARIES IR RDSET 4 19. ILMAX NO. OF LIBRARY 1 RUCLIDBS C*t
HTYPB O/1/>1 LIBRARY TYPE 1 20. IAMAX NO. OF LIBRARY 2 NUCLIDES 102
RORP -R/O/R NTRN GRP STRUCTURE 1 21. IFMAX NO OF LIBRARY 3 NUCLIDES 122
ROUT PRNT OUTPUT UNIT NUMBER 6 22. UMAX NO. OF OFF DIAO ELEMENTS 6515
HPCTAB 0/1 YES/RO AIR,WATER RtRDS 1 23. RREACT MAX. NO. OF REACS/HUCLIDE 0
INPT 0/1 PHTN LIB FROM RDSET 0 24. RFISO NO. OF FISSILE ISOTOPES S
IR 1/0 PRRT TRANS.MATRIX Y/N 0 25. HELEN MAX. ATOMIC NO. IN CALC. 99
LPU 0/N ACTINIDE CARDS/NDSET N 0 2(. HMO MONTH IN DATE OF LIBRARY 24
10. NN1 1/0 PRRT 1ST LIB. TBLE Y/R 0 27. HDAY DAY IR DATE •
II. RR2 1/0 PRRT 2RD LIB. TSLE Y/N 0 21. HTR YEAR IN OATS . II
12. HH3 1/0 PRNT 3RD LIB. TBLE Y/R 0 29. HBRAC NO. ACTINIDE PRTM E GRPS II
11. NR4 1/0 PRRT 4TH LIB. TBLE Y/N 0 30. RCMLE NO. OF LIGHT EL. PRTR GRP 12
14. HHS 1/0 PRNT STH LIB. TBLE Y/N 0 31. RERFP NO. FISSION »RD PHTR GRPS 12
15. NH6 1/0 PRNT 6Tit LIB. TBLE Y/R 0 32. RVERT 0/-N/N INTEGRAL OPTION 0
16. HR7 0/1/2/3 CONC. UNITS 2 33. HO NUMBER OF ENERGY GROUPS 1
17. RNI -1/0 PRIHT LIB. PROLOG H/Y -1

S$ LIBRARY POSITION RUMBER

1. HLIBC REACTOR LIB. POS. IN NDSET

1/2/3/4 HTOR/LWR/LMFBR/MSBR

Page D.1S
 Zircaloy Activation Products

54$ SPECIAL OPTIONS - OPTION I REQUESTED IF J O P T U ) <> 0

1. JOPTU) PP F7.6.25 SCALE BOOK 2 0 7. JOPT(7) PP F7.6.25 SCALE BOOK 2

2. JOPT(2) PUNCH STRT CON. OF SUBCAS 0 8. JOPT(ft) HOT USED
3. JOPTI3) PP F7.6.25 SCALE BOOK 2 0 9. JOPT(9) PP F7.6.2S SCALE BOOK 2
4. JOPTU) PP F7.6.25 SCALE BOOK 2 0 10. JOPT(IO) DO ADJOINT CALCULATIONS
5. JOPT(S) PP F7.6.25 IN SCALE BOOK 0 11. JOPT(ll) NOT USED
«. JOPT(fi) PP F7.6.25 SCALE BOOK 2 0 12. JOPT(12) KODEL REMOVABLE HEAT/FIS

56$ - SUBCASE INTEGER CONTROL CONSTANTS

1. MMN NO. OF IRRADIATION INTERVA 5 11. STERN <NO. Or EXP EXPANSION TER 21
2. MOUT TINS INTERVALS IN SUBCASE S 12. NSHRT 100
3. INDEX 0/1 1 13. NXCMP NO. OF NUCLIDE OR EL.CONC 25
4. NTABLE 0/1 OUTPUT/SUMMARY TABLES 0 14. NttNIT 1/2/3/4/5/6 TIME 4
5. HSTAR TIME FOB CUTOFF PHOT SOURC 0 15. NT I 0/1/2/3 0/TITLE/BASIS/BOT 0
6. NGO -1/0/1/2/3 NEXT PROBLEM 3 16. NPUN 0/N NO PUNCHES/PUNCH ON N 0
7. MPROS PP F7.6.11 SCALE BOOK 2 0 17. JTO PP F7.6.11 IN SCALE BOOK 1
a. NPROS 0 IF MPROS°0/N>MAX QRP. # 0 IS. NUC PP F7.6.12 SCALE BOOK 2 0
9. HFEED NUCLIDCS FED TO SYSTEM 0 19. NCL SAME AS NUC FOR ELB TABLE 0
10. MSUB PP F7.6.11 IN SCALE BOOK 2 0 20. KBLEND PP F7.6.11 IN SCALE BOOK 0

57* - SUBCASE FLOATING POINT CONSTANTS

1. TMO T I M S I D - T M O FIRST INTERVAL. 00000E+00 4. FRACPW TIME OF ALL IRRAD SUBCASE.10000E+01
2. RHO TOTAL MATERIAL DENSITY . O000OE+O0 5. TCONST SECS IN SPECIAL TIME UNIT.§64001+05
3. CUT FRACTION CUTOFF IN DECAY .OOOOOE+GO

3$ ARRAY 33 ENTRIES READ

2T
DATA LIBRARY VERIFICATION INFORMATION
DEFAULT DIRECTORY : AECL$SAB: [WILKIN.FWF1
UNIT
NUMBER DATA SET MAMS UNIT FUNCTION

5 ORJINPCLAD CARD INPUT

( ORIOUTCLAD OUTPUT PRINT
13 ORIFIDCLAD FIDO EDIT OUTPUT
(0 AECLlSABl:[SAB CODES.ICALELIBIFNOMAST60.DAT MASTER PROTON D/R
0 |und«fln»d) NEUTRON ENEROY GROUPS
105 ASCDSABl: I SAB CODBS . SCALELIB) CPUFAC. D M era NORMALIXATION
0 (undaflnad) CARD PUNCt
11 (ICR«1AB: (WILK1NIFOR011.DAT tCRATCR
SI (und«fln«d) BINARY QAMMA SOURCE
22 AECL*»AB1: (SAB SHIELD. LIBRARY) SRVCtCY2m.il. IZ1I LIBRARY DATA SSI NUMBER

Pftg* D.16
 Zircaloy Activation Products

LIBRARY INFORMATION...

COUPLE PROCESSED CROSS SECTIONS WITH

ORIGEB-S DATA LIBRARIES FOR CANDU REACTOR
BRUCE FUEL ASSEMBLY BURNUP CALCULATIONS
UPDATE LIBRARY WITH PU243 CAPTURE DATA
UPDATE LIBRARY WITH CORRECTED NP236 DECAY DATA

ORIOEN-S INPUT DATA

3$ LIBRARY CONSTANTS
1. NDSET LIBRARY UNIT NUMBER 22 It. ITMAX NUMBER OF LIBRARY NUCLIDE 1610
2. NOLIB NO. OF LIBRARIES IN NDSET 4 19. ILMAX NO. OF LIBRARY 1 NUCLIDES 688
3. NTYPE O/1/>1 LIBRARY TYPE 1 20. IAMAX NO. OF LIBRARY 2 NUCLIDES 102
4. NGRP -N/O/N NTRN SRP STRUCTURE 1 21. IFMAX NO OF LIBRARY 3 HUCLIDES 822
5. KOUT PRNT OUTPUT UNIT NUMBER 6 22. IZMAX NO. OF OFF DIAQ ELEMENTS 6585
6. MPCTAB 0/1 YES/NO AIR,WATER HZRDS 1 23. NREACT MAX. NO. OF REACS/NUCilDE 0
7. INPT 0/1 PHTN LIB FROM NDSET 0 24. HFISO NO. OF FISSILE ISOTOPES 5
8. IR 1/0 PRNT TRANS.MATRIX Y/N 0 25. NELCM MAX. ATOMIC NO. IN CALC. 99
9. LPU 0/N ACTINIDE CARDS/HDSET N 0 26. NMO MONTH IN DATE OF LIBRARY 25
10. NN1 1/0 PRNT 1ST LIB. TBLE Y/N 0 27. NDAY DAY IN DATS 8
11. NN2 1/0 PRNT 2ND LIB. TBLE Y/N 0 28. NYR YEAR IN DATE 88
12. NN3 1/0 PUNT 3RD LIB. TBLE Y/N 0 29. NENAC NO. ACTINIDE PHTN E GRPS It
13. NN4 1/0 PRNT 4TH LIB. TBLE Y/N 0 30. NENLE NO. OF LIGHT EL. PHTN GRP 12
14. NNS 1/0 PRNT 3TH LIB. TBLE Y/N 0 31. NENFP NO. FISSION PRO PHTN GRPS 12
15. NN6 1/0 PRNT 6TH LIB. TBLE Y/N 0 32. NVEXT 0/-N/N INTEGRAL OPTION 0
16. NN7 0/1/2/3 CONC. UNITS 2 33. NO NUMBER OF ENERGY GROUPS 1
17. NNS -1/0 PRINT LIB. PROLOG N/Y -1

5$ LIBRARY POSITION NUMBER

1. NLIBE REACTOR LIB. POS. IR NDSET
1/2/3/4 HTOR/LWR/LMFBR/M8BR

54$ SPECIAL OPTIONS - OPTION I REQUESTED IF JOPT(I) <> 0

1. JOPT(l) PP F7.6.25 SCALE BOOK 2 0 7. JOPTI7) PP F7.6.25 SCALE BOOK 2 0
1. JOPT<2> PUNCH STRT COR. Of SVBCAS 0 *. JOFT(I) ROT USED . 0
3. JOPTI3) PP F7.6.2S SCALE BOOK 2 0 9. JOPTI9) PP F7.6.2S SCALE BOOK 2 0
4. JOPTI4) PP F7.6.25 SCALE BOOK 2 0 10. JOPT(IO) DO ADJOINT CALCULATIONS 0
5. JOPT(S) PP F7.6.25 IN SCALE BOOK 0 11. JOPTU1) NOT USED 0
6. JOPT(6) PP F7.6.2S SCALE BOOK 2 0 12. JOPTI12) MODEL REMOVABLE HEAT/FIS 1

Page D.17
 Zircaloy Activation Products

56$ - SUBCASE INTEGER CONTROL CONSTANTS

1. MMN NO. OF IRRADIATION INTERVA 5 11. NTERM <NO. OF EXP EXPANSION TER 21
2. MOUT TIME INTERVALS IN SUBCASE 5 12. NSHRT 100
3. INDEX 0/1 1 13. NXCMP NO. OF NUCLIDG OR ET.. CONC 0
4. NTABLE 0/1 OUTPUT/SUHHARV TABLES 0 14. HUN1T 1/2/3/4/5/6 TIME 4
5. HSTAR TIME FOR CUTOFF PHOT SOURC 0 15. RTI 0/1/2/3 0/TITtE/BASIS/BOT 0
6. NGO -1/0/1/2/3 NEXT PROBLEM 1 16. NPUN 0/R NO PUNCHES/PUNCH ON N 0
7. HPROS PP F7.6.11 SCALE BOOK 2 O 17. JTO PP F7.6.11 IN SCALE BOOK 1
8. NPROS 0 IF MPROS»0/N*MAX GRP. * 0 18. NUC PP F7.6.12 SCALE BOOK 2 0
9. MFEED NUCLIDES PED TO SYSTEM 0 19. REL SAME AS NUC FOX ELE TABLE 0
10. MSUB PP F7.6.11 IN SCALE BOOK 2 5 20. KBLEHD PP F7.6.11 IR SCALE BOOK 0

57« - SUBC.
1. TMO TIME(I)-TMO FIRST INTERVAL.00000E+00 4. FRACPW TIME OF ALL IRRAD SUBCASE.10000E+01
2. RHO TOTAL MATERIAL DENSITY .OOOOOE+00 5. TCONST SECS IN SPECIAL TIME UNIT.S6400E+05
3. CUT FRACTION CUTOFF IN DECAY .00000E+00

56$ - SUBC

1. turn NO. OF IRRADIATION INTERVA 0 11. RTERM <HO. OF EXP EXPANSION TER 0
2. MOUT TIME INTERVALS IN SUBCASE 8 12. NSHRT 0
3. INDEX 0/1 0 13. RXCMP NC. OP NUCLIDE OR EL.CORC 0
4. STABLE 0/1 OUTPUT/SUMMARY TABLES 0 14. RUNIT 1/2/3/4/5/6 TIME S
5. HSTAR TIME FOR CUTOFF PHOT SOURC 1 15. RTI 0/1/2/3 0/TITLE/BASIS/BOT 3
6. NGO -1/0/1/2/3 NEXT PROBLEM 0 16. RPUN 0/R NO PUNCHES/PUNCH ON R 0
7. NPROS PP F7.6.11 SCALE BOOK 2 0 17. JTO PP F7.6.11 IR SCALE BOOK 4
8. NPROS 0 ir MPROS*0/N*MAX ORP. » 0 18. RUC PP F7.6.12 SCALE BOOK 2 0
9. MFEED NUCLIDES FED TO SYSTEM 0 19. REL SAME AS RUC FOR ELE TABLE 0
10. MSUB PP F7.6.11 IR SCALE BOOK 2 5 20. KBLBND PP F7.6.11 IR SCALE BOOK 0

SUBCASE FLOATING POIHT CONSTANTS

1. TMO TIMEID-TMO FIRST INTERVAL.OOOOOE+00 4. FRACPW TIME OF ALL IRRAD SUBCASE.10000E+01

2. SHO TOTAL MATERIAL DENSITY .O00OOE+00 5. TCONST SSCS IR SPECIAL TIMS UNIT.86400E+05
3. COT FRACTION CUTOFF IR DECAY .00000E+00

Page D.18
 - E.I -

APPENDIX E
CREATION AND BENCHMARKING OF ORIGEN-S CROSS-SECTION DATA LIBRARIES
FOR USE IN BRUCE "A" CANDU FUEL BURNUP CALCULATIONS

CONTENTS

Page

E.I INTRODUCTION E.3

E.2 OVERVIEW OF METHODS E.3

E.2.1 ORIGEN-S CODE E.3

E.2.2 VIMS CODE E.5

E.3 UPDATING THE NUCLEAR DATA LIBRARY E.5

E.4 LIBRARY CROSS-SECTION PROCESSING E.6

E.4.1 UNIRRADIATED-FUEL LIBRARY E.V
E.4.2 BURNUP-DEPENDENDENT LIBRARIES E.8
E.5 LIBRARY BENCHMARKING E.9
E.5.1 TRANSPORT COMPARISON WITH VIMS E.9
E.5.2 UNIRRADIATED-FUEL CROSS-SECTION LIBRARY B.1O
E.5.3 BURNUP-DEPENDENT LIBRARIES E.ll

E.6 CONCLUSIONS B.12

continued...
 - E.2 -

CONTENTS (concluded)

REFERENCES E.IA

TABLES E.15

FIGURES E.18
 - E.3 -

E.I INTRODUCTION

This appendix describes the codes and procedures used in creating Bruce "A" cross-section data libraries
used by ORIGEN-S to calculate used-fuel isotope inventories. All changes that have been made to the as-
delivered version of the ORIGEN-S nuclear data library are also documented here. The ORIGEN-S isotope
inventory results obtained using the libraries are compared to CANIGEN results (Smith et al., 1987). The
ORIGEN-S results are also numerically benchmarked against VIMS (Askew et al., 1966; Donnelly, 1986), a
detailed physics lattice-cell transport and burnup code.

E.2 OVERVIEW OF METHODS

This section briefly describes the ORIGEN-S and VIMS codes, the cross-section processing codes and
outlines the sequences used in preparing a CANDU library.

E.2.1 ORIGEN-S CODE

The ORIGEN-S computer code (NUREG, 1982) is used to estimate time-dependent compositions and sources of
isotopes generated or depleted through neutron transmutation, fission, and radioactive decay. ORIGEN-S
requires the initial composition and specified burnup, and details of the neutron-flux spectrum. The
code then solves the coupled set of differential equations that describes the generation and depletion of
all isotopes involved to arrive at the final composition. The numerical method of solution is
essentially unchanged from the earlier ORIGEN and 0RIGEN2 codes, and all three codes use virtually
identical nuclide decay data.
 - E.4 -

The reaction rate cross-sections for each isotope in the ORIGEN-S library (NUREG, 1982) are described in
a three-energy-group format. The effective total cross-sections are derived from the three-group values
by weighting vith the three-group flux parameters THERM, RES, and FAST. These three flux factors are
used to partially account for neutron-flux spectral differences betveen those used to collapse the
original three-group cross-sections, and those in the problem being solved. Hovever, a sore rigorous
treatment is allowed in the SCALIAS-3.1 system (RSIC, 1986) whereby ORIGEN-S cross-sections are replaced
by those calculated from the multigroup ENDF/B databases.

Cross-sections of the multigroup ENDF/B database libraries (NUREG, 1982) are adjusted for resonance self-
shielding using the SCALIAS-3.1 processing codes BONAMI-S and NITAVL-S (NUREG, 1982). Execution of these
codes is controlled using the CSAS4 control module (NUREG, 1982), which creates resonance self-shielded
cross-section sets from an ENDF/B standard composition library. These cross-sections are subsequently
used in XSDRNPM-S, a one-dimensional S M lattice-cell transport code (NUREG, 1982). The wiltigroup cross-
sections for each material are collapsed by XSDRNPM-S into the ORIGEN-S three-group structure using the
neutron-flux spectrum in that material. The resulting cross-sections reflect the lattice environment
more accurately than if the standard three-group cross-sections and flux weighting factors are used
alone.

The COUPLE code (NUREG, 1982) is used to replace the general ORIGEN-S cross-sections vith those from the
XSDRNPM-S calculation, veighted for the specific lattice. COUPLE creates a binary version of the updated
library for use by ORIGEN-S. COUPLE also allows all the cross-section and decay data to be updated vith
revised information and permits the addition of nev precursors and daughter nuclides within the library.
 - E.5 -

E.2.2 VIMS CODE

VIMS is a multigroup neutron transport code used within AECL for reactor design and development. The
application of VIMS to lattice-cell-type reactor physics calculations has been validated for pin-cell
lattices (Donnelly, 1988) using an 89-neutron-group ENDF/B-V cross-section library (Craig and Festarini,
1985). As VIMS is primarily a reactor physics code, the burnable isotopes in the library are currently
limited to 54 individual fission products and 21 actinides that are of greatest significance to reactor
calculations. The VIMS library also ignores production through alpha decay since neutron reactions
dominate production and removal channels during reactor irradiations. Although this does not effect the
accuracy of the eigenvalues and flux distributions in reactor calculations, it can lead to significant
errors in the isotopic concentrations predicted tolloving periods of decay, when alpha decay becomes
important.

E.3 UPDATING THE NUCLEAR DATA LIBRARY

Two shortcomings were believed to exist in
predicted 23< Pu isotope concentrations were
tests against results from CANIGEN (Smith
production channel from the decay of 236 Np.
lover than expected.
the as-delivered ORIGEN-S nuclear data libraries. The
found to be consistently low in preliminary benchmarking
et al., 1987). This was thought to be due to a missing
The 244 Pu and daughter concentrations were also significantly

An analysis of the ORIGEN-S data library revealed that
the half-life and branching ratio assignment to "«Np.
isomeric states, one vith a half-life of more than 10 s
ORIGEN-S library assumed the long-lived isomeric state
production through beta decay. The underprediction in
result of missing capture data for " 3 P u .
low 2JS Pu concentrations were due most likely to
Beta decay to 236 Pu occurs from two separate 21*Np
a, and the other with a half-life of 22.5 h. The
for "*Np, which virtually eliminates 2J*Pu
244
Pu concentrations was found to be a probable
 - E.6 -

The binary ORIGEN-S working library vas updated using the COUPLE code. The 236 Np half-life vas altered
to 22.5 h, vith a beta decay branching ratio to 236 Pu of 50% (Lederer and Shirley, 1978), and the
243
Pu(n,r) 244 Pu transition vas also added. The thermal capture cross-section of 87 barns and resonance
integral of 270 barns vere obtained from BNL data (Mughabghab, 1984). The 243 Pu fission cross-section,
already included in the library, vas unaltered.

E.4 LIBRARY CROSS-SECTION PROCESSING

The SCALE cross-section library used in the lattice-cell transport calculation vas the 27-neutron-group
transport library, 27GROUPSHLD (NUREG, 1982). The 27GROUPSHLD library is based on ENDF/B-IV data and
extends the 27GROUPNDF4 library to include a number of fission producr isotopes seldom used in
criticality analyses. The library is the most extensive in the SCALE collection and contains over 230
isotopes.

Resonance processing of the ENDF/B-IV cross-sections vas performed by the BONAMI-S and NITAVL-S codes
through the CSAS4 control module. The CSASN control sequence vas invoiced vithin CSAS4, vhich halts
execution after producing the resonance-corrected cross-sections. The fuel-element pitch vas calculated
based on the average pin density inside the pressure tube. The unit cell used in the resonance
processing included the fuel element, cladding, and heavy vater coolant/moderator.

The neutron transport calculation vas earned out using the XSDRNPM-S one-dimensional S R transport code
and the resonance-processed library. The unit cell used in the calculation included the entire fuel
assembly, flow tubes and surrounding moderator. The fuel assembly vas modelled vith the central fuel
 - E.7 -

element surrounded by three concentric annular rings to approximate the outer fuel elements. The annular
ring midpoints vere equal to the true fuel ring radii, and the fuel cross-sectional area of each ring vas
conserved. The fuel diaensions vere obtained fro* Saith et al. (1987) and are listed in Table 2 of the
main body of this report. The unit cell radius of 16.122 ca is based on the equivalent fuel assembly
square pitch in the core of 28.575 cm. The cladding, moderator, and initial Bruce fuel data used in the
XSDRNPN-S calculations are listed in Table E-l.

The XSDRNPN-S code vas executed using a buckling search eigenvalue calculation, vith an initial buckling
height of 250 cm. The insulating gap betveen the pressure tube and calandria tube vas modelled as a
void. Two heavy-water cross-section sets, created in CSAS4, vere used to reflect the different operating
temperatures of the coolant and moderator. Region veighting vas employed in collapsing the 27GROUPSHLD
cross-sections, whereby one set of cross-sections vas generated for each isotope based on the neutron
spectrum in the zones in vhich the isotope resides.

The COUPLE code vas used to interface the collapsed 27GROUPSHLD cross sections, vhich are specifically
applicable to the Bruce "A" CANDU reactor operating conditions, vith the cross-sections of the original
ORIGEN-S library. This involved replacing over 230 individual isotope cross-sections in the ORIGEN-S
library. COUPLE also calculates the flux veighting factors THERM, RES and FAST froa the XSDRNPM-S
vorking library and applies these factors to those isotopes not in the XSDRNPM-S produced library.

E.4.1 UNIRRADIATED-FUEL LIBRARY

Initial coaparisons of ORIGEN-S inventory calculations vith CANIGEN and VIMS calculations vere perforaed
using a single cross-section library created based on an unirradiated-fuel composition of
99.29 X vt. *"U, and 0.71 X vt. 219 U. The initial fuel composition did not include the "*U isotope
 - E.8 -

since the CANIGEN data (Smith et al., 1987) did not include this isotope in the initial fuel composition.
In addition to the unirradiated-fuel isotopes, all other actinides and fission products in the
27GROUPSBLD library were also included at trace concentrations in the fuel, so that the new working
library vould contain all these isotopes.

E.4.2 BURNUP-DEPENDENT LIBRARIES

The unirradiated-fuel ORIGEN-S cross-section library, described above, assumes infinite dilution cross-
sections for all isotopes not initially present in the fuel. Therefore, the self-shielding effects of
the strong resonance-absorbing nuclides are not correctly accounted for as the concentrations of these
isotopes increases with burnup.

In an effort to assess the magnitude of the self-shielding effects, two burnup-dependent libraries for
the sane Bruce "A" burnup case were created. The first irradiation cycle was performed to half-burnup
using a cross-section library generated based on fuel compositions representative of the cycle midpoint,
i.e., at 2SX burnup. The cycle midpoint compositions were obtained using the unirradiated-fuel library
vsection 4.1). The second irradiation cycle was continued using a separate library created based on the
second-cycle midpoint compositions. The cross-sections of the following 17 actinides were updated at the
cycle midpoints with resonance-processed ENDF/B-IV data from the 27GROUPSHLD SCALE library: 234 U, 235 U,
"«U, »»U, » 7 Np, "«Pu, 23»Pu, 140 Pu, 241 Pu, 242 Pu, 241Am, 243Am, and i44 Cm. This isotope list is based on
an earlier study (Ryman ct al., 1982).

The sequence of codes used in creating problem-dependent cross-section libraries using the SCALIAS-3.1
system is illustrated in Figure E.I.
 - E.9 -

E.5 LIBRARY BENCHMARKING

To benchmark the Bruce "A" burnup libraries created using the SCALIAS-3.1 system, the exit burnup isotope
inventories calculated using ORIGEN-S were compared with those calculated using the CANIGEN and VIMS
codes.

The CANIGEN data were taken from a report by Smith et al. (1987) for a typical Bruce "A" exit burnup of
685 GJ/kg U and a cooling time of one year. This report did not state the specific power or irradiation
time of the assembly; hovever, archived records indicated that, most likely, an irradiation time of
228.7 d vas used, vhich would result in a specific power of 34.664 kV/kg U. These data were also assumed
for the comparison of ORIGEN-S and VIMS cases.

As mentioned previously, the initial fuel composition used to produce the CANIGEN results (Smith et al.,
1987) did not include the 234 U isotope. p or consistency, in the comparative runs, 234 U was also omitted
in the ORIGEN-S and VIMS initial fuel compositions.

E.5.1 TRANSPORT COMPARISON WITH VIMS

Prior to comparing the burnup inventory results from the different codes, a comparison was made between
the neutron spectra in the Bruce fuel elements calculated by XSDRNPM-S, and that of VIMS. The comparison
was made for unirradiated-fuel compositions. An accurate determination of the neutron spectral shape is
essential since it is used to collapse the aultigroup cross-section library. The neutron spectrum was
compared in terms of the spectral weighting factors THERM, RES and FAST. The thermal weighting parameter
THERM was found to agree with that calculated using VIMS to within 10X, while the RES and PAST parameters
agreed to within 1% and 13%, respectively. The reactivities calculated by XSDRNPM-S and VIMS were also
compared and found to agree to within 0.1 mk.
 - E.10 -

E.5.2 UNIRRADIATED-FUEL CROSS-SECTION LIBRARY

The isotopic concentrations of Bruce "A" fuel were calculated using ORIGEN-S with the unirradiated-fuel
cross-section library (Sections E.4.1). The results, in units of grams per kilograms of initial U, are
listed in Table 1 of the main body of the report, along with the VIMS and CANIGEN results. The ratios of
the inventories from ORIGEN-S and CANIGEN are compared for most of the 226 fission product and actinide
isotopes listed in the CANIGEN report (Smith et al., 1987), and for the 58 isotopes common to the ORIGEN-
S and VIMS libraries. Three actinides, 246Am, 246 Pu, and 237 Pu, do not currently exist in the ORIGEN-S or
VIMS libraries and so have not been presented. However, the concentrations of these isotopes are
insignificant and fall to essentially zero at times exceeding 10 years.

The inventories calculated by ORIGEN-S using the updated cross-section library are in good agreement vith
the results of CANIGEN vith the exception of the actinides in the uranium decay chains, vhere differences
of typically a factor of five or more are observed. Generally, the results agree to better than 50X for
the uranium and transuranic isotopes, and to better than 10% for the fission product nudides. Only tvo
fission products, l29 Xe and 152 Gd, differ by significantly more than 503:. In both actinide and fission
product groups, the ORIGEN-S predicted concentrations are generally greater than those of CANIGEN.

The effect of adding the 243 Pu(n,r) transition reaction vas a significant increase in the predicted 24*Pu
concentrations, to vithin about 30* of the CANIGEN value. The concentrations of 240 "Wp and "°U, both
daughters of 244 Pu, also increased to agree to vithin 30*. Altering the " s N p isomeric state decay data
also resulted in a significant increase in the 23< Pu concentration. The concentrations of " 2 U , 22l Th,
"«Ra, 220 Rn, "«Po, " 2 P b , 2 " B i , " 2 P o , m T l , and stable a0l Pb, all created through alpha and beta decay
from 23'Pu, similarly increased due to the decay data revision. The ORIGEN-S results for these daughter
isotopes arc still approximately seven times lover than the CANIGEN values. The concentration of the
2i3
\J isotope is of particular interest to used-fuel reprocessing since it produces dominant hard gamma
radiation during decay.
 - E.ll -

The code results are seen to be in excellent agreement for most of the 58 isotopes common to the three
libraries. The concentration of 239 Np, calculated by WINS, is lov by over seven orders of magnitude
compared to the other codes because of the missing alpha decay data for the 243 Am parent in the VIMS
library. The 2 3 4 U inventory calculated by VIMS is also lov for the same reason, although the magnitude
of the error is much smaller. The missing source contribution to 234 U from the decay of 23s Pu is
estimated to be about 3.34 x 10~s over the one-year cooling time, based on the 23*Pu half-life of
87.74 a. Adding this to the 3.62 x 10~5 inventory calculated by VIMS, which is based on neutron reaction
transitions only, results in a corrected 6.96 x 10" 5 total 2 3 4 U inventory. This corrected value is vithin
10X of the ORIGEN-S result and indicates a potential underprediction of 2 3 4 U and its daughters by
CANIGEN.

For all the other VIMS actinides and fission products, the difference betveen codes is generally less
than 10%. The largest difference in the actinides is in the predicted concentration for 23< Pu, vhere the
VIMS result indicates that the CANIGEN value for 236 Pu is significantly higher and tends to support the
ORIGEN-S value, vhich is vithin about 50* of the VIMS result. This suggests that all the 236 Pu daughters
discussed above are also likely to be predicted high by CANIGEN by a similar amount.

The only other isotopes differing by more than about SOZ from VIMS results are l51 Gd and 242"Am. The
ORIGEN-S and CANIGEN results are about a factor of 3 and 6 higher than VIMS for 157 Gd. The VIMS results
indicate that the ORIGEN-S 242- Am concentrations may be high by a factor of over tvo.

E.5.3 BURNUP-DEPBNDENT LIBRARIES

To assess the effect of self-shielding on predicted nuclide concentrations, ORIGEN-S vas executed using
•ultiple-burnup libraries (Section E.4.2). Table E-2 compares the actinide inventories, calculated using
 - E.12 -

the multiple burnup-dependent libraries (BDL), with those calculated using the single burnup library
(Section E.4.1). The CANIGEN and VIMS results are also presented for comparison. (Fission product
inventories vere not compared since only the actinide cross-sections were updated with BNDF/B-IV data for
this study). Most of the actinides in the uranium decay chains have also been omitted as their
inventories are largely unchanged by using the nultipie-burnup libraries.

The effect of using tvo irradiation cycles to approximate the variation in composition during burnup is
seen to be most significant in the Pu and Am isotopes. Most notably, the isotopes 242 Pu, 241 Pu, 240 Pu,
242-
Am, 242 Am and 241Am, which differed by as much as 80Z from the CANIGEN results, are seen to agree to
vithin 30% when tvo burnup steps are used. The other significant change occurs with 237 U, where earlier
differences of 60X have been reduced to less than 20*. These changes are a direct result of replacing
the infinite dilution cross-sections used in the unirradiated-fuel library with the resonance-corrected
cross-sections for those actinides listed above (Section 4.2) and, to a lesser degree, of accounting for
the change in the neutron-flux spectrum with time.

The change in the remaining isotope inventories was generally much smaller than those discussed above,
vith some isotopes shoving moderately better agreement with CANIGEN and others being moderately poorer.
The effect on these isotopes vas generally less than a 20% change from the unirradiated-fuel library
values.

E.6 CONCLUSIONS

The results of the unirradiated-fuel library evaluation have shovn that good overall agreement vas
obtained between the ORIGEN-S, CANIGEN, and VIMS codes. The largest discrepancies between ORIGEN-S and
the CANIGEN values occurred in the uranium decay chains, typically the daughters of "Ml and "*U decay.
 - E.13 -

The deviation in these chains generally occurs with the first or second daughter in the chain, and the
difference is propagated through to the stable isotopes at about the same ratio. This suggests that the
discrepancies in these chains may be limited to a few isotope cross-section or decay data differences
between the libraries.

The VIMS results support the predicted ORIGEN-S concentrations for 23*Pu, and hence, 2 3 2 U and its
subsequent daughters. Similarly, the VIMS results for 234 U, when corrected for the alpha decay source
term from 23*Pu, also tend to support the ORIGEN-S results and indicate that CANIGEN may be predicting
higher values for these isotopes and their daughters.

The use of multiple burnup-dependent libraries significantly improved the agreement in the actinide
inventories predicted by ORIGEN-S and CANIGEN. The largest improvements vere observed in the isotopes of
Am and Pu. Based on these results, it is recommended that future inventory calculations be carried out
using cycled libraries to correctly account for the time dependence of resonance self-shielding.

The results of this benchmarking work vith VIMS and CANIGEN indicate that ORIGEN-S, executed using the
ENDF/B-IV updated burnup-dependent cross-sections, produces isotopic inventories for Bruce "A" CANDU fuel
that are in good overall agreement vith the more rigorous methods of VIMS and the long-standing
experience base of CANIGEN. Furthermore, it has been demonstrated that the ORIGEN-S library data can be
easily accessed for any given nuclide and the cross-section and decay information revised and updated as
required.
 - E.14 -

REFERENCES

Askev, J.R., F.J. Payers, and P.B. Kemshell. 1966. A General Description of the Lattice Code VIMS.
JBNES 4, 564.
Craig, D.S. and G.L. Festarini. 1985. The ENDF/B-V VIMS Library, Chalk River Nuclear Laboratories
Report, CRNL-2784.
Donnelly, J.V. 1986. VIMS-CRNL: A Users Manual for the Chalk River Version of VIMS. Atomic Energy of
Canada Limited Report, AECL-8955.
Donnelly, J.V. 1988. Validation of VIMS with ENDF/B-V Data for Pin-Cell Lattices. Atonic Energy of
Canada Report, AECL-9564 (in press).
Lederer, CM., V.S. Shirley, and E. Browne (eds.). 1978. In Table of Isotopes, 7 t h ed., John Viley and
Sons Inc., New York.
Mughabghab, S.F. 1984. In Neutron Resonance Parameters and Thermal Neutron Cross Sections, Vol. 1,
Academic Press, Toronto.
NUREG. 1982. SCALE: A Modular Code System for Performing Standardized Computer Analyses for Licensing
Evaluation. Oak Ridge National Laboratory Report, NUREG/CR-0200, Volumes I, II, and III. Revised
1983 and 1984.
RSIC. 1986. SCALIAS 3.1: Selected FORTRAN 77 Modules From SCALE 3.1. RSIC Code Package CCC-475.
Ryman, J.C., O.V. Hermann, C.C. Vebster and C.V. Parks. 1982. Fuel Inventory and Afterheat Pover
Studies of Uranium-Fueled Pressurized-Vater-Reactor Fuel Assemblies Using the SAS2 and ORIGEN-S
Modules of SCALE vith an ENDF/B-V Updated Cross Section Library. NUREG/CR-2397, ORNL/CSD-90.
Smith, H.J., J.C. Tait and R. von Massov. 1987. Radioactive Decay Properties of BRUCE "A" CANDU™ U0 2
Fuel and Fuel Recycle Vaste. Atomic Energy of Canada Limited Report, AECL-9072.
 - E.15 -

TABLE E-l
XSDPNPM-S UNIT CELL COMPOSITIONS

Material Temp Density Isotope Atomic Density

(K) (g/cm3) (b^-cnr 1 )*
Fuel 1155 10.359 234U 1.0998e-06
235(j 1.6425e-04
238U 2.2936e-02
16Q 4.6204e-02
Zircaloy-4 549 6.550 Zr 4.2337e-02
Sn 5.2840e-04
Fe 3.5313e-04
X
Heavy vater 359 1.074 2
H 1.7958e-04
(moderator) H 6.4433e-02
16Q 3.2298e-02
Heavy vater 549 0.836 *H 1.3988e-04
2
(coolant) H 5.0188e-02
2.5157e-02
* Note: 1 b-^cm- 1 - 1 atom-cm"3 x 10~ 24 cm'-b"1
(b - barn, a unit of cross-section of a nuclear target)
 - E.16 -

TABLE E-2
BRUCE UP, FUEL - BURNUP 685 GJ/kg U
MASS, g / k g INITIAL URANIUM, 1-YEAR COOLED
ORIGEN-S CALCUUTED USING SINGLE(*) AND BURNUP-DBPBNDBNT(**) LIBRARIES

Mass, g/kg U Ratios

Isotope CANIGEN" ORIGEN-S* ORIGEN-S** VIMS ORIGEN-S*/ ORIGEN-S**/ ORIGEN-S**/
CANIGEN CANIGEN VIMS
Cf Z51 2.39e-15 1.92e-15 2.32e-15 0.80 0.97
Cf 250 1.57e-14 7.70e-15 9.02e-15 0.49 0.57
Cf 249 4.92e-14 2.60e-U 3.07e-14 0.53 0.62
Bk 249 3.84e-14 2.04e-14 2.41e-14 0.53 0.63
Cm 248 2.86e-ll 1.43e-ll 1.56e-ll 0.50 0.55
Cm 247 1.31e-09 6.04e-10 6.32e-10 0.46 0.48
Cm 246 2.22e-07 1.90e-07 1.8U-07 0.86 0.82
Cm 245 2.29e-06 1.99e-06 1.87e-06 0.87 0.82
Cm 244 2.34e-04 2.37e-04 2.04e-04 1.01 0.87
Cm 243 4.81e-06 4.43e-06 3.31e-06 0.92 0.69
Cm 242 1.12e-04 1.12e-04 8.20e-05 1.00 0.73
Am 243 2.87e-03 3.19e-03 2.54e-03 3.67e-03 1.11 0.89 0.69
Am 242M 1.73e-05 3.19e-05 2.28e-05 1.42e-05 1.84 1.32 1.61
Am 242 2.08e-10 3.82e-10 2.73e-10 1.84 1.31
Am 241 l.lle-02 1.64e-02 1.2Oe-O2 1.27e-O2 1.48 1.08 0.94
Pu 244 1.35c-06 1.01e-06 8.27e-07 0.75 0.61
Pu 243 4.75«-20 2.15e-20 2.25e-20 0.45 0.47
Pu 242 6.65c-02 8.18e-02 5.90e-02 7.44e-02 1.23 0.89 0.79
Pu 241 1.99e-01 2.93c-01 2.14e-01 2.25e-01 1.47 1.08 0.95
Pu 240 1.14e+00 9.02e-01 l.OAe+00 1.06e+00 0.79 0.91 0.98
Pu 239 2.7Oe+OO 2.56e+OO 2.77«+O0 2.61e+00 0.95 1.03 1.06
Pu 238 4.53t-03 4.68e-03 4.99e-03 4.24e-03 1.03 1.10 1.18
Pu 236 1.45t-07 2.31e-08 3.03«-08 1.39e-08 0.16 0.21 2.18
Np 240M 2.28«-19 1.69.-19 1.38c-19 0.74 0.61
Np 239 2.47t-09 2.74t-09 2.18«-09 2.73e-16 1.11 0.88 7977506
Np 237 3.09e-02 3.45e-02 3.75e-02 2.84c-02 1.12 1.21 1.32
continued...
 - E.17 -

TABLE E-2 (concluded)

Mass, g/kg U Ratios

Isotope CANIGEN ORIGEN-S* ORIGEN-S** VIMS ORIGEN-S* ORIGEN-S**/ ORIGEN-S**/
CANIGEN CANIGEN VIMS
U 240 2.57e-17 1.93e-17 1.58e-17 0.75 0.61
U 238 9.85e+02 9.85e+02 9.85e+02 9.85e+02 1.00 1.00 1.00
U 237 5.68e-09 9.08e-09 6.62e-09 1.60 1.17
U 236 7.64e-01 7.65e-01 7.66e-01 7.58e-01 1.00 1.00 1.01
U 235 2.O7e-rOO 2.00e+00 2.02e+00 2.12e+00 0.97 0.98 0.95
U 234 3.99e-05 7.54e-05 8.42e-05 3.62e-05 1.89 2.11 2.33
U 233 1.62e-08 3.2Oe-08 3.56e-08 1.98 2.20
U 232 4.63e-08 7.93e-09 1.02e-08 0.17 0.22
Pa 234H 4.82e-13 4.82e-13 4.82e-13 1.00 1.00
Pa 233 1.05e-09 1.17e-09 1.27e-09 1.11 1.21
Pa 231 3.96e-09 3.81e-09 3.83e-09 0.96 0.97
Th 234 1.43e-08 1.43e-08 1.43e-08 1.00 1.00
Th 232 3.04e-08 3.06e-08 3.05e-08 1.01 1.00
Th 231 8.43e-12 8.15e-12 8.20e-12 0.97 0.97
Th 230 6.53e-ll 1.97e-10 2.23e-10 3.02 3.42
Th 229 4.88e-14 2.89e-13 3.27e-13 5.92 6.70
Th 228 2.36e-10 4.27e-ll S.44c-ll 0.18 0.23
Th 227 1.63«-16 1.72e-16 1.72e-16 1.06 1.06
a) Saith et al., 1987
 FIGURE E-l
ORIGEN-S BURNUP-DEPENDENT LIBRARIES

COMPOSITION

SCALE •• NITAWL
LIBRARY
Each cycle creates
one burnup-dependent
XSDRNPM working library.

SCALE
WORKING
LIBRARY

w ORIGEN COUPLE
I LIBRARY

ORIGEN
WORKING ORIGEN Complete
LIBRARIES calculation.

1 INVENTORIES
N/y SOURCES
ORIGEN ACTIVITIES

COMPOSITION
 - F.I -

APPENDIX F

CALCULATION OF THE ACTINIDE, FISSION PRODUCT, AMD NEUTRON ACTIVATION PRODUCT

INVENTORIES IN USED BRUCE "A" CANDU FUEL

The radioactive inventory in used nuclear fuel results froa three mechanisms: actinides and fission
products produced during the fission process; activation products froa neutron transautation of the
uranium oxide fuel, fuel inpurjties, the Zircaloy-4 cladding, and ladding iapurities; and radioactive
decay of all unstable isotopes. The used-fuel characterization aethod aust account for the generation
and depletion of all relevant isotopes during both the irradiation and cooling phases of the fuel
history.

The fission process produces actinides and fission products in the used fuel and neutron transautation
alters these inventories, creating other isotopes in the process. Activation of the fuel and cladding in
a fuel bundle is caused by the neutron transautation of the materials and impurities contained in the
bundle vhen it is first placed into the reactor. The ORIGEN-S computer code (Hermann, 1986) vas used to
estiaate the final bundle isotopic coaposition after discharge froa the reactor and the accompanying
activity and heat that results froa decay of the radioactive isotopes. ORIGEN-S requires the user to
supply the initial coaposition, the specific power produced or the irradiating flux, and the irradiation
and cooling tiaes. The code then solves the coupled set of differential equations that describe the
generation and depletion of all isotopes involved to arrive at the final composition. Decay tables are
then used to detcraine the activity and decay heat.

ORIGEN-S determines the reaction rate for each nuclear reaction for which data is available as follows:
 - F.2 -

where R * reaction rate, cores' 1

N * atomic density of the target nucleus, b ^ - c r 1
a # f f » effective reaction cross-section, barn (b)
•th * absolute thermal neutron flux, E < E t h , the thermal energy
CUtOff, CB^'S"1

The effective reaction cross-section is defined as

a,tt B (THERM)a0 + (RES)I + (FAST)^

where a0 » 2200 m/s cross-section

I * resonance integral
al • fission-spectrum-averaged cross-section for threshold
reactions, E > E ( , the fast energy cutoff

These three items, oo, I, alf are contained in the ORIGEN-S master data library for each target isotope
and reaction handled by the code. The energy cutoffs are taken as 0.5 eV and 1.0 NeV for E t h and E e ,
respectively. The three flux veighting factors, THERM, RES, and FAST, used to describe the flux spectral
shape, are generated by the SCALIAS-3.1 system (NUREG, 1982; RSIC, 1986) and are contained in the vorking
library. This formulation allows a three-energy-group equivalent specification of the cross-sections and
irradiating flux. The user supplies ORIGEN-S with the specific pover in fixed-pover mode (used to model
the fission process) and supplies the irradiating thermal-neutron flux in fixed-flux mode (used to model
fuel and cladding activation).
 - F.3 -

The first step in the analysis is the creation of the ORIGEN-S working library. For the present work,
two burnup-dependent libraries were used, one from the start of irradiation to the burnup Midpoint, and a
second to the end of irradiation. This approach allows a midpoint correction to the cross-sections and
the irradiating flux and more accurately models the resonance self-shielding. This is particularly
important for the strong resonance absorbing nuclides. Appendix E contains the details of producing a
single working library and a comparison of results to other codes, as veil as a review of the production
of the two-cycle burnup-dependent libraries and a comparison of the actinide results to other codes.
Note that the two burnup-dependent libraries used in these calculations were created by replacing both
actinide and fission product cross-sections with appropriately collapsed ENDF/B-IV data, as discussed in
Appendix E.

Three separate 0RI6EN-S calculations were performed: one for the fuel fission process, and one each for
the fuel activation and cladding activation. The fission calculation assumed a specific power of
34.664 MW-(Mg initial U ) " 1 and an irradiation period of 228.72 d to produce the reference burnup of
685 GJ*(kg initial U)~ l . The thermal-neutron fluxes for the activation calculations were determined with
the VIMS lattice cell code (Donnelly, 1986) to be 1.665 x 1 0 " and 1.719 x 1 0 " cm'-s"1 for the fuel and
cladding, respectively, using the above specific power.

The initial fuel composition for the fission calculation, which did not include impurities, and the fuel
and cladding (Zircaloy-4) compositions, including impurities, are discussed in the main body of this
report. Note that the fissile elements (thorium in the fuel and uranium in the cladding) were excluded
from the activation calculations. The initial compositions are included in Tables 3 to 6 of the main
body of this report and the ORIGEN-S input files art given in Appendix D.

The ORIGEN-S results are listed in Appendix A (actinides and fission products from the fission process),
Appendix B (neutron activation products in the fuel), and Appendix C (neutron activation products in the
 - F.4 -

cladding), for cooling times ranging from one year to 10 6 years. Note that a numerical cutoff of 10~ 20
was used in producing the tables to limit the amount of output.

A general discussion on the accuracy of these ORIGEN-S results can be found in the main body of this
report and detailed comparisons with other codes can be found in Appendix E. Extensive experimental
analysis on CANDU fuel is required to refine ORIGEN-S accuracy estimates for both individual isotopes and
for the very long decay times that are important in disposal projects.

REFERENCES

Donnelly, J.V. 1986. VIMS-CRNL: A Users Manual for the Chalk River Version of VIMS. Atomic Energy of
Canada Limited Report, AECL-89S5.
Hermann, O.V., C.V. Parks, J.C. Ryman. 1986. Spent Fuel Decay Heat Calculations Using ORIGEN-S.
Presented at the Third International Spent Fuel Storage Technology Symposium/Workshop, April 8-10,
1986, Seattle, VA.
NUREG. 1982. SCALE: A Modular Code System for Performing Standardized Computer Analyses for Licensing
Evaluation. NUREG/CR-0200, Oak Ridge National Laboratory Report. Volumes I, II, and III. Revised
1983 and 1984.
RSIC. 1986. SCALIAS 3.1: Selected FORTRAN 77 Modules From SCALE 3.1. RSIC Code Package CCC-475.
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