Professional Documents
Culture Documents
Abstract. In the east of China, recent haze pollution has been 1 Introduction
severe and damaging. In addition to anthropogenic emis-
sions, atmospheric circulations and local meteorological con- Because of its enormous adverse effects, haze pollution has
ditions were conducive factors. The number of December become one of the most serious environmental problems in
haze days over North China and the Huanghuai area has in- China, attracting considerable scientific and social attention.
creased sharply since 2010 and was greatest in 2016. Dur- Increasing anthropogenic emissions have been contributing
ing 2016, the most aggressive control measures for anthro- to severe haze pollution in China and have mainly impacted
pogenic emissions were implemented from 16 to 21 Decem- on the long-term trend of haze days (Wang et al., 2013).
ber, but the most severe haze pollution still occurred, cover- However, interannual variations of haze days were affected
ing approximately 25 % of the land area of China and last- by meteorological conditions (Wang et al., 2015; Yang et al.,
ing for 6 days. The atmospheric circulations must play crit- 2016; Wang and Chen, 2016). At present, aerosols have ap-
ical roles in the sub-seasonal haze events. Actually, the pos- proached saturation in the atmosphere (Zhang et al., 2013).
itive phase of the East Atlantic–West Russia pattern in the When the horizontal and vertical dispersion of atmospheric
middle troposphere strengthened the anomalous anti-cyclone particulates is impeded, haze weather tends to occur (Yin et
over the NH area that confined vertical motion below. The al., 2015a). Therefore, anomalous atmospheric circulations
associated southerly anomalies made the cold air and surface play a key role in the formation of heavy haze pollution in
wind speed weaker, but enhanced the humid flow. Thus, the winter (December–February; Chen and Wang, 2015). From
horizontal and vertical dispersion of atmospheric particulates the hemispheric and regional perspective, the positive phase
was suppressed and the pollutants gathered within a narrow of the Arctic Oscillation (Yin et al., 2015b), the weak East
space. In December 2016, these key indices were strongly Asia winter monsoon (Li et al., 2015; Yin et al., 2015b), and
beneficial for haze occurrence and combined to result in the the positive phase of the East Atlantic–West Russia (EA/WR)
severest haze pollution. The influences of the preceding au- teleconnection (Yin et al., 2017) contribute to the occurrence
tumn sea surface temperature near the Gulf of Alaska and the of winter haze by modulating local anti-cyclone anomalies
subtropical eastern Pacific, October–November snow cover over North China. As a key local circulation, this anomalous
in western Siberia, and associated physical processes on haze anti-cyclone resulted in descending motion (Wu et al., 2017)
pollution are also discussed. that contributed to a reduction in the height of the planetary
boundary layer (PBL). Other conducive weather conditions
include reduced surface wind speed and enhanced humidity
in the lower atmosphere (Ding et al., 2014). Such weather
conditions trap abundant atmospheric particles and moisture,
Days
On the sub-seasonal timescale, haze pollution in Decem-
ber is quite serious and has distinct characteristics, but it has
not received adequate attention. As shown in Fig. 1, there 15
were eight wide-scale haze pollution events in China in 2016.
During six of these events, the highest PM2.5 concentration
was observed in North China. During 2016, haze pollution
10
was most severe during 16–21 December, with the highest 1979 1984 1989 1994 1999
Year
2004 2009 2014
severe haze was 710 000 km2 , which was close to the total 4 4
200 1000
area of the preceding seven episodes in 2016. In addition, its
105 km2
3 3 3 3 3
duration was 6 days, which was approximately twice as long 150 750
as the other haze episodes (Fig. 1b). Furthermore, for the past
38 years, the number of December haze days (DHD) over 100 500
Table 1. Correlation coefficients between the DHDNH and key indices from 1979 to 2016 and the ranks of key indices in 2016. The Corr
Coe1 and Corr Coe2 indicated that correlation coefficients were calculated after and before detrending. The IAC was the anti-cyclone index
that was defined as the mean Z500 over 105–125, 30–50◦ E. The local PBL, surface wind speed, and relative humidity were calculated as the
mean over the NH area. All the correlation coefficients were above the 99 % confidence level. The rank was sorted from largest to smallest,
when the Corr Coe was positive. If the Corr Coe was negative, the rank was calculated from smallest to largest.
o o
o
o
o o
Figure 2. Distribution of the global atmospheric circulation anomalies, (a) Z500 (shading) and U200 (contour) and (b) SLP (shading) and
SAT (contour) in December 2016. The anomalies here are calculated with respect to the period from 1981 to 2010.
the observed visibility and relative humidity. Hourly PM2.5 than that with winter haze days (i.e., 0.43), as analyzed by
concentration data were downloaded from the website of the Yin et al. (2017). Specific to the positive Z500 anomalies
Ministry of Environmental Protection of China. Definitions over 105–125, 30–50◦ E (i.e., the easternmost center of the
of anomalies are described in the captions for each figure. EA/WR pattern), the correlation coefficient was 0.62 (Ta-
ble 1). Thus, the anomalous anti-cyclone over the NH area in
December 2016 could efficiently weaken the vertical motion,
3 Associated atmospheric circulations in December resulting in a shallower PBL (Fig. 3a). Furthermore, possible
2016 conducive local weather conditions that included the shallow
PBL (impacting vertical dispersion), low surface wind speed
Figure 2 shows the distribution of atmospheric circulation
(impacting horizontal dispersion), and high relative humid-
anomalies in December 2016. In the upper troposphere, the
ity (impacting moisture absorption), whose correlation co-
East Asia jet stream (EAJS) was weaker and northward rel-
efficients with DHDNH were −0.59, −0.63, and 0.49 from
ative to the mean status, indicating that meridional cold air
1979 to 2016, all passed the 99 % confidence test (Table 1).
activity in East Asia was restricted (Chen et al., 2015). As a
Near the surface, the SLP gradient between Eurasia and the
result, the land surface of East China was warmer (Fig. 2b).
western Pacific decreased (Fig. 2b) and the southerly was in-
On the mid-level, there were positive anomalies of Z500
duced over the east of China. Warm and humid airflow from
over Europe and North China and negative centers over the
the south caused the surface wind speed to be slower and
central–North Atlantic and to the north of the Caspian Sea
the surface relative humidity to be higher (Fig. 3b). Physi-
(Fig. 2a). This Rossby wave train resembled the positive
cally, the positive phase of the EA/WR pattern strengthened
phase of the EA/WR pattern. To verify the relationship be-
the anomalous anti-cyclone over the NH area and the Japan
tween the DHDNH and the EA/WR pattern, the correlation
Sea from the surface to the middle troposphere, resulting in
coefficient was calculated: it was 0.66 from 1979 to 2016
confined vertical motion. The southerly anomalies made the
after removing the linear trend and exceeded the 99 % confi-
cold air and surface wind speed weaker but enhanced the hu-
dence level (Table 1). This positive correlation was stronger
o
o
o
o o o o o o o o
o o o o
o
o o
o
o o o o o
20 100
10 80
0 60
−10 40
T Inv Vis Ws Rhums
Figure 5. The variation of area-mean visibility (black), surface wind speed (blue), and surface relative humidity (red, right y-axis). The
intensity of the temperature inversion (T925 –T1000 ) in Beijing is shown as a gray bar.
o o
o
o
o o
Figure 6. Distribution of the global atmospheric circulation anomalies, (a) Z500 (shading) and U200 (contour); the white dots indicate Z500
anomalies exceeding the 95 % confidence level (t test), and (b) SLP (shading) and SAT (contour) during 16–21 December 2016; the white
dots indicate SLP anomalies exceeding the 95 % confidence level (t test). The anomalies here are calculated with respect to the period of
1981–2010.
200
PBLH (unit: m)
−200
−400
−600
−800
1 6 11 16 21 26 31
Date
Figure 8. The variation of the area-mean anomalous height of the PBL in December 2016. The anomalies here are twice a day and calculated
with respect to the December mean PBLH from 1981 to 2010.
o
o
o
o
o o o o
o
o
o o o
o o o o o o o o
6 1.5
EA/WR DHD SST
NH EP
4 1
2 0.5
0 0
−2 −0.5
−4 −1
−6 −1.5
1979 1984 1989 1994 1999 2004 2009 2014
the surface, the positive phase of the AO pattern made the Figure 13. Variation of the DHDNH (black) and SnowWS (blue) in-
cold air move southward. The anomalous southerly not only dices from 1979 to 2016. The solid lines indicate the indices whose
weakened the surface wind speed, but also led to high hu- linear trends were removed and the symbols without lines are the
midity over the NH area. The atmospheric circulations were original indices.
very conducive to severe haze pollution over the NH area.
During all of December, the number of DHDNH increased
sharply from 2010 and was greatest in 2016. The associ- The preceding autumn SST in the Pacific significantly in-
ated atmospheric circulations that were verified by climatic fluenced the winter haze days in North China (Yin et al.,
correlation analysis were similar. In other words, there was 2016) and could partly explain the severe haze pollution dur-
a weaker EAJS in the upper troposphere, a positive phase ing the winter of 2014 (Yin et al., 2017). For December,
of the EA/WR pattern in the middle troposphere, and con- the significantly correlated SST with DHDNH was located
ducive local weather conditions (lower PBL, low surface near the Gulf of Alaska and the subtropical eastern Pacific
wind speed, and abundant moisture). (Fig. 10a). The preceding autumn SST of these two areas
was averaged as an index (SSTEP ), and the correlation coeffi- the winter haze days in the east of China. The climatic re-
cients with December Z500 were calculated and are shown in lationship between the Arctic sea ice and DHDNH and the
Fig. 10b. The EA/WR pattern, especially the anomalous anti- anomalies in December were also examined and found to be
cyclone over NH and Japan, was obvious. The correlation insignificant (figure omitted). This may be due to the rela-
coefficient between SSTEP and the EA/WR index (DHDNH) tionship being different in the early and late winter, which re-
was 0.48 (0.55) after detrending; thus, we speculated that the quires more research in the future. The detailed mechanisms
SSTEP influenced DHDNH by modulating the EA/WR pat- between the external forcings and haze pollution should be
tern. The positive SST anomalies near the Gulf of Alaska studied physically and dynamically in future work. Further-
and the subtropical eastern Pacific could impact the wave ac- more, although anthropogenic emissions were limited dur-
tivity flux (WAF) and (Fig. 10b) stimulated a Rossby wave- ing haze pollution events, there were still aerosols being dis-
like pattern propagating from the eastern Pacific, through charged into the atmosphere by the dense population and
North America and the Atlantic, and to East Asia. The atmo- industry before and during 16–21 December. There is lit-
spheric action centered over the North Atlantic and Eurasia tle doubt that the high concentration of PM2.5 was the fun-
overlapped with that of the EA/WR teleconnection pattern. damental cause of haze pollution, and the associated atmo-
Therefore, the positive phase of the EA/WR pattern could spheric anomalies played key roles in the severe haze pollu-
be stimulated or enhanced by positive SSTEP and then lead tion events. The previous accumulation of atmospheric par-
to weak ventilation conditions that were beneficial for the ticles also contributed to the occurrence of haze pollution
occurrence of haze. In 2016, the positive SSTEP in autumn events. As revealed in this study, it was difficult to modify the
were consistent with the positive correlation fields, leading simultaneous atmospheric circulations, which significantly
to more DHDNH . Furthermore, the DHDNH varied with an contributed to the haze. Therefore, the controlling measures
obvious decreasing trend from 2006 to 2010, and with a of anthropogenic emissions should be implemented in ad-
dramatic increasing trend after 2010. The variation of the vance to reduce the stock of aerosols in the atmosphere.
EA/WR and SSTEP index exhibited similar features. During
the most recent 10 years, the EA/WR pattern was distributed
as its strongest negative phase in 2010 and strongest positive Data availability. Atmospheric data are available from the
phase in 2016, which was consistent with the variation of NCEP/NCAR data archive: http://www.esrl.noaa.gov/psd/
DHDNH (Fig. 11). The variation of the EA/WR pattern could data/gridded/data.ncep.reanalysis.html (NCEP/NCAR, 2017).
largely explain the trend break of DHDNH . As shown by Gao SST data are downloaded from http://www.esrl.noaa.gov/psd/
data/gridded/data.noaa.ersst.v4.html (NOAA, 2017). Snow
and Chen (2017), October SST anomalies near the Gulf of
cover data can be downloaded from Rutgers University:
Alaska and the subtropical eastern Pacific contributed to the http://climate.rutgers.edu/snowcover/ (Rutgers, 2017). The
haze pollution over North China in October 2016. Impacts of monthly EA/WR and WP indices (CPC, 2017) can be downloaded
the SSTEP on ventilation conditions were robust and could from NOAA’s Climate Prediction Center: http://www.cpc.ncep.
continue into December. Furthermore, the relationships with noaa.gov/data/teledoc/telecontents.shtml. The ground observations
autumn SST in the Atlantic were also found to be weaker and are from the website http://data.cma.cn/ (CMA, 2017). The
significant only in small regions (figure omitted). monthly PBLH data are available on the ERA-Interim website:
The Eurasian snowpack and atmospheric circulation http://www.ecmwf.int/en/research/climate-reanalysis/era-interim
dominant modes were stably coupled from autumn to (ERA-Interim, 2017). The atmospheric composition data can be
the subsequent spring (Sun, 2017), so the role of obtained from the authors.
the preceding October–November (ON) snow cover was
also examined (Fig. 12). The snow cover over western
Siberia (SnowWS ) was significantly correlated with DHDNH Competing interests. The authors declare that they have no conflict
of interest.
(EA/WR; Fig. 12a); i.e., the correlation coefficient was 0.52
(0.45) after detrending (Table 1). More snow was correlated
with a higher albedo, resulting in a colder land surface. When
Acknowledgements. This research was supported by the National
there was higher SnowWS , negative Z500 anomalies over
Key Research and Development Plan (2016YFA0600703), the Na-
western Siberia and positive anomalies over eastern China, tional Natural Science Foundation of China (41421004, 41705058),
i.e., the two active centers of the EA/WR pattern in the east, the CAS-PKU Partnership Program, the Startup Foundation for
were significantly stimulated. The WAF associated with pos- Introducing Talent of Nanjing University of Information Sci-
itive SnowWS anomalies was evidently induced near western ence and Technology (20172007), the KLME Open Foundation
Siberia and efficiently propagated westwards, and stimulated (KLME1607), and the Priority Academic Program Development of
an obvious anti-cyclone over Baikal Lake and the NH area Jiangsu Higher Education Institutions (PAPD).
(Fig. 12b). The SnowWS varied similarly with DHDNH and
achieved its maximum (minimum) in 2016 (2010). As re- Edited by: Jianping Huang
vealed by Wang et al. (2015) and Yin et al. (2017), the pre- Reviewed by: two anonymous referees
ceding autumn Arctic sea ice has a close relationship with